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Low-temperature control of nanoscale molecular dynamics
A novel in situ probe of the nanoscale molecular dynamics of organic-molecule and fullerene-tube nanostructures is proposed. General and consistent results for the nonlinear-current coupling to the nanostructure excitations are presented to document a frequency-selective electrostatic control of thi...
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| Main Author: | |
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| Format: | Article |
| Language: | English |
| Published: |
Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України
2001
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| Series: | Физика низких температур |
| Subjects: | |
| Online Access: | http://dspace.nbuv.gov.ua/handle/123456789/128699 |
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| Summary: | A novel in situ probe of the nanoscale molecular dynamics of organic-molecule and fullerene-tube nanostructures is proposed. General and consistent results for the nonlinear-current coupling to the nanostructure excitations are presented to document a frequency-selective electrostatic control of this current stimulation and optimal operation as a local source of current-induced molecular excitations Ωi. The control is possible for temperatures T≪Ωi. Finally, it is explained in detail how Raman measurements of this molecular dynamics would probe the nanoscale excitations within organic and fullerene nanostructures under nonlinear transport conditions. |
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