ESR studies of nitrogen atoms stabilized in aggregates of krypton–nitrogen nanoclusters immersed in superfluid helium

Impurity–helium condensates (IHCs) containing nitrogen and krypton atoms immersed in superfluid ⁴He
 have been studied via a CW electron spin resonance (ESR) technique. The IHCs are gel-like aggregates of nanoclusters
 composed of impurity species. It was found that the addition of k...

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Veröffentlicht in:Физика низких температур
Datum:2012
Hauptverfasser: Mao, S., Boltnev, R.E., Khmelenko, V.V., Lee, D.M.
Format: Artikel
Sprache:Englisch
Veröffentlicht: Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України 2012
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Online Zugang:https://nasplib.isofts.kiev.ua/handle/123456789/117923
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Zitieren:ESR studies of nitrogen atoms stabilized in aggregates
 of krypton–nitrogen nanoclusters immersed in superfluid helium / S. Mao, R.E. Boltnev, V.V. Khmelenko, D.M. Lee // Физика низких температур. — 2012. — Т. 38, № 11. — С. 1313–1319. — Бібліогр.: 45 назв. — англ.

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Digital Library of Periodicals of National Academy of Sciences of Ukraine
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author Mao, S.
Boltnev, R.E.
Khmelenko, V.V.
Lee, D.M.
author_facet Mao, S.
Boltnev, R.E.
Khmelenko, V.V.
Lee, D.M.
citation_txt ESR studies of nitrogen atoms stabilized in aggregates
 of krypton–nitrogen nanoclusters immersed in superfluid helium / S. Mao, R.E. Boltnev, V.V. Khmelenko, D.M. Lee // Физика низких температур. — 2012. — Т. 38, № 11. — С. 1313–1319. — Бібліогр.: 45 назв. — англ.
collection DSpace DC
container_title Физика низких температур
description Impurity–helium condensates (IHCs) containing nitrogen and krypton atoms immersed in superfluid ⁴He
 have been studied via a CW electron spin resonance (ESR) technique. The IHCs are gel-like aggregates of nanoclusters
 composed of impurity species. It was found that the addition of krypton atoms to the nitrogen–helium
 gas mixture used for preparation of IHCs increases efficiency of stabilization of nitrogen atoms. We have
 achieved high average (5·10¹⁹ cm⁻³) and local (2·10²¹ cm⁻³) concentrations of nitrogen atoms in kryptonnitrogen–helium
 condensates. The analysis of ESR lines shows that three different sites exist for stabilization of
 nitrogen atoms in krypton-nitrogen nanoclusters. Nitrogen atoms are stabilized in the krypton core of nanoclusters,
 in the nitrogen molecular layer which covers the Kr core and on the surface of the nanoclusters. High concentrations
 of nitrogen atoms achieved in IHCs provide an important step in the search for magnetic ordering effects
 at low temperatures.
first_indexed 2025-11-29T11:57:15Z
format Article
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institution Digital Library of Periodicals of National Academy of Sciences of Ukraine
issn 0132-6414
language English
last_indexed 2025-11-29T11:57:15Z
publishDate 2012
publisher Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України
record_format dspace
spelling Mao, S.
Boltnev, R.E.
Khmelenko, V.V.
Lee, D.M.
2017-05-27T13:27:16Z
2017-05-27T13:27:16Z
2012
ESR studies of nitrogen atoms stabilized in aggregates
 of krypton–nitrogen nanoclusters immersed in superfluid helium / S. Mao, R.E. Boltnev, V.V. Khmelenko, D.M. Lee // Физика низких температур. — 2012. — Т. 38, № 11. — С. 1313–1319. — Бібліогр.: 45 назв. — англ.
0132-6414
PACS: 67.80.–s, 61.46–w, 76.30.Rn, 76.30.–v
https://nasplib.isofts.kiev.ua/handle/123456789/117923
Impurity–helium condensates (IHCs) containing nitrogen and krypton atoms immersed in superfluid ⁴He
 have been studied via a CW electron spin resonance (ESR) technique. The IHCs are gel-like aggregates of nanoclusters
 composed of impurity species. It was found that the addition of krypton atoms to the nitrogen–helium
 gas mixture used for preparation of IHCs increases efficiency of stabilization of nitrogen atoms. We have
 achieved high average (5·10¹⁹ cm⁻³) and local (2·10²¹ cm⁻³) concentrations of nitrogen atoms in kryptonnitrogen–helium
 condensates. The analysis of ESR lines shows that three different sites exist for stabilization of
 nitrogen atoms in krypton-nitrogen nanoclusters. Nitrogen atoms are stabilized in the krypton core of nanoclusters,
 in the nitrogen molecular layer which covers the Kr core and on the surface of the nanoclusters. High concentrations
 of nitrogen atoms achieved in IHCs provide an important step in the search for magnetic ordering effects
 at low temperatures.
We take this opportunity to thank Adil Meraki, Patrick
 McColgan and Trevor Dragon for assembling experimental
 setup and participation in the experiments.
 The work was supported by grant № 010366-0137-2009
 Norman Hackerman Advanced Research Program, CRDF
 grant RUP1-7025-CG-11, RFBR grant 11-02-92500-CRDFE_a,
 and federal contract 11.519.11.6021 with Russian
 Federation Ministry of Education and Science.
en
Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України
Физика низких температур
К 75-летию Л.П. Межова-Деглина
ESR studies of nitrogen atoms stabilized in aggregates of krypton–nitrogen nanoclusters immersed in superfluid helium
Article
published earlier
spellingShingle ESR studies of nitrogen atoms stabilized in aggregates of krypton–nitrogen nanoclusters immersed in superfluid helium
Mao, S.
Boltnev, R.E.
Khmelenko, V.V.
Lee, D.M.
К 75-летию Л.П. Межова-Деглина
title ESR studies of nitrogen atoms stabilized in aggregates of krypton–nitrogen nanoclusters immersed in superfluid helium
title_full ESR studies of nitrogen atoms stabilized in aggregates of krypton–nitrogen nanoclusters immersed in superfluid helium
title_fullStr ESR studies of nitrogen atoms stabilized in aggregates of krypton–nitrogen nanoclusters immersed in superfluid helium
title_full_unstemmed ESR studies of nitrogen atoms stabilized in aggregates of krypton–nitrogen nanoclusters immersed in superfluid helium
title_short ESR studies of nitrogen atoms stabilized in aggregates of krypton–nitrogen nanoclusters immersed in superfluid helium
title_sort esr studies of nitrogen atoms stabilized in aggregates of krypton–nitrogen nanoclusters immersed in superfluid helium
topic К 75-летию Л.П. Межова-Деглина
topic_facet К 75-летию Л.П. Межова-Деглина
url https://nasplib.isofts.kiev.ua/handle/123456789/117923
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AT khmelenkovv esrstudiesofnitrogenatomsstabilizedinaggregatesofkryptonnitrogennanoclustersimmersedinsuperfluidhelium
AT leedm esrstudiesofnitrogenatomsstabilizedinaggregatesofkryptonnitrogennanoclustersimmersedinsuperfluidhelium