Structure and photoluminescence of helium-intercalated fullerite C₆₀

Intercalation of C₆₀ single crystals with helium was studied by powder x-ray diffractometry. It was established that the intercalation is a two-stage process, octahedral cavities are filled first and then tetrahedral ones, the chemical pressure being negative during both stages. For the first time l...

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Veröffentlicht in:Физика низких температур
Datum:2002
Hauptverfasser: Legchenkova, I.V., Prokhvatilov, A.I., Stetsenko, Yu.E., Strzhemechny, M.A., Yagotintsev, K.A., Avdeenko, A.A., Eremenko, V.V., Zinoviev, P.V., Zoryansky, V.N., Silaeva, N.B., Ruoff, R.S.
Format: Artikel
Sprache:English
Veröffentlicht: Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України 2002
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Online Zugang:https://nasplib.isofts.kiev.ua/handle/123456789/128766
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Zitieren:Structure and photoluminescence of helium-intercalated fullerite C₆₀ / I.V. Legchenkova, A.I. Prokhvatilov, Yu. E. Stetsenko, M.A. Strzhemechny, K.A. Yagotintsev, A.A. Avdeenko, V.V. Eremenko, P.V. Zinoviev, V.N. Zoryansky, N.B. Silaeva, R.S. Ruoff // Физика низких температур. — 2002. — Т. 28, № 12. — С. 1320-1323. — Бібліогр.: 16. назв. — англ.

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Digital Library of Periodicals of National Academy of Sciences of Ukraine
id nasplib_isofts_kiev_ua-123456789-128766
record_format dspace
spelling Legchenkova, I.V.
Prokhvatilov, A.I.
Stetsenko, Yu.E.
Strzhemechny, M.A.
Yagotintsev, K.A.
Avdeenko, A.A.
Eremenko, V.V.
Zinoviev, P.V.
Zoryansky, V.N.
Silaeva, N.B.
Ruoff, R.S.
2018-01-13T19:40:31Z
2018-01-13T19:40:31Z
2002
Structure and photoluminescence of helium-intercalated fullerite C₆₀ / I.V. Legchenkova, A.I. Prokhvatilov, Yu. E. Stetsenko, M.A. Strzhemechny, K.A. Yagotintsev, A.A. Avdeenko, V.V. Eremenko, P.V. Zinoviev, V.N. Zoryansky, N.B. Silaeva, R.S. Ruoff // Физика низких температур. — 2002. — Т. 28, № 12. — С. 1320-1323. — Бібліогр.: 16. назв. — англ.
0132-6414
PACS: 61.48.+c, 61.66.-f, 71.35.Aa, 78.55.-m
https://nasplib.isofts.kiev.ua/handle/123456789/128766
Intercalation of C₆₀ single crystals with helium was studied by powder x-ray diffractometry. It was established that the intercalation is a two-stage process, octahedral cavities are filled first and then tetrahedral ones, the chemical pressure being negative during both stages. For the first time low-temperature (5 K) photoluminescence spectra of helium-intercalated fullerite C₆₀ were studied. The presence of helium in lattice voids was shown to reduce that part of the luminescent intensity which is due to the emission of covalently bound pairs of C₆₀ molecules, the socalled "deep traps" with the 0-0 transition energy close to 1.69 eV. The mechanism of the effect of the intercalation with helium on the pair formation in fullerite C₆₀ is discussed.
en
Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України
Физика низких температур
Письма pедактоpу
Structure and photoluminescence of helium-intercalated fullerite C₆₀
Article
published earlier
institution Digital Library of Periodicals of National Academy of Sciences of Ukraine
collection DSpace DC
title Structure and photoluminescence of helium-intercalated fullerite C₆₀
spellingShingle Structure and photoluminescence of helium-intercalated fullerite C₆₀
Legchenkova, I.V.
Prokhvatilov, A.I.
Stetsenko, Yu.E.
Strzhemechny, M.A.
Yagotintsev, K.A.
Avdeenko, A.A.
Eremenko, V.V.
Zinoviev, P.V.
Zoryansky, V.N.
Silaeva, N.B.
Ruoff, R.S.
Письма pедактоpу
title_short Structure and photoluminescence of helium-intercalated fullerite C₆₀
title_full Structure and photoluminescence of helium-intercalated fullerite C₆₀
title_fullStr Structure and photoluminescence of helium-intercalated fullerite C₆₀
title_full_unstemmed Structure and photoluminescence of helium-intercalated fullerite C₆₀
title_sort structure and photoluminescence of helium-intercalated fullerite c₆₀
author Legchenkova, I.V.
Prokhvatilov, A.I.
Stetsenko, Yu.E.
Strzhemechny, M.A.
Yagotintsev, K.A.
Avdeenko, A.A.
Eremenko, V.V.
Zinoviev, P.V.
Zoryansky, V.N.
Silaeva, N.B.
Ruoff, R.S.
author_facet Legchenkova, I.V.
Prokhvatilov, A.I.
Stetsenko, Yu.E.
Strzhemechny, M.A.
Yagotintsev, K.A.
Avdeenko, A.A.
Eremenko, V.V.
Zinoviev, P.V.
Zoryansky, V.N.
Silaeva, N.B.
Ruoff, R.S.
topic Письма pедактоpу
topic_facet Письма pедактоpу
publishDate 2002
language English
container_title Физика низких температур
publisher Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України
format Article
description Intercalation of C₆₀ single crystals with helium was studied by powder x-ray diffractometry. It was established that the intercalation is a two-stage process, octahedral cavities are filled first and then tetrahedral ones, the chemical pressure being negative during both stages. For the first time low-temperature (5 K) photoluminescence spectra of helium-intercalated fullerite C₆₀ were studied. The presence of helium in lattice voids was shown to reduce that part of the luminescent intensity which is due to the emission of covalently bound pairs of C₆₀ molecules, the socalled "deep traps" with the 0-0 transition energy close to 1.69 eV. The mechanism of the effect of the intercalation with helium on the pair formation in fullerite C₆₀ is discussed.
issn 0132-6414
url https://nasplib.isofts.kiev.ua/handle/123456789/128766
citation_txt Structure and photoluminescence of helium-intercalated fullerite C₆₀ / I.V. Legchenkova, A.I. Prokhvatilov, Yu. E. Stetsenko, M.A. Strzhemechny, K.A. Yagotintsev, A.A. Avdeenko, V.V. Eremenko, P.V. Zinoviev, V.N. Zoryansky, N.B. Silaeva, R.S. Ruoff // Физика низких температур. — 2002. — Т. 28, № 12. — С. 1320-1323. — Бібліогр.: 16. назв. — англ.
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first_indexed 2025-12-07T20:52:03Z
last_indexed 2025-12-07T20:52:03Z
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