Heat transfer in crystalline clathrate hydrates at low temperatures

The experimental results on the thermal conductivity k(T) of crystalline Xe, CH₄, and THF clathrate hydrates have been analyzed. In a wide region of temperatures above 2 K, k(T) exhibits a behavior typical of disordered solids, which depends weakly on their chemical composition, crystalline struct...

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Veröffentlicht in:Физика низких температур
Datum:2007
Hauptverfasser: Krivchikov, A.I., Korolyuk, O.A., Romantsova, O.O.
Format: Artikel
Sprache:English
Veröffentlicht: Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України 2007
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Online Zugang:https://nasplib.isofts.kiev.ua/handle/123456789/121797
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Zitieren:Heat transfer in crystalline clathrate hydrates at low temperatures / A.I. Krivchikov, O.A. Korolyuk, O.O. Romantsova // Физика низких температур. — 2007. — Т. 33, № 6-7. — С. 798-804. — Бібліогр.: 31 назв. — англ.

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Digital Library of Periodicals of National Academy of Sciences of Ukraine
id nasplib_isofts_kiev_ua-123456789-121797
record_format dspace
spelling Krivchikov, A.I.
Korolyuk, O.A.
Romantsova, O.O.
2017-06-16T08:14:27Z
2017-06-16T08:14:27Z
2007
Heat transfer in crystalline clathrate hydrates at low temperatures / A.I. Krivchikov, O.A. Korolyuk, O.O. Romantsova // Физика низких температур. — 2007. — Т. 33, № 6-7. — С. 798-804. — Бібліогр.: 31 назв. — англ.
0132-6414
PACS: 66.70.+f; 63.20.–e; 63.20.Pw; 63.50.+x
https://nasplib.isofts.kiev.ua/handle/123456789/121797
The experimental results on the thermal conductivity k(T) of crystalline Xe, CH₄, and THF clathrate hydrates have been analyzed. In a wide region of temperatures above 2 K, k(T) exhibits a behavior typical of disordered solids, which depends weakly on their chemical composition, crystalline structure and microstructure. The results are discussed in the context of phenomenological models of phonon scattering by local modes. It has been found that the Xe clathrate has a feature unusual for glasses, namely, k(T) decreases almost two-fold as the temperature increases from 50–100 K. The behavior of k(T) is presumably determined mainly by the strong phonon scattering on water molecules.
The study was partially supported with a Grant of President of Ukraine for young scientists engaged in scientific research (GP/F13/0037). We thank Prof. Vadim Manzhelii, Prof. Werner Press, and Prof. Javier Bermejo for fruitful discuss.
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Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України
Физика низких температур
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Heat transfer in crystalline clathrate hydrates at low temperatures
Article
published earlier
institution Digital Library of Periodicals of National Academy of Sciences of Ukraine
collection DSpace DC
title Heat transfer in crystalline clathrate hydrates at low temperatures
spellingShingle Heat transfer in crystalline clathrate hydrates at low temperatures
Krivchikov, A.I.
Korolyuk, O.A.
Romantsova, O.O.
Related Topics
title_short Heat transfer in crystalline clathrate hydrates at low temperatures
title_full Heat transfer in crystalline clathrate hydrates at low temperatures
title_fullStr Heat transfer in crystalline clathrate hydrates at low temperatures
title_full_unstemmed Heat transfer in crystalline clathrate hydrates at low temperatures
title_sort heat transfer in crystalline clathrate hydrates at low temperatures
author Krivchikov, A.I.
Korolyuk, O.A.
Romantsova, O.O.
author_facet Krivchikov, A.I.
Korolyuk, O.A.
Romantsova, O.O.
topic Related Topics
topic_facet Related Topics
publishDate 2007
language English
container_title Физика низких температур
publisher Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України
format Article
description The experimental results on the thermal conductivity k(T) of crystalline Xe, CH₄, and THF clathrate hydrates have been analyzed. In a wide region of temperatures above 2 K, k(T) exhibits a behavior typical of disordered solids, which depends weakly on their chemical composition, crystalline structure and microstructure. The results are discussed in the context of phenomenological models of phonon scattering by local modes. It has been found that the Xe clathrate has a feature unusual for glasses, namely, k(T) decreases almost two-fold as the temperature increases from 50–100 K. The behavior of k(T) is presumably determined mainly by the strong phonon scattering on water molecules.
issn 0132-6414
url https://nasplib.isofts.kiev.ua/handle/123456789/121797
citation_txt Heat transfer in crystalline clathrate hydrates at low temperatures / A.I. Krivchikov, O.A. Korolyuk, O.O. Romantsova // Физика низких температур. — 2007. — Т. 33, № 6-7. — С. 798-804. — Бібліогр.: 31 назв. — англ.
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first_indexed 2025-12-07T15:57:59Z
last_indexed 2025-12-07T15:57:59Z
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