Ferrimagnetic spin-1/2 chain of alternating Ising and Heisenberg spins in arbitrarily oriented magnetic field

• Видавець: Інститут фізики конденсованих систем НАН України
• Дата: 2012
• Автори: Strečka, J., Hagiwara, M., Han, Y., Kida, T., Honda, Z., Ikeda, M.
• Формат: Стаття
• Мова: English
• Опубліковано: Інститут фізики конденсованих систем НАН України 2012
• Назва видання: Condensed Matter Physics
• Онлайн доступ: http://dspace.nbuv.gov.ua/handle/123456789/120296
• Цитувати: Ferrimagnetic spin-1/2 chain of alternating Ising and Heisenberg spins in arbitrarily oriented magnetic field / J. Strečka, M. Hagiwara, Y. Han, T. Kida, Z. Honda, M. Ikeda // Condensed Matter Physics. — 2012. — Т. 15, № 4. — С. 43002:1-11. — Бібліогр.: 15 назв. — англ.

The ferrimagnetic spin-1/2 chain composed of alternating Ising and Heisenberg spins in an arbitrarily oriented magnetic field is exactly solved using the spin-rotation transformation and the transfer-matrix method. It is shown that the low-temperature magnetization process depends basically on a spatial orientation of the magnetic field. A sharp stepwise magnetization curve with a marked intermediate plateau, which emerges for the magnetic field applied along the easy-axis direction of the Ising spins, becomes smoother and the intermediate plateau shrinks if the external field is tilted from the easy-axis direction. The magnetization curve of a polycrystalline system is also calculated by performing powder averaging of the derived magnetization formula. The proposed spin-chain model brings an insight into high-field magnetization data of 3d-4f bimetallic polymeric compound Dy(NO₃)(DMSO)₂Cu(opba)(DMSO)₂, which provides an interesting experimental realization of the ferrimagnetic chain composed of two different but regularly alternating spin-1/2 magnetic ions Dy³+ and Cu²+ that are reasonably approximated by the notion of Ising and Heisenberg spins, respectively.