On the dense plasma decay within the electron concentration range of 10¹⁷ cm⁻³≤Ne≤10²² cm⁻³

The paper presents the results of comparison between the experimental decay coefficients of the dense plasma produced by pulsed discharges in water with theoretical coefficients calculated using all the known formulas for the three-particle recombination with the plasma ionization taken into account...

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Published in:Вопросы атомной науки и техники
Date:2013
Main Authors: Fedorovich, О.А., Voitenko, L.M.
Format: Article
Language:English
Published: Національний науковий центр «Харківський фізико-технічний інститут» НАН України 2013
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Online Access:https://nasplib.isofts.kiev.ua/handle/123456789/112166
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Cite this:On the dense plasma decay within the electron concentration range of 10¹⁷ cm⁻³≤Ne≤10²² cm⁻³ / О.А. Fedorovich, L.M. Voitenko // Вопросы атомной науки и техники. — 2013. — № 4. — С. 217-222. — Бібліогр.: 24 назв. — англ.

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Digital Library of Periodicals of National Academy of Sciences of Ukraine
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author Fedorovich, О.А.
Voitenko, L.M.
author_facet Fedorovich, О.А.
Voitenko, L.M.
citation_txt On the dense plasma decay within the electron concentration range of 10¹⁷ cm⁻³≤Ne≤10²² cm⁻³ / О.А. Fedorovich, L.M. Voitenko // Вопросы атомной науки и техники. — 2013. — № 4. — С. 217-222. — Бібліогр.: 24 назв. — англ.
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container_title Вопросы атомной науки и техники
description The paper presents the results of comparison between the experimental decay coefficients of the dense plasma produced by pulsed discharges in water with theoretical coefficients calculated using all the known formulas for the three-particle recombination with the plasma ionization taken into account. The best agreement was obtained in the calculations of the ternary recombination with taking into account only the levels realized in the dense plasma and with taking into account the ionization using the experimental decay coefficients of the dense plasma. Наведено результати порівняння експериментальних коефіцієнтів розпаду густої плазми імпульсних розрядів у воді з теоретичними коефіцієнтами, розрахованими за всіма відомими формулами для тричасткової рекомбінації з урахуванням іонізації плазми. Найкращу згоду з експериментальними коефіцієнтами розпаду густої плазми отримано при розрахунку коефіцієнтів потрійної рекомбінації з урахуванням тільки тих рівнів, які реалізувалися в щільній плазмі із урахуванням іонізації. Приведены результаты сравнения экспериментальных коэффициентов распада плотной плазмы импульсных разрядов в воде с теоретическими, рассчитанными по всем известным формулам коэффициентами для трехчастичной рекомбинации с учетом ионизации плазмы. Наилучшее согласие получено при расчете коэффициентов тройной рекомбинации с учетом только реализовавшихся в плотной плазме уровней и учетом ионизации с экспериментальными коэффициентами распада плотной плазмы.
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fulltext ISSN 1562-6016. ВАНТ. 2013. №4(86) 217 ON THE DENSE PLASMA DECAY WITHIN THE ELECTRON CONCENTRATION RANGE OF 1017 cm-3≤Ne≤1022 cm-3 О.А. Fedorovich, L.M. Voitenko Institute for Nuclear Research of National Academy of Sciences of Ukraine, Kiev, Ukraine E-mail: oafedorovich@kinr.kiev.ua The paper presents the results of comparison between the experimental decay coefficients of the dense plasma produced by pulsed discharges in water with theoretical coefficients calculated using all the known formulas for the three-particle recombination with the plasma ionization taken into account. The best agreement was obtained in the calculations of the ternary recombination with taking into account only the levels realized in the dense plasma and with taking into account the ionization using the experimental decay coefficients of the dense plasma. PACS: 52.80.-s. 52.20.Dq INTRODUCTION Processes of the dense plasma decay are studied not satisfactory. In recent years a series of theoretical works were published presenting the results of numerical simulation on recombination processes in the dense plasma [1 - 4]. There the corrections were introduced into the classical Gurevich-Pitaevsky formula for calcula- tion of a three-particle recombination in the rarefied plasma [5, 6]. The corrections leaded to the slight de- crease in the values of dense plasma recombination coef- ficients. But the calculated corrections enclose different models of the electron-ion interaction. The authors of [1 - 3] have made an assumption that there are existing cou- pled states of atoms; an energy region adjacent to the ionization limit where pairing states, practically, are ab- sent (a ”gap” between the pairing coupled and free elec- tron states); free electron states. In [1 - 3] the effect of atomic level unrealization in the high electric microfields was taken into account. In [4] the corrections to the Gurevich-Pitaevsky formula for the ultracold nonideal plasma were calculated. Here it has been supposed the following: “The previously existing viewpoint, asserting that in the course of the degree of nonideality increasing in the distribution function a gap arises because of the pairing state absence, is not quite right” (gap absence). The authors of [7, 8] proposed a model for the bi- nary recombination in the dense plasma and derived a corresponding formula for the strongly nonideal plasma recombination coefficient. An interaction between the electron and the nearest ion in the nonideal plasma was described in the nearest neighbor approximation and by the cellular model. In the theoretical work [9] the corrections to the Gurevich-Pitaevsky formula [5, 6] were derived too. The corrections to the coefficient of the three-particle recombination depending on the temperature (T) and electron concentration (Ne) were calculated. Independ- ently on the charged particle concentration in the plasma, there obtained were three variants of corrections to the formula showing the recombination coefficient decreasing versus Ne. According to [9] the three-particle electron recombination rate decreases by a factor of ė (2.718) occurs, when Г ee≥ 0.55 (Гee is the degree of plasma nonideality). This is the condition for almost full closing of the three-particle electron recombination channel (by Pitaevsky) [9]. It should be also noted, that the magnetic field influence on the dense (nonideal) plasma recombination rate is insignificant [9]. In [10] the decrease of the nonideal plasma recom- bination coefficient as a result of upper level unrealiza- tion in the high microfields was estimated. There it has been assumed that the levels, onto which the recombina- tion can occur, are not broadened. Before, the decay and recombination coefficients were determined experimentally for the electron con- centrations to Ne ≤ 2⋅1017 сm-3 at 64⋅103 K [11]. Dis- crepancies between the predicted and experimental val- ues were insignificant. However, a slight decrease of experimental values in comparison with theoretical cal- culations by the formula for three-particle recombina- tion has been already observed [5, 6]. The subsequent investigations on the hydrogen-oxygen plasma produced the high-voltage pulse discharges in water [12 - 16] have revealed a significant disagreement between ex- perimental and theoretical results at high values of Ne. For the electron concentration Ne ≤ 2⋅1017 сm-3 the ex- perimental values of the decay coefficient are practi- cally coinciding with the theory, as in [11]. For higher Ne the values of the decay coefficient obtained experi- mentally were lower than the calculated values by 6 orders of magnitude and more. And the difference was increasing with electron concentration increasing, the calculations being carried out with the use of the three- particle recombination model. The purpose of the pre- sent work is to compare the experimental results with calculation results obtained by different theoretical models and to determine dependences of the decay coef- ficient on plasma temperature, electron concentration, degree of plasma nonideality within the ranges of elec- tron concentration of 1017 сm-3 ≤ Ne ≤ 1022 сm-3 and temperature of 5⋅103 К ≤ Т ≤ 5⋅104 К. EXPERIMENTAL RESULTS AND DISCUSSION Experimental investigations of dense plasma decay coefficients at electron concentrations of 1017сm-3 ≤ Ne ≤ 1022 сm-3 were carried out under condi- tions of relaxation of the plasma produced by pulsed discharges in water. To obtain a good reproducibility and high electron densities, the discharges in water were initiated by the thin exploding wires. The diameter of tungsten conductors initiating discharges was varying from 20 to 500 μm. The storage battery capacity С = 14.6 μF, discharge circuit inductance was 0.43 μH. The discharge period under short-circuit conditions was 15.5 μs. The initial voltage on the battery was varying ISSN 1562-6016. ВАНТ. 2013. №4(86) 218 from 3 to 37 kV, and the maximum accumulated energy did not exceed 10 kJ. The discharge gap length was changing from 10 to 100 mm. The discharges in water were initiated by conductors of iron, molybdenum, cop- per, brass, constantan, carbon, nickel and other materi- als. The most interesting were discharges initiated by the tungsten conductor. A peculiarity of such discharges consisted in that the tungsten conductors might be heated before the metal vapor breakdown to the tem- perature of 13⋅103 К [17] at tungsten melting tempera- ture of 3689 K and boiling temperature of 5930 K. The metal heating to such high temperatures permits to ob- tain, rather easily, free electrons in vapors and to gener- ate discharges without a current pause with a very high degree of ionization and concentrations to the densities electrons of 1022 сm-3. Besides, the first ionization po- tential W is 8 eV, the second is 14 eV and the third is 24 eV [18]. For hydrogen the ionization potential Eи = 13.6 eV; for oxygen the first potential is 13.6 eV and the second is 35.1 eV. Also, for the water molecule dissociation it is necessary to use 9.5 eV. Therefore, when the discharge occurs in the tungsten vapors, the second tungsten ion ionization is possible and the plasma with a high temperature and electron concentra- tion can be obtained. If for the discharge initiation in water the conductors of other metals are used it is im- possible to obtain the plasma with such a high concen- tration. When the discharge initiation in water is per- formed with the conductors of carbon, constantan, nickel, these materials are heated up to moderate tem- peratures. Therefore, the vapor breakdowns are delayed for long times and, consequently, the low values of the plasma channel temperature and comparatively low electron concentrations are observed. In addition, for investigations of decay coefficients the discharges cho- sen have contributed a maximum energy into the chan- nel in the first half-period, practically, without energy supplements into the plasma in the second and subse- quent half-periods [13, 14]. Thus, it was possible to ob- tain minimum errors when determining the decay coef- ficients. The most interesting were discharges with a discharge gap length of 100 mm initiated by tungsten exploding conductors with wire diameter of 20 μm, voltage U0 =30 kV, as well as, a tungsten exploding wire of 320 μm in diameter, conductor length of 40 mm and voltage of 20 kV. The experimental plasma decay coefficient is deter- mined from the relation 2 e e r Nt N K ⋅Δ Δ = , where eNΔ is the electron concentration decrease for the time interval tΔ , and eN − the electron concentration. The theoreti- cal calculation of the decay coefficient is determined from the principle of detailed balancing i e a 2 e e Nb N N Ndt dN ⋅α−= ⋅ , where aN is the atomic concen- tration in plasma, b − the ionization coefficient, iN⋅α − the recombination coefficient. In this case the decay coefficient is determined with taking into account the plasma ionization that can be rather high at a tempera- ture of (7…45)⋅103 К. Just such temperatures are ob- served in the case of pulsed discharges in water. As is shown in [15, 16] the unambiguous depend- ence of the decay coefficient on the plasma temperature is not observed. This contradicts to the classical formula for three-particle plasma recombination by the electron- electron-ion collision model. The temperature depend- ence in this model is very strong ~Т-9/2 [5, 6]. When the temperature changes from 7000 to 64000 K the experi- mental value of K at equal values of concentration Ne has practically the same value [15, 16]. According to [5, 6] the recombination coefficient should be different by a factor of ~ 2.1⋅104 (twenty one thousands times). Comparison of experimental results on K with val- ues calculated by the recombination model [7, 8] shows a satisfactory coincidence only at the electron concen- tration Ne < 1019 сm-3 [16]. Fig. 1 presents the decay coefficient values Kr versus time determined experimentally in comparison with theoretical values calculated by the classical formula for the three particle recombination. Here also given are the calculated values of b N N e a ⋅ , being less by an order of magnitude and more than the recombination coefficient. Therefore, in such a discharge regime practically there is no ionization influence on the calculation results and the decay coefficient coincides with the recombination coefficient (an overestimation error < 10 %). The ap- proach of results goes with concentration decreasing and sequential appearance of Нα (656.3 nm), Нβ (486.1 nm) andНγ (434.06 nm) lines in the radiation. Then the plasma in the continuous spectrum becomes transparent. Fig. 1. The dependence on time the decay coefficient Comparison of experimental values Кр with these calculated by the Gurevich-Pitaevsky formula [5, 6], calculations by Johnson and Hinnov [20], as well as, Lankin-Norman [1 - 3] is given in Fig. 2. In [20] the hydrogen plasma opacity in the Layman series radiation lines and the ionization was taken into account. Thus the approach of experimental and experimental results was slightly improved (Fig. 2). The calculation results by the formulas of [1 - 3] practically coincide with the calcula- tion results for the nonideal plasma formulas at electron concentrations Ne less than 1019 сm-3 or Гее ≤ 0.6…7, as it follows from the formulas given in the present paper. But they are significantly higher than the experimental values of Kr. According to [19] the decay coefficient Kr can be determined by the time dependence of the ratio between the maximum electron concentration max eN and the current concentration Ne. ISSN 1562-6016. ВАНТ. 2013. №4(86) 219 Fig. 2. The dependence on time the decay coefficient Fig. 3 presents the ratio e max e NN as a function of time. One can see that to 70 µs the curve slope was neg- ligibly small. Beginning from 70 µs the curve depend- ence increases and after 80 µs it increases once again. This can evidence on the recombination type change with electron concentration decreasing in the dense plasma. Fig. 3. Dependence on time the ratio e max e NN The results on the time dependence of experimental values of rК and calculated values obtained by different models for the nonideal plasma are presented in Fig. 4. Fig. 4. The dependence on time the decay coefficient The calculation results do not show significant ap- proach of theoretical and experimental values of rК . If the ionization is taken into account, the approach of experimental and theoretical results also is not improved because the ionization values are < 10% in comparison with the recombination values, and the calculation re- sults are practically coinciding. It should be noted that the used ionization calculation was taken from [20]. But there one does not take into account the effects of line level unrealization in the high electrical dense plasma microfields. The value of rК is slowly changing with time. Fig. 5,a presents the results of comparison between the experimental values of rК and the calculation data with corrections taking into account the influence of the de- gree of plasma nonideality on the Gurevich-Pitaevsky formula. Fig. 5,a. The dependence of the decay of the degree of nonideality Depending on the degree of plasma nonideality in the case of Гее < 1 the corrections do not lead to the sig- nificant decrease of calculated values of decay coeffi- cients in all the three theoretical models [1 - 4, 9]. To 50 µs the value of rК is practically unchangeable. The electron concentration changing with time in this case was calculated by the Sakha formula. The total electron concentration in the plasma was determined from the pressure. The pressure dependence on time was calcu- lated by the hydrodynamic characteristics of the plasma channel. The pressure was calculated by the quasi- incompressible liquid [21]. The radiance temperature was taken from the plasma channel radiation measure- ments by comparison with a standard source EV-45 [22]. In calculations of the partition function only the levels observed experimentally were taken into account. The ionization potential decrease was not taken into account [1 - 3]. The plasma channel has radiated a con- tinuous spectrum but its radiation strongly differs from the radiation of an absolutely black body [23]. In the present case the temperature was measured on the wave- length of 400 nm. As the plasma is decaying and the intensity of the continuous spectrum is decreasing, from this spectrum an emission linear spectrum begins to appear. At 50 µm a strongly broadened Нα (656.3 nm) line appears and at 63 µm it is the Нγ (434.06 nm) line. Therefore, beginning from 65 µm it has been succeeded to measure the electron concentration change in time by the Stark broadening of Нα line [24]. With appearance of Нα, Нβ and Нγ lines the plasma decay rate quickly increases (see Fig. 2). The value of Кr increases and the approach between the theoretical calculation results for the triple recombination and experimental values of Кr ISSN 1562-6016. ВАНТ. 2013. №4(86) 220 takes place. It is explained by the fact that in the hydro- gen atom new levels arise onto which the electron re- combination is observed leading to the Кp increase. Be- sides, when the electron concentration Ne decreases, the line broadening and electron orbits in atoms become more stable that leads to rК increasing. When plotting rК against the degree of nonideality a peculiarity is ob- served. As the degree of nonideality decreases from 0.6 (at the plasma decay beginning) to 0.3 then the region of experimental values of rК arises, where Гее is not changing and the decay coefficient increases from 10-16 до 10-13 сm3/s. It is due to the appearance of Нα, Нβ and Нγ line levels and to the beginning of the sharp re- combination rate increase. The nonideality parameter Гее includes the temperature-electron concentration rela- tion. Therefore different values of Ne and T can corre- spond to the same value of Гее. At the same time in the calculation curves a kind of a “hysteresis loop” is ob- served for the dependence of Кr on Гee. The unambiguous temperature dependence of Кr in the dense plasma was not revealed. Only the unambigu- ous dependence on the electron concentration was ob- served [15]. Evidently, the nonideality parameter is not a main and unique parameter on which the dense plasma decay coefficient depends. Indeed, at high degrees of nonideality there is a correlation between the rК de- crease and Гее increase (Fig. 5,b). Fig. 5,b. The dependence of the decay of the degree of nonideality Comparison between the experimental results ob- tained for rК versus Г and the theoretical data shows that all the calculated values are significantly higher in the case of Г ≤ 5. The most close values were obtained in [1 - 3], particularly, if it is assumed that the ion charge Z = 2. Nevertheless, it is necessary to estimate additionally the theoretical corrections to the formula for the three-particle recombination. As is noted in [9] at high Ne the “three-particle recombination channel is closed”. In [9] the values of Ne, are lower as compared to these given in our paper. Also, the results are not im- proved even if the ionization is taken into account when the real recombination coefficients are determined. The ionization coefficient is changing approximately from 10% at Ne concentrations of 1020 сm-3 and T of 45·103 K to 0.1% at Ne = 1017…1018 сm-3 and Т < 7⋅103 K. So, at plasma temperatures lower than <20⋅103 К for the pulsed discharges in water the decay coefficients are almost coinciding with the recombination coefficients. And the error does not exceed 10% towards the recom- bination coefficient overestimation. Taking into account that none of the corrections to the three-particle recom- bination formula [1 - 4, 9] leads to a good agreement with the experimental data on the dense plasma decay coefficient at the electron concentration Ne > 1019 сm-3, it is necessary to consider other possible recombination mechanisms. Besides, it should be kept in mind that the calculated values are by several orders of magnitude higher than the experimental values. To be exact, the triple shock-radiation recombination is by 4-5 orders is higher than the coefficient corresponding to the electron capture as a result of triple collisions into the ground atomic state [19]. The calculation results for the triple recombination onto the ground hydrogen atomic state and their comparison with the experimental data are presented in Fig. 6. Fig. 6. The dependence on time the decay coefficient One can see from the figure that the values calcu- lated by this formula really are less by three orders than these calculated by the Gurevich-Pitaevsky formula, but still exceed by several orders the experimental values at electron densities of > 3·1018 сm-3 and coincides with the experimental values obtained at Ne = 2·1017 сm-3. If the ionization coefficient is plotted, it is by an order higher than the coefficient of recombination onto the ground state. From the plasma radiation spectra is known that the second excitation level is not observed (there is no Нα line in the radiation spectrum) to 50 μs. Therefore we decided to calculate the recombination coefficient onto the first level with the excitation energy of 10.2 eV. The results of calculations on the ionization coefficient and the recombination coefficient practically are coinciding. The summation of recombination coeffi- cient values by two levels increases its total value by 10% (see Fig. 6). And the difference between the ioni- zation values and recombination values is so negligible that, apparently, in this connection the experimental values of the decay coefficients are lower by several orders of magnitude. For comparison the results of calculations on the time dependence of photorecombination coefficients for one of the discharge regime are given in Fig. 7. ISSN 1562-6016. ВАНТ. 2013. №4(86) 221 Fig. 7. The dependence on time the decay coefficient They are sufficiently close to the decay coefficient values at the initial discharge stage. However, the calcu- lated ionization coefficients are by three-four orders higher than the photorecombination coefficients and at Ne = 2·1018 сm-3 they are meeting. But in experiments the decay coefficient values were higher than the ioniza- tion coefficient values. Once more contradiction to the experimental fact takes place. It is shown in [15] that there is a dependence of rК on the electron concentra- tion during the decay of the plasma produced by the pulsed discharge in water. And in the case of the photo- recombination the recombination coefficient does not depend on Ne. Consequently, in the dense plasma the ternary combination occurs, but the recombination coef- ficients should be calculated only with taking into ac- count the experimentally observed atomic levels, as well as, the calculation results for ionization in the dense plasma. CONCLUSIONS The degree of nonideality is not an unambiguous pa- rameter describing the corrections for recombination coefficient calculations by the Gurevich-Pitaevsky for- mula. None of formulas with plasma nonideality correc- tions to the Gurevich-Pitaevsky formula gives a good agreement between the calculated values and experi- mental values of the decay coefficients even if the ioni- zation is taken into account. The corrections on the elec- tron density are necessary. The best coincidence with the experimental values of decay coefficients has been obtained in the calculations of the coefficients of ternary electron recombination only onto the experimentally observed atomic levels and when the ionization was taken into account. REFERENCES 1. A.V. Lankin, G.E. Norman. Self-consistent descrip- tion of free and coupled states in the nonideal plasma. Fluctuation approach // Reports of the Acad- emy of Sciences. 2008, v. 418, № 3, p. 466-472. 2. A.V. Lankin, G.E. Norman. Recombination in the dense ion plasma // Reports of the Academy of Sci- ences. 2012, v. 446, № 3, p. 1-5. 3. A.V. Lankin. 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M.: «Nauka», 1987, 592 p. (in Russian). 20. L.C. Johnson, E. Hinnov. Ionization, recombination and population of excited levels in hydrogen plas- mas // J. Quant. Spectrosc. аnd Radiat. Transfer. 1973, v. 13, p. 333-337. 21. N.М. Beskaravayniy, V.А. Posdeev. Wave problems on the cavity widening in liquid with taking into ac- count the boundary displacement finiteness // Phys- ico-fur processes at a high voltage discharge in liq- uid. Kiev: «Naukova dumka», 1980, p. 88-97. 22. А.N. Demidov, N.N. Оgurzova, I.V. Pоdmoschen- sky. Pulsed light source with radiation similar to the absolute black body radiation at temperature of 40000 K // Opto-mechanical industry. 1960, № 1, p. 2-7. 23. L.L. Pasechnik, P.D. Starchik, O.A. Fedorovich. Investigation of the continuous radiation from the pulsed discharge in water within the range of 400…700 nm // Proc. Reports. 6-Union Conf. on the physics of low-temperature plasma. L. 1983, v. 1, p. 501-503. 24. V.V. Matvienko, A.Yu. Popov, O.A. Fedorovich. On the problem of radiation line use for measuring the parameters of plasma produced by pulsed-discharges in water // Collection. Theory, experiment, practice razryadnoimpulsnoy technology. Kiev: "Naukova Dumka", 1987, p. 14-22 (in Ukrainian). Article received 21.05.2013. О РАСПАДЕ ПЛОТНОЙ ПЛАЗМЫ В ДИАПАЗОНЕ КОНЦЕНТРАЦИЙ ЭЛЕКТРОНОВ 1017 см-3 ≤ Ne ≤ 1022 см-3 О.А. Федорович, Л.М. Войтенко Приведены результаты сравнения экспериментальных коэффициентов распада плотной плазмы импульс- ных разрядов в воде с теоретическими, рассчитанными по всем известным формулам коэффициентами для трехчастичной рекомбинации с учетом ионизации плазмы. Наилучшее согласие получено при расчете ко- эффициентов тройной рекомбинации с учетом только реализовавшихся в плотной плазме уровней и учетом ионизации с экспериментальными коэффициентами распада плотной плазмы. ПРО РОЗПАД ГУСТОЇ ПЛАЗМИ В ДІАПАЗОНІ КОНЦЕНТРАЦІЙ ЕЛЕКТРОНІВ 1017 см-3 ≤ Nе ≤ 1022 см-3 О.А. Федорович, Л.М. Войтенко Наведено результати порівняння експериментальних коефіцієнтів розпаду густої плазми імпульсних роз- рядів у воді з теоретичними коефіцієнтами, розрахованими за всіма відомими формулами для тричасткової рекомбінації з урахуванням іонізації плазми. Найкращу згоду з експериментальними коефіцієнтами розпаду густої плазми отримано при розрахунку коефіцієнтів потрійної рекомбінації з урахуванням тільки тих рів- нів, які реалізувалися в щільній плазмі із урахуванням іонізації.
id nasplib_isofts_kiev_ua-123456789-112166
institution Digital Library of Periodicals of National Academy of Sciences of Ukraine
issn 1562-6016
language English
last_indexed 2025-12-01T11:03:50Z
publishDate 2013
publisher Національний науковий центр «Харківський фізико-технічний інститут» НАН України
record_format dspace
spelling Fedorovich, О.А.
Voitenko, L.M.
2017-01-17T19:52:29Z
2017-01-17T19:52:29Z
2013
On the dense plasma decay within the electron concentration range of 10¹⁷ cm⁻³≤Ne≤10²² cm⁻³ / О.А. Fedorovich, L.M. Voitenko // Вопросы атомной науки и техники. — 2013. — № 4. — С. 217-222. — Бібліогр.: 24 назв. — англ.
1562-6016
PACS: 52.80.-s. 52.20.Dq
https://nasplib.isofts.kiev.ua/handle/123456789/112166
The paper presents the results of comparison between the experimental decay coefficients of the dense plasma produced by pulsed discharges in water with theoretical coefficients calculated using all the known formulas for the three-particle recombination with the plasma ionization taken into account. The best agreement was obtained in the calculations of the ternary recombination with taking into account only the levels realized in the dense plasma and with taking into account the ionization using the experimental decay coefficients of the dense plasma.
Наведено результати порівняння експериментальних коефіцієнтів розпаду густої плазми імпульсних розрядів у воді з теоретичними коефіцієнтами, розрахованими за всіма відомими формулами для тричасткової рекомбінації з урахуванням іонізації плазми. Найкращу згоду з експериментальними коефіцієнтами розпаду густої плазми отримано при розрахунку коефіцієнтів потрійної рекомбінації з урахуванням тільки тих рівнів, які реалізувалися в щільній плазмі із урахуванням іонізації.
Приведены результаты сравнения экспериментальных коэффициентов распада плотной плазмы импульсных разрядов в воде с теоретическими, рассчитанными по всем известным формулам коэффициентами для трехчастичной рекомбинации с учетом ионизации плазмы. Наилучшее согласие получено при расчете коэффициентов тройной рекомбинации с учетом только реализовавшихся в плотной плазме уровней и учетом ионизации с экспериментальными коэффициентами распада плотной плазмы.
en
Національний науковий центр «Харківський фізико-технічний інститут» НАН України
Вопросы атомной науки и техники
Плазменно-пучковый разряд, газовый разряд и плазмохимия
On the dense plasma decay within the electron concentration range of 10¹⁷ cm⁻³≤Ne≤10²² cm⁻³
Про розпад густої плазми в діапазоні концентрацій електронів 10¹⁷ см⁻³ ≤ Nе ≤ 10²² см⁻³
О распаде плотной плазмы в диапазоне концентраций электронов 10¹⁷ см⁻³ ≤ Nе ≤ 10²² см⁻³
Article
published earlier
spellingShingle On the dense plasma decay within the electron concentration range of 10¹⁷ cm⁻³≤Ne≤10²² cm⁻³
Fedorovich, О.А.
Voitenko, L.M.
Плазменно-пучковый разряд, газовый разряд и плазмохимия
title On the dense plasma decay within the electron concentration range of 10¹⁷ cm⁻³≤Ne≤10²² cm⁻³
title_alt Про розпад густої плазми в діапазоні концентрацій електронів 10¹⁷ см⁻³ ≤ Nе ≤ 10²² см⁻³
О распаде плотной плазмы в диапазоне концентраций электронов 10¹⁷ см⁻³ ≤ Nе ≤ 10²² см⁻³
title_full On the dense plasma decay within the electron concentration range of 10¹⁷ cm⁻³≤Ne≤10²² cm⁻³
title_fullStr On the dense plasma decay within the electron concentration range of 10¹⁷ cm⁻³≤Ne≤10²² cm⁻³
title_full_unstemmed On the dense plasma decay within the electron concentration range of 10¹⁷ cm⁻³≤Ne≤10²² cm⁻³
title_short On the dense plasma decay within the electron concentration range of 10¹⁷ cm⁻³≤Ne≤10²² cm⁻³
title_sort on the dense plasma decay within the electron concentration range of 10¹⁷ cm⁻³≤ne≤10²² cm⁻³
topic Плазменно-пучковый разряд, газовый разряд и плазмохимия
topic_facet Плазменно-пучковый разряд, газовый разряд и плазмохимия
url https://nasplib.isofts.kiev.ua/handle/123456789/112166
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