Dynamics of the emission spectrum of the hydrogenoxygen plasma of pulsed discharge in water in the range of the Balmer series with a minimum of impurities

The results of experimental investigations of the spectral distribution of radiation of hydrogen - oxygen plasma pulsed discharges in water in a minimum difference of radiation from the blackbody radiation (BBR) are given. The pressure in the plasma channel was changed from 5000 to 80 atm, the brigh...

Full description

Saved in:
Bibliographic Details
Published in:Вопросы атомной науки и техники
Date:2015
Main Authors: Fedorovich, O.A., Voitenko, L.M.
Format: Article
Language:English
Published: Національний науковий центр «Харківський фізико-технічний інститут» НАН України 2015
Subjects:
Online Access:https://nasplib.isofts.kiev.ua/handle/123456789/112196
Tags: Add Tag
No Tags, Be the first to tag this record!
Journal Title:Digital Library of Periodicals of National Academy of Sciences of Ukraine
Cite this:Dynamics of the emission spectrum of the hydrogenoxygen plasma of pulsed discharge in water in the range of the Balmer series with a minimum of impurities / O.A. Fedorovich, L.M. Voitenko // Вопросы атомной науки и техники. — 2015. — № 4. — С. 189-193. — Бібліогр.: 21 назв. — англ.

Institution

Digital Library of Periodicals of National Academy of Sciences of Ukraine
_version_ 1859943809385758720
author Fedorovich, O.A.
Voitenko, L.M.
author_facet Fedorovich, O.A.
Voitenko, L.M.
citation_txt Dynamics of the emission spectrum of the hydrogenoxygen plasma of pulsed discharge in water in the range of the Balmer series with a minimum of impurities / O.A. Fedorovich, L.M. Voitenko // Вопросы атомной науки и техники. — 2015. — № 4. — С. 189-193. — Бібліогр.: 21 назв. — англ.
collection DSpace DC
container_title Вопросы атомной науки и техники
description The results of experimental investigations of the spectral distribution of radiation of hydrogen - oxygen plasma pulsed discharges in water in a minimum difference of radiation from the blackbody radiation (BBR) are given. The pressure in the plasma channel was changed from 5000 to 80 atm, the brightness temperature of 24·10³ to 7·10³ K. The difference in brightness temperatures of the violet and the red area does not exceed ± 2000 K of the average temperature. With the relaxation of plasma electron density decreased from 2·10²⁰ to 10¹⁷ cm⁻³. It is shown that at high concentrations of electron spectral distribution of the radiation in the spectral range of the Balmer series differs little from the blackbody radiation is not observed and none of the hydrogen Balmer line. This indicates "non-realization" even the top level line Hα. (656.2 nm, with excitation energy of the upper level of 12.09 eV). As the relaxation of the plasma to be consistent line Нα, Нβ, Нγ. There is a redistribution of the broadening of the hydrogen lines of the Bal-mer series. At Ne ≤ 10¹⁷ сm⁻³ hydrogen emission spectrum coincides with the traditional. Наведено результати експериментальних досліджень спектральних розподілів випромінювання воднево-кисневої плазми імпульсних розрядів у воді (ІРВ) в умовах мінімальної відмінності випромінювання від випромінювання абсолютно чорного тіла (АЧТ). Тиск у плазмовому каналі змінювався від 5 тис. атмосфер до 80 атмосфер, яскравістна температура – від 24·10³ до 7·10³ К. Різниця яскравісних температур у фіолетовій і червоній областях не перевищувала ± 2000 К від середньої температури. При релаксації плазми концентрація електронів зменшувалася від 2·10²⁰ до 10¹⁷ см⁻³. Показано, що при високих концентраціях електронів спектральний розподіл випромінювання в діапазоні спектра серії Бальмера мало відрізняється від випромінювання АЧТ і не спостерігається ні одна лінія водню серії Бальмера Hα. Це свідчить про «нереалізацію» навіть самого верхнього рівня лінії Нα (656,2 нм, з енергією збудження верхнього рівня 12,09 еВ). По мірі релаксації плазми проявляються послідовно лінії Нα, Нβ, Нγ. Спостерігається перерозподіл розширення ліній водню серії Бальмера. При Ne ≤ 10¹⁷ см⁻³ спектр випромінювання водню збігається з традиційним. Приведены результаты экспериментальных исследований спектральных распределений излучения водородно-кислородной плазмы импульсных разрядов в воде (ИРВ) в условиях минимального отличия этого излучения от излучения абсолютно черного тела (АЧТ). Давление в плазменном канале менялось от 5 тыс. атмосфер до 80 атмосфер, яркостная температура от 24·10³ до 7·10³ К. Различие яркостных температур в фиолетовой и красной областях не превышало ± 2000 К от средней температуры. При релаксации плазмы концентрация электронов уменьшалась от 2·10²⁰ до 10¹⁷ см⁻³. Показано, что при высоких концентрациях электронов спектральное распределение излучения в диапазоне спектра серии Бальмера мало отличается от излучения АЧТ и не наблюдается ни одна линия водорода серии Бальмера. Это свидетельствует о «нереализации» даже самого верхнего уровня линии Нα (656,2 нм, с энергией возбуждения верхнего уровня 12,09 эВ). По мере релаксации плазмы проявляются последовательно линии Нα, Нβ, Нγ. Наблюдается перераспределение уширения линий водорода серии Бальмера. При Ne ≤ 10¹⁷ см⁻³ спектр излучения водорода совпадает с традиционным спектром.
first_indexed 2025-12-07T16:12:39Z
format Article
fulltext ISSN 1562-6016. ВАНТ. 2015. №4(98) 189 DYNAMICS OF THE EMISSION SPECTRUM OF THE HYDROGEN- OXYGEN PLASMA OF PULSED DISCHARGE IN WATER IN THE RANGE OF THE BALMER SERIES WITH A MINIMUM OF IMPURITIES O.A. Fedorovich, L.M. Voitenko Institute for Nuclear Research NASU, Kiev, Ukraine E-mail: oafedorovich@kinr.kiev.ua The results of experimental investigations of the spectral distribution of radiation of hydrogen - oxygen plasma pulsed discharges in water in a minimum difference of radiation from the blackbody radiation (BBR) are given. The pressure in the plasma channel was changed from 5000 to 80 atm, the brightness temperature of 24⋅103 to 7⋅103 K. The difference in brightness temperatures of the violet and the red area does not exceed ± 2000 K of the average temper- ature. With the relaxation of plasma electron density decreased from 2⋅1020 to 1017 cm-3. It is shown that at high con- centrations of electron spectral distribution of the radiation in the spectral range of the Balmer series differs little from the blackbody radiation is not observed and none of the hydrogen Balmer line. This indicates "non-realization" even the top level line Hα. (656.2 nm, with excitation energy of the upper level of 12.09 eV). As the relaxation of the plasma to be consistent line Нα, Нβ, Нγ. There is a redistribution of the broadening of the hydrogen lines of the Bal- mer series. At Ne ≤ 1017 сm-3 hydrogen emission spectrum coincides with the traditional. PACS: 52.80.-s. 52.20. Dq INTRODUCTION Optical radiation nonideal plasma is practically the only source of information on plasma parameters, the structure of the plasma channel, the mean free path of photons, radiant thermal conductivity, line broadening in a plasma, "optical reduction of the ionization poten- tial", reducing the oscillator strengths, "non-realization" of individual, high-lying levels, and so on [1]. The study of the spectral distribution of radiation is necessary for the calculation of the energy and the particles balance in the channel of a pulsed discharge in water, revealing the influence of non-ideal effects on the emission spectra of hydrogen-oxygen plasma, the development and testing of the methods for measuring the basic plasma parame- ters and to identify the range of applicability of these methods depending on the electrons concentration in the plasma. The hydrogen-oxygen plasma produced in a pulsed discharge in water (PDW) on 2/3 is composed of atoms and ions of hydrogen. It is one of the significant advantages in the study of such plasma to determine the effects of nonideality influence on the emission spectra and their dependence on the electron concentration and temperature. The spectrum hydrogen is the simplest for theoreti- cal description as a hydrogen atom consists of a single electron and proton. But the published data on the hy- drogen spectra at high electron densities are insufficient and they often contradictory (see in particular [2 - 8]). This is due to the fact that these data have been obtained at essentially different research facilities parameters, different methods of nonideal plasma obtaining and different initial conditions. Theoretical estimates of the non-ideal properties of the plasma are given in (see in particular [1, 10, 12]). This paper presents the results of experimental in- vestigations of the spectral distribution of radiation of hydrogen-oxygen plasma, and the evolution of the emis- sion spectra at the stage of relaxation, depending on the temperature and on the optical thickness reducing. Also, presents the results of testing of different methods to determine the main parameters of the plasma. One technique for obtaining spectral scans over time and the dynamics of the emission spectrum of the hy- drogen-oxygen plasma in the PDW, in the Hα, Hβ lines region, was considered in [6, 13]. A second technique for obtaining spectra scans in time and space, as well as calibration of the film in intensity from source EV-45 [14] is given in [15]. Previously, it was noted that in the initial stage of the discharge emission of the hydrogen-oxygen plasma essentially differs from the black body (BB) radiation [3]. The violet region of the spectrum there was a signif- icant exceeding of brightness temperature Tb measured in the red region of the spectrum. The degree of differ- ence from the BB radiation increases with the rate of energy input into the plasma channel. EXPERIMENTAL RESULTS AND DISCUSSION For studies was selected the discharge mode in which there is the smallest deviation of the radiation from the BB radiation. The emission spectrum of the investigated plasma in the initial stage of discharge is continuous, and the intensity changes are little over time. With the expan- sion of the plasma channel, and with the decrease in its electrons concentration and pressure, a continuous spec- trum of radiation is transformed into a line spectrum, and the duration of the last essentially depends on the energy input into the channel [15]. This reduces the optical thickness of the plasma and plasma becomes optically transparent [16, 17]. Let us consider in more detail the dynamics of the spectrum in the Balmer lines Hα, Hβ, Hγ in near and- threshold region for one discharge regime and estimate influence on the spectrum of non-ideal effects. Figs. 1-8 shows the spectral radiation distribution of the hydro- gen-oxygen plasma at different times, as the relaxation of the plasma. To do this, select the category with a minimal amount of metal impurities (emission spectrum which often leads to the inability to obtain lines of hy- drogen [15]). ISSN 1562-6016. ВАНТ. 2015. №4(98) 190 Fig. 1. The intensity of the radiation I = f (λ) hydrogen- oxygen plasma in the Balmer series. W, d = 20 µm; U0 = 30 кV; l0 = 100 mm; t = (9 ± 2) µs To eliminate the influence of impurities of metal va- pors coming from the electrodes [15] we chosen for study the spectrum of the discharge with electrode gap length 100 mm and investigated the middle of the channel. Fig. 2. The dependence of the radiation intensity I = f (λ) hydrogen-oxygen plasma. W, d = 20 µm; U0 = 30 кV; l0 = 100 mm; t = (12 ± 2) µs As follows from Fig. 1 the emission spectrum of the hydrogen-oxygen plasma at an initial stage of the dis- charge (9 ± 2) microseconds) differs little from the blackbody radiation at a temperature (20 ± 1)⋅103 K. In near and-threshold region, as well as in the area of the most intense spectral Hα lines of hydrogen Balmer series no singularities of the spectrum is observed. The plasma pressure, calculated by the hydrodynam- ic characteristics of the channel and model of quasi- incompressible fluid is ~ 2⋅103 at, and the electron den- sity is less than Ne ~ 5⋅1019 сm-3 at a concentration of atoms Na ~ 5⋅1020 сm-3 [18]. In the wall region of the plasma channel is always a colder region. The degree of ionization of the plasma in the colder region not exceeding 10%, and at this tem- perature there is always excited hydrogen atoms. In this case, inevitably had be observed in the absorption lines of hydrogen Hα (λ = 656.2 nm). However, as shown in Fig. 1, this does not occur, which indicates the manifes- tation of the effect of "non-realization" of the upper level of the most intense line of the Balmer series. Over time, as the pressure reduction in the emission intensity at the spectrum-threshold and begins to rise somewhat, while in other areas it is somewhat reduced (Fig. 2), (t = (12 ± 2) µs). To detect absorption in the Hα line also fails. At the time (t = (22 ± 2) µs) is already clearly seen in the absorption line Hα (Fig. 3). Fig. 3. The dependence of the radiation intensity I = f (λ) hydrogen-oxygen plasma. W, d = 20 µm; U0 = 30 кV; l0 = 100 mm; t =(22 ± 2) µs In the wall region of the plasma channel is always a colder region. The degree of ionization of the plasma in the colder region not exceeding 10%, and at this tem- perature there is always excited hydrogen atoms. In this case, inevitably had be observed in the absorption lines of hydrogen Hα (λ = 656.2 nm). However, as shown in Fig. 1, this does not occur, which indicates the manifes- tation of the effect of "non-realization" of the upper level of the most intense line of the Balmer series. Over time, as the pressure reduction in the emission intensity at the spectrum-threshold and begins to rise somewhat, while in other areas it is somewhat reduced (see Fig. 2), (t = (12 ± 2) µs). To detect absorption in the Hα line also fails. At the time (t = (22 ± 2) µs) is already clearly seen in the absorption line Hα (see Fig. 3). The intensity of the emission spectrum in the supercritical region corresponds to (22 ± 2)⋅103 К. If at the same time to measure the tem- perature in the center of the reabsorb line Hα it is ~14.5⋅103 К. The pressure in the plasma channel at the same time about ~ 300 at and Ne ~ 3 ⋅ cm-3 (γ ~ 0.27). Under these conditions, Hβ line is not yet observed. chan-nel in the wall region. In the supercritical region while there is a small rise in intensity. The brightness tempera-ture Tb = 20⋅103 К (Wing line Hα Тя=17⋅103 К). Hγ line under these conditions has not yet been shown (Fig. 4). The plasma in this case is still optically opaque. Fig. 4 shows the emission spectrum of the hydrogen-oxygen plasma at a pressure of about 150 at and a tem-perature of 20⋅103 К (t = (48 ± 2) µs). Under these con-ditions, Ne ~ ISSN 1562-6016. ВАНТ. 2015. №4(98) 191 ing of lines which are at a higher power level in com- parison with the calculated. Fig. 4. The dependence of the radiation intensity I = f (λ) hydrogen-oxygen plasma. W, d = 20 µm; U0 = 30 кV; l0 = 100 mm; t = (48 ± 2) µs These results indicate an inaccuracy of theoretical calculations of line broadening at high values of the micro-fields [15], in spite of the Debye screening ac- counting for the electron and ion components and the line broadening at high concentrations. Fig. 5. The dependence of the radiation intensity I = f (λ) hydrogen-oxygen plasma. tungsten, d = 20 µm; U0 = 30 кV; l0 = 100 mm; t =(57 ± 2) µs As already noted, the pressure drop as the optical thickness and temperature of the plasma decreases and continuous emission spectrum is transformed into a line spectrum. Fig. 5 shows the emission spectrum of the hydrogen-oxygen plasma, when the lines Hα, Hβ, Hγ become prominent in a continuous spectrum of radia- tion. The optical thickness in the distant wing of the line Hα, is reduced to τ = 1.5…2 [13, 17]. Note that the values of τ, obtained by the method of plasma transillumination under PRW give overestimat- ed 5…8 times values. This is due to the passage of the rays through the plasma. Plasma is in the water with a refractive index n = 1.34, while for n = 1 the plasma [20]. This cylindrical plasma channel works as a cylin- drical lens. Given that the boundary of the channel are not al- ways strictly cylindricity due to instabilities of the plasma channel is correctly taken into account in deter- mining the curvature of the intensity of the transmitted beam is not possible. Fig. 6. The dependence of the radiation intensity I = f (λ) hydrogen-oxygen plasma. W, d = 20 µm; U0 = 30 кV; l0 = 100 mm; t = (64 ± 2) µs Because of this value of τ, obtained by the method transillumination essentially overestimated and they can not be used, although plasma is possible to enlighten in the later stages the discharge. In violet part of the continuous spectrum of the value of τ should be even smaller. The parameters of the plas- ma channel, defined by several independent methods are: P = 120 bar, Ne = 1019 cm-3, T = 17·103 K. At the same time temperature as determined by the intensity at the maximum reabsorbs line Hα [13] and in the threshold of the Balmer series of the spectrum are the same. The temperature obtained by I for the line Hβ somewhat higher. A characteristic feature of the emission spectrum is the fact that the half-width of the line Hα more than Hβ and Hγ, although according to the theory of line broad- ening [15] should be the opposite. The same effect is observed upon further reduction of P and T (Fig. 6). Here the half-width of the line Hα, Hβ is 150, 140 A, Hγ 65 A. The optical thickness in the red region of the con- tinuous spectrum τ < 1 [15]. Therefore, the effect of the near-wall cold regions of the plasma can be neglected. They partially affect reab- sorption in the central region of the line Hα, where τ more (τ > 10), but their influence on the radiation in the violet part of the spectrum should be negligible. The parameters of the plasma channel are follows: P = 100 atm, Tmax = 15.5⋅103K, Ne = 6⋅1018 cm-3, the bore diameter d = 23.4 mm. In Figs. 7, 8 show the dynamics of the emission spec- trum at lower plasma concentrations and low temperatures. These figures show that the half-width of the lines Hα and Hβ are compared, and then, when at Ne ≤2⋅1017 cm-3 lines Hβ are wider than Hα, as predicted by the theory [19], and the values of Ne, obtained by the half-widths of these lines are virtually identical. Decreases while the intensity Hβ line and T defined poney becomes smaller than de- fined by certain intensity in Hα, which could be evidence of small optical thickness in line Hβ. In the adjacent and threshold areas of the series spectrum regions intensity is slightly higher than in oth- er areas. In the near-threshold areas and threshold areas a se- ries of intensity of the spectrum is somewhat higher than in other areas. Line Hγ observed only a few microsec- ISSN 1562-6016. ВАНТ. 2015. №4(98) 192 onds, and its half width is less than Hβ. microseconds, and its half width is less than the line Hβ [5, 6]. Line Hδ from the continuous spectrum was unable to locate. Fig. 7. The dependence of the radiation intensity I = f (λ) hydrogen-oxygen plasma. W, d = 20 µm; U0 = 30 кV; l0 = 100 mm; t =(71 ± 2) µs Fig. 8. The dependence of the radiation intensity I = f (λ) hydrogen-oxygen plasma. W, d = 20 µm; U0 = 30 кV; l0 = 100 mm; t = (86 ± 2) µs Note that if the appearance of lines Hβ, and Hγ re- sponsible colder outer region of the plasma, the effect of reducing the line broadening is even stronger. To detect the influence of this effect it is necessary to obtain the radial distribution of the temperature and make intensity correction taking into account the refraction at the plas- ma-water interface. In [20] the radial temperature distribution for this mode of discharge by 77 ms. It shows almost plateau- like temperature distribution along the radius (cross section) of the channel, which should not significantly affect the electrons distribution and concentration in the channel cross section and the absorption in the near-wall plasma regions. According to [10, 11] Hα line should "not be real- ized" when the electron density Ne ≥ 2⋅1019 cm-3, Hβ when Ne ≥ (1.5…3)⋅1018 cm-3, Hγ when Ne ≥ 0.9⋅1018 cm- 3. These Ne values are somewhat lower than those ob- tained experimentally by several methods [20]. Perhaps this is due to colder regions near the walls, and realization of the lines with higher levels just in them. The above results indicate a decrease or redistribu- tion of oscillator strength, predicted in [21], and the "non-realization" of lines level in the micro-fields, com- parable in magnitude to the strength of intra-atomic fields, and in this range includes most intense level of Hα lines. CONCLUSIONS The plasma parameters can be measured outside the boundaries of the series or on lines that are not affected by non-realization, as predicted theoretically in [5, 6]. Especially strongly last effect is manifested with in- creasing rate of energy input into the channel [3]. From the above results and results in [13] it can also be concluded that it is permissible to determine the elec- tron density from the Stark broadening of the lines Hα when Ne < 1019 cm-3 and Hβ when Ne < 1018 cm-3. To measure the maximum temperature along the line monitoring the intensity of the radiation maximum Hα line can be reabsorbed immediately after discharge from the continuous spectrum. REFERENCES 1. V. Fortov, I. Iakubov, A. Khrapak. Fizika neidealnoi plazmy. M.: “Fizmatlit”, 2004, 326 p. (in Russian). 2. A.A. Kon'kov. Izluchenie plotnoy vodorodnoy termycheskoy plasma // Teplofizika vysokikh tem- peratur (TVT). 1979, v. 17, №4, p. 678-684 (in Rus- sian). 3. L.L. Pasechnik, P.D. Starchik, O.A. Fedorovich. Study of continuous pulsed discharge in water in the range of 400…700 nm // Abstracts of the VI All- Union Conference on the Physics of low- temperature plasma, Leningrad: 1983, v. I, p. 501- 503 (in Russian). 4. P.D. Starchyk, P.V. Porytskyy. On the optical prop- erties of the nonideal plasma of electrical pulse dis- charge in water // Problems of Atomic Science and Technology. Series “Plasma Physics”. 2007, № 1, p. 182-184. 5. O.A. Fedorovich. Empirical formula for the depend- ence of the “optical gap” value on the electron con- centration Ne within the range of 1017 cm-3≤Ne≤1017 cm-3 // Problems of Atomic Science and Technology. Series “Plasma Electronics and New Methods of Acceleration”. 2013, №4, p. 223-228. 6. O.A. Fedorovich. Experimental Investigation of Op- tical Properties of Nonideal Plasma within the Elec- tron Concentration Range 1017 cm−3<Ne<1022 cm−3 // TPHT. 2014, v. 52. № 4, p. 524-534 (in Russian). 7. T.V. Gavrilova, V.P. Aver’yanov, Y. Vitel, L.G. D’yachkov, Yu.K. Kurilenkov. Spectrum of ab- sorption of dense hydrogenic plasmas in Balmer’s re- gion // Opt. Spectrosc. 1997, v. 82, № 5, p. 757-764. 8. Y. Vitel, M. El. Bezzari, L.G. D’yachkov, Yu.K. Kurilenkov. Emission from weakly nonideal http://lib.mipt.ru/search/?q=authors%3A+Fortov http://lib.mipt.ru/search/?q=authors%3A+Iakubov http://lib.mipt.ru/search/?q=authors%3A+Khrapak http://lib.mipt.ru/search/?q=authors%3A+Khrapak ISSN 1562-6016. ВАНТ. 2015. №4(98) 193 helium plasmas produced in flash lamps // Phys. Rev. E. 1998, v. 58, № 6, p. 7855-7863. 9. T.V. Gavrilova, V.P. Averyanov, I. Vittel, L.G. Diachkov, Yu.K. Kurilenkov. Optical spectra of hydrogen plasma at electron concentrations over 1019cm3 // Optics and Spectroscopy. 2001, v. 91, № 5, p. 667-674. 10. G.E. Norman. Continuous emission spectra (absorp- tion) nonideal plasma // TVT. 1979, v. 17, № 3, p. 453-460 (in Russian). 11. G.A. Kobzev, Yu.K. Kurilenkov, G.E. Norman. Theory of the optical properties of strongly coupled plasma // TVT. 1979, v. 15, № 1, p. 193-196 (in Rus- sian). 12. L.G. Diachkov. "Continuous spectrum", Encyclopedia of low-temperature plasma / red. V.E. Fortov. Mos- cow: “Nauka”, 2000. v. 1, p. 391-395 (in Russian). 13. V.V. Matvienko, A.Y. Popov, O.A. Fedorovich. To a question about the use of the emission lines for measuring plasma pulsed discharge in water // Col- lection. Theory, experiment, practice razryadnoim- pulsnoy technology. Kiev: "Naukova Dumka", 1987, p. 14-22 (in Russian). 14. А.N. Demidov, N.N. Оgurzova, I.V. Pоdmoschensky. Pulsed light source with radiation similar to the abso- lute black body radiation at temperature of 40000 K // Optico-mechanical industry. 1960, № 1, p. 2-7. 15. L.L. Pasechnik, P.D. Starchik, O.A. Fedorovich. Temporal evolution of the emission spectra PDW // Collection. Theory, experiment, practice of pulsed discharge technology. Kiev: "Naukova Dumka", 1987, p. 6-9 (in Russian). 16. O.A. Fedorovich. Technique of experimental defini- tion of optical thickness of the plasma channel by the method of lightening and possibilities of its appli- cation for pulsing discharge in water // Nuclear Phys- ics and Atomic Energy. 2008, № 2, p. 86-96. 17. O.A. Fedorovich. Methods of experimental determi- nation of the optical thickness of the plasma channel PDW on a contour line reabsorb hydrogen Нα // Nu- clear Physics and Atomic Energy. 2010, v. 11, № 1, p. 97-107. 18. O.A. Fedorovich, L.M. Voitenko. Coefficients col- lapse of strongly coupled plasma concentrations of electrons at PDW 2⋅1017см-3 ≤ Ne ≤ 2⋅1020cм-3 // Problems of Atomic Science and Technology. Series “Plasma Electronics and New Methods of Accelera- tion”. 2008, № 4, p. 288-293. 19. G. Grim. The broadening of the spectral lines in plasma. M.: «Mir», 492 p. (in Russian). 20. О.А. Fedorovich. On peculiarities of the radial tem- perature distribution in a channel of pulsed discharge in water at the relaxation stage // Ukr. J. Phys. 2008, v. 53, № 5, р. 458-464. 21. V.T. Gurovich, V.L. Spectorov, V.S. Engelsht. On the degeneration of spectral series of hydrogen plasma // TVT. 1979, v. 17, № 6, p. 1128-1132 (in Russian). Article received 30.04.2015 ДИНАМИКА СПЕКТРА ИЗЛУЧЕНИЯ ВОДОРОДНО-КИСЛОРОДНОЙ ПЛАЗМЫ ИРВ В ДИАПАЗОНЕ СЕРИИ БАЛЬМЕРА С МИНИМАЛЬНЫМ КОЛИЧЕСТВОМ ПРИМЕСЕЙ О.А. Федорович, Л.М. Войтенко Приведены результаты экспериментальных исследований спектральных распределений излучения водо- родно-кислородной плазмы импульсных разрядов в воде (ИРВ) в условиях минимального отличия этого излучения от излучения абсолютно черного тела (АЧТ). Давление в плазменном канале менялось от 5 тыс. атмосфер до 80 атмосфер, яркостная температура от 24⋅103 до 7⋅103 К. Различие яркостных температур в фи- олетовой и красной областях не превышало ± 2000 К от средней температуры. При релаксации плазмы кон- центрация электронов уменьшалась от 2⋅1020 до 1017 см-3. Показано, что при высоких концентрациях элек- тронов спектральное распределение излучения в диапазоне спектра серии Бальмера мало отличается от из- лучения АЧТ и не наблюдается ни одна линия водорода серии Бальмера. Это свидетельствует о «нереализа- ции» даже самого верхнего уровня линии Нα (656,2 нм, с энергией возбуждения верхнего уровня 12,09 эВ). По мере релаксации плазмы проявляются последовательно линии Нα, Нβ, Нγ. Наблюдается перераспределе- ние уширения линий водорода серии Бальмера. При Ne ≤ 1017 см-3 спектр излучения водорода совпадает с традиционным спектром. ДИНАМІКА СПЕКТРА ВИПРОМІНЮВАННЯ ВОДНЕВО-КИСНЕВОЇ ПЛАЗМИ IPВ У ДІАПАЗОНІ СЕРІЇ БАЛЬМЕРА З МІНІМАЛЬНОЮ КІЛЬКІСТЮ ДОМІШОК О.А. Федорович, Л.М. Войтенко Наведено результати експериментальних досліджень спектральних розподілів випромінювання воднево- кисневої плазми імпульсних розрядів у воді (ІРВ) в умовах мінімальної відмінності випромінювання від ви- промінювання абсолютно чорного тіла (АЧТ). Тиск у плазмовому каналі змінювався від 5 тис. атмосфер до 80 атмосфер, яскравістна температура – від 24⋅103 до 7⋅103 К. Різниця яскравісних температур у фіолетовій і червоній областях не перевищувала ± 2000 К від середньої температури. При релаксації плазми концентра- ція електронів зменшувалася від 2⋅1020 до 1017 см-3. Показано, що при високих концентраціях електронів спектральний розподіл випромінювання в діапазоні спектра серії Бальмера мало відрізняється від випромі- нювання АЧТ і не спостерігається ні одна лінія водню серії Бальмера Hα. Це свідчить про «нереалізацію» навіть самого верхнього рівня лінії Нα (656,2 нм, з енергією збудження верхнього рівня 12,09 еВ). По мірі релаксації плазми проявляються послідовно лінії Нα, Нβ, Нγ. Спостерігається перерозподіл розширення ліній водню серії Бальмера. При Ne ≤ 1017 см-3 спектр випромінювання водню збігається з традиційним. introduction references
id nasplib_isofts_kiev_ua-123456789-112196
institution Digital Library of Periodicals of National Academy of Sciences of Ukraine
issn 1562-6016
language English
last_indexed 2025-12-07T16:12:39Z
publishDate 2015
publisher Національний науковий центр «Харківський фізико-технічний інститут» НАН України
record_format dspace
spelling Fedorovich, O.A.
Voitenko, L.M.
2017-01-17T20:33:34Z
2017-01-17T20:33:34Z
2015
Dynamics of the emission spectrum of the hydrogenoxygen plasma of pulsed discharge in water in the range of the Balmer series with a minimum of impurities / O.A. Fedorovich, L.M. Voitenko // Вопросы атомной науки и техники. — 2015. — № 4. — С. 189-193. — Бібліогр.: 21 назв. — англ.
1562-6016
PACS: 52.80.-s. 52.20. Dq
https://nasplib.isofts.kiev.ua/handle/123456789/112196
The results of experimental investigations of the spectral distribution of radiation of hydrogen - oxygen plasma pulsed discharges in water in a minimum difference of radiation from the blackbody radiation (BBR) are given. The pressure in the plasma channel was changed from 5000 to 80 atm, the brightness temperature of 24·10³ to 7·10³ K. The difference in brightness temperatures of the violet and the red area does not exceed ± 2000 K of the average temperature. With the relaxation of plasma electron density decreased from 2·10²⁰ to 10¹⁷ cm⁻³. It is shown that at high concentrations of electron spectral distribution of the radiation in the spectral range of the Balmer series differs little from the blackbody radiation is not observed and none of the hydrogen Balmer line. This indicates "non-realization" even the top level line Hα. (656.2 nm, with excitation energy of the upper level of 12.09 eV). As the relaxation of the plasma to be consistent line Нα, Нβ, Нγ. There is a redistribution of the broadening of the hydrogen lines of the Bal-mer series. At Ne ≤ 10¹⁷ сm⁻³ hydrogen emission spectrum coincides with the traditional.
Наведено результати експериментальних досліджень спектральних розподілів випромінювання воднево-кисневої плазми імпульсних розрядів у воді (ІРВ) в умовах мінімальної відмінності випромінювання від випромінювання абсолютно чорного тіла (АЧТ). Тиск у плазмовому каналі змінювався від 5 тис. атмосфер до 80 атмосфер, яскравістна температура – від 24·10³ до 7·10³ К. Різниця яскравісних температур у фіолетовій і червоній областях не перевищувала ± 2000 К від середньої температури. При релаксації плазми концентрація електронів зменшувалася від 2·10²⁰ до 10¹⁷ см⁻³. Показано, що при високих концентраціях електронів спектральний розподіл випромінювання в діапазоні спектра серії Бальмера мало відрізняється від випромінювання АЧТ і не спостерігається ні одна лінія водню серії Бальмера Hα. Це свідчить про «нереалізацію» навіть самого верхнього рівня лінії Нα (656,2 нм, з енергією збудження верхнього рівня 12,09 еВ). По мірі релаксації плазми проявляються послідовно лінії Нα, Нβ, Нγ. Спостерігається перерозподіл розширення ліній водню серії Бальмера. При Ne ≤ 10¹⁷ см⁻³ спектр випромінювання водню збігається з традиційним.
Приведены результаты экспериментальных исследований спектральных распределений излучения водородно-кислородной плазмы импульсных разрядов в воде (ИРВ) в условиях минимального отличия этого излучения от излучения абсолютно черного тела (АЧТ). Давление в плазменном канале менялось от 5 тыс. атмосфер до 80 атмосфер, яркостная температура от 24·10³ до 7·10³ К. Различие яркостных температур в фиолетовой и красной областях не превышало ± 2000 К от средней температуры. При релаксации плазмы концентрация электронов уменьшалась от 2·10²⁰ до 10¹⁷ см⁻³. Показано, что при высоких концентрациях электронов спектральное распределение излучения в диапазоне спектра серии Бальмера мало отличается от излучения АЧТ и не наблюдается ни одна линия водорода серии Бальмера. Это свидетельствует о «нереализации» даже самого верхнего уровня линии Нα (656,2 нм, с энергией возбуждения верхнего уровня 12,09 эВ). По мере релаксации плазмы проявляются последовательно линии Нα, Нβ, Нγ. Наблюдается перераспределение уширения линий водорода серии Бальмера. При Ne ≤ 10¹⁷ см⁻³ спектр излучения водорода совпадает с традиционным спектром.
en
Національний науковий центр «Харківський фізико-технічний інститут» НАН України
Вопросы атомной науки и техники
Плазменно-пучковый разряд, газовый разряд и плазмохимия
Dynamics of the emission spectrum of the hydrogenoxygen plasma of pulsed discharge in water in the range of the Balmer series with a minimum of impurities
Динаміка спектра випромінювання воднево-кисневої плазми ІРВ у діапазоні серії Бальмера з мінімальною кількістю домішок
Динамика спектра излучения водородно-кислородной плазмы ИРВ в диапазоне серии Бальмера с минимальным количеством примесей
Article
published earlier
spellingShingle Dynamics of the emission spectrum of the hydrogenoxygen plasma of pulsed discharge in water in the range of the Balmer series with a minimum of impurities
Fedorovich, O.A.
Voitenko, L.M.
Плазменно-пучковый разряд, газовый разряд и плазмохимия
title Dynamics of the emission spectrum of the hydrogenoxygen plasma of pulsed discharge in water in the range of the Balmer series with a minimum of impurities
title_alt Динаміка спектра випромінювання воднево-кисневої плазми ІРВ у діапазоні серії Бальмера з мінімальною кількістю домішок
Динамика спектра излучения водородно-кислородной плазмы ИРВ в диапазоне серии Бальмера с минимальным количеством примесей
title_full Dynamics of the emission spectrum of the hydrogenoxygen plasma of pulsed discharge in water in the range of the Balmer series with a minimum of impurities
title_fullStr Dynamics of the emission spectrum of the hydrogenoxygen plasma of pulsed discharge in water in the range of the Balmer series with a minimum of impurities
title_full_unstemmed Dynamics of the emission spectrum of the hydrogenoxygen plasma of pulsed discharge in water in the range of the Balmer series with a minimum of impurities
title_short Dynamics of the emission spectrum of the hydrogenoxygen plasma of pulsed discharge in water in the range of the Balmer series with a minimum of impurities
title_sort dynamics of the emission spectrum of the hydrogenoxygen plasma of pulsed discharge in water in the range of the balmer series with a minimum of impurities
topic Плазменно-пучковый разряд, газовый разряд и плазмохимия
topic_facet Плазменно-пучковый разряд, газовый разряд и плазмохимия
url https://nasplib.isofts.kiev.ua/handle/123456789/112196
work_keys_str_mv AT fedorovichoa dynamicsoftheemissionspectrumofthehydrogenoxygenplasmaofpulseddischargeinwaterintherangeofthebalmerserieswithaminimumofimpurities
AT voitenkolm dynamicsoftheemissionspectrumofthehydrogenoxygenplasmaofpulseddischargeinwaterintherangeofthebalmerserieswithaminimumofimpurities
AT fedorovichoa dinamíkaspektravipromínûvannâvodnevokisnevoíplazmiírvudíapazoníserííbalʹmerazmínímalʹnoûkílʹkístûdomíšok
AT voitenkolm dinamíkaspektravipromínûvannâvodnevokisnevoíplazmiírvudíapazoníserííbalʹmerazmínímalʹnoûkílʹkístûdomíšok
AT fedorovichoa dinamikaspektraizlučeniâvodorodnokislorodnoiplazmyirvvdiapazoneseriibalʹmerasminimalʹnymkoličestvomprimesei
AT voitenkolm dinamikaspektraizlučeniâvodorodnokislorodnoiplazmyirvvdiapazoneseriibalʹmerasminimalʹnymkoličestvomprimesei