Experimental cross-section evaluation data for ⁷Be photoproduction by ¹²C, ¹⁴N, ¹⁶O nuclei in the energy range between 40…90 MeV

The ⁷Be isotope produced in the upper atmosphere under the action of cosmic radiation is an important factor in population radiation load. A correct determination of the radiation dose coming from this isotope calls for consideration of the photonuclear mechanism of ⁷Be production by the nuclei of o...

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Published in:Вопросы атомной науки и техники
Date:2013
Main Authors: Dovbnya, A.N., Deyev, O.S., Kushnir, V.A., Malyshevsky, V.S., Malykhina, T.V., Mitrochenko, V.V., Perezhogin, S.A., Torgovkin, A.V., Fomin, G.V., Shramenko, B.I.
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Language:English
Published: Національний науковий центр «Харківський фізико-технічний інститут» НАН України 2013
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Online Access:https://nasplib.isofts.kiev.ua/handle/123456789/112085
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Journal Title:Digital Library of Periodicals of National Academy of Sciences of Ukraine
Cite this:Experimental cross-section evaluation data for ⁷Be photoproduction by ¹²C, ¹⁴N, ¹⁶O nuclei in the energy range between 40…90 MeV / A.N. Dovbnya1, O.S. Deyev, V.A. Kushnir, V.S. Malyshevsky, T.V. Malykhina, V.V. Mitrochenko, S.A. Perezhogin, A.V. Torgovkin, G.V. Fomin, B.I. Shramenko1 // Вопросы атомной науки и техники. — 2013. — № 6. — С. 192-195. — Бібліогр.: 7 назв. — англ.

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Digital Library of Periodicals of National Academy of Sciences of Ukraine
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author Dovbnya, A.N.
Deyev, O.S.
Kushnir, V.A.
Malyshevsky, V.S.
Malykhina, T.V.
Mitrochenko, V.V.
Perezhogin, S.A.
Torgovkin, A.V.
Fomin, G.V.
Shramenko, B.I.
author_facet Dovbnya, A.N.
Deyev, O.S.
Kushnir, V.A.
Malyshevsky, V.S.
Malykhina, T.V.
Mitrochenko, V.V.
Perezhogin, S.A.
Torgovkin, A.V.
Fomin, G.V.
Shramenko, B.I.
citation_txt Experimental cross-section evaluation data for ⁷Be photoproduction by ¹²C, ¹⁴N, ¹⁶O nuclei in the energy range between 40…90 MeV / A.N. Dovbnya1, O.S. Deyev, V.A. Kushnir, V.S. Malyshevsky, T.V. Malykhina, V.V. Mitrochenko, S.A. Perezhogin, A.V. Torgovkin, G.V. Fomin, B.I. Shramenko1 // Вопросы атомной науки и техники. — 2013. — № 6. — С. 192-195. — Бібліогр.: 7 назв. — англ.
collection DSpace DC
container_title Вопросы атомной науки и техники
description The ⁷Be isotope produced in the upper atmosphere under the action of cosmic radiation is an important factor in population radiation load. A correct determination of the radiation dose coming from this isotope calls for consideration of the photonuclear mechanism of ⁷Be production by the nuclei of oxygen and nitrogen. The paper gives the experimental yields from A(γ, X)⁷Be nuclear reactions in the bremsstrahlung beam versus the end-point energies of electrons (from 40 to 90 MeV). The mathematical model approach with the GEANT4 class library was used to calculate the spectra of bremsstrahlung incident on the targets. Based on the experimental results, we have calculated the A(γ, X)⁷Be reaction cross-sections for oxygen, nitrogen and carbon. Calculated values of photonuclear reaction cross-sections for ⁷Be production by ¹²C, ¹⁴N, ¹⁶O nuclei were obtained with the use of the TALYS package. Agreement between experimental and calculated results only for ¹²C and ¹⁴N is shown. Ізотоп ⁷Be, що утворюється у верхніх шарах атмосфери під впливом космічного випромінювання, є важливим чинником радіаційного навантаження на людину. Для правильного визначення дози опромінення від цього ізотопу потрібно ураховувати фотоядерний механізм утворення ⁷Be на ядрах кисню та азоту. Наведено експериментальні залежності виходів ядерних реакцій А(γ, Х) Ве⁷ на пучку гальмівного випромінювання для наступних граничних енергій електронів: 40, 50, 60, 70, 80, 90 МеВ. Методом математичного моделювання з використанням GEANT4 розраховані спектри гальмівного випромінювання, що падає на мішені, за результатами експерименту були обчислені перерізи реакцій А(γ, Х) ⁷Ве на кисні, азоті і вуглеці. За допомогою пакету TALYS отримані розрахункові залежності перерізів фотоядерних реакцій утворення 7Ве на ядрах ¹²C, ¹⁴N, ¹⁶O. Показано частково задовільне узгодження експериментальних та розрахункових результатів. Изотоп ⁷Ве, образующийся в верхних слоях атмосферы под действием космического излучения, является важным фактором радиационной нагрузки на человека. Для правильного определения дозы облучения от этого изотопа необходим учет фотоядерного механизма образования ⁷Ве на ядрах кислорода и азота. Приведены экспериментальные зависимости выходов ядерных реакций А(γ, Х) ⁷Ве на пучке тормозного излучения для следующих граничных энергий электронов: 40, 50, 60, 70, 80, 90 МэВ. Методом математического моделирования с использованием библиотеки классов GEANT4 рассчитаны спектры тормозного излучения, падающего на мишени, по результатам эксперимента были вычислены сечения реакций А(γ, Х) ⁷Ве на кислороде, азоте и углероде. При помощи пакета TALYS получены расчетные зависимости сечения фотоядерных реакций образования ⁷Ве на ядрах ¹²C, ¹⁴N, ¹⁶O. Показано частично удовлетворительное согласие экспериментальных и расчетных результатов.
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fulltext ISSN 1562-6016. ВАНТ. 2013. №6(88) 192 EXPERIMENTAL CROSS-SECTION EVALUATION DATA FOR 7Be PHOTOPRODUCTION BY 12C, 14N, 16O NUCLEI IN THE ENERGY RANGE BETWEEN 40…90 MeV A.N. Dovbnya1, O.S. Deyev1, V.A. Kushnir1, V.S. Malyshevsky2, T.V. Malykhina3, V.V. Mitrochenko1, S.A. Perezhogin1, A.V. Torgovkin1, G.V. Fomin2, B.I. Shramenko1 1National Science Center “Kharkov Institute of Physics and Technology”, Kharkov, Ukraine; 2Southern Federal University, Rostov-on-Don; 3V.N. Karazin Kharkov National University, Kharkov, Ukraine E-mail: bshram@kipt.kharkov.ua The 7Be isotope produced in the upper atmosphere under the action of cosmic radiation is an important factor in population radiation load. A correct determination of the radiation dose coming from this isotope calls for considera- tion of the photonuclear mechanism of 7Be production by the nuclei of oxygen and nitrogen. The paper gives the experimental yields from A(γ, X)7Be nuclear reactions in the bremsstrahlung beam versus the end-point energies of electrons (from 40 to 90 MeV). The mathematical model approach with the GEANT4 class library was used to cal- culate the spectra of bremsstrahlung incident on the targets. Based on the experimental results, we have calculated the A(γ, X)7Be reaction cross-sections for oxygen, nitrogen and carbon. Calculated values of photonuclear reaction cross-sections for 7Be production by 12C, 14N, 16O nuclei were obtained with the use of the TALYS package. Agreement between experimental and calculated results only for 12C and 14N is shown. PACS: 07.85.-m, 87.53.-j INTRODUCTION At present, the monitoring of radionuclides content in the air-ground interface suggests the conclusion that the radioactivity of ground air is essentially contributed by a short-lived isotope 7Be of cosmic origin. The 7Be isotope presents interest not only from the standpoint of its radioactive effect on biological systems, but also because it can serve as an indicator of the build-up of air-supplied pollutants by natural environments [1]. The last-mentioned property may be conveniently used for estimating a possible atmospheric pollution and air ex- change in the environment. Therefore, the investigation into the mechanisms and regularities of the processes of 7Be generation, transport and migration in the ecosphere objects and at their interfaces appears rather urgent. It is considered that the main reactions leading to beryllium isotope generation in the terrestrial atmosphere take place at interaction of cosmic rays with nitrogen and oxygen nuclei [2], which are the principal constituents of the atmospheric air: 7N14(p, X) 4Be7, 8O16(p, X) 4Be7, 7N14(n, X) 4Be7 and 8O16(n, X) 4Be7. Another possible mechanism of 7Be generation in the upper atmosphere may lie in photonuclear reactions. The literature comprises scarce data on the reactions of multiparticle photodisintegration of nuclei. For ex- ample, details for the 6C12(γ, nα) 4Be7 reaction cross- section can be found in ref. [3], whereas no data on the reactions 7N14(n, X) 4Be7 and 8O16(n, X) 4Be7 are avail- able in the literature. Since the mentioned nuclei are the basic components of atmospheric air, it is just these re- actions are of particular interest for the analysis of the photonuclear mechanism of 7Be production in the at- mosphere. 1. EXPERIMENT To determine the 7Be photoproduction cross-section in the А(γ, X)4Be7 reaction, experiments were made to expose a set of targets comprising oxygen, nitrogen and carbon to bremsstrahlung at the electron linear accelera- tor LUE-40 [7]. The energy of accelerated electrons was varied with a 10 MeV step from 40 to 90 MeV, the cur- rent being about 4.2 μA. In total, six target irradiation sessions were carried out. The time of exposure was varied in order to attain the same dose (charge) in all the sessions, namely, 12.5 μA·h. The design of the target assembly is presented in Fig. 1. The target beam is incident on the converter consist- ing of 4 tantalum plates, 4 mm in total thickness, with air gaps in-between to improve heat removal. e - Converter 1 2 3 4 Fig. 1. Target assembly for exposure at the accelerator Immediately behind the converter there were the tar- gets comprising the nuclei under study: 1-16О, 2-12С, 3-14N, and the molybdenum target 4-Mo used as a check test piece. To ensure thermal resistance in the process of expo- sure, the following materials were used as targets: co- rundum (Al2O3), high-purity graphite (C) and a highly compressed aluminum nitride powder (AlN). The de- sign of the target assembly has made it possible to dis- pense with water cooling, using instead air blast cool- ing, which provided prompt access to the targets before and after their irradiation. The activity of each target after its irradiation was measured using the spectrometer complex CANBERRA InSpector 2000 with an energy resolution of 1.74 keV in mailto:bshram@kipt.kharkov.ua ISSN 1562-6016. ВАНТ. 2013. №6(88) 193 the 1332 keV line and a relative activity measurement error no more than 6%. 2. CALCULATION AND SIMULATION RESULTS To calculate the cross-section for isotope 7Be photo- production, it is necessary to know the flux density of bremsstrahlung photons at the site of target location. For this purpose, a computational modeling was performed to describe the passage of primary electrons of energies ranging from 40 to 90 MeV with a 10 MeV step through the target assembly model having the parameters, which correspond to the parameters of the experimental target assembly. For computation purposes, a computer pro- gram “KIPT” has been developed. The program is writ- ten in the C++ language in OC Linux with the use of the Geant 4 class library, version 9.4. The electron beam diameter was set to be 10 mm, the electron beam distri- bution was determined using class G4UniformRand. The parameters of the target assembly model were described with the use of the methods of class G4DetectorConstruction (defined were the component parts of the target assembly model, in particular, the geometrical parameters and materials, visualization pa- rameters, etc.). In the description of visualization op- tions we have put to be visible only tantalum plates (turquoise blue), alumina (red), carbon (orange), and aluminum nitride (violet) (Fig. 2). Fig. 2. OpenGL-visualization of the facility fragment (theta=85°, phi=178°) For the description of physical processes, the low- energy electromagnetic process model “Livermore” was used. In modeling, the gamma-quanta that have passed through the Al2O3, C and AlN targets were traced. Fig. 3 shows typical computed energy spectra of gamma-quanta of energies between 18 and 40 MeV, which have passed through different targets. The prima- ry electron energy was Ee = 40 MeV, the number of primary electrons amounted to Nevents= 6.24⋅106. Similar spectra have been computed for energies 50, 60, 70, 80 and 90 MeV. Later on, these results were used to calcu- late cross-sections for 7Be photoproduction by the nu- clei under study using the “photon-difference” method. 18 20 22 24 26 28 30 32 34 36 38 40 0,0 2,0x104 4,0x104 6,0x104 8,0x104 1,0x105 1,2x105 Air 4mm (before Al2O3) Al2O3 C AlN Eγ, MeV Primary electrons, Ee=40 MeV, Nevents = 6.24*106 N g am m a Fig. 3. Energy spectra of bremsstrahlung gamma- quanta for Ee-= 40 MeV 3. RESULTS AND DISCUSSION On the basis of target activity measurements, the 7Be yield curves were plotted as functions of electron beam energy for all the targets under study (Figs. 4-7). 40 50 60 70 80 90 500 750 1000 1250 1500 1750 Ac tiv ity , k Bq Ee, MeV Mo Fig. 4. 99Mo activity (yield) in the check test target versus electron energy The simulated bremsstrahlung spectrum was con- volved with the known experimental cross-section for the 100Мо(γ, n) 99Mo reaction [6] and with the cross- section, obtained using the program TALYS-1.4, with the result that the calculated values of 99Mo activity in the check test target were obtained. The difference be- tween the measured 99Mo activity value (see Fig. 4) and the simulated result does not exceed 5…8 %. This con- firms the adequacy of the technique applied. 40 50 60 70 80 90 25 50 75 100 125 150 175 A ct iv ity 7 B e, k Bq Ee, MeV C Fig. 5. 7Be activity in 12C-target vs electron energy ISSN 1562-6016. ВАНТ. 2013. №6(88) 194 40 50 60 70 80 90 0 3 6 9 12 A ct iv ity 7 B e, k B q Ee, MeV N Fig. 6. 7Be activity in 14N-target vs electron energy 40 50 60 70 80 90 0 1 2 3 4 5 6 7 8 9 10 A ct iv ity 7 B e, k B q Ee, MeV O Fig. 7. 7Be activity in 16O-target vs electron energy The experimental data on 7Be activity in the C, N, O targets were corrected for the 99Mo yield. In this way the errors due to nonidentical conditions of different irradia- tion sessions were reduced in the determination of the cross-section for 7Be production. The averaged cross-sections for the 7Be isotope pro- duction from different targets were calculated by the following formula: ( ) 24 0 0 101 −⋅− ⋅−⋅⋅⋅Φ ⋅ = îáët AV m eNm AA λσ , (1) where σ − is the cross-section (b); Ф0 − is the γ-quantum flux density (1/cm2·s); А0 − is the target activity (Bq); Аm − is the atomic weight of the target isotope; NAv − is the Avogadro number; m − is the isotopic mass in the target (g); λ − is the decay constant of 7Be. The density of nuclear-active bremsstrahlung gam- ma-quantum flux was calculated for each energy inter- val (10 MeV) by subtracting simulated brems-strahlung spectras for nearby end-point energy value of electron. The activity difference for boundary energies of each interval was calculated in a similar way. The resulting reaction cross-sections σ(E) for 7Be production present the values averaged over the 10 MeV interval. It should be noted that the application of the classi- cal technique of spectrum subtraction, i.e., the photon- difference method, permits one to obtain a more mono- chromatic spectrum as compared to the initial brems- strahlung photon spectrum. A substantial thickness of the tantalum converter brings up problems concerning the low-energy part of the difference spectrum, namely, it ceases to be zero and introduces a significant error into the cross-section evaluation. So, the determination of the reaction cross-section σ(E) from the experimental yield (target activity) actually provides information on the evaluative cross-section σо(Е)= ∫ dEEEEF i )()(' σ , (2) that essentially differs from the sought-for cross-section σ(E) by the value, by which the difference spectrum F′(Ei, E) differs from the Schiff residue in the limit of the δ-function [4]. It is obvious that to estimate the validity of the ob- tained results, it is necessary to have an independent method of evaluating cross-sections for the reactions under study. The program TALYS [5] has been used to plot 7Be production cross-sections as functions of the photon energy for carbon, nitrogen and oxygen nuclear targets (solid curves in Figs. 8-10). 25 30 35 40 45 50 55 60 65 70 75 80 85 90 0,00 0,05 0,10 0,15 0,20 0,25 0,30 cr os s- se ct io n. m b Energy ( Eγ) , MeV target: 12 C 7Be production Fig. 8. Cross-section for 7Ве production by 12C nuclei 30 35 40 45 50 55 60 65 70 75 80 85 90 0,00 0,01 0,02 0,03 0,04 0,05 0,06 cr os s- se cti on . m b Energy ( Eγ) , MeV target: 14 N 7Be production Fig. 9. Cross-section for 7Ве production by 14N nuclei 30 35 40 45 50 55 60 65 70 75 80 85 90 0,000 0,005 0,010 0,015 0,020 0,025 0,030 0,035 cr os s- se ct io n. m b Energy ( Eγ) , MeV target: 16O 7Be production Fig. 10. Cross-section for 7Ве production by 16O nuclei The points in the plots show the calculated values of the evaluative cross-section σ(E). For the 12C nuclei the cross-section σ(E) for the 7Be ISSN 1562-6016. ВАНТ. 2013. №6(88) 195 production reactions is in satisfactory agreement with the cross-section calculated by the TALYS program and with data [3]. However, for the 14N nuclei (below 60 MeV) and 16O nuclei (in the whole energy range), it appeared impossible to attain a satisfactory agreement even with the use of the yield-curve smoothing proce- dure. Ishkhanov et al. have described [5] the technique of reconstructing the Ta photodisintegration reaction yield with the use of the cross-sections calculated by the TALYS code. In our case with the use of this technique for reconstructing the yields from the reactions 7N14(γ, X) 4Be7, 8O16(γ, X) 4Be7, the reaction yields (and hence, the TALYS cross-section) turn out to be essentially lower than the experimental reaction yields (σ(E) val- ues, accordingly). The reasons for this discrepancy may be attributed to both the experimental and calculation procedure errors, namely, no consideration was given to the cluster structure of the emitted reaction products and to TALYS working peculiarities at escape of a great amount of nucleons [5]. This work was supported by the National Academy of Sciences of Ukraine and by Russian Foundation for Basic Research Grants № 02-08-12(У) 35-2012. REFERENCES 1. M.V. Bezuglov, V.S. Malyshevsky, T.V. Malykhina, G.V. Fomin, A.V. Torgovkin, B.I. Shramenko. Photonuclear channel of cosmogenic 7Be production in the terrestrial atmosphere // Yadernaya Fizika. 2012, v. 75, № 4, p. 427-43 (in Russian). 2. M.V. Bezuglov, V.S. Malyshevsky, G.V. Fomin. T.V. Malykhina, A.V. Torgovkin, B.I. Shramenko. Photonuclear production of cosmogenic beryllium-7 in the terrestrial atmosphere // Physical Review C 86 024609(2012). 3. V.V. Kirichenko, A.F. Khodyachikh, P.I. Vatset, et al. // Yadernaya Fizika. 1979, v. 29, p. 572 (in Rus- sian). 4. V.V. Varlamov, B.S. Ishkhanov, I.M. Kapitonov. Photonuclear reactions. Present status of experi- mental data // MGU publ. Moscow. 2008, 304 p. 5. B.S. Ishkhanov, V.N. Orlin, S.Yu. Troshchiyev. Tantalum photodisintegration // Yadernaya Fizika. 2012, v. 75, № 3, p. 283-292 (in Russian). 6. H. Naik, S.V. Suryanarayana, K.C. Jagadeesan, et al. An alternative route for the preparation of the medi- cal isotope 99Mo from the 238U(γ, f) and 100Mo(γ, n) reactions // Journal of Radioanalytical and Nuclear Chemistry. 2013, v. 295, iss. 1, p. 807-816. 7. A.N. Dovbnya, M.I. Ayzatskiy, V.A. Kushnir, et al. Beam parameters of an S-band electron linac with beam energy of 30…100 MeV // Problems of Atom- ic Science and Technology. Ser. “Nuclear Physics Investigations”. 2006, № 2, p. 11-13. Article received 16.10.2013 ЭКСПЕРИМЕНТАЛЬНЫЕ РЕЗУЛЬТАТЫ ОПРЕДЕЛЕНИЯ СЕЧЕНИЯ ФОТОРОЖДЕНИЯ 7Ве НА ЯДРАХ 12С, 14N,16O В ДИАПАЗОНЕ ЭНЕРГИЙ 40…90 МэВ А.Н. Довбня, А.С. Деев, В.А. Кушнир, В.С. Малышевский, Т.В. Малыхина, В.В. Митроченко, С.А. Пережогин, А.В. Торговкин, Г.В. Фомин, Б.И. Шраменко Изотоп 7Ве, образующийся в верхних слоях атмосферы под действием космического излучения, является важным фактором радиационной нагрузки на человека. Для правильного определения дозы облучения от этого изотопа необходим учет фотоядерного механизма образования 7Ве на ядрах кислорода и азота. Приве- дены экспериментальные зависимости выходов ядерных реакций А(γ, Х) 7Ве на пучке тормозного излучения для следующих граничных энергий электронов: 40, 50, 60, 70, 80, 90 МэВ. Методом математического моде- лирования с использованием библиотеки классов GEANT4 рассчитаны спектры тормозного излучения, па- дающего на мишени, по результатам эксперимента были вычислены сечения реакций А(γ, Х) 7Ве на кисло- роде, азоте и углероде. При помощи пакета TALYS получены расчетные зависимости сечения фотоядерных реакций образования 7Ве на ядрах 12С, 14N, 16O. Показано частично удовлетворительное согласие экспери- ментальных и расчетных результатов. ЕКСПЕРИМЕНТАЛЬНІ РЕЗУЛЬТАТИ ВИЗНАЧЕННЯ ПЕРЕРІЗІВ ФОТОУТВОРЕННЯ 7Вe НА ЯДРАХ 12С, 14N, 16O В ДІАПАЗОНІ ЕНЕРГІЙ 40…90 МeВ А.М. Довбня, О.С. Дeєв, В.А. Кушнір, В.С. Малишевський, Т.В. Малихіна, В.В. Митроченко, С.О. Пережогін, О.В. Торговкін, Г.В. Фомін, Б.І. Шраменко Ізотоп 7Ве, що утворюється у верхніх шарах атмосфери під впливом космічного випромінювання, є важ- ливим чинником радіаційного навантаження на людину. Для правильного визначення дози опромінення від цього ізотопу потрібно ураховувати фотоядерний механізм утворення 7Ве на ядрах кисню та азоту. Наведено експериментальні залежності виходів ядерних реакцій А(γ, Х) Ве7 на пучку гальмівного випромінювання для наступних граничних енергій електронів: 40, 50, 60, 70, 80, 90 МеВ. Методом математичного моделювання з використанням GEANT4 розраховані спектри гальмівного випромінювання, що падає на мішені, за результатами експерименту були обчислені перерізи реакцій А(γ, Х) 7Ве на кисні, азоті і вуглеці. За допомогою пакету TALYS отримані розрахункові залежності перерізів фотоядерних реак- цій утворення 7Ве на ядрах 12С, 14N, 16O. Показано частково задовільне узгодження експериментальних та розрахункових результатів. http://link.springer.com/search?facet-author=%22H.+Naik%22 http://link.springer.com/search?facet-author=%22S.+V.+Suryanarayana%22 http://link.springer.com/search?facet-author=%22K.+C.+Jagadeesan%22 http://link.springer.com/journal/10967 http://link.springer.com/journal/10967 http://link.springer.com/journal/10967/295/1/page/1
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institution Digital Library of Periodicals of National Academy of Sciences of Ukraine
issn 1562-6016
language English
last_indexed 2025-12-07T15:29:25Z
publishDate 2013
publisher Національний науковий центр «Харківський фізико-технічний інститут» НАН України
record_format dspace
spelling Dovbnya, A.N.
Deyev, O.S.
Kushnir, V.A.
Malyshevsky, V.S.
Malykhina, T.V.
Mitrochenko, V.V.
Perezhogin, S.A.
Torgovkin, A.V.
Fomin, G.V.
Shramenko, B.I.
2017-01-17T14:51:35Z
2017-01-17T14:51:35Z
2013
Experimental cross-section evaluation data for ⁷Be photoproduction by ¹²C, ¹⁴N, ¹⁶O nuclei in the energy range between 40…90 MeV / A.N. Dovbnya1, O.S. Deyev, V.A. Kushnir, V.S. Malyshevsky, T.V. Malykhina, V.V. Mitrochenko, S.A. Perezhogin, A.V. Torgovkin, G.V. Fomin, B.I. Shramenko1 // Вопросы атомной науки и техники. — 2013. — № 6. — С. 192-195. — Бібліогр.: 7 назв. — англ.
1562-6016
PACS: 07.85.-m, 87.53.-j
https://nasplib.isofts.kiev.ua/handle/123456789/112085
The ⁷Be isotope produced in the upper atmosphere under the action of cosmic radiation is an important factor in population radiation load. A correct determination of the radiation dose coming from this isotope calls for consideration of the photonuclear mechanism of ⁷Be production by the nuclei of oxygen and nitrogen. The paper gives the experimental yields from A(γ, X)⁷Be nuclear reactions in the bremsstrahlung beam versus the end-point energies of electrons (from 40 to 90 MeV). The mathematical model approach with the GEANT4 class library was used to calculate the spectra of bremsstrahlung incident on the targets. Based on the experimental results, we have calculated the A(γ, X)⁷Be reaction cross-sections for oxygen, nitrogen and carbon. Calculated values of photonuclear reaction cross-sections for ⁷Be production by ¹²C, ¹⁴N, ¹⁶O nuclei were obtained with the use of the TALYS package. Agreement between experimental and calculated results only for ¹²C and ¹⁴N is shown.
Ізотоп ⁷Be, що утворюється у верхніх шарах атмосфери під впливом космічного випромінювання, є важливим чинником радіаційного навантаження на людину. Для правильного визначення дози опромінення від цього ізотопу потрібно ураховувати фотоядерний механізм утворення ⁷Be на ядрах кисню та азоту. Наведено експериментальні залежності виходів ядерних реакцій А(γ, Х) Ве⁷ на пучку гальмівного випромінювання для наступних граничних енергій електронів: 40, 50, 60, 70, 80, 90 МеВ. Методом математичного моделювання з використанням GEANT4 розраховані спектри гальмівного випромінювання, що падає на мішені, за результатами експерименту були обчислені перерізи реакцій А(γ, Х) ⁷Ве на кисні, азоті і вуглеці. За допомогою пакету TALYS отримані розрахункові залежності перерізів фотоядерних реакцій утворення 7Ве на ядрах ¹²C, ¹⁴N, ¹⁶O. Показано частково задовільне узгодження експериментальних та розрахункових результатів.
Изотоп ⁷Ве, образующийся в верхних слоях атмосферы под действием космического излучения, является важным фактором радиационной нагрузки на человека. Для правильного определения дозы облучения от этого изотопа необходим учет фотоядерного механизма образования ⁷Ве на ядрах кислорода и азота. Приведены экспериментальные зависимости выходов ядерных реакций А(γ, Х) ⁷Ве на пучке тормозного излучения для следующих граничных энергий электронов: 40, 50, 60, 70, 80, 90 МэВ. Методом математического моделирования с использованием библиотеки классов GEANT4 рассчитаны спектры тормозного излучения, падающего на мишени, по результатам эксперимента были вычислены сечения реакций А(γ, Х) ⁷Ве на кислороде, азоте и углероде. При помощи пакета TALYS получены расчетные зависимости сечения фотоядерных реакций образования ⁷Ве на ядрах ¹²C, ¹⁴N, ¹⁶O. Показано частично удовлетворительное согласие экспериментальных и расчетных результатов.
This work was supported by the National Academy of Sciences of Ukraine and by Russian Foundation for Basic Research Grants № 02-08-12(У) 35-2012.
en
Національний науковий центр «Харківський фізико-технічний інститут» НАН України
Вопросы атомной науки и техники
Применение ускоренных пучков. Детекторы и детектирование ядерных излучений
Experimental cross-section evaluation data for ⁷Be photoproduction by ¹²C, ¹⁴N, ¹⁶O nuclei in the energy range between 40…90 MeV
Експериментальні результати визначення перерізів фотоутворення ⁷Be на ядрах ¹²C, ¹⁴N, ¹⁶O в діапазоні енергій 40…90 МeВ
Экспериментальные результаты определения сечения фоторождения ⁷Be на ядрах ¹²C, ¹⁴N, ¹⁶O в диапазоне энергий 40…90 МэВ
Article
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spellingShingle Experimental cross-section evaluation data for ⁷Be photoproduction by ¹²C, ¹⁴N, ¹⁶O nuclei in the energy range between 40…90 MeV
Dovbnya, A.N.
Deyev, O.S.
Kushnir, V.A.
Malyshevsky, V.S.
Malykhina, T.V.
Mitrochenko, V.V.
Perezhogin, S.A.
Torgovkin, A.V.
Fomin, G.V.
Shramenko, B.I.
Применение ускоренных пучков. Детекторы и детектирование ядерных излучений
title Experimental cross-section evaluation data for ⁷Be photoproduction by ¹²C, ¹⁴N, ¹⁶O nuclei in the energy range between 40…90 MeV
title_alt Експериментальні результати визначення перерізів фотоутворення ⁷Be на ядрах ¹²C, ¹⁴N, ¹⁶O в діапазоні енергій 40…90 МeВ
Экспериментальные результаты определения сечения фоторождения ⁷Be на ядрах ¹²C, ¹⁴N, ¹⁶O в диапазоне энергий 40…90 МэВ
title_full Experimental cross-section evaluation data for ⁷Be photoproduction by ¹²C, ¹⁴N, ¹⁶O nuclei in the energy range between 40…90 MeV
title_fullStr Experimental cross-section evaluation data for ⁷Be photoproduction by ¹²C, ¹⁴N, ¹⁶O nuclei in the energy range between 40…90 MeV
title_full_unstemmed Experimental cross-section evaluation data for ⁷Be photoproduction by ¹²C, ¹⁴N, ¹⁶O nuclei in the energy range between 40…90 MeV
title_short Experimental cross-section evaluation data for ⁷Be photoproduction by ¹²C, ¹⁴N, ¹⁶O nuclei in the energy range between 40…90 MeV
title_sort experimental cross-section evaluation data for ⁷be photoproduction by ¹²c, ¹⁴n, ¹⁶o nuclei in the energy range between 40…90 mev
topic Применение ускоренных пучков. Детекторы и детектирование ядерных излучений
topic_facet Применение ускоренных пучков. Детекторы и детектирование ядерных излучений
url https://nasplib.isofts.kiev.ua/handle/123456789/112085
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