Phonon Drag Thermopower in Quantum Wire with Parabolic Confinement Potential

The quantitative theory of phonon drag thermopower for the one-dimensional electron gas in a quantum wire with a parabolic confinement potential is developed. The temperature gradient is directed along the axis of a quantum wire. As assumed, the Fermi level is located between the zero and first leve...

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Datum:2017
Hauptverfasser: Abbasov, I.I., Hasanov, Kh.A., Huseynov, J.I.
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Veröffentlicht: Інститут металофізики ім. Г.В. Курдюмова НАН України 2017
Schriftenreihe:Металлофизика и новейшие технологии
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spelling irk-123456789-1304032018-02-13T03:03:28Z Phonon Drag Thermopower in Quantum Wire with Parabolic Confinement Potential Abbasov, I.I. Hasanov, Kh.A. Huseynov, J.I. Строение и свойства наноразмерных и мезоскопических материалов The quantitative theory of phonon drag thermopower for the one-dimensional electron gas in a quantum wire with a parabolic confinement potential is developed. The temperature gradient is directed along the axis of a quantum wire. As assumed, the Fermi level is located between the zero and first levels of a size quantization. Using the Boltzmann kinetic equation, the phonon and electronic parts of a thermoelectric power are calculated. For comparison, numerical calculations of the temperature and concentration dependences of the phonon and diffusion parts of a thermoelectric power are carried out. As shown, the phonon drag makes a main contribution in thermopower within the temperature interval 2–20 K. Разработана количественная теория термоэдс фононного увлечения для одномерного электронного газа в квантовой проволоке с параболическим ограничивающим потенциалом. Градиент температуры направлен вдоль оси квантовой проволоки. Предполагается, что уровень Ферми расположен между нулевым и первым уровнями размерного квантования. С использованием кинетического уравнения Больцмана вычислены фононная и электронная части термоэдс. Для сравнения были проведены численные расчёты температурной и концентрационной зависимостей фононной и диффузионной частей термоэдс. Показано, что фононное увлечение вносит основной вклад в термоэдс в интервале температур 2–20 К. Розроблено кількісну теорію термоерс фононного перетягання для одновимірного електронного газу в квантовому дроті з параболічним обмежувальним потенціялом. Ґрадієнт температури спрямовано уздовж осі квантового дроту. Передбачається, що рівень Фермі розташований між нульовим і першим рівнями розмірного квантування. З використанням Больцманнового кінетичного рівняння обчислено фононну й електронну частини термоерс. Для порівняння було проведено чисельні розрахунки температурної та концентраційної залежностей фононної й дифузійної частин термоерс. Показано, що фононне перетягання дає основний внесок у термоерс в інтервалі температур 2–20 К. 2017 Article Phonon Drag Thermopower in Quantum Wire with Parabolic Confinement Potential / I.I. Abbasov, Kh.A. Hasanov, J.I. Huseynov // Металлофизика и новейшие технологии. — 2017. — Т. 39, № 9. — С. 1165-1171. — Бібліогр.: 12 назв. — англ. 1024-1809 PACS: 63.20.K-, 72.15.Jf, 72.15.Nj, 72.20.Pa, 73.21.Hb, 73.63.Nm, 85.80.Fi http://dspace.nbuv.gov.ua/handle/123456789/130403 DOI: https://doi.org/10.15407/mfint.39.09.1165 en Металлофизика и новейшие технологии Інститут металофізики ім. Г.В. Курдюмова НАН України
institution Digital Library of Periodicals of National Academy of Sciences of Ukraine
collection DSpace DC
language English
topic Строение и свойства наноразмерных и мезоскопических материалов
Строение и свойства наноразмерных и мезоскопических материалов
spellingShingle Строение и свойства наноразмерных и мезоскопических материалов
Строение и свойства наноразмерных и мезоскопических материалов
Abbasov, I.I.
Hasanov, Kh.A.
Huseynov, J.I.
Phonon Drag Thermopower in Quantum Wire with Parabolic Confinement Potential
Металлофизика и новейшие технологии
description The quantitative theory of phonon drag thermopower for the one-dimensional electron gas in a quantum wire with a parabolic confinement potential is developed. The temperature gradient is directed along the axis of a quantum wire. As assumed, the Fermi level is located between the zero and first levels of a size quantization. Using the Boltzmann kinetic equation, the phonon and electronic parts of a thermoelectric power are calculated. For comparison, numerical calculations of the temperature and concentration dependences of the phonon and diffusion parts of a thermoelectric power are carried out. As shown, the phonon drag makes a main contribution in thermopower within the temperature interval 2–20 K.
format Article
author Abbasov, I.I.
Hasanov, Kh.A.
Huseynov, J.I.
author_facet Abbasov, I.I.
Hasanov, Kh.A.
Huseynov, J.I.
author_sort Abbasov, I.I.
title Phonon Drag Thermopower in Quantum Wire with Parabolic Confinement Potential
title_short Phonon Drag Thermopower in Quantum Wire with Parabolic Confinement Potential
title_full Phonon Drag Thermopower in Quantum Wire with Parabolic Confinement Potential
title_fullStr Phonon Drag Thermopower in Quantum Wire with Parabolic Confinement Potential
title_full_unstemmed Phonon Drag Thermopower in Quantum Wire with Parabolic Confinement Potential
title_sort phonon drag thermopower in quantum wire with parabolic confinement potential
publisher Інститут металофізики ім. Г.В. Курдюмова НАН України
publishDate 2017
topic_facet Строение и свойства наноразмерных и мезоскопических материалов
url http://dspace.nbuv.gov.ua/handle/123456789/130403
citation_txt Phonon Drag Thermopower in Quantum Wire with Parabolic Confinement Potential / I.I. Abbasov, Kh.A. Hasanov, J.I. Huseynov // Металлофизика и новейшие технологии. — 2017. — Т. 39, № 9. — С. 1165-1171. — Бібліогр.: 12 назв. — англ.
series Металлофизика и новейшие технологии
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AT hasanovkha phonondragthermopowerinquantumwirewithparabolicconfinementpotential
AT huseynovji phonondragthermopowerinquantumwirewithparabolicconfinementpotential
first_indexed 2025-07-09T13:29:45Z
last_indexed 2025-07-09T13:29:45Z
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fulltext СТРОЕНИЕ И СВОЙСТВА НАНОРАЗМЕРНЫХ И МЕЗОСКОПИЧЕСКИХ МАТЕРИАЛОВ PACS numbers: 63.20.K-, 72.15.Jf, 72.15.Nj, 72.20.Pa, 73.21.Hb, 73.63.Nm, 85.80.Fi Phonon Drag Thermopower in Quantum Wire with Parabolic Confinement Potential I. I. Abbasov, Kh. A. Hasanov*, and J. I. Huseynov* Azerbaijan State Oil and Industrial University, 20 Azadliq, Baku, Azerbaijan *Azerbaijan State Pedagogical University, 34 U. Hajibayov Str., Baku, Azerbaijan The quantitative theory of phonon drag thermopower for the one-dimen- sional electron gas in a quantum wire with a parabolic confinement potential is developed. The temperature gradient is directed along the axis of a quan- tum wire. As assumed, the Fermi level is located between the zero and first levels of a size quantization. Using the Boltzmann kinetic equation, the pho- non and electronic parts of a thermoelectric power are calculated. For com- parison, numerical calculations of the temperature and concentration de- pendences of the phonon and diffusion parts of a thermoelectric power are carried out. As shown, the phonon drag makes a main contribution in ther- mopower within the temperature interval 2–20 K. Key words: quantum wire, phonon drag, parabolic potential, energy spec- trum, thermoelectric effects, diffusion thermopower, phonon thermopower. Розроблено кількісну теорію термоерс фононного перетягання для одно- вимірного електронного газу в квантовому дроті з параболічним обмежу- вальним потенціялом. Ґрадієнт температури спрямовано уздовж осі кван- тового дроту. Передбачається, що рівень Фермі розташований між нульо- вим і першим рівнями розмірного квантування. З використанням Больц- Corresponding author: Ibrahim I. Abbasov E-mail: ibrahimabbasov179@gmail.com Please cite this article as: I. I. Abbasov, Kh. A. Hasanov, and J. I. Huseynov, Phonon Drag Thermopower in Quantum Wire with Parabolic Confinement Potential, Metallofiz. Noveishie Tekhnol., 39, No. 9: 1165–1171 (2017), DOI: 10.15407/mfint.39.09.1165. Ìåòàëëîôèç. íîâåéøèå òåõíîë. / Metallofiz. Noveishie Tekhnol. 2017, т. 39, № 9, сс. 1165–1171 / DOI: 10.15407/mfint.39.09.1165 Îттиски доступнû непосредственно от издателя Фотокопирование разрешено только в соответствии с лицензией  2017 ÈÌФ (Èнститут металлофизики им. Ã. Â. Êурдюмова ÍÀÍ Óкраинû) Íапечатано в Óкраине. 1165 https://doi.org/10.15407/mfint.39.09.1165 https://doi.org/10.15407/mfint.39.09.1165 1166 I. I. ABBASOV, Kh. A. HASANOV, and J. I. HUSEYNOV маннового кінетичного рівняння обчислено фононну й електронну части- ни термоерс. Для порівняння було проведено чисельні розрахунки темпе- ратурної та концентраційної залежностей фононної й дифузійної частин термоерс. Показано, що фононне перетягання дає основний внесок у тер- моерс в інтервалі температур 2–20 Ê. Ключові слова: квантовий дріт, фононне перетягання, параболічний по- тенціял, енергетичний спектер, термоелектричні ефекти, термодинаміка дифузії, теплова енергія фононів. Разработана количественная теория термоэдс фононного увлечения для одномерного электронного газа в квантовой проволоке с параболическим ограничивающим потенциалом. Ãрадиент температурû направлен вдоль оси квантовой проволоки. Предполагается, что уровень Ферми располо- жен между нулевûм и первûм уровнями размерного квантования. С ис- пользованием кинетического уравнения Больцмана вûчисленû фононная и электронная части термоэдс. Для сравнения бûли проведенû численнûе расчётû температурной и концентрационной зависимостей фононной и диффузионной частей термоэдс. Показано, что фононное увлечение вно- сит основной вклад в термоэдс в интервале температур 2–20 Ê. Ключевые слова: квантовая проволока, фононное увлечение, параболиче- ский потенциал, энергетический спектр, термоэлектрические эффектû, термодинамика диффузии, тепловая энергия фононов. (Received August 5, 2017) 1. INTRODUCTION In recent years, a significant number of papers were devoted to exper- imental and theoretical investigations of thermopower in low-dimen- sional systems have appeared [1–3]. The limited motion of electrons in such systems leads to the fact that the kinetic phenomena in them sharply differ from the electronic transport phenomena in bulk sam- ples. Quantum-size structures produced in recent decades have attracted attention also because of possibility of their using in thermoelements with high thermoelectric efficiency. Studies in this field have shown that it is possible to increase the thermoelectric efficiency two or three times by preparing thermoelectric structures with quantum wells [4]. In this paper, we discuss the temperature dependence of the thermo- electric power of a degenerate electron gas in a quantum wire with a parabolic confinement potential in the low-temperature range of 1–20 K, where the phonon drag effect plays an important role. Due to con- finement, the energy spectrum and the wave function of the electron essentially change. A numerical calculation of the thermoelectric pow- er is carried out for the quantum wire GaAs/AlxGa1−xAs with a parabol- ic well. PHONON DRAG THERMOPOWER IN QUANTUM WIRE 1167 2. THEORETICAL DETAILS To obtain an analytical expression for various physical quantities, it is advisable to use a specific model of a potential quantum well. For this purpose, a parabolic potential of the U(x) = 2 2 0 /2m xω form that re- stricts the motion of electrons in the direction of the x-axis, is often used, where m is the effective mass of the conduction electrons, and ω0 is the parabolic potential parameter. In a present work, the phonon drag thermopower for one- dimensional degenerated electron gas in quantum wire (QW) with a parabolic confinement potential is calculated. Spectrum and wave functions of the system ground state under consideration are given in [5]: 2 2 0,0, , 2k k m ε = + ω   (1) 2 0,0, 2 1 exp , 2k r ikz RR L   ψ = − +  p   (2) where ω is a parabolic potential parameter, ( )R m= ω is an oscilla- tory length, L is a QW length. It is supposed that the Fermi level ζ is localized between zero level and first one of dimensional quantization. Moreover, necessary condition for the existence of a strong degenera- tion is 0k T << ζ − ω < ω  , where T is temperature, k0 is the Boltz- mann constant. Earlier, the phonon drag thermopower for one- dimensional electron gas was calculated in the framework of the rec- tangular confinement potential model [6]. There are both theoretical calculations [3, 7] and experimental results [8, 9] confirming the dom- inating contribution of phonon drag thermopower in the total ther- mopower for a two-dimensional electron gas. 3. RESULTS Thermopower α associated with a temperature gradient along the QW axis consists of diffusion αe and phonon αph parts: α = αe + αph = βe/σ + + βph/σ [10]. Here, σ is the specific conductivity of the QW along the wire axis: 2 ( ) .Fn e k m τ σ = (3) As evaluations show, at low temperatures, the dominating scatter- ing mechanism for strongly degenerated electron gas is scattering on ionized impurities and scattering on a sample boundary for phonons. 1168 I. I. ABBASOV, Kh. A. HASANOV, and J. I. HUSEYNOV The expression for the electron-momentum relaxation time has the form: ( ) ( ) ( ) 23 2 2 2 2 2 21 ( ) ( ) exp 0, 2 F F F F F I k Z e k k R k R k N m −   τ = ε Γ χ   ; (4) for phonons, / ,ph L sτ = where s is the sound velocity in the wire. The electron concentration n and the Fermi wave number kF are re- lated by the following expression: 2 2 2 ( ) ,Fn k m= = ζ − ω p p   (5) 2 2 2 2 2 2 2 ( ) 1 exp(2 ) (0,2 ),F F F F m e k R k R k k ε = + Γ p χ (6) where ( )Fkε is the dielectric function, χ is the static dielectric con- stant, Γ(0, õ) is the incomplete gamma function, 2 2 0 1 ( ) , 3e k T eT p ∂σ β = − ∂ζ (7) 0 ,ph ph k A e β = − σ (8) ( ) 2 2 2 2 2 2 2 2 2 00 2 2 2 4 (1 (1 )) exp( 2 ) ( ) (exp( 1 ) exp( 1 )) , F ph F F m e L sk A a x R k x k T k b x b x xdx ∞ − β = + + − × p ρ ε × + − − + ∫  (9) where the following notations are introduced: 12 ,Fk E a e = β 0 .Fs k b k T =  (10) Here. e is the elementary charge, E1 is the deformation-potential con- stant, and β is the parameter characterizing the piezo acoustic poten- tial. The contributions from electron interactions with acoustic phonons in the phonon drag thermopower are taken into account in [9] by means of the deformational potential E1 and the piezo-acoustic one 140.8 /eβ = χ [11]. 4. DISCUSSION Numerical calculations are performed for the GaAs/AlxGa1−xAs QW PHONON DRAG THERMOPOWER IN QUANTUM WIRE 1169 with the following GaAs parameter values: mass of electrons m = = 0.067 m0, where m0 is the free-electron mass, the crystal mass density ρ = 3.3⋅104 kg/m3, s = 5⋅105 m/s, E1 = 7.4 eV, e14 = 0.16 C/m3, the QW length L = 3⋅10−4 m, the linear density of electrons n = 1.6⋅108 m −1, ω = = 7⋅1013 s −1. The calculated temperature dependence of the phonon drag ther- mopower (a solid line) is shown in Fig. 1. For comparison, the tempera- ture-dependent thermopower diffusion component (a dotted line) is also given. The parabolic potential parameter for GaAs/AlxGa1−x As is inversely proportional to the wire thickness ω = 14.6 eV/d(Å) [12]. Our choice corresponds to thicknesses of about 100 Å. The diffusion thermopower component value is larger than the pho- non one in the temperature interval 1–20 K. The phonon drag strongly Fig. 2. Concentration dependences of the phonon drag thermopower (solid line) and the diffusion thermopower (dotted line). Fig. 1. Temperature dependences of the phonon drag thermopower (solid line) and the diffusion thermopower (dotted line). 1170 I. I. ABBASOV, Kh. A. HASANOV, and J. I. HUSEYNOV grows with temperature increasing, exceeding the diffusion ther- mopower by one order. The concentration dependences of the phonon drag thermopower (a solid line) and the diffusion thermopower (a dotted line) are shown in Fig. 2. The diffusion component of the thermopower is approximately inversely proportional to the concentration and phonon component is inversely proportional to the concentration squared. Kubakaddi’s expression for the phonon drag thermopower for the QW model with a rectangular potential [6] differs from our expression, but both qualitative results are similar. 5. CONCLUSION The theoretical results obtained are applied to the analysis of a ther- mopower with phonon drag of a one-dimensional degenerate electron gas in a quantum wire with a parabolic confinement potential. For comparison, the temperature dependence of the diffusion component of the thermoelectric power is also given. Numerical calculations are given for the QW GaAs/AlxGa1−xAs. In the temperature range 1–2 K, the diffusion thermoelectric power exceeds the phonon one. With tem- perature increasing, the phonon thermoelectric power increases sharp- ly, exceeding the diffusion one by an order of magnitude. The diffu- sion component of the thermoelectric power is approximately inversely proportional to the concentration, and the phonon component is in- versely proportional to the concentration squared. In the temperature range 2–20 K, the main contribution to the thermoelectric power is given by the phonon drag. REFERENCES 1. M.-T. Rieder, T. Micklitz, A. Levchenko, and K. A. Matveev, Phys. Rev. B, 90: 165405 (2014). 2. J. Mao, Z. Liu, and Z. Ren, NPJ Quantum Materials, 1, Article number: 16028 (2016). 3. Kh. A. Hasanov, J. I. Huseynov, V. V. Dadashova, and F. F. Aliyev, Semiconductors, 50, Iss. 3: 295 (2016). 4. L. D. Hicks and M. S. Dresselhaus, Phys. Rev. B, 47: 12727 (1993). 5. V. M. Galitskiy, B. M. Karnakov, and V. I. Kogan, Zadachi po Kvantovoy Mekhanike [Problems in Quantum Mechanics] (Moscow: Nauka: 1992) (in Russian). 6. S. S. Kubakaddi and P. N. Butcher, J. Phys.: Condens. Matter, 1: 3939 (1989). 7. S. K. Lyo, Phys. Rev. B, 38: 6345 (1988). 8. R. Fletcher, J. C.Maan, and G. Weimann, Phys. Rev. B, 32: 8477 (1985). 9. R. Fletcher, J. J. Harris, C. T.Foxon, M. Tsaousidou, and P. N. Butcher, Phys. Rev. B, 50: 14991 (1994). 10. B. M. 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Sokovich, Fizika Tverdogo Tela, 42, No. 9: 1695 (2000) (in Russian). https://doi.org/10.1142/1926 << /ASCII85EncodePages false /AllowTransparency false /AutoPositionEPSFiles true /AutoRotatePages /None /Binding /Left /CalGrayProfile (Dot Gain 20%) /CalRGBProfile (sRGB IEC61966-2.1) /CalCMYKProfile (U.S. Web Coated \050SWOP\051 v2) /sRGBProfile (sRGB IEC61966-2.1) /CannotEmbedFontPolicy /Error /CompatibilityLevel 1.4 /CompressObjects /Tags /CompressPages true /ConvertImagesToIndexed true /PassThroughJPEGImages true /CreateJobTicket false /DefaultRenderingIntent /Default /DetectBlends true /DetectCurves 0.0000 /ColorConversionStrategy /CMYK /DoThumbnails false /EmbedAllFonts true /EmbedOpenType false /ParseICCProfilesInComments true /EmbedJobOptions true /DSCReportingLevel 0 /EmitDSCWarnings false /EndPage -1 /ImageMemory 1048576 /LockDistillerParams false /MaxSubsetPct 100 /Optimize true /OPM 1 /ParseDSCComments true /ParseDSCCommentsForDocInfo true /PreserveCopyPage true 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