Magnetic and resonance properties of the two-dimensional S = 1 compound Ni₅(TeO₃)₄Cl₂ with frustrated geometry

The magnetic and magnetoresonance properties of a new single-crystal compound Ni₅(TeO₃)₄Cl₂ are studied. The measurements of the magnetization and magnetic susceptibility of the crystal in a wide temperature range (5–300 K) made it possible to conclude that Ni₅(TeO₃)₄Cl₂ is a quasi-two-dimensional...

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Published in:Физика низких температур
Date:2008
Main Authors: Gnatchenko, S.L., Kobets, M.I., Khatsko, E.N., Baran, M., Szymczak, R., Lemmens, P., Berger, H.
Format: Article
Language:English
Published: Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України 2008
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Online Access:https://nasplib.isofts.kiev.ua/handle/123456789/117392
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Journal Title:Digital Library of Periodicals of National Academy of Sciences of Ukraine
Cite this:Magnetic and resonance properties of the two-dimensional S = 1 compound Ni₅(TeO₃)₄Cl₂ with frustrated geometry / S.L. Gnatchenko, M.I. Kobets, E.N. Khatsko, M. Baran, R. Szymczak, P. Lemmens, H. Berger // Физика низких температур. — 2008. — Т. 34, № 8. — С. 798–803. — Бібліогр.: 7 назв. — англ.

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Digital Library of Periodicals of National Academy of Sciences of Ukraine
id nasplib_isofts_kiev_ua-123456789-117392
record_format dspace
spelling Gnatchenko, S.L.
Kobets, M.I.
Khatsko, E.N.
Baran, M.
Szymczak, R.
Lemmens, P.
Berger, H.
2017-05-23T10:15:06Z
2017-05-23T10:15:06Z
2008
Magnetic and resonance properties of the two-dimensional S = 1 compound Ni₅(TeO₃)₄Cl₂ with frustrated geometry / S.L. Gnatchenko, M.I. Kobets, E.N. Khatsko, M. Baran, R. Szymczak, P. Lemmens, H. Berger // Физика низких температур. — 2008. — Т. 34, № 8. — С. 798–803. — Бібліогр.: 7 назв. — англ.
0132-6414
PACS: 76.50.+g;75.50.Ee
https://nasplib.isofts.kiev.ua/handle/123456789/117392
The magnetic and magnetoresonance properties of a new single-crystal compound Ni₅(TeO₃)₄Cl₂ are studied. The measurements of the magnetization and magnetic susceptibility of the crystal in a wide temperature range (5–300 K) made it possible to conclude that Ni₅(TeO₃)₄Cl₂ is a quasi-two-dimensional antiferromagnet with the easy magnetization axis a* directed perpendicular crystallographic plane bc and a magnetic ordering temperature TN≈21 K. The resonance measurements at 4.2 K in wide range of frequencies (25–105 GHz) and magnetic field (up to 200 kOe) permitted us to obtain the frequency–field dependence of AFMR spectrum for a field applied along the easy magnetization axis a*. It is shown that the magnetic field directed along the antiferromagnetism axis (H||a*) induces the magnetic phase transition of a spin-flop type which is found to be Hsf≈120 kOe. The magnetic resonance experimental data are described qualitatively in model of the biaxial antiferromagnet.
The authors would like to thank Dr. V.I. Fomin and Dr. V.P. Gnezdilov for fruitful discussions. This work has been supported in part by Ukrainian-Russian grant № 8-2008.
en
Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України
Физика низких температур
Низкотемпеpатуpный магнетизм
Magnetic and resonance properties of the two-dimensional S = 1 compound Ni₅(TeO₃)₄Cl₂ with frustrated geometry
Article
published earlier
institution Digital Library of Periodicals of National Academy of Sciences of Ukraine
collection DSpace DC
title Magnetic and resonance properties of the two-dimensional S = 1 compound Ni₅(TeO₃)₄Cl₂ with frustrated geometry
spellingShingle Magnetic and resonance properties of the two-dimensional S = 1 compound Ni₅(TeO₃)₄Cl₂ with frustrated geometry
Gnatchenko, S.L.
Kobets, M.I.
Khatsko, E.N.
Baran, M.
Szymczak, R.
Lemmens, P.
Berger, H.
Низкотемпеpатуpный магнетизм
title_short Magnetic and resonance properties of the two-dimensional S = 1 compound Ni₅(TeO₃)₄Cl₂ with frustrated geometry
title_full Magnetic and resonance properties of the two-dimensional S = 1 compound Ni₅(TeO₃)₄Cl₂ with frustrated geometry
title_fullStr Magnetic and resonance properties of the two-dimensional S = 1 compound Ni₅(TeO₃)₄Cl₂ with frustrated geometry
title_full_unstemmed Magnetic and resonance properties of the two-dimensional S = 1 compound Ni₅(TeO₃)₄Cl₂ with frustrated geometry
title_sort magnetic and resonance properties of the two-dimensional s = 1 compound ni₅(teo₃)₄cl₂ with frustrated geometry
author Gnatchenko, S.L.
Kobets, M.I.
Khatsko, E.N.
Baran, M.
Szymczak, R.
Lemmens, P.
Berger, H.
author_facet Gnatchenko, S.L.
Kobets, M.I.
Khatsko, E.N.
Baran, M.
Szymczak, R.
Lemmens, P.
Berger, H.
topic Низкотемпеpатуpный магнетизм
topic_facet Низкотемпеpатуpный магнетизм
publishDate 2008
language English
container_title Физика низких температур
publisher Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України
format Article
description The magnetic and magnetoresonance properties of a new single-crystal compound Ni₅(TeO₃)₄Cl₂ are studied. The measurements of the magnetization and magnetic susceptibility of the crystal in a wide temperature range (5–300 K) made it possible to conclude that Ni₅(TeO₃)₄Cl₂ is a quasi-two-dimensional antiferromagnet with the easy magnetization axis a* directed perpendicular crystallographic plane bc and a magnetic ordering temperature TN≈21 K. The resonance measurements at 4.2 K in wide range of frequencies (25–105 GHz) and magnetic field (up to 200 kOe) permitted us to obtain the frequency–field dependence of AFMR spectrum for a field applied along the easy magnetization axis a*. It is shown that the magnetic field directed along the antiferromagnetism axis (H||a*) induces the magnetic phase transition of a spin-flop type which is found to be Hsf≈120 kOe. The magnetic resonance experimental data are described qualitatively in model of the biaxial antiferromagnet.
issn 0132-6414
url https://nasplib.isofts.kiev.ua/handle/123456789/117392
citation_txt Magnetic and resonance properties of the two-dimensional S = 1 compound Ni₅(TeO₃)₄Cl₂ with frustrated geometry / S.L. Gnatchenko, M.I. Kobets, E.N. Khatsko, M. Baran, R. Szymczak, P. Lemmens, H. Berger // Физика низких температур. — 2008. — Т. 34, № 8. — С. 798–803. — Бібліогр.: 7 назв. — англ.
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first_indexed 2025-11-29T03:29:16Z
last_indexed 2025-11-29T03:29:16Z
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