Resonance generation of sum harmonic in static electric field

Using the group theory considerations, we investigate the nonlinear effect tensor (NET) for a crystal in a static electric field when a harmonic or the initial emission frequency approaches that of the excitonic absorption band. The dependence of additional terms in NET (resulting from the electric...

Ausführliche Beschreibung

Gespeichert in:
Bibliographische Detailangaben
Veröffentlicht in:Semiconductor Physics Quantum Electronics & Optoelectronics
Datum:1999
Hauptverfasser: Venger, E.F., Griban, V.M., Melnichuk, A.V.
Format: Artikel
Sprache:English
Veröffentlicht: Інститут фізики напівпровідників імені В.Є. Лашкарьова НАН України 1999
Online Zugang:https://nasplib.isofts.kiev.ua/handle/123456789/119876
Tags: Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
Назва журналу:Digital Library of Periodicals of National Academy of Sciences of Ukraine
Zitieren:Resonance generation of sum harmonic in static electric field / E.F. Venger, V.M. Griban, A.V. Melnichuk // Semiconductor Physics Quantum Electronics & Optoelectronics. — 1999. — Т. 2, № 3. — С. 98-102. — Бібліогр.: 4 назв. — англ.

Institution

Digital Library of Periodicals of National Academy of Sciences of Ukraine
id nasplib_isofts_kiev_ua-123456789-119876
record_format dspace
spelling Venger, E.F.
Griban, V.M.
Melnichuk, A.V.
2017-06-10T08:08:17Z
2017-06-10T08:08:17Z
1999
Resonance generation of sum harmonic in static electric field / E.F. Venger, V.M. Griban, A.V. Melnichuk // Semiconductor Physics Quantum Electronics & Optoelectronics. — 1999. — Т. 2, № 3. — С. 98-102. — Бібліогр.: 4 назв. — англ.
1560-8034
PACS: 78.20.Jq
https://nasplib.isofts.kiev.ua/handle/123456789/119876
Using the group theory considerations, we investigate the nonlinear effect tensor (NET) for a crystal in a static electric field when a harmonic or the initial emission frequency approaches that of the excitonic absorption band. The dependence of additional terms in NET (resulting from the electric field applied) on the electric field components is found. Their form is shown to differ from that of usual NET. The results obtained are illustrated by considering the case of the D₂d crystal symmetry.
en
Інститут фізики напівпровідників імені В.Є. Лашкарьова НАН України
Semiconductor Physics Quantum Electronics & Optoelectronics
Resonance generation of sum harmonic in static electric field
Article
published earlier
institution Digital Library of Periodicals of National Academy of Sciences of Ukraine
collection DSpace DC
title Resonance generation of sum harmonic in static electric field
spellingShingle Resonance generation of sum harmonic in static electric field
Venger, E.F.
Griban, V.M.
Melnichuk, A.V.
title_short Resonance generation of sum harmonic in static electric field
title_full Resonance generation of sum harmonic in static electric field
title_fullStr Resonance generation of sum harmonic in static electric field
title_full_unstemmed Resonance generation of sum harmonic in static electric field
title_sort resonance generation of sum harmonic in static electric field
author Venger, E.F.
Griban, V.M.
Melnichuk, A.V.
author_facet Venger, E.F.
Griban, V.M.
Melnichuk, A.V.
publishDate 1999
language English
container_title Semiconductor Physics Quantum Electronics & Optoelectronics
publisher Інститут фізики напівпровідників імені В.Є. Лашкарьова НАН України
format Article
description Using the group theory considerations, we investigate the nonlinear effect tensor (NET) for a crystal in a static electric field when a harmonic or the initial emission frequency approaches that of the excitonic absorption band. The dependence of additional terms in NET (resulting from the electric field applied) on the electric field components is found. Their form is shown to differ from that of usual NET. The results obtained are illustrated by considering the case of the D₂d crystal symmetry.
issn 1560-8034
url https://nasplib.isofts.kiev.ua/handle/123456789/119876
citation_txt Resonance generation of sum harmonic in static electric field / E.F. Venger, V.M. Griban, A.V. Melnichuk // Semiconductor Physics Quantum Electronics & Optoelectronics. — 1999. — Т. 2, № 3. — С. 98-102. — Бібліогр.: 4 назв. — англ.
work_keys_str_mv AT vengeref resonancegenerationofsumharmonicinstaticelectricfield
AT gribanvm resonancegenerationofsumharmonicinstaticelectricfield
AT melnichukav resonancegenerationofsumharmonicinstaticelectricfield
first_indexed 2025-11-25T23:28:33Z
last_indexed 2025-11-25T23:28:33Z
_version_ 1850581058795339776
fulltext 98 © 1999, Institute of Semiconductor Physics, National Academy of Sciences of Ukraine Semiconductor Physics, Quantum Electronics & Optoelectronics. 1999. V. 2, N 3. P. 98-102. 1. Introduction The sum harmonic generation is among the nonlinear opti- cal effects in crystals. It involves emission at a sum fre- quency, ω1(k1) + ω2(k2), due to emission at frequencies ω1(k1) and ω2(k2). The well -known frequency doubling, i.e. the second harmonic generation, is a special case of the above effect. When theoretically investigating the sum harmonic gen- eration, it is convenient to use the nonlinear effect tensor (NET) α. NET is a factor in the expression for the matrix element corresponding to an elementary act of the above process. The generation intensity is proportional to the NET modulus squared. The NET α form was determined in the paper [1] using the polariton theory. The latter takes into account the retardation of interaction. This enables one to correctly analyze resonance phenomena that occur when an emission frequency approaches the excitonic absorption band fre- quency. The NET form in crystals of various symmetries was also investigated in the above paper. Using the technique developed in the paper [1], one of the authors of the present paper has found the NET form for crystals in a static electric field E [2]. It was shown that the effect of the electric field results in appearance of an additional term α(E) in the NET α. The form of this addi- tional term, α(E), differs from that of α. This means that, at PACS: 78.20.Jq Resonance generation of sum harmonic in static electric field E.F. Venger*, V.M. Griban, A.V. Melnichuk *Institute of Semiconductor Physics, NAS of Ukraine, 45, prospekt Nauki, Kyiv, 252028, Ukraine Phone: (38044) 265 25 93; Fax: (38044) 265 83 42; E-mail: mickle@semicond.kiev.ua Mykola Gogol State Pedagogic University, 2 Kropyv�yans�kogo Str., Nizhin, 251200, Ukraine Abstract. Using the group theory considerations, we investigate the nonlinear effect tensor (NET) for a crystal in a static electric field when a harmonic or the initial emission frequency approaches that of the excitonic absorption band. The dependence of additional terms in NET (resulting from the electric field applied) on the electric field components is found. Their form is shown to differ from that of usual NET. The results obtained are illustrated by considering the case of the D2d crystal symmetry. Keywords: sum harmonic, nonlinear effect tensor, group theory considerations. Paper received 29.01.99; revised manuscript received 01.06.99; accepted for publication 11.10.99. some emission polarization, the harmonic generation is due to the field action only. The tensor α(E) was found in the first order of the per- turbation theory, so in general case the intensity of the sum harmonic generation due to it has to be much less than that due to the tensor α. The tensor α(E), however, has resonance terms in denominators. This means that, when an emission frequency approaches the resonance, the effect of an elec- tric field is to grow abruptly. Hence it follows that in the case of the resonance it is of both interest and importance to study the structure of the tensor α(E) and its transformation properties. The same is also true for the dependence of the tensor α(E) form on the symmetry type of the exciton state whose frequency is resonant. It is the above problems the present paper deals with. 2. Results and discussion Let us give, first of all, the explicit form of the tensor α(E). According to the paper [2], it is a product of the vec- tor E and a tensor β of rank four: ∑= i ijjjijjj E .2121 )( βα E (1) The tensor β has 16 rather complicated components. For the following analysis it will be sufficient to give ex- plicitly only one of them: E.F. Venger et al.: Resonance generation of sum harmonic... 99SQO, 2(3), 1999 [ ]∑     × − −= ',',, '2 2,22 21 2 21 )'()( )',')(','0( k kk kkk µµµ µµ µµµ β EE pj N i ijjj [ ][ ] . )()()( )0,)(,,( 212122 211211122 12     ⋅⋅⋅+ +−+− ++ × ωωω µµµ µµ hh kkk kkkkk EE jj (2) Here N is the number of crystal unit cells; Εµ(k), |µ, k) are, respectively, the energy and wave function of a Coulomb exciton with wave vector k that belongs to the µ-th band; |0) is the wave function for the ground state of the crystal; j, j1, j2 index the projections of polarization vectors for the harmonic and initial emission (they may take the values x, y, z); pi(i = x, y, z) is the i-th component of the electric dipole moment for a unit cell; (µ1, k1|jn| µ2, k2) is the matrix element of the operator nj I m e (where e, m, I are, respectively, the electron charge, mass and momentum operator). The other terms in expression (2) differ from the above one by the place of the matrix element for the component pi and the differences (sums) in the denominators. The frequencies ω1 and ω2 can be considered as interchangeable, i.e., the right hand side of expression (2) is symmetric about interchang- ing the indices 1 and 2. The form of the tensor α(E) depends on that of the ten- sor β. When determining the latter form, one has to keep in mind that the exciton states |µ, k) are classified according to the irreducible representations of the point group of crystal symmetry, while the expressions of the type . )( ,)(,∑ ±µ µ µ ω µ hk kk E transform according to the entire symmetry representations [2]. So it follows from expression (2) that the tensor β is isomorphic to (jj1j2i)0: 02121 )( ijjjijjj →β . (3) Here index 0 means that the product of coordinates, jj1j2i, is projected onto the entire symmetry representation of the point symmetry group. Basing on expression (3), the form of the tensor α(E) was determined in the paper [2] for crystals of various symmetries. Now let us consider the form of the tensor α(E) when the sum frequency, ω1 + ω2, approaches the excitonic band absorption frequency, 1/h ⋅Εµ(k1+ k2). (The case h (ω1+ ω2) = Εµ(k1+ k2) is, however, excluded. Such a two-photon absorption will be considered elsewhere.) First of all, it should be noted that generally the terms with different µ1 make different contributions to different components of tensor β, depending on the |µ1, k1 + k2) state symmetry. To demonstrate this, let us separate out those terms in expression (2) for which µ1 = µ: [ ]∑     × − −= ',', '2 2,22)( 2 2 21 )'()( )',')(','0( k kk kkk µµ µµ µ µµµ β EE pj N i ijjj [ ][ ] . )()()( )0,)(,,( 212122 2121122 2     ⋅⋅⋅+ +−+− ++ × ωωω µµµ µµ hh kkk kkkkk EE jj (4) There is no summation over µ here, and hence the quantity [ ].)()( ,)(, 2121 2121 ωω µµ µ +−+ ++ hkk kkkk E is not of full symmetry. This means that the term given in an explicit form in (4) is isomorphic not to (jj1j2i)0 but to the product (j2ij1)µ(j)µ where index µ signifies projection onto the irreducible representation to which the |µ1, k1 + k2) state belongs. An analysis made for the rest of terms in (4) (denoted by dots) shows that tensor β(µ) is isomorphic to the following sum: .)()()()( 2112 )( 21 µµµµ µβ jjijijjjijjj +→ (5) After summing over µ one gets the relation (3) (as it was to be expected). Identifying the index µ with designation of the corre- sponding irreducible representation, one can determine the factors in the right-hand side of expression (5) and obtain first the tensor β(µ) and then the tensor α(µ)(E): .)( )()( 2121 ∑= i ijjjijjj E µµ βα E (6) After summing the corresponding tensor α(µ)(E) components over all the irreducible representations, one can get the tensor α(E). Its form is to be the same as that fol- lowing from expression (3). Now let us return to the resonance conditions when h (ω1+ ω2)→Εµ(k1+ k2). In this case the terms in β(µ) with µ = µ1 will prevail. As a result, the components α(µ)(E) of the tensor α(E) will prevail. Thus under resonance conditions one can write down: ( ) ( ) ( ) ( ) ( ) ( ) ( ) ( ) ( ) ( ) β β β β α α α α µ µ µ µ µ µ µ µ µ µ µµ = = + = = + ∑ ∑ ∑∑ ≠ ≠ 1 1 1 1 1 1 11 , .E E E E According to the above considerations, the non- resonance components may be neglected and therefore α(E) ≈ α(µ)(E). This means that under resonance conditions the tensor α(E) retains its form; α(µ)(E), however, become the governing components. Similar reasoning was used in paper [3] to analyze the Raman scattering tensor under resonance conditions. E.F. Venger et al.: Resonance generation of sum harmonic... 100 SQO, 2(3), 1999 To illustrate the above results, let us consider a crystal of D2d symmetry. For it the usual NET has the following non-zero components: αxyz = αxzy = αyxz = αyzx, αzxy = αzyx. In a static electric field the tensor α(E) appears whose form follows from expression (3). It is given in Table 2 - see the row designated by µ ∑ . Let us determine the tensor α(µ)(E). The D2d group has four one-dimensional (1D) irreducible representations, A1, A2, B1, B2, and a 2D irreducible representation, E, with two rows, E(x) and E(y), after which the coordinates x, y trans- form. Using expression (5), one can find the form of the ten- sor β(µ). To this end one has to determine the irreducible representations of the D2d group after which the coordinates x, y, z, as well as their double and triple products, trans- form. The corresponding technique is discussed in the pa- pers [3,4]. The results of our calculations are given in Table 1. Let us consider the case µ = A1, i.e. the wave function of the intermediate state, |µ1, k1+k2), corresponds to the irreducible representation A1. One can conclude from Table 1 that projections of coordinates x, y, z onto the representation A1 are zero. Therefore, the first term in the right-hand side of expression (5) drops out. For the second term the non-zero projections of double products are (x1x2)A1 = (y1y2)A1 and (z1z2)A1. Thus, according to expression (5), the non-zero components of the tensor β(µ) are the following: 1 )1()1()1( aA yyxx A xxyy A xxxx === βββ , 2 )1( aA zzzz =β , 3 )1()1( aA yyzz A xxzz == ββ , 4 )1()1( aA zzyy A zzxx == ββ . (7) Thereafter, using (6), one can determine the form of the tensor ( )E)( 1Aα : xEaA xxx 1)()1( =Eα , yEaA yyy 1)()1( =Eα , zEaA zzz 2)()1( =Eα , yEaA yxx 1)()1( =Eα , xEaA xyy 1)()1( =Eα , zEaA zxx 3)()1( =Eα , z A zyy Ea3 )( )(1 =Eα , xEaA xzz 4)()1( =Eα , yEaA yzz 4)()1( =Eα . (8) All the other components are zero. The same procedure can be used to find the tensor α(µ)(E) components for other irreducible representations of the D2d group. The corresponding results are given in Table 2. (There the numbers 1, 2, ... are used instead of a1, a2, ..., and the relations between components correspond to the only representation.) After performing summation of the corresponding components over all the irreducible representations, one can obtain the tensor form in the case when there is no resonance (it is given in the row designated with ∑ µ ). Now let us consider the case when the frequency ω2 approaches the frequency of the excitonic absorption band. One can show that an isomorphism at the initial emission frequency follows from expression (2): .)()()()( 1212 )( 21 µµµµ µβ jijjjjjjijjj +→ (9) If µ = A2, then, basing on expressions (9) and (1) and Table 1, we get: yEaA xyx 1)()2( =Eα , yEaA yxx 1)()2( −=Eα , xEaA yxy 1)()2( =Eα , xEaA xyy 1)()2( −=Eα . (10) All the other components are zero. The form of the tensor α(µ)(E) in this case is given in Table 3. This tensor is non-symmetric in respect to the indi- ces j1, j2, because there is no symmetry now between the frequencies ω1 and ω2: ω2 is the resonance frequency, while ω1 is not. When the resonance occurs at a frequency ω1, then one has to interchange the components )( 21 µα jjj and )( 12 µα jjj in Table 3. If frequency is doubled (ω1 = ω2 = ω), then one has to take )()( 1221 µµ αα jjjjjj = . µ Coordinates and their products A1 x1x2 + y1y2 z1z2 x1y2z3 + y1x2z3 x1z2y3+ y1z2x3 z1x2y3 + z1y2x3 A2 x1y2 - y1x2 x1x2z3 - y1y2z3 x1z2x3 - y1z2y3 z1x2x3 - z1y2y3 B1 x1x2 - y1y2 x1y2z3 - y1x2z3 x1z2y3 - y1z2x3 z1x2y3 - z1y2x3 B2 z z1z2z3 x1x2z3 + y1y2z3 x1z2x3 + y1z2y3 z1x2x3 + z1y2y3 E(x) x y1z2 z1y2 x1x2x3 y1y2x3 y1x2y3 x1y2y3 z1z2x3 z1x2z3 x1z2z3 E(y) y x1z2 z1x2 y1y2y3 x1x2y3 x1y2x3 y1x2x3 z1z2y3 z1y2z3 y1z2z3 Table 1. Coordinates and their products that transform according to the irreducible representations of the D2d group. E.F. Venger et al.: Resonance generation of sum harmonic... 101SQO, 2(3), 1999 jj 1j2 µ xxx yyy zzz xxz xzx zxx zzy zyz yzz xxy xyx yxx yyz yzy zyy xyz xzy zxy yyx yxy xyy zzx zxz xzz yxz yzx zyx 1Ex 1Ey 2Ez 0 0 3Ez 0 0 4Ez A1 0 0 1Ey 0 0 3Ez 0 0 0 0 0 1Ex 0 0 4Ex 0 0 0 0 0 4Ey 0 0 0 0 0 0 A2 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 1Ex 1Ey 0 0 0 0 0 0 0 B1 0 0 -1Ey 0 0 0 0 0 0 0 0 -1Ex 0 0 0 0 0 0 0 0 1Ez 0 0 3Ez 4Ey 4Ey 0 B2 2Ey 2Ey 0 0 0 3Ez 0 0 0 2Ex 2Ex 0 4Ex 4Ex 0 0 0 0 1Ex 0 0 4Ez 4Ez 0 7Ey 7Ey 0 E(x) 2Ey 2Ey 0 5Ez 5Ez 0 0 0 0 0 0 3Ex 0 0 6Ex 0 0 0 0 1Ey 0 4Ez 4Ez 0 0 0 7Ey E(y) 0 0 2Ey 5Ez 5Ez 0 0 0 0 3Ex 3Ex 0 6Ex 6Ex 0 0 0 0 1Ex 2Ey 3Ez 8Ez 8Ez 9Ez 14Ey 14Ey 15Ey ∑ µ 4Ey 6Ex 4Ey 6Ex 5Ey 7Ex 10Ez 12Ex 10Ez 12Ex 11Ez 13Ex 0 0 0 0 0 0 Table 3. Form of the tensor α(µ)(E) for the resonance frequency ω2. µ jj 1j2 xxx yyy zzz xxz xzx zxx zzy zyz yzz xxy xyx yxx yyz yzy zyy xyz xzy zxy yyx yxy xyy zzx zxz xzz yxz yzx zyx 1Ex 1Ey 2Ez 0 3Ez 0 0 0 0 A1 0 1Ey 0 0 3Ez 0 0 0 0 0 1Ex 0 0 4Ex 0 0 0 0 0 0 0 0 0 0 0 0 0 A2 1Ey 0 -1Ey 0 0 0 0 0 0 1Ex 0 -1Ex 0 0 0 0 0 0 1Ex 1Ey 0 0 0 0 0 0 0 B1 0 -1Ey 0 0 0 0 0 0 0 0 -1Ex 0 0 0 0 0 0 0 0 0 1Ez 0 3Ez 0 4Ey 0 5Ey B2 2Ey 0 0 0 3Ez 0 0 0 0 2Ex 0 0 4Ex 0 5Ex 0 0 0 1Ex 0 0 5Ez 0 6Ez 10Ey 0 11Ey E(x) 2Ey 0 3Ey 7Ez 0 8Ez 0 0 0 0 4Ex 0 0 9Ex 0 0 0 0 0 1Ey 0 5Ez 0 6Ez 0 11Ey 0 E(y) 0 2Ey 0 7Ez 0 8Ez 0 0 0 3Ex 0 4Ex 9Ex 0 10Ex 0 0 0 Table 2. Form of the tensor α(µ)(E) for the resonance frequency ω1 +ω2. E.F. Venger et al.: Resonance generation of sum harmonic... 102 SQO, 2(3), 1999 3. Conclusions From the above results it follows that, under the resonance generation of the sum harmonic in a static electric field, the nonlinear effect tensor involves a term α(µ)(E) that depends on both the field E and the symmetry type of the exciton state whose frequency is the resonance one. The form of the tensor α(µ)(E) differs from that of the non-resonance nonlinear effect tensor. Besides, it is different at the fre- quencies of the harmonic and initial emission. References 1. L.N. Ovander, Nonlinear optical effects in crystals // Uspekhi Fiz. Nauk 86 (1), pp. 1-39 (1965) (in Russian). 2. V.M. Griban, On sum harmonic generation in crystals with inversion center (in Russian) // Izv. Vuzov SSSR. Fizika N 6, pp.107-110 (1969). 3. L.D. Landau, E.M. Lifshits, Quantum Mechanics, Nauka, Moscow, p.443 (1989) (in Russian). 4. M.I. Petrashen, E.D. Trifonov, Group Theory Applications in Quantum Mechanics, Nauka, Moscow (1967) (in Russian).