Intercalation of fullerite C₆₀ with N₂ molecules. An investigation by x-ray powder diffraction

The lattice parameter a of fullerite C₆₀ intercalated with N₂ molecules is investigated in the temperature interval 6–295 K by x-ray diffraction. It is found that the interstitial molecular N₂ has a considerable effect on both the temperatures, Tc of the orientational phase transition and Tg of...

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Published in:Физика низких температур
Date:2007
Main Authors: Galtsov, N.N., Prokhvatilov, A.I., Dolgova, G.N., Cassidy, D., Gadd, G.E., Moricca, S., Sundqvist, B.
Format: Article
Language:English
Published: Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України 2007
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Online Access:https://nasplib.isofts.kiev.ua/handle/123456789/120957
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Journal Title:Digital Library of Periodicals of National Academy of Sciences of Ukraine
Cite this:Intercalation of fullerite C₆₀ with N₂ molecules. An investigation by x-ray powder diffraction / N.N. Galtsov, A.I. Prokhvatilov, G.N. Dolgova, D. Cassidy, G.E. Gadd, S. Moricca, B. Sundqvist // Физика низких температур. — 2007. — Т. 33, № 10. — С. 1159–1165. — Бібліогр.: 37 назв. — англ.

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Digital Library of Periodicals of National Academy of Sciences of Ukraine
id nasplib_isofts_kiev_ua-123456789-120957
record_format dspace
spelling Galtsov, N.N.
Prokhvatilov, A.I.
Dolgova, G.N.
Cassidy, D.
Gadd, G.E.
Moricca, S.
Sundqvist, B.
2017-06-13T11:02:42Z
2017-06-13T11:02:42Z
2007
Intercalation of fullerite C₆₀ with N₂ molecules. An investigation by x-ray powder diffraction / N.N. Galtsov, A.I. Prokhvatilov, G.N. Dolgova, D. Cassidy, G.E. Gadd, S. Moricca, B. Sundqvist // Физика низких температур. — 2007. — Т. 33, № 10. — С. 1159–1165. — Бібліогр.: 37 назв. — англ.
0132-6414
PACS: 61.10.Nz, 81.05.Tp, 64.70.–p
https://nasplib.isofts.kiev.ua/handle/123456789/120957
The lattice parameter a of fullerite C₆₀ intercalated with N₂ molecules is investigated in the temperature interval 6–295 K by x-ray diffraction. It is found that the interstitial molecular N₂ has a considerable effect on both the temperatures, Tc of the orientational phase transition and Tg of the orientational glass formation. Hysteresis of a(T) has been detected in the Tc and Tg regions, besides, the abrupt change in the volume over the region defining Tc. Complete intercalation of C₆₀ with N₂ molecules results in a 0.2% increase in the lattice parameter, which persists over the whole temperature range. Evidence is also obtained that the interstitial guest molecular N₂ induces a slight deformation of the cubic symmetry of the host C₆₀ lattice.
The authors are indebted to M.A. Strzhemechny for helpful discussions at every stage of the investigation and helpful advice in the course of the paper preparation and to T.Yu. Shcherban’ for help in carrying out the experiments. The study was partially supported by the International STCU Foundation, Grant ¹ 2669.
en
Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України
Физика низких температур
Динамика кристаллической решетки
Intercalation of fullerite C₆₀ with N₂ molecules. An investigation by x-ray powder diffraction
Article
published earlier
institution Digital Library of Periodicals of National Academy of Sciences of Ukraine
collection DSpace DC
title Intercalation of fullerite C₆₀ with N₂ molecules. An investigation by x-ray powder diffraction
spellingShingle Intercalation of fullerite C₆₀ with N₂ molecules. An investigation by x-ray powder diffraction
Galtsov, N.N.
Prokhvatilov, A.I.
Dolgova, G.N.
Cassidy, D.
Gadd, G.E.
Moricca, S.
Sundqvist, B.
Динамика кристаллической решетки
title_short Intercalation of fullerite C₆₀ with N₂ molecules. An investigation by x-ray powder diffraction
title_full Intercalation of fullerite C₆₀ with N₂ molecules. An investigation by x-ray powder diffraction
title_fullStr Intercalation of fullerite C₆₀ with N₂ molecules. An investigation by x-ray powder diffraction
title_full_unstemmed Intercalation of fullerite C₆₀ with N₂ molecules. An investigation by x-ray powder diffraction
title_sort intercalation of fullerite c₆₀ with n₂ molecules. an investigation by x-ray powder diffraction
author Galtsov, N.N.
Prokhvatilov, A.I.
Dolgova, G.N.
Cassidy, D.
Gadd, G.E.
Moricca, S.
Sundqvist, B.
author_facet Galtsov, N.N.
Prokhvatilov, A.I.
Dolgova, G.N.
Cassidy, D.
Gadd, G.E.
Moricca, S.
Sundqvist, B.
topic Динамика кристаллической решетки
topic_facet Динамика кристаллической решетки
publishDate 2007
language English
container_title Физика низких температур
publisher Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України
format Article
description The lattice parameter a of fullerite C₆₀ intercalated with N₂ molecules is investigated in the temperature interval 6–295 K by x-ray diffraction. It is found that the interstitial molecular N₂ has a considerable effect on both the temperatures, Tc of the orientational phase transition and Tg of the orientational glass formation. Hysteresis of a(T) has been detected in the Tc and Tg regions, besides, the abrupt change in the volume over the region defining Tc. Complete intercalation of C₆₀ with N₂ molecules results in a 0.2% increase in the lattice parameter, which persists over the whole temperature range. Evidence is also obtained that the interstitial guest molecular N₂ induces a slight deformation of the cubic symmetry of the host C₆₀ lattice.
issn 0132-6414
url https://nasplib.isofts.kiev.ua/handle/123456789/120957
citation_txt Intercalation of fullerite C₆₀ with N₂ molecules. An investigation by x-ray powder diffraction / N.N. Galtsov, A.I. Prokhvatilov, G.N. Dolgova, D. Cassidy, G.E. Gadd, S. Moricca, B. Sundqvist // Физика низких температур. — 2007. — Т. 33, № 10. — С. 1159–1165. — Бібліогр.: 37 назв. — англ.
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