Thermal conductivity of solid parahydrogen with methane admixtures

The thermal conductivity of solid parahydrogen crystal with methane admixtures has been measured in the temperature range 1.5 to 8 K. Solid samples were grown from the gas mixture at 13 K. Concentration of CH₄ admixture molecules in the gas varied from 5 to 570 ppm. A very broad maximum of thermal c...

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Veröffentlicht in:Физика низких температур
Datum:2003
Hauptverfasser: Krivchikov, A.I., Sumarokov, V.V., Mucha, J., Stachowiak, P., Jezowski, A., Korolyuk, O.A.
Format: Artikel
Sprache:English
Veröffentlicht: Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України 2003
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Online Zugang:https://nasplib.isofts.kiev.ua/handle/123456789/128871
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Назва журналу:Digital Library of Periodicals of National Academy of Sciences of Ukraine
Zitieren:Thermal conductivity of solid parahydrogen with methane admixtures / A.I. Krivchikov, V.V. Sumarokov, J. Mucha, P. Stachowiak, A. Jezowski, O.A. Korolyuk // Физика низких температур. — 2003. — Т. 29, № 6. — С. 706-709. — Бібліогр.: 18 назв. — англ.

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Digital Library of Periodicals of National Academy of Sciences of Ukraine
id nasplib_isofts_kiev_ua-123456789-128871
record_format dspace
spelling Krivchikov, A.I.
Sumarokov, V.V.
Mucha, J.
Stachowiak, P.
Jezowski, A.
Korolyuk, O.A.
2018-01-14T11:04:15Z
2018-01-14T11:04:15Z
2003
Thermal conductivity of solid parahydrogen with methane admixtures / A.I. Krivchikov, V.V. Sumarokov, J. Mucha, P. Stachowiak, A. Jezowski, O.A. Korolyuk // Физика низких температур. — 2003. — Т. 29, № 6. — С. 706-709. — Бібліогр.: 18 назв. — англ.
0132-6414
PACS: 66.70.+f, 67.80.Gb, 67.80.Mg
https://nasplib.isofts.kiev.ua/handle/123456789/128871
The thermal conductivity of solid parahydrogen crystal with methane admixtures has been measured in the temperature range 1.5 to 8 K. Solid samples were grown from the gas mixture at 13 K. Concentration of CH₄ admixture molecules in the gas varied from 5 to 570 ppm. A very broad maximum of thermal conductivity with absolute value of about 110 W/(m×K) is observed at 2.6 K. The data are interpreted by Callaway model considering phonons resonant scattering on quasi-local vibrations of CH₄ molecules, phonon-grain boundary and phonon-phonon scattering processes. The increase of grain boundary scattering leads to the decrease of the maximum broadening. The analysis shows that the solid mixture of p-H₂ and CH₄ is a heterogeneous solution for CH₄ concentration higher than 0.1 ppm.
We are grateful to Prof. V.G. Manzhelii, Dr. B.Ya. Gorodilov for helpful discussions. The study described in this publication was made possible in part Grant N 2M/78-2000 of Ukrainian Min. of Education and Science.
en
Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України
Физика низких температур
3-й Международный семинар по физике низких температур в условиях микрогравитации
Thermal conductivity of solid parahydrogen with methane admixtures
Article
published earlier
institution Digital Library of Periodicals of National Academy of Sciences of Ukraine
collection DSpace DC
title Thermal conductivity of solid parahydrogen with methane admixtures
spellingShingle Thermal conductivity of solid parahydrogen with methane admixtures
Krivchikov, A.I.
Sumarokov, V.V.
Mucha, J.
Stachowiak, P.
Jezowski, A.
Korolyuk, O.A.
3-й Международный семинар по физике низких температур в условиях микрогравитации
title_short Thermal conductivity of solid parahydrogen with methane admixtures
title_full Thermal conductivity of solid parahydrogen with methane admixtures
title_fullStr Thermal conductivity of solid parahydrogen with methane admixtures
title_full_unstemmed Thermal conductivity of solid parahydrogen with methane admixtures
title_sort thermal conductivity of solid parahydrogen with methane admixtures
author Krivchikov, A.I.
Sumarokov, V.V.
Mucha, J.
Stachowiak, P.
Jezowski, A.
Korolyuk, O.A.
author_facet Krivchikov, A.I.
Sumarokov, V.V.
Mucha, J.
Stachowiak, P.
Jezowski, A.
Korolyuk, O.A.
topic 3-й Международный семинар по физике низких температур в условиях микрогравитации
topic_facet 3-й Международный семинар по физике низких температур в условиях микрогравитации
publishDate 2003
language English
container_title Физика низких температур
publisher Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України
format Article
description The thermal conductivity of solid parahydrogen crystal with methane admixtures has been measured in the temperature range 1.5 to 8 K. Solid samples were grown from the gas mixture at 13 K. Concentration of CH₄ admixture molecules in the gas varied from 5 to 570 ppm. A very broad maximum of thermal conductivity with absolute value of about 110 W/(m×K) is observed at 2.6 K. The data are interpreted by Callaway model considering phonons resonant scattering on quasi-local vibrations of CH₄ molecules, phonon-grain boundary and phonon-phonon scattering processes. The increase of grain boundary scattering leads to the decrease of the maximum broadening. The analysis shows that the solid mixture of p-H₂ and CH₄ is a heterogeneous solution for CH₄ concentration higher than 0.1 ppm.
issn 0132-6414
url https://nasplib.isofts.kiev.ua/handle/123456789/128871
citation_txt Thermal conductivity of solid parahydrogen with methane admixtures / A.I. Krivchikov, V.V. Sumarokov, J. Mucha, P. Stachowiak, A. Jezowski, O.A. Korolyuk // Физика низких температур. — 2003. — Т. 29, № 6. — С. 706-709. — Бібліогр.: 18 назв. — англ.
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