Small-angle neutron scattering and magnetization study of HoNi₂B₂C

The superconducting and magnetic properties of HoNi₂B₂C single crystals are investigated through transport, magnetometry and small-angle neutron scattering (SANS) measurements. In the magnetic phases that enter below the superconducting critical temperature, the small-angle neutron scattering data u...

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Hauptverfasser: Ramazanoglu, M., Laver, M., Yagmurcu, A., Cho, E.-M., Lee, S.-I., Knigavko, A., Gaulin, B.D.
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Veröffentlicht: Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України 2014
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spelling irk-123456789-1194322017-06-07T03:05:46Z Small-angle neutron scattering and magnetization study of HoNi₂B₂C Ramazanoglu, M. Laver, M. Yagmurcu, A. Cho, E.-M. Lee, S.-I. Knigavko, A. Gaulin, B.D. К восьмидесятилетию антиферромагнетизма ІІ. Эксперимент The superconducting and magnetic properties of HoNi₂B₂C single crystals are investigated through transport, magnetometry and small-angle neutron scattering (SANS) measurements. In the magnetic phases that enter below the superconducting critical temperature, the small-angle neutron scattering data uncover networks of magnetic surfaces. These likely originate from uncompensated moments, e.g., at domain walls pinned to crystallographic grain boundaries. The field and temperature dependent behavior of SANS appears consistent with the metamagnetic transitions reported in earlier works. 2014 Article Small-angle neutron scattering and magnetization study of HoNi₂B₂C / M. Ramazanoglu, M. Laver, A. Yagmurcu, E.-M. Choi, S.-I. Lee, A. Knigavko, B.D. Gaulin // Физика низких температур. — 2014. — Т. 40, № 2. — С. 205-210. — Бібліогр.: 31 назв. — англ. 0132-6414 PACS 72.10.D, 72.15.Eb, 72.15.Jf, 74.25.–q, 75.30.Kz http://dspace.nbuv.gov.ua/handle/123456789/119432 en Физика низких температур Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України
institution Digital Library of Periodicals of National Academy of Sciences of Ukraine
collection DSpace DC
language English
topic К восьмидесятилетию антиферромагнетизма ІІ. Эксперимент
К восьмидесятилетию антиферромагнетизма ІІ. Эксперимент
spellingShingle К восьмидесятилетию антиферромагнетизма ІІ. Эксперимент
К восьмидесятилетию антиферромагнетизма ІІ. Эксперимент
Ramazanoglu, M.
Laver, M.
Yagmurcu, A.
Cho, E.-M.
Lee, S.-I.
Knigavko, A.
Gaulin, B.D.
Small-angle neutron scattering and magnetization study of HoNi₂B₂C
Физика низких температур
description The superconducting and magnetic properties of HoNi₂B₂C single crystals are investigated through transport, magnetometry and small-angle neutron scattering (SANS) measurements. In the magnetic phases that enter below the superconducting critical temperature, the small-angle neutron scattering data uncover networks of magnetic surfaces. These likely originate from uncompensated moments, e.g., at domain walls pinned to crystallographic grain boundaries. The field and temperature dependent behavior of SANS appears consistent with the metamagnetic transitions reported in earlier works.
format Article
author Ramazanoglu, M.
Laver, M.
Yagmurcu, A.
Cho, E.-M.
Lee, S.-I.
Knigavko, A.
Gaulin, B.D.
author_facet Ramazanoglu, M.
Laver, M.
Yagmurcu, A.
Cho, E.-M.
Lee, S.-I.
Knigavko, A.
Gaulin, B.D.
author_sort Ramazanoglu, M.
title Small-angle neutron scattering and magnetization study of HoNi₂B₂C
title_short Small-angle neutron scattering and magnetization study of HoNi₂B₂C
title_full Small-angle neutron scattering and magnetization study of HoNi₂B₂C
title_fullStr Small-angle neutron scattering and magnetization study of HoNi₂B₂C
title_full_unstemmed Small-angle neutron scattering and magnetization study of HoNi₂B₂C
title_sort small-angle neutron scattering and magnetization study of honi₂b₂c
publisher Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України
publishDate 2014
topic_facet К восьмидесятилетию антиферромагнетизма ІІ. Эксперимент
url http://dspace.nbuv.gov.ua/handle/123456789/119432
citation_txt Small-angle neutron scattering and magnetization study of HoNi₂B₂C / M. Ramazanoglu, M. Laver, A. Yagmurcu, E.-M. Choi, S.-I. Lee, A. Knigavko, B.D. Gaulin // Физика низких температур. — 2014. — Т. 40, № 2. — С. 205-210. — Бібліогр.: 31 назв. — англ.
series Физика низких температур
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fulltext Low Temperature Physics/Fizika Nizkikh Temperatur, 2014, v. 40, No. 2, pp. 205–210 Small-angle neutron scattering and magnetization study of HoNi2B2C M. Ramazanoglu1,2, M. Laver3, A. Yagmurcu4, E.-M. Choi5, S.-I. Lee5, A. Knigavko6, and B.D. Gaulin1,7 1Department of Physics and Astronomy, McMaster University, Hamilton, Ontario L8S 4M1, Canada 2Faculty of Engineering, Istanbul Technical University, Maslak, Istanbul 34469, Turkey E-mail: mr.mehmet.ramazanoglu@gmail.com 3Department of Metallurgy and Materials, University of Birmingham Edgbaston, Birmingham B15 2TT, United Kingdom 4Ministery of Development, Ankara 06100, Turkey 5National Creative Research Initiative Center for Superconductivity and Department of Physics, Pohang University of Science and Technology, Pohang 790-784, Republic of Korea 6Department of Physics, Brock University, St. Catharines, Ontario L2S 3A1, Canada 7Canadian Institute for Advanced Research, 180 Dundas St. W., Toronto, Ontario M5G 1Z8, Canada Received August 6, 2013 The superconducting and magnetic properties of HoNi2B2C single crystals are investigated through transport, magnetometry and small-angle neutron scattering (SANS) measurements. In the magnetic phases that enter be- low the superconducting critical temperature, the small-angle neutron scattering data uncover networks of mag- netic surfaces. These likely originate from uncompensated moments, e.g., at domain walls pinned to crystallo- graphic grain boundaries. The field and temperature dependent behavior of SANS appears consistent with the metamagnetic transitions reported in earlier works. PACS: 72.10.Di Scattering by phonons, magnons, and other nonlocalized excitations; 72.15.Eb Electrical and thermal conduction in crystalline metals and alloys; 72.15.Jf Thermoelectric and thermomagnetic effects; 74.25.–q Properties of type I and type II superconductors; 75.30.Kz Magnetic phase boundaries (including magnetic transitions, metamagnetism, etc.). Keywords: superconductivity, magnetism, metamagnetic transitions. 1. Introduction The rare-earth nickel borocarbide compounds RNi2B2C exhibit superconductivity even when the rare-earth element R is a magnetic ion [1–5]. Due to the possibility of study- ing the interplay between superconductivity and mag- netism, these materials have remained at the forefront of condensed matter physics research for over a decade fol- lowing their discovery [6,7]. For the non-magnetic ions R = Y and Lu, the superconducting critical temperatures are = 15cT and 16 K, respectively [2,7,8]. For the magne- tic ions R = Ho, Tm or Er, Néel states enter at temperatures below cT , whereas for R = Dy superconductivity is stable only within the antiferromagnetic region [1,2,9–16]. All the rare-earth nickel borocarbides share a nominally tetrago- nal crystal structure, though orthorhombic distortions can appear due to magnetoelastic effects [1,5]. The unit cell is formed of alternating RC and Ni2B2 layers, with supercon- ductivity understood to originate in the latter [2–5,7]. In HoNi2B2C, the superconductivity appears at ~ 9cT K. Subsequently, a cascade of different magnetic structures within a narrow range of temperatures 6.0 to 5.2 K results in a near-reentrant behavior of the superconducting phase [9–11,17,18]. The interplay between magnetism and super- conductivity in HoNi2B2C has been succinctly probed by Bitter decoration measurements by Vinnikov et al. [19], © M. Ramazanoglu, M. Laver, A. Yagmurcu, E.-M. Choi, S.-I. Lee, A. Knigavko, and B.D. Gaulin, 2014 mailto:mr.mehmet.ramazanoglu@gmail.com M. Ramazanoglu, M. Laver, A. Yagmurcu, E.-M. Choi, S.-I. Lee, A. Knigavko, and B.D. Gaulin where it was demonstrated that magnetic domain boundaries strongly pin superconducting vortices, at least in the com- mensurate magnetic phase at low temperatures ( < 5.2T K). Similar pinning to magnetic domain boundaries was also observed in ErNi2B2C [19]. Intriguingly, the antiferromag- netic state for < 6T K in ErNi2B2C develops a ferromag- netic component below 2.3 K [20] raising the possibility of a subsequent spontaneous formation of superconducting vortices [20]. It would be intriguing to see if similar effects should occur at the metamagnetic transitions in HoNi2B2C. This article is the first report of a small-angle neutron scat- tering (SANS) study on this material. At zero and low ap- plied fields we find sharply increasing SANS as the sam- ples are cooled through ~ 5T K. We associate this signal to scattering from magnetic surfaces (i.e., domain walls) in the low-temperature collinear magnetic phases. This article is continued as follows: in the following section (Sec. 2) we outline the materials and methods; in the Results section (Sec. 3) we report the results of our resistivity (Sec. 3.1), magnetization (Sec. 3.2) and SANS (Sec. 3.3) measurements. A short summary and discussion is provided in the concluding section (Sec. 4). 2. Experimental details Single crystals of HoNi2B2C were grown using a slow- cooling flux method with isotropic enrichment of 11B in order to reduce the neutron absorption in our SANS experi- ments. The details can be found elsewhere [21]. Magnetiza- tion and transport measurements were performed in the physics laboratories at McMaster University using a quan- tum design magnetic properties measurement system and a quantum design physical properties measurement system, respectively. Resistance was measured by the standard four- point probe technique. The SANS experiments were carried out at the NIST Center for Neutron Research using the NG3- SANS and NG7-SANS instruments [22]. In a typical setup, 9≈ Å wavelength neutrons were used and the small-angle scattering detected with a 2D area detector placed ~ 13.7 m away from the sample. Two HoNi2B2C single crystals (8×5×1 and 5×4×1 mm) were co-aligned on an Al sample holder by x-ray Laue diffraction. The holder was mounted into a superconducting cryomagnet so that the samples’ c axes, applied field (H) and neutron beam directions were all initially coincident, with the [110] and [110] crystallogra- phic axes were aligned horizontal and vertical, respectively. The field direction H of the cryomagnet was initially aligned relative to the neutron beam using the vortex lattice in a Nb single crystal. The HoNi2B2C scattering measure- ments detailed herein were carried out with c turned away by ~ 45, so that H and the neutron beam direction were ~ 45 to c in the (110) plane. Datasets as a function of tem- perature were collected by applying the desired field at high temperatures > cT T , cooling to base temperature ( 3 K) and then measuring at selected temperatures on warming. 3. Results 3.1. Resistivity Figure 1(a) shows a plot of electrical resistivity ρ as a function of temperature at zero field. The current created by the four probe measurement lies in the ab plane of the crystal. As can be seen in this figure, the onset of super- conductivity appears at ~ 9cT K. Overall metallic behavior can also be seen for cT T> in the limited temperature range probed. In Fig. 1(b), ρ at low temperatures is shown as a function of applied field H in the two directions, 0 and ~ 45 from the crystallographic c axis, for direct compari- son with the SANS measurements. At = 2T K and H || c, the upper critical field is found at 0 2( = 2 K)cH Tµ ~ 0.7 T, in agreement with previous works [10,23]. The coherence length at = 2T K from this value is 200ξ Å. A kink at lower fields ~ 0.4 T can also be observed in this figure. We note that the slope of ( )Hρ steepens with increasing field Fig. 1. (Color online) Resistivity ρ measurements as functions of temperature T and of magnetic field H : (a) shows ( )Tρ at zero field; (b) shows ( )Hρ at = 2T and 3.5 K, with fields H applied parallel to c and also at 45 to c in the (110) plane. The arrow shows the point for 2cH (T = 2 K) of the previous study [10]. In (a) the yellow background shading highlights the superconduct- ing region. (a) (b) 0 2 4 6 8 10 12 14 16 18 20 22 T, K 0 0.3 0.6 0.9 1.2 1.5 1.8 30 20 10 0 25 20 15 10 5 0 T = 2 K, T = 3.5 K, T = 3.5 K, 206 Low Temperature Physics/Fizika Nizkikh Temperatur, 2014, v. 40, No. 2 Small-angle neutron scattering and magnetization study of HoNi2B2C through the kink, implying that the superconductivity ab- ruptly weakens. This can be associated with increased fluc- tuations arising from the lower 2( )cT H of the reentrant region. Similar kinks are observed at 0.35≈ T in the = 3.5T K datasets. For H || c, we see that 0 2( = 3.5 K)cH Tµ ~ 0.5 T in agreement with the expected form of 2( )cH T [10]. A slight decrease in 2cH is anticipated on rotation of H from c towards the tetragonal basal plane [23], and indeed a small leftwards shift of ( )Hρ in the upper critical field region may be discerned going from H || c to H applied 45 from c. In the latter, the ( )Hρ further rises into a broad maximum at fields above 2cH . This may be a consequence of the metamagnetic transitions to be discussed in Sec. 3.3; similar features in the resistivity have previously been re- ported for fields applied in the basal plane [23]. 3.2. Magnetization Figure 2 illustrates our magnetometry data. In Fig. 2(a), the zero field cooled (ZFC) and field cooled (FC) magnetic responses in a small applied field of 1 mT are plotted as a function of temperature. The reentrant superconductivity manifests itself as a reduced superconducting response in the region = 5T to 6 K. In Fig. 2(b) we show the magneti- zation at 2 K as a function of increasing field applied paral- lel to c after cooling in zero field. The overall signal is dominated by the linear paramagnetic response of a com- ponent of the ( 10 B≈ µ ) Ho3+ moments, but one can esti- mate the value of the upper critical field from the point of departure from the linear normal state behavior illustrated by the dashed line; one then obtains 0 2 ~ 0.7cHµ T in agreement with our resistivity measurements [Fig. 1(b)] and previous Hall probe results [10]. The ( )M H data in Fig. 2(b) can also be used to estimate the lower critical field value as 0 1 ~ 4cHµ mT at = 2T K, though this esti- mate does not take into account sample demagnetization or Ho3+ moment alignment effects. In Fig. 2(b) we measure a linear paramagnetic response of 1750 emu·mol–1·T–1, or 0.31 Bµ T–1 per Ho3+ ion. It is interesting to compare this with previously published val- ues. Ref. 24 reports 0.3 Bµ T–1/ion in agreement with our measurement. In contrast, a smaller value of 0.1 Bµ T–1/ion is reported in Ref. 18. It should be noted that all works report comparable M values at the metamagnetic transi- tions present for H ⊥ c; this is expected for an intensive quantity like magnetization. The possible non-intensive nature of M for H || c suggests that its origin may not be an intrinsic property of the bulk of samples. In the next section, we moot the possibility that this magnetization arises from more easily polarizable Ho3+ moments at crys- tallographic grain boundaries and dislocations. 3.3. Small-angle neutron scattering (SANS) We now turn to the main results of this manuscript. Figures 3 and 4 summaries the dependences of the small- angle neutron scattering (SANS) on temperature, applied field and scattering vector q. As a function of applied field, HoNi2B2C exhibits a series of metamagnetic transitions with magnetic structures depending on the field direction [8,10–12,23,25–27]. At low temperatures 5T  K with H applied along the [110] easy axis, the magnetic structures are constructed from ferromagnetic sheets, with each sheet being a basal plane, within which all Ho3+ moments co- align along one of the four 110〈 〉 directions [18]. The zero- field structure consists of antiferromagnetically coupled basal plane sheets, denoted by ↑↓ . At the first me- tamagnetic transition at 0.41 T at 2 K, a jump in the mag- netization signals that two thirds of the basal plane sheets align along H || [110] and only one along [110]; this is Fig. 2. (Color online) Magnetometry M as functions of tempera- ture T and of magnetic field H . (a) The temperature dependence of /M H , measured after cooling in zero field (ZFC) and field- cooling (FC) using a small applied field of 1 mT. (b) ( )M H at = 2T K. The dashed line indicates the linear paramagnetic re- sponse of a component of the Ho3+ moments at high fields. The inset in each panel shows a magnified region of the main figure. In these measurements, the magnetic field is applied parallel to the c axis. For clarity, yellow background shading has been added to highlight the superconducting region. Low Temperature Physics/Fizika Nizkikh Temperatur, 2014, v. 40, No. 2 207 M. Ramazanoglu, M. Laver, A. Yagmurcu, E.-M. Choi, S.-I. Lee, A. Knigavko, and B.D. Gaulin denoted ↑↑↓ . Subsequently this becomes the high-field ↑↑↑ phase with another magnetization jump at the second metamagnetic transition at 1.07 T at 2 K. Fields applied away from [110] in the basal plane yield a second interme- diate field phase ↑↑→ . The → indicates that the magnetic structure is non-collinear; it has a wave vector ≈(4/7 0 0) r.l.u. [26,27]. A recent torque magnetometry study [8] con- firms that this phase does not appear for H applied within 1° of [110], in support of the results of mean-field theory accounting for the crystalline electric field and Ruderman– Kittel–Kasuya–Yosida exchange interaction [28]. For fields applied along the hard c axis, there are no metamagnetic transitions over this field regime. Therefore, for our orientation of field direction 45≈  from c in the (110) plane, we anticipate two clear metamagnetic transi- tions; the first from ↑↓ to ↑↑↓ at 0.41/ cos45 = 0.58 T and the second to ↑↑↑ at 1.51 T. Figure 3 shows the SANS intensity integrated over the 2D detector (this corresponds to a q-range of 3(3 14)·10q −≤ ≤ Å–1). We see there are indeed three dif- ferent field regimes that correspond to the expected metamagnetic transitions. First, at low fields < 0.58 T and including zero field, the SANS temperature dependences share a common form, with intensity at low temperatures entering abruptly, rather like an order parameter with a transition temperature of 5≈ K. Then, at an intermediate applied field of 1.5 T, the magnitude of this order-parame- ter-like response appears somewhat increased compared to the low field regime. Finally at high fields > 1.51 T the SANS intensity rises smoothly with falling temperature, and also increases with increasing field. To understand the origin of the SANS intensity appear- ing at low temperatures, we first consider the possibility that the SANS signal at fields 2< cH arises from superconduct- ing vortices in the sample. To check for sharp Bragg reflec- tions from a well-defined superconducting vortex lattice, at selected low applied fields we also collected data as the samples were rocked through the expected Bragg angles. The field direction of the cryomagnet was initially aligned relative to the neutron beam using the vortex lattice in a Nb single crystal. No angular dependence was observed in the rocking scans on our HoNi2B2C samples, precluding a well- defined vortex lattice. At zero field, a SANS signal is ob- served even when no superconducting vortices are present (no spontaneously forming vortices are anticipated because the magnetic ground state is antiferromagnetic). Hence su- perconducting vortices, even in a disordered ensemble, can- not account for the observed SANS response. Next we turn to the possibility that temperature-induced SANS is generated by multiple Bragg scattering between slightly misoriented crystallites in the samples. This possi- bility would be completely excluded by working at neutron wavelengths λ above the Bragg cutoff max> 2dλ , where maxd is the maximum d-spacing of the Bragg diffraction planes. For HoNi2B2C, max = 10.53d Å, corresponding to the (001) magnetic Bragg reflection that appears at < 5.2T K in the commensurate Néel state. Unfortunately working at > 21λ Å is infeasible due to the lack of flux at these wave- lengths at even the best of today's neutron facilities. In- stead we used 9λ ≈ Å. Nonetheless we may defenestrate multiple Bragg scattering since this usually manifests itself as isolated spots on the small-angle detector that typically change rapidly with rotations of the sample or with neutron wavelengths. Here, in contrast, we observe a smooth SANS profile (c.f. Fig. 4) that is insensitive to small changes in angle or wavelength. Figure 4 shows the typical scattering vector = | |q q de- pendence of the SANS intensity I induced at low tempera- Fig. 3. (Color online) Integrated detector counts, summed over the range of (~ 3 14q≤ ≤ )·10–3 Å–1 as a function of temperature at various magnetic fields applied 45° from c in the (110) plane. The zero field data collected in a separate experimental setup have their own intensity scale (right). Fig. 4. Intensity I as a function of scattering vector q at low temperatures and 0 = 0.08Hµ T. A high temperature background has been subtracted. The red line shows the power-law behavior of nI q−∝ with the fitted = 4.0 0.2n ± . 208 Low Temperature Physics/Fizika Nizkikh Temperatur, 2014, v. 40, No. 2 Small-angle neutron scattering and magnetization study of HoNi2B2C tures. In this figure we plot the behavior at 0.08 T (high temperature > 9 K backgrounds have been subtracted) but a similar behavior for the induced SANS intensity I is ob- served at all fields. The data fit well to a Porod law nI q−∝ with the fitted exponent ~ 4n at all fields. At 0.08 T, for example, we find = 4.0 0.2n ± . The atomic form factor ( )AF q of the Ho3+ moments is essentially constant at low q, and the SANS profile probes directly how these moments arrange. The Porod behavior implies a network of interfaces or surfaces, with the ~ 4n signifying that these interfaces are smooth. Our experiments do not probe sufficiently small scattering vectors to access the Guinier regime of the ( )I q profile and we therefore deduce a lower bound 1300D Å for the characteristic size D of the net- work. In the high field region, we find that the anisotropy of the temperature-induced SANS is very similar to that of the crystallographic background, as characterized by the angular dependence of q measured over the 2D SANS de- tector. The same can be said for the low field region, alt- hough here there are fewer counts with which to make this evaluation. Like the temperature-induced foreground SANS intensity, the crystallographic background exhibits a Porod law 4| |q −∝ , indicative of grain boundaries and dis- location surfaces. It is likely that the temperature-induced SANS also originates at these crystal grain boundaries and dislocations. In the antiferromagnetic ↑↓ region at zero and low fields, we conjecture that the grain boundaries and dislocations serve as pinning sites for antiferromagnetic domain walls that carry a net magnetic moment. Due to the crystal electric field, at high fields the Ho3+ moments align to the [110] direction that is nearest to the applied field H; we postulate that additional small-angle scattering appears at decreasing temperatures from interfacial moments at the grain boundaries and dislocations that are susceptible to align directly along H instead of along [110]. As mooted in Sec. 3.2, these free moments at extrinsic interfaces may also account for the discrepancies between the reported values of the paramagnetic magnetization for H || c. 4. Discussion To summarize, we have performed magnetometry, transport and small-angle neutron scattering (SANS) mea- surements on HoNi2B2C single crystals. Additional SANS intensity I appearing at low temperatures is observed at all fields. In a low field region 0 < 0.58Hµ T that includes zero field, the temperature dependence of the signal is or- der-parameter-like with a transition at 5T ≈ K. At high fields 0 > 1.51Hµ T, the SANS increases continuously on cooling across the temperature range probed (from 3 K to 25 K). At low but finite fields, superconducting vortices will exist in the sample with an arrangement that is known to be rather disordered from previous local Hall probe [10] and Bitter decoration work [19]. SANS ( )I q profiles similar to those observed here were previously reported on polycrys- talline Sr0.9La0.1CuO2 and interpreted as scattering from disordered vortices [29]. Such an interpretation cannot account for our HoNi2B2C scattering data since we also observe a SANS signal at zero field. The agreement between the observed field regimes and the expected metamagnetic transitions, plus the Porod-law behavior exhibited in ( )I q , lead us to conclude that the low-temperature SANS stems from uncompensated mo- ments at crystallographic grain boundaries and disloca- tions. At low fields, these uncompensated moments are associated with domain walls in the antiferromagnetic ↑↓ phase, while at high fields they are suggested to stem from paramagnetic moments at the interfaces that align along the field direction rather than along the nearest [110] easy axis in the bulk ferromagnetic structure. We emphasize that these magnetic structures form a network of large length scales 1300D Å. Magnetic contrast over similar scales has already been observed in Bitter decoration of non-superconducting TbNi2B2C and of the normal state of ErNi2B2C [30]. In these high-resolution decoration studies, the lamellar magnetic flux structures observed were thought to be linked to crystallographic twin boundaries by magnetoelastic stresses. In HoNi2B2C magnetoelastic ef- fects lead to an orthorhombic distortion such that the unit cell length along the [110] (tetragonal) direction closest to H shrinks by ≈0.2% compared to [110] [1]. These large magnetoelastic strains would likely favour the location of magnetic domain walls at crystallographic grain bounda- ries and dislocations [31]. It would be extremely interest- ing to explore, in future work, the physics of antiferromag- netic magnetoelastic domain wall boundaries using high- resolution microscopy techniques in HoNi2B2C and in other materials. Acknowledgments We acknowledge the support of the National Institute of Standards and Technology, U.S. Department of Commerce, in providing the neutron research facilities used in this work. M.L. acknowledges support from DanScatt. 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/NLD (Gebruik deze instellingen om Adobe PDF-bestanden te maken die moeten worden gecontroleerd of die moeten voldoen aan PDF/A-1b, een ISO-standaard voor de langetermijnopslag \(archivering\) van elektronische documenten. Zie voor meer informatie over het maken van PDF/A-compatibele PDF-documenten de Acrobat-gebruikershandleiding. PDF-documenten kunnen worden geopend met Acrobat en Adobe Reader 5.0 en hoger.) /NOR 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/ENU (Use these settings to create Adobe PDF documents that are to be checked or must conform to PDF/A-1b, an ISO standard for the long-term preservation \(archival\) of electronic documents. For more information on creating PDF/A compliant PDF documents, please refer to the Acrobat User Guide. Created PDF documents can be opened with Acrobat and Adobe Reader 5.0 and later.) >> >> setdistillerparams << /HWResolution [2400 2400] /PageSize [612.000 792.000] >> setpagedevice