Quantum property of solid hydrogen as revealed by high-resolution laser spectroscopy

Pure vibrational overtone transitions of solid parahydrogen were studied using high-resolution laser spectroscopy. Extremely narrow spectral linewidth (~20 MHz) allowed us to observe rich spectral structure that originates in subtle intermolecular interactions in the crystal. It was found that aniso...

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Veröffentlicht in:Физика низких температур
Datum:2003
Hauptverfasser: Hiroyuki Katsuki, Mizuho Fushitani, Takamasa Momose
Format: Artikel
Sprache:Englisch
Veröffentlicht: Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України 2003
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Online Zugang:https://nasplib.isofts.kiev.ua/handle/123456789/128935
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Zitieren:Quantum property of solid hydrogen as revealed by high-resolution laser spectroscopy / Hiroyuki Katsuki, Mizuho Fushitani, Takamasa Momose // Физика низких температур. — 2003. — Т. 29, № 9-10. — С. 1093-1100. — Бібліогр.: 25 назв. — англ.

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Digital Library of Periodicals of National Academy of Sciences of Ukraine
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author Hiroyuki Katsuki
Mizuho Fushitani
Takamasa Momose
author_facet Hiroyuki Katsuki
Mizuho Fushitani
Takamasa Momose
citation_txt Quantum property of solid hydrogen as revealed by high-resolution laser spectroscopy / Hiroyuki Katsuki, Mizuho Fushitani, Takamasa Momose // Физика низких температур. — 2003. — Т. 29, № 9-10. — С. 1093-1100. — Бібліогр.: 25 назв. — англ.
collection DSpace DC
container_title Физика низких температур
description Pure vibrational overtone transitions of solid parahydrogen were studied using high-resolution laser spectroscopy. Extremely narrow spectral linewidth (~20 MHz) allowed us to observe rich spectral structure that originates in subtle intermolecular interactions in the crystal. It was found that anisotropy of the distribution of zero-point lattice vibration of hydrogen molecules perturbs the energy levels of the vibrationally excited states significantly. Large amplitude of the zero-point lattice vibration being an intrinsic nature of quantum solids, was directly observed from the present high-resolution spectroscopy. The first observation of a pure vibrational overtone transition of solid orthodeuterium is also discussed.
first_indexed 2025-11-26T22:53:25Z
format Article
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institution Digital Library of Periodicals of National Academy of Sciences of Ukraine
issn 0132-6414
language English
last_indexed 2025-11-26T22:53:25Z
publishDate 2003
publisher Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України
record_format dspace
spelling Hiroyuki Katsuki
Mizuho Fushitani
Takamasa Momose
2018-01-14T13:13:20Z
2018-01-14T13:13:20Z
2003
Quantum property of solid hydrogen as revealed by high-resolution laser spectroscopy / Hiroyuki Katsuki, Mizuho Fushitani, Takamasa Momose // Физика низких температур. — 2003. — Т. 29, № 9-10. — С. 1093-1100. — Бібліогр.: 25 назв. — англ.
0132-6414
PACS: 33.20.Ea, 63.50.+x, 67.80.-s
https://nasplib.isofts.kiev.ua/handle/123456789/128935
Pure vibrational overtone transitions of solid parahydrogen were studied using high-resolution laser spectroscopy. Extremely narrow spectral linewidth (~20 MHz) allowed us to observe rich spectral structure that originates in subtle intermolecular interactions in the crystal. It was found that anisotropy of the distribution of zero-point lattice vibration of hydrogen molecules perturbs the energy levels of the vibrationally excited states significantly. Large amplitude of the zero-point lattice vibration being an intrinsic nature of quantum solids, was directly observed from the present high-resolution spectroscopy. The first observation of a pure vibrational overtone transition of solid orthodeuterium is also discussed.
The work described herein was supported in part by the Grant-in Aid for Scientific Research of the Ministry of Education, Science, Culture, and Sports of Japan. The authors would like to thank Prof. H. Meyer who drew our attention to the problems of solid deuterium. Further, H. Katsuki would also like to acknowledge the support from JSPS Research Fellowships for Young Scientists.
en
Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України
Физика низких температур
Spectroscopy in Cryocrystals and Matrices
Quantum property of solid hydrogen as revealed by high-resolution laser spectroscopy
Article
published earlier
spellingShingle Quantum property of solid hydrogen as revealed by high-resolution laser spectroscopy
Hiroyuki Katsuki
Mizuho Fushitani
Takamasa Momose
Spectroscopy in Cryocrystals and Matrices
title Quantum property of solid hydrogen as revealed by high-resolution laser spectroscopy
title_full Quantum property of solid hydrogen as revealed by high-resolution laser spectroscopy
title_fullStr Quantum property of solid hydrogen as revealed by high-resolution laser spectroscopy
title_full_unstemmed Quantum property of solid hydrogen as revealed by high-resolution laser spectroscopy
title_short Quantum property of solid hydrogen as revealed by high-resolution laser spectroscopy
title_sort quantum property of solid hydrogen as revealed by high-resolution laser spectroscopy
topic Spectroscopy in Cryocrystals and Matrices
topic_facet Spectroscopy in Cryocrystals and Matrices
url https://nasplib.isofts.kiev.ua/handle/123456789/128935
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