Nonlinear optical response of the nematic liquid crystal doped with polymer-azo-dye complex under picosecond laser pulses excitation
The nonlinear optical (NLO) response of the heterosystem based on nematic liquid crystal (LC) with incorporated polymer-azo-dye complex (PADC) was studied within the self-action of picosecond laser pulses at 532 nm. It was shown the enhancement of the refractive NLO response efficiency up to 20 % at...
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| Date: | 2015 |
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НТК «Інститут монокристалів» НАН України
2015
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| Cite this: | Nonlinear optical response of the nematic liquid crystal doped with polymer-azo-dye complex under picosecond laser pulses excitation/ A.V.Uklein, E.V.Ouskova, V.Ya.Gayvoronsky// Functional Materials. — 2015. — Т. 22, № 1. — С. 20-26. — Бібліогр.: 17 назв. — англ. |
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Uklein, A.V. Ouskova, E.V. Gayvoronsky, V.Ya. 2017-06-04T13:47:42Z 2017-06-04T13:47:42Z 2015 Nonlinear optical response of the nematic liquid crystal doped with polymer-azo-dye complex under picosecond laser pulses excitation/ A.V.Uklein, E.V.Ouskova, V.Ya.Gayvoronsky// Functional Materials. — 2015. — Т. 22, № 1. — С. 20-26. — Бібліогр.: 17 назв. — англ. 1027-5495 DOI: http://dx.doi.org/10.15407/fm22.01.020 https://nasplib.isofts.kiev.ua/handle/123456789/119113 The nonlinear optical (NLO) response of the heterosystem based on nematic liquid crystal (LC) with incorporated polymer-azo-dye complex (PADC) was studied within the self-action of picosecond laser pulses at 532 nm. It was shown the enhancement of the refractive NLO response efficiency up to 20 % at lower excitation level (0.5-20 MW/cm2) and up to 5 times at higher excitation level (20-600 MW/cm2) for the PADC doped LC versus the components response and conventional azo-dye doped LC. The manifestation of three photoinduced mechanisms was observed with the rise of the PADC concentration in LC matrix: 1) orientation of the PADC; 2) trans-cis-trans isomerization; 3) cooperative response/aggregation effect. Each mechanism defines the heterosystem NLO response at corresponding PADC concentration range. The proposed smart material is promising for photonic application due to NLO properties control with variation of the PADC concentration. en НТК «Інститут монокристалів» НАН України Functional Materials Characterization and properties Nonlinear optical response of the nematic liquid crystal doped with polymer-azo-dye complex under picosecond laser pulses excitation Article published earlier |
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Digital Library of Periodicals of National Academy of Sciences of Ukraine |
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| title |
Nonlinear optical response of the nematic liquid crystal doped with polymer-azo-dye complex under picosecond laser pulses excitation |
| spellingShingle |
Nonlinear optical response of the nematic liquid crystal doped with polymer-azo-dye complex under picosecond laser pulses excitation Uklein, A.V. Ouskova, E.V. Gayvoronsky, V.Ya. Characterization and properties |
| title_short |
Nonlinear optical response of the nematic liquid crystal doped with polymer-azo-dye complex under picosecond laser pulses excitation |
| title_full |
Nonlinear optical response of the nematic liquid crystal doped with polymer-azo-dye complex under picosecond laser pulses excitation |
| title_fullStr |
Nonlinear optical response of the nematic liquid crystal doped with polymer-azo-dye complex under picosecond laser pulses excitation |
| title_full_unstemmed |
Nonlinear optical response of the nematic liquid crystal doped with polymer-azo-dye complex under picosecond laser pulses excitation |
| title_sort |
nonlinear optical response of the nematic liquid crystal doped with polymer-azo-dye complex under picosecond laser pulses excitation |
| author |
Uklein, A.V. Ouskova, E.V. Gayvoronsky, V.Ya. |
| author_facet |
Uklein, A.V. Ouskova, E.V. Gayvoronsky, V.Ya. |
| topic |
Characterization and properties |
| topic_facet |
Characterization and properties |
| publishDate |
2015 |
| language |
English |
| container_title |
Functional Materials |
| publisher |
НТК «Інститут монокристалів» НАН України |
| format |
Article |
| description |
The nonlinear optical (NLO) response of the heterosystem based on nematic liquid crystal (LC) with incorporated polymer-azo-dye complex (PADC) was studied within the self-action of picosecond laser pulses at 532 nm. It was shown the enhancement of the refractive NLO response efficiency up to 20 % at lower excitation level (0.5-20 MW/cm2) and up to 5 times at higher excitation level (20-600 MW/cm2) for the PADC doped LC versus the components response and conventional azo-dye doped LC. The manifestation of three photoinduced mechanisms was observed with the rise of the PADC concentration in LC matrix: 1) orientation of the PADC; 2) trans-cis-trans isomerization; 3) cooperative response/aggregation effect. Each mechanism defines the heterosystem NLO response at corresponding PADC concentration range. The proposed smart material is promising for photonic application due to NLO properties control with variation of the PADC concentration.
|
| issn |
1027-5495 |
| url |
https://nasplib.isofts.kiev.ua/handle/123456789/119113 |
| citation_txt |
Nonlinear optical response of the nematic liquid crystal doped with polymer-azo-dye complex under picosecond laser pulses excitation/ A.V.Uklein, E.V.Ouskova, V.Ya.Gayvoronsky// Functional Materials. — 2015. — Т. 22, № 1. — С. 20-26. — Бібліогр.: 17 назв. — англ. |
| work_keys_str_mv |
AT ukleinav nonlinearopticalresponseofthenematicliquidcrystaldopedwithpolymerazodyecomplexunderpicosecondlaserpulsesexcitation AT ouskovaev nonlinearopticalresponseofthenematicliquidcrystaldopedwithpolymerazodyecomplexunderpicosecondlaserpulsesexcitation AT gayvoronskyvya nonlinearopticalresponseofthenematicliquidcrystaldopedwithpolymerazodyecomplexunderpicosecondlaserpulsesexcitation |
| first_indexed |
2025-12-07T16:19:39Z |
| last_indexed |
2025-12-07T16:19:39Z |
| _version_ |
1850867061321891840 |