EXAFS studies of the trapping site structure for molecules isolated in cryogenic matrices

We present here results concerning the first attempt of determining the trapping site structure of molecules isolated in inert matrices at low temperature by the EXAFS (Extended X-ray Absorption Fine Structure) method. The experiments have been performed at the K edge of argon, silicon, sulfur, and...

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Veröffentlicht in:Физика низких температур
Datum:2000
Hauptverfasser: Roubin, P., Varin, S., Gauthier-Roy, B., Crépin, C., Flank, A.-M., Lagarde, P., Ténégal, F.
Format: Artikel
Sprache:English
Veröffentlicht: Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України 2000
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Online Zugang:https://nasplib.isofts.kiev.ua/handle/123456789/129212
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Zitieren:EXAFS studies of the trapping site structure for molecules isolated in cryogenic matrices / P. Roubin, S. Varin, B. Gauthier-Roy, C. Crépin, A.-M. Flank, P. Lagarde, F. Ténégal // Физика низких температур. — 2000. — Т. 26, № 9-10. — С. 937-946. — Бібліогр.: 30 назв. — англ.

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Digital Library of Periodicals of National Academy of Sciences of Ukraine
id nasplib_isofts_kiev_ua-123456789-129212
record_format dspace
spelling Roubin, P.
Varin, S.
Gauthier-Roy, B.
Crépin, C.
Flank, A.-M.
Lagarde, P.
Ténégal, F.
2018-01-16T20:00:30Z
2018-01-16T20:00:30Z
2000
EXAFS studies of the trapping site structure for molecules isolated in cryogenic matrices / P. Roubin, S. Varin, B. Gauthier-Roy, C. Crépin, A.-M. Flank, P. Lagarde, F. Ténégal // Физика низких температур. — 2000. — Т. 26, № 9-10. — С. 937-946. — Бібліогр.: 30 назв. — англ.
0132-6414
PACS: 33.20.Rm, 61.10.Ht
https://nasplib.isofts.kiev.ua/handle/123456789/129212
We present here results concerning the first attempt of determining the trapping site structure of molecules isolated in inert matrices at low temperature by the EXAFS (Extended X-ray Absorption Fine Structure) method. The experiments have been performed at the K edge of argon, silicon, sulfur, and chlorine for pure solid argon, and for SiH4, OCS and HCl isolated in different cryogenic matrices. The EXAFS technique is sensitive to the local environment around the absorbing atom and the spectral features induced by the matrix material (Ar, Xe, N₂ and CH₄) are clearly evidenced here. The data allow a characterization of the double substitutional site for OCS in argon and xenon while no structure can be determined for the accommodation of SiH₄ in argon. A discussion of the best choice for the guest/host system to obtain a good EXAFS signal is included.
en
Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України
Физика низких температур
Low-Temperature Physics and Chemistry in Cryomatrice
EXAFS studies of the trapping site structure for molecules isolated in cryogenic matrices
Article
published earlier
institution Digital Library of Periodicals of National Academy of Sciences of Ukraine
collection DSpace DC
title EXAFS studies of the trapping site structure for molecules isolated in cryogenic matrices
spellingShingle EXAFS studies of the trapping site structure for molecules isolated in cryogenic matrices
Roubin, P.
Varin, S.
Gauthier-Roy, B.
Crépin, C.
Flank, A.-M.
Lagarde, P.
Ténégal, F.
Low-Temperature Physics and Chemistry in Cryomatrice
title_short EXAFS studies of the trapping site structure for molecules isolated in cryogenic matrices
title_full EXAFS studies of the trapping site structure for molecules isolated in cryogenic matrices
title_fullStr EXAFS studies of the trapping site structure for molecules isolated in cryogenic matrices
title_full_unstemmed EXAFS studies of the trapping site structure for molecules isolated in cryogenic matrices
title_sort exafs studies of the trapping site structure for molecules isolated in cryogenic matrices
author Roubin, P.
Varin, S.
Gauthier-Roy, B.
Crépin, C.
Flank, A.-M.
Lagarde, P.
Ténégal, F.
author_facet Roubin, P.
Varin, S.
Gauthier-Roy, B.
Crépin, C.
Flank, A.-M.
Lagarde, P.
Ténégal, F.
topic Low-Temperature Physics and Chemistry in Cryomatrice
topic_facet Low-Temperature Physics and Chemistry in Cryomatrice
publishDate 2000
language English
container_title Физика низких температур
publisher Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України
format Article
description We present here results concerning the first attempt of determining the trapping site structure of molecules isolated in inert matrices at low temperature by the EXAFS (Extended X-ray Absorption Fine Structure) method. The experiments have been performed at the K edge of argon, silicon, sulfur, and chlorine for pure solid argon, and for SiH4, OCS and HCl isolated in different cryogenic matrices. The EXAFS technique is sensitive to the local environment around the absorbing atom and the spectral features induced by the matrix material (Ar, Xe, N₂ and CH₄) are clearly evidenced here. The data allow a characterization of the double substitutional site for OCS in argon and xenon while no structure can be determined for the accommodation of SiH₄ in argon. A discussion of the best choice for the guest/host system to obtain a good EXAFS signal is included.
issn 0132-6414
url https://nasplib.isofts.kiev.ua/handle/123456789/129212
citation_txt EXAFS studies of the trapping site structure for molecules isolated in cryogenic matrices / P. Roubin, S. Varin, B. Gauthier-Roy, C. Crépin, A.-M. Flank, P. Lagarde, F. Ténégal // Физика низких температур. — 2000. — Т. 26, № 9-10. — С. 937-946. — Бібліогр.: 30 назв. — англ.
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last_indexed 2025-12-07T19:48:34Z
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