Phase transitions in TbMnO₃ manganites

X-ray diffraction and magnetic measurements of polycrystalline and nanosize TbMnO₃ manganites have been performed. All the compounds studied crystallize in the orthorhombic crystal structure (space group Pnma) at room temperature. The nanosize manganites were synthesized with a sol-gel method at d...

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Veröffentlicht in:Физика низких температур
Datum:2012
Hauptverfasser: Dyakonov, V., Szytuła, A., Szymczak, R., Zubov, E., Szewczyk, A., Kravchenko, Z., Bażela, W., Dyakonov, K., Zarzycki, A., Varyukhin, V., Szymczak, H.
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Sprache:English
Veröffentlicht: Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України 2012
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Online Zugang:https://nasplib.isofts.kiev.ua/handle/123456789/116948
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Zitieren:Phase transitions in TbMnO₃ manganites / V. Dyakonov, A. Szytuła, R. Szymczak, E. Zubov,A. Szewczyk, Z. Kravchenko, W. Bażela, K. Dyakonov,A. Zarzycki, V. Varyukhin, H. Szymczak // Физика низких температур. — 2012. — Т. 38, № 3. — С. 273-277. — Бібліогр.: 19 назв. — англ.

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Digital Library of Periodicals of National Academy of Sciences of Ukraine
id nasplib_isofts_kiev_ua-123456789-116948
record_format dspace
spelling Dyakonov, V.
Szytuła, A.
Szymczak, R.
Zubov, E.
Szewczyk, A.
Kravchenko, Z.
Bażela, W.
Dyakonov, K.
Zarzycki, A.
Varyukhin, V.
Szymczak, H.
2017-05-18T14:56:26Z
2017-05-18T14:56:26Z
2012
Phase transitions in TbMnO₃ manganites / V. Dyakonov, A. Szytuła, R. Szymczak, E. Zubov,A. Szewczyk, Z. Kravchenko, W. Bażela, K. Dyakonov,A. Zarzycki, V. Varyukhin, H. Szymczak // Физика низких температур. — 2012. — Т. 38, № 3. — С. 273-277. — Бібліогр.: 19 назв. — англ.
0132-6414
PACS: 61.05.cp, 61.46.–w, 75.75.–c, 75.47.Lx, 73.63.Bd
https://nasplib.isofts.kiev.ua/handle/123456789/116948
X-ray diffraction and magnetic measurements of polycrystalline and nanosize TbMnO₃ manganites have been performed. All the compounds studied crystallize in the orthorhombic crystal structure (space group Pnma) at room temperature. The nanosize manganites were synthesized with a sol-gel method at different (800 and 900°C) temperatures. The average size of synthesized nanoparticles (from 45 to 70 nm) was estimated by using the x-ray diffraction and low-temperature adsorption of argon methods. An information on the evolution of properties of TbMnO₃ with changing grain size, temperature and magnetic field was obtained. The crystal structure parameters of nanospecimens change slightly with changing the nanoparticle size. The peculiarities of magnetic ordering in polycrystalline and nanosize TbMnO₃ were compared. Magnetization and the Nèel temperature corresponding to antiferromagnetic ordering of the Tb³⁺ sublattice decrease as the particle size is reduced. The inverse magnetic susceptibility of the nanoparticle samples deviates from the Curie–Weiss law below 50 K, that is connected with the magnetic ordering of the Mn³⁺ moments. Specific heat of the nanosize samples exhibits anomalies related to the magnetic ordering of the Tb³⁺ and Mn³⁺ sublattices.
en
Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України
Физика низких температур
Низкотемпеpатуpный магнетизм
Phase transitions in TbMnO₃ manganites
Article
published earlier
institution Digital Library of Periodicals of National Academy of Sciences of Ukraine
collection DSpace DC
title Phase transitions in TbMnO₃ manganites
spellingShingle Phase transitions in TbMnO₃ manganites
Dyakonov, V.
Szytuła, A.
Szymczak, R.
Zubov, E.
Szewczyk, A.
Kravchenko, Z.
Bażela, W.
Dyakonov, K.
Zarzycki, A.
Varyukhin, V.
Szymczak, H.
Низкотемпеpатуpный магнетизм
title_short Phase transitions in TbMnO₃ manganites
title_full Phase transitions in TbMnO₃ manganites
title_fullStr Phase transitions in TbMnO₃ manganites
title_full_unstemmed Phase transitions in TbMnO₃ manganites
title_sort phase transitions in tbmno₃ manganites
author Dyakonov, V.
Szytuła, A.
Szymczak, R.
Zubov, E.
Szewczyk, A.
Kravchenko, Z.
Bażela, W.
Dyakonov, K.
Zarzycki, A.
Varyukhin, V.
Szymczak, H.
author_facet Dyakonov, V.
Szytuła, A.
Szymczak, R.
Zubov, E.
Szewczyk, A.
Kravchenko, Z.
Bażela, W.
Dyakonov, K.
Zarzycki, A.
Varyukhin, V.
Szymczak, H.
topic Низкотемпеpатуpный магнетизм
topic_facet Низкотемпеpатуpный магнетизм
publishDate 2012
language English
container_title Физика низких температур
publisher Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України
format Article
description X-ray diffraction and magnetic measurements of polycrystalline and nanosize TbMnO₃ manganites have been performed. All the compounds studied crystallize in the orthorhombic crystal structure (space group Pnma) at room temperature. The nanosize manganites were synthesized with a sol-gel method at different (800 and 900°C) temperatures. The average size of synthesized nanoparticles (from 45 to 70 nm) was estimated by using the x-ray diffraction and low-temperature adsorption of argon methods. An information on the evolution of properties of TbMnO₃ with changing grain size, temperature and magnetic field was obtained. The crystal structure parameters of nanospecimens change slightly with changing the nanoparticle size. The peculiarities of magnetic ordering in polycrystalline and nanosize TbMnO₃ were compared. Magnetization and the Nèel temperature corresponding to antiferromagnetic ordering of the Tb³⁺ sublattice decrease as the particle size is reduced. The inverse magnetic susceptibility of the nanoparticle samples deviates from the Curie–Weiss law below 50 K, that is connected with the magnetic ordering of the Mn³⁺ moments. Specific heat of the nanosize samples exhibits anomalies related to the magnetic ordering of the Tb³⁺ and Mn³⁺ sublattices.
issn 0132-6414
url https://nasplib.isofts.kiev.ua/handle/123456789/116948
citation_txt Phase transitions in TbMnO₃ manganites / V. Dyakonov, A. Szytuła, R. Szymczak, E. Zubov,A. Szewczyk, Z. Kravchenko, W. Bażela, K. Dyakonov,A. Zarzycki, V. Varyukhin, H. Szymczak // Физика низких температур. — 2012. — Т. 38, № 3. — С. 273-277. — Бібліогр.: 19 назв. — англ.
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first_indexed 2025-12-07T15:57:18Z
last_indexed 2025-12-07T15:57:18Z
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