Spectroscopy of nanosized composites silicon-organic polymer/nanoporous silicas

Fluorescence and excitation spectra (T = 5–290 K) of nanosized silicon–organic polymers poly(di-n-hexylsilane) and poly(methyl(phenyl)silane) incorporated into porous silica materials MCM-41 and SBA-15 have been studied with varying pore diameter from 2.8 to 10 nm. The controlled variation of the...

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Veröffentlicht in:Физика низких температур
Datum:2006
Hauptverfasser: Ostapenko, N., Kozlova, N., Suto, S., Watanabe, A.
Format: Artikel
Sprache:English
Veröffentlicht: Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України 2006
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Online Zugang:https://nasplib.isofts.kiev.ua/handle/123456789/120881
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Назва журналу:Digital Library of Periodicals of National Academy of Sciences of Ukraine
Zitieren:Spectroscopy of nanosized composites silicon-organic polymer/nanoporous silicas / N. Ostapenko, N. Kozlova, S. Suto, A. Watanabe // Физика низких температур. — 2006. — Т. 32, № 11. — С. 1363–1371. — Бібліогр.: 18 назв. — англ.

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Digital Library of Periodicals of National Academy of Sciences of Ukraine
id nasplib_isofts_kiev_ua-123456789-120881
record_format dspace
spelling Ostapenko, N.
Kozlova, N.
Suto, S.
Watanabe, A.
2017-06-13T08:55:05Z
2017-06-13T08:55:05Z
2006
Spectroscopy of nanosized composites silicon-organic polymer/nanoporous silicas / N. Ostapenko, N. Kozlova, S. Suto, A. Watanabe // Физика низких температур. — 2006. — Т. 32, № 11. — С. 1363–1371. — Бібліогр.: 18 назв. — англ.
0132-6414
PACS: 78.55.Qr, 79.60.Jv
https://nasplib.isofts.kiev.ua/handle/123456789/120881
Fluorescence and excitation spectra (T = 5–290 K) of nanosized silicon–organic polymers poly(di-n-hexylsilane) and poly(methyl(phenyl)silane) incorporated into porous silica materials MCM-41 and SBA-15 have been studied with varying pore diameter from 2.8 to 10 nm. The controlled variation of the pore diameter in the wide range (2.8–10 nm) permitted us, for the first time, to investigate the optical properties of the polymers on their transition from isolated macromolecules to a film. It is found that this transition depends on polymer type and occurs via the formation of new spatially independent structures of the polymers not observed in the spectra of the film, namely, via the formation of disordered and (or) ordered conformations of polymer chains and clusters.
We gratefully acknowledge Dr. G. Telbiz for preparation of the specimens used. The work was partially supported by the Ministry of Education and Science, grant No. M/128-2005.
en
Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України
Физика низких температур
Molecular Solids
Spectroscopy of nanosized composites silicon-organic polymer/nanoporous silicas
Article
published earlier
institution Digital Library of Periodicals of National Academy of Sciences of Ukraine
collection DSpace DC
title Spectroscopy of nanosized composites silicon-organic polymer/nanoporous silicas
spellingShingle Spectroscopy of nanosized composites silicon-organic polymer/nanoporous silicas
Ostapenko, N.
Kozlova, N.
Suto, S.
Watanabe, A.
Molecular Solids
title_short Spectroscopy of nanosized composites silicon-organic polymer/nanoporous silicas
title_full Spectroscopy of nanosized composites silicon-organic polymer/nanoporous silicas
title_fullStr Spectroscopy of nanosized composites silicon-organic polymer/nanoporous silicas
title_full_unstemmed Spectroscopy of nanosized composites silicon-organic polymer/nanoporous silicas
title_sort spectroscopy of nanosized composites silicon-organic polymer/nanoporous silicas
author Ostapenko, N.
Kozlova, N.
Suto, S.
Watanabe, A.
author_facet Ostapenko, N.
Kozlova, N.
Suto, S.
Watanabe, A.
topic Molecular Solids
topic_facet Molecular Solids
publishDate 2006
language English
container_title Физика низких температур
publisher Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України
format Article
description Fluorescence and excitation spectra (T = 5–290 K) of nanosized silicon–organic polymers poly(di-n-hexylsilane) and poly(methyl(phenyl)silane) incorporated into porous silica materials MCM-41 and SBA-15 have been studied with varying pore diameter from 2.8 to 10 nm. The controlled variation of the pore diameter in the wide range (2.8–10 nm) permitted us, for the first time, to investigate the optical properties of the polymers on their transition from isolated macromolecules to a film. It is found that this transition depends on polymer type and occurs via the formation of new spatially independent structures of the polymers not observed in the spectra of the film, namely, via the formation of disordered and (or) ordered conformations of polymer chains and clusters.
issn 0132-6414
url https://nasplib.isofts.kiev.ua/handle/123456789/120881
citation_txt Spectroscopy of nanosized composites silicon-organic polymer/nanoporous silicas / N. Ostapenko, N. Kozlova, S. Suto, A. Watanabe // Физика низких температур. — 2006. — Т. 32, № 11. — С. 1363–1371. — Бібліогр.: 18 назв. — англ.
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AT kozlovan spectroscopyofnanosizedcompositessiliconorganicpolymernanoporoussilicas
AT sutos spectroscopyofnanosizedcompositessiliconorganicpolymernanoporoussilicas
AT watanabea spectroscopyofnanosizedcompositessiliconorganicpolymernanoporoussilicas
first_indexed 2025-11-30T10:07:45Z
last_indexed 2025-11-30T10:07:45Z
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