The content of natural radioactive isotopes in soil of Kharkov region

The content and migration of natural radioactive isotopes in some lot of the surface soil of the Kharkiv region have been studied by the help of low background gamma spectroscopy. The migration series of radioactive elements (Ra > U > Th) in the soil of the Kharkiv region is determined, which...

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Опубліковано в: :Вопросы атомной науки и техники
Дата:2017
Автори: Dikiy, N.P., Lyashko, Yu.V., Medvedeva, E.P., Medvedev, D.V., Parhomenko, Yu.G., Fedorets, I.D.
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Мова:Англійська
Опубліковано: Національний науковий центр «Харківський фізико-технічний інститут» НАН України 2017
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Онлайн доступ:https://nasplib.isofts.kiev.ua/handle/123456789/136096
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Цитувати:The content of natural radioactive isotopes in soil of Kharkov region / N.P. Dikiy, Yu.V. Lyashko, E.P. Medvedeva, D.V. Medvedev, Yu.G. Parhomenko, I.D. Fedorets // Вопросы атомной науки и техники. — 2017. — № 3. — С. 55-59. — Бібліогр.: 10 назв. — англ.

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Digital Library of Periodicals of National Academy of Sciences of Ukraine
_version_ 1860260106901389312
author Dikiy, N.P.
Lyashko, Yu.V.
Medvedeva, E.P.
Medvedev, D.V.
Parhomenko, Yu.G.
Fedorets, I.D.
author_facet Dikiy, N.P.
Lyashko, Yu.V.
Medvedeva, E.P.
Medvedev, D.V.
Parhomenko, Yu.G.
Fedorets, I.D.
citation_txt The content of natural radioactive isotopes in soil of Kharkov region / N.P. Dikiy, Yu.V. Lyashko, E.P. Medvedeva, D.V. Medvedev, Yu.G. Parhomenko, I.D. Fedorets // Вопросы атомной науки и техники. — 2017. — № 3. — С. 55-59. — Бібліогр.: 10 назв. — англ.
collection DSpace DC
container_title Вопросы атомной науки и техники
description The content and migration of natural radioactive isotopes in some lot of the surface soil of the Kharkiv region have been studied by the help of low background gamma spectroscopy. The migration series of radioactive elements (Ra > U > Th) in the soil of the Kharkiv region is determined, which corresponds to the humid type of climate. A high radium mobility as respect to uranium and thorium has been found. A high correlation between ⁴⁰K vs ²³²Th was found. Therefore, as a result of low mobility of thorium, it is possible to assume that thorium and potassium enter into the composition of the mother minerals. Correlation of ¹³⁷Cs with other radioactive isotopes was not significant in the soil of the Kharkiv region. This apparently indicates specifies in that a high mobility clay minerals can sorbing of cesium. Вміст і міграція природних радіоактивних ізотопів у деяких ділянках поверхневого грунту Харківської області вивчалися за допомогою низькофонової гамма-спектроскопії. Визначена міграційна серія радіоактивних елементів (Ra > U > Th) у грунті Харківської області, що відповідає гумідному типу клімату. Виявлена висока рухливість радію по відношенню до урану і торію. Виявлена висока кореляція між ⁴⁰K vs ²³²Th, яка підтверджує, що торій і калій входять до складу материнських мінералів через низьку рухливость торію. Кореляція ¹³⁷Cs з іншими радіоактивними ізотопами не є суттєвою в грунті Харківської області. Це, мабуть, вказує на те, що високомобільні глинисті мінерали можуть сорбувати цезій. Содержание и миграция природных радиоактивных изотопов в некоторых участках поверхностной почвы Харьковской области изучались с помощью низкофоновой гамма-спектроскопии. Определена миграционная серия радиоактивных элементов (Ra > U > Th) в почве Харьковской области, что соответствует гумидному типу климата. Обнаружена высокая подвижность радия по отношению к урану и торию. Обнаружена высокая корреляция между ⁴⁰K vs ²³²Th, которая подтверждает, что торий и калий входят в состав материнских минералов из-за низкой подвижности тория. Корреляция ¹³⁷Cs с другими радиоактивными изотопами не существенна в почве Харьковской области. Это, по-видимому, указывает на то, что высокомобильные глинистые минералы могут сорбировать цезий.
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fulltext THE CONTENT OF NATURAL RADIOACTIVE ISOTOPES IN SOIL OF KHARKOV REGION N.P.Dikiy1∗, Yu.V.Lyashko1, E.P.Medvedeva1, D.V.Medvedev1, Yu.G.Parhomenko1, I.D.Fedorets2 1National Science Center "Kharkiv Institute of Physics and Technology", 61108, Kharkiv, Ukraine; 2V.N. Karazin Kharkiv National University, 61077, Kharkiv, Ukraine (Received May 10, 2017) The content and migration of natural radioactive isotopes in some lot of the surface soil of the Kharkiv region have been studied by the help of low background gamma spectroscopy. The migration series of radioactive elements (Ra > U > Th) in the soil of the Kharkiv region is determined, which corresponds to the humid type of climate. A high radium mobility as respect to uranium and thorium has been found. A high correlation between 40K vs 232Th was found. Therefore, as a result of low mobility of thorium, it is possible to assume that thorium and potassium enter into the composition of the mother minerals. Correlation of 137Cs with other radioactive isotopes was not signi�cant in the soil of the Kharkiv region. This apparently indicates speci�es in that a high mobility clay minerals can sorbing of cesium. PACS: 89.60.-k 1. INTRODUCTION Soil radioactivity is formed by geochemical pro- cesses in the biosphere. The parent rock generally determines a concentration of radioactive elements in soil. In Tab. 1 shows typical concentrations of natural radionuclides in di�erent soil types. Biological pro- cesses in the formation of soils lead to a greater ac- cumulation of radionuclides in chernozems compared to gray forest or sod-podzolic soils. The leaching and precipitation of radionuclides by soil waters de- termine the uneven distribution of nuclide activity along the depth of the soil. For example, uranium has a high concentration in the deep layers due to the washing out of soluble fractions from the sur- face horizons, and thorium, on the contrary, tends to increase in the surface layers due to low solubil- ity and greater weathering of other components from the soil surface. Potassium tends to a greater extent to surface layers as it characterizes by relatively high biological activity (see Table 1) [1]. Many radionuclides, especially analogs of calcium and actinides, have osteotropic properties and are be- ing detected in the human body. This particularly applies to radium isotopes. Radium and its com- pounds are widely distributed in nature and are a major source of natural radiation. During the weath- ering, and migration of radium from rock to soil, it can 'move out' in the particulate phase, to be trans- ported and deposited as loess, silt placers, and ter- tiary soil. However, that part of radium which tends to be solubilized in water � either with a ground or river water � moves along with the water stream until it is �nally deposited in the soil through chemical or biological action. The range of 226Ra concentrations for soil in normal areas varies from 3.7 to 125.8 Bq/kg [2]. It is known that the content and distribution of radium in soils a�ects the radon emanation. Table 1. The concentration of natural radionuclides in soils, Bq/kg Type of soil 238U 232Th 40K Serozems 31.5 48.1 666 Gray-brown 27.8 40.7 703 Chestnut 26.6 37 555 Chernozems 21.6 35.9 407 Gray forest 17.8 26.6 370 Sod-podzolic 15.2 22.2 300 Podzolic 8.9 12.2 148 Peaty 6.3 6.3 89 Thorium exists in soils mainly as thorite (ThSiO4), monazite [(Ce,La,Th,Nd)PO4], and thori- anite (ThO2). Although they are very resistant after extreme weathering, monazite and thorite end up be- ing dissolved and then precipitates as thorianite. Our planet displays the results of an uninten- tional, multibillion-year experiment between biota and Earth materials. One of the exciting frontiers in the geosciences is the investigation of how biota impacts chemical and physical processes in the Crit- ical Zone. Understanding the feedbacks between life and Earth materials is important for society as well, because humans, a relatively recent addition to the ∗Corresponding author E-mail address: ndikiy@kipt.kharkov.ua ISSN 1562-6016. PROBLEMS OF ATOMIC SCIENCE AND TECHNOLOGY, 2017, N3(109). Series: Nuclear Physics Investigations (68), p.55-59. 55 Earth's biota, are increasingly testing the resilience of the Critical Zone. The response of Critical Zone processes to these stresses will ultimately impact the whole of the Earth's biosphere, and thereby, humans themselves [1]. The biotechnological introduction of microbial genes coding for toxic proteins against insects, weed species or other pests in the genome of crop plants is another important topic in the study of the environ- mental and health consequences of protein�mineral interactions in soil. Some of the best known and most controversial genetically modi�ed plants are those containing the Bacillus thuringiensis (Bt) toxin. Commercially available Bt plants include maize, cot- ton, potato, tobacco and rice. Nevertheless, the bal- ance between these clear advantages in the short- and medium-terms and the possible pernicious ef- fects in the longer term needs to be studied. With the introduction of toxins, such as Bt and an in- creasing number of other potentially valuable insec- ticidal molecules, the risk of the development of re- sistance increases. This could have major negative consequences for agriculture, equivalent to bacterial resistance to antibiotics in medicine. Thus, studies on the long-term fate and side e�ects of Bt toxins in soil need to be pursued [3]. 500 1000 1500 101 102 103 214Bi 214Bi 228Ac 208Tl 214Pb 40K co un ts energy , keV soil 212Pb 137Cs 511 keV Fig.1. The energy spectrum of soil sample Modern ideas about the formation of chernozems con�rm the hypothesis of plant-terraneous origin. The most important processes of formation of cher- nozems are sodding and eluvial. The latter is ex- pressed mainly in the pro�le migration of calcium bicarbonate, which is formed by the decomposition of plant remains rich in calcium. These processes de- velop under the perennial vegetation of grassy steppes in the forest-steppe and steppe zones under condi- tions of periodically washing and non-washable wa- ter regimes and form humus and carbonate pro�les of chernozem [4]. Dust �ux is greater than 10% of global sediment. Therefore the deposition from the atmosphere plays an important role in the biogeo- chemistry of soils worldwide [5]. The study of the content of 40K, 232Th, 238U and their radioactive products in soils of a neighborhood of the Kharkiv region and an establishment of cor- relative connections between radioelements were the purposes of the present investigation. 2. MATERIALS AND METHODS Samples of soils (15x15 cm2 and h=10 cm) were collected in the neighborhood of Kharkiv on virgin soil or in the forest. Two samples were taken on arable land. Soil samples were dried at room tem- perature, then sieved through a 1-mm mesh to re- move the roots of plants and stones and homogenized prior to analysis. Determination of the radionuclides in soil samples was performed by gamma spectrome- ter method on Ge(Li)-detector with the volume of 50 cm3 and resolution of 3.2 keV at 1332 keV line. The measurement time of the gamma spectrum of each soil sample was about 24 hours. To reduce the in�u- ence of background, the detector is equipped with a three-layer Pb-Cu-Al protection [6] (Fig.1). The er- rors in determining the activity of radionuclides 40K and 137Cs do not exceed 20%. The same errors are found for 228Ac, 212Pb, 208Tl from the family 232Th and 214Pb, 214Bi (which is determined the parent 226Ra) from the family 238U. The more signi�cant error is for 238U, the activity of which was calculated from the activity of 235U (line of 186 keV is equal sum's of lines from 226Ra+235U). 0,0 0,1 0,2 0,01 0,02 0,03 0,04 Kharkiv region Askaniya-Nova ac tiv ity 22 6 R a, B q/ g activity 238U, Bq/g A Ra =0.31 A U Fig.2. Dependence of activity of 226Ra vs 238U in the soil of the Kharkiv region and Askaniya-Nova 3. RESULTS AND DISCUSSION It is known that the content of radioactive iso- topes in the soil is largely determined by the parent rocks. However, environmental conditions have a sig- ni�cant e�ect on the migration of uranium, thorium and their decay products. For example, the migra- tion of radium (an analog of calcium) depends most strongly on the environmental conditions. In Fig.2 shows the dependence of activity of 226Ra on the ac- tivity of 238U for various samples of soil from di�erent regions of Ukraine. The data from Askaniya-Nova is taken from [7]. The Kharkiv region is characterized by a humid climate, which, apparently, determines the greater removal of radium from a given territory in the sea. Askaniya-Nova is characterized by a more 56 arid climate. It can be assumed that the Askaniya- Nova region was often �ooded with water (its height above sea level is 30 m). Therefore, the content of 226Ra in the soil of Askaniya-Nova is somewhat higher than in the humid zone of the Kharkiv region. We note that in the soil, which is closer to the parent rock, there is a 226Ra/238U equilibrium. In our case, the content of radium for the Kharkiv region is much smaller (see Fig.2). 0,02 0,04 0,06 0,08 0,2 0,4 0,6 0,8 activity 238U, Bq/g 40K ac tiv ity 40 K, B q/ g Fig.3. Dependence of activity of 40K vs 238U in the soil of the Kharkiv region 0,01 0,02 0,03 0,2 0,4 0,6 0,8 ac tiv ity 40 K, B q/ g activity 214Bi, Bq/g Fig.4. Dependence of activity of 40K vs 214Bi (226Ra) in the soil of the Kharkiv region In Figs.3-5 the dependencies of activity 40Ê vs 238U, 40Ê vs 214Bi (corresponds 226Ra) and 40Ê vs 208Tl (corresponds 232Th) in soil of the Kharkov re- gion are given. Approximation of the above depen- dencies is carried out by a linear function. It is pos- sible to see that the most smaller straggling of the values concerning a linear function is observed for de- pendence 40K/232Th. As stated above, it is caused by high fastness of thorium minerals in the soil. Small enough straggling of value is observed and for depen- dence 40Ê/214Bi. We will notice that points values of 40Ê which strongly di�er from a linear dependence, correspond to samples which had been taken from an arable land. The greatest straggling of values is re- alized for dependence 40Ê/238U. In general, uranium is more closely associated with iron and manganese, due to its strong sorption by iron oxides. Radium, on the other hand, is more related to Ca and Ba in its behavior [4]. 0,00 0,02 0,04 0,0 0,2 0,4 0,6 0,8 ac tiv ity 40 K, B q/ g activity 208Tl(232Th), Bq/g 40K Fig.5. Dependence of activity of 40K vs 208Tl (232Th) in the soil of the Kharkiv region 0,02 0,04 0,06 0,01 0,02 0,03 0,04 Kharkiv region Askaniya-Nova ac tiv ity 21 4 Pb , B q/ g activity 212Pb, Bq/g Fig.6. Dependence of activity of 214Pb vs 212Pb in the soil of the Kharkiv region and Askaniya-Nova The intensity of migration of radioactive elements by of water under oxidizing conditions forms the fol- lowing series: 238U > 226Ra > 232Th. Due to the di�erent migration mobility of natural radioactive el- ements, a redistribution of these elements between the conjugate landscapes is observed. Thus, U(VI) is removed from eluvial landscapes and concentrates on geochemical barriers such as �oodplain, marsh and swampy soils, where it is restored to a relatively in- active U(IV). In humid eluvial and trans-eluvial land- scapes, soils are depleted of uranium in favor of ra- dium in comparison with their equilibrium ratio. Hy- dromorphic soils of accumulative landscapes are en- riched uranium. In alluvial sediments, the concen- trations of U and Ra are low due to their leaching and removing by water. The ratio Ra/U in alluvial sediments is high since U is more mobility and is pre- dominated in the water. The shift of radioisotope ratios in soils of conjugate landscapes is observed for Th/U and Th/Ra since thorium is characterized by much lower migration mobility in comparison with U and Ra [8]. For soils of the humid zone, the migra- tion series of elements Ra > U > Th were determined. 57 In our case, Ra is more mobile, which con�rms the humid climate of the Kharkiv region [4] (see Fig.2). The dependence of 214Pb vs 212Pb, which is re- lated to the ratio of uranium vs thorium and in a greater degree to the ratio of radium vs thorium, is shown in Fig.6. In our case, a signi�cant amount of radium is washed out by water (see Fig.2). Therefore, it can be assumed that a signi�cant amount of ra- dium is found in minerals containing thorium. A cer- tain con�rmation of this is the dependence of 214Pb vs 212Pb for the Askaniya-Nova soil (see Fig.6), in which an analogous dependence take place only for large values of 212,214Pb. The dependence of 40K vs 214Pb shows In Fig.7 (214Pb is the decay product of 238U → 226Ra). More reliably, this dependence is due to 226Ra. The con- tent of 238U and 40K is greater for the dark chestnut soil of Askaniya-Nova than for chernozems [9]. The 40K content is especially great in the soil of Askaniya- Nova (see Fig.7). 0,01 0,02 0,03 0,04 0,2 0,4 0,6 0,8 Kharkiv region Askaniya-Nova ac tiv ity 40 K Bq /g activity 214Pb, Bq/g Fig.7. Dependence of activity of 40K vs 214Pb in the soil of the Kharkiv region and Askaniya-Nova 0,02 0,04 0,06 0,2 0,4 0,6 0,8 Kharkiv region Askaniya-Nova ac tiv ity 40 K Bq /g activity 212Pb, Bq/g Fig.8. Dependence of activity of 40K vs 212Pb in the soil of the Kharkiv region and Askaniya-Nova The dependence of 40K vs 212Pb is shown in Fig.8 (212Pb product of the decay of 232Th). The mobility of Th in soil is low, so the dependence of 40K vs 212Pb for the soil of Askaniya-Nova is similar it's for the soil of Kharkiv region, which corresponds to the conven- tional value of thorium content in the dark chestnut soil [10]. The dependence of 40K vs 137Cs is shown in Fig.9. It can be seen that there are no correlation links. It can be assumed that the 137Cs content is due to its sorption by illite of soil. Due to water erosion, the caesium moves from the humid area or it is trans- ported to deeper horizons of the soil. 0,00 0,02 0,04 0,06 0,2 0,4 0,6 0,8 ac tiv ity 40 K Bq /g activity 137Cs, Bq/g K40 Fig.9. Dependence of activity of 40K vs 137Cs in the soil of the Kharkiv region 4. CONCLUSIONS 1. The series of migration elements (Ra > U > Th) in the soil of the Kharkiv region is determined by gamma spectrometer method. These series of mi- gration elements corresponds to the humid type of climate. A high mobility of radium as respect to ura- nium and thorium has been found. 2. A high correlation between 40K vs 232Th was found. Therefore, as a result of low mobility of tho- rium, it is possible to assume that thorium and potas- sium enter into the composition of the mother min- erals. 3. Correlation of 137Cs with other radioactive iso- topes was not signi�cant in the soil of the Kharkiv region. This apparently indicates speci�es in that a high mobility clay minerals can sorbing of cesium. References 1. R.Amundson, D.D.Richter, G.S.Humphreys, et al. Coupling between Biota and Earth Materi- als in the Critical Zone // Elements. 2007, v.3, p.327-332. 2. M.J. Frissel, H.W.Koster. Radium in soil // The environmental behavior of radium v.1, IAEA, Austria, Vienna: 1990, 600 p. 3. H.Quiquampoix, R.G.Burns. Interactions be- tween Proteins and Soil Mineral Surfaces: En- vironmental and Health Consequences // Ele- ments. 2008, v.3, p.401-406. 4. V.P.Kovrigo, I.S.Kaurichev, L.M.Burlakova // Soil science with the basics of geology, Moscow, "Kolos". 2000, 416 p. (in Russian). 58 5. L.A.Derry, O.A.Chadwick. Contributions from Earth's Atmosphere to Soil // Elements. 2007, v.3, p.333�338. 6. N.P.Dikiy, Yu.V. Lyashko, D.S.Katalevskaya, et al. Anthropogenic genomic radionuclides and mi- croelements in the soil and cleanliness of the city of Kharkiv // PAST. Ser. "Nuclear Physics In- vestigations" (93). 2014, N5(63), p.54�58. 7. V.S. Bulkln, I.A.Malluk, A.F.Ogorodnik, et al. Micro elements composition of soils and veg- etation in Askania-Nova preservez: Preprint. KINR-94-10, Kiev, 1994, 23 p. (in Russian). 8. G.D.Belitsina, V.D.Vasilevsky, L.A.Grishin, et al. Soil science, Moscow: "The higher school". 1988, 400 p. (in Russian). 9. E.M.Morgun, T.I. Ushacheva. In�uence of pyro- genic factor on humus content in steppe dark- chestnut soils of Askiniya-Nova Nature Reserve // Vist. Biosfer. Zapovid. Askaniya-Nova. 2008, v.10, p.127�130. 10. S.P.Anderson, F. vonBlanckenburg, A.F.White. Physical and Chemical Controls on the Critical Zone // Elements. 2007, v.3, p.315�319. ÑÎÄÅÐÆÀÍÈÅ ÏÐÈÐÎÄÍÛÕ ÐÀÄÈÎÀÊÒÈÂÍÛÕ ÈÇÎÒÎÏΠ ÏÎ×ÂÅ ÕÀÐÜÊÎÂÑÊÎÉ ÎÁËÀÑÒÈ Í.Ï. Äèêèé, Þ.Â. Ëÿøêî, Å.Ï. Ìåäâåäåâà, Ä.Â. Ìåäâåäåâ, Þ.Ã. Ïàðõîìåíêî, È.Ä. Ôåäîðåö Ñîäåðæàíèå è ìèãðàöèÿ ïðèðîäíûõ ðàäèîàêòèâíûõ èçîòîïîâ â íåêîòîðûõ ó÷àñòêàõ ïîâåðõíîñòíîé ïî÷âû Õàðüêîâñêîé îáëàñòè èçó÷àëèñü ñ ïîìîùüþ íèçêîôîíîâîé ãàììà-ñïåêòðîñêîïèè. Îïðåäåëåíà ìèãðàöèîííàÿ ñåðèÿ ðàäèîàêòèâíûõ ýëåìåíòîâ (Ra > U > Th) â ïî÷âå Õàðüêîâñêîé îáëàñòè, ÷òî ñîîòâåòñòâóåò ãóìèäíîìó òèïó êëèìàòà. Îáíàðóæåíà âûñîêàÿ ïîäâèæíîñòü ðàäèÿ ïî îòíîøåíèþ ê óðàíó è òîðèþ. Îáíàðóæåíà âûñîêàÿ êîððåëÿöèÿ ìåæäó 40K vs 232Th, êîòîðàÿ ïîäòâåðæäàåò, ÷òî òîðèé è êàëèé âõîäÿò â ñîñòàâ ìàòåðèíñêèõ ìèíåðàëîâ èç-çà íèçêîé ïîäâèæíîñòè òîðèÿ. Êîððåëÿöèÿ 137Cs ñ äðóãèìè ðàäèîàêòèâíûìè èçîòîïàìè íå ñóùåñòâåííà â ïî÷âå Õàðüêîâñêîé îáëàñòè. Ýòî, ïî- âèäèìîìó, óêàçûâàåò íà òî, ÷òî âûñîêîìîáèëüíûå ãëèíèñòûå ìèíåðàëû ìîãóò ñîðáèðîâàòü öåçèé. ÂÌIÑÒ ÏÐÈÐÎÄÍÈÕ ÐÀÄIÎÀÊÒÈÂÍÈÕ IÇÎÒÎÏIÂ Ó ÃÐÓÍÒI ÕÀÐÊIÂÑÜÊÎ� ÎÁËÀÑÒI Ì.Ï. Äèêèé, Þ.Â. Ëÿøêî, Î.Ï. Ìåäâåä¹âà, Ä.Â. Ìåäâåä¹â, Þ.Ã. Ïàðõîìåíêî, I.Ä. Ôåäîðåöü Âìiñò i ìiãðàöiÿ ïðèðîäíèõ ðàäiîàêòèâíèõ içîòîïiâ ó äåÿêèõ äiëÿíêàõ ïîâåðõíåâîãî ãðóíòó Õàðêiâñü- êî¨ îáëàñòi âèâ÷àëèñÿ çà äîïîìîãîþ íèçüêîôîíîâî¨ ãàììà-ñïåêòðîñêîïi¨. Âèçíà÷åíà ìiãðàöiéíà ñåðiÿ ðàäiîàêòèâíèõ åëåìåíòiâ (Ra > U > Th) ó ãðóíòi Õàðêiâñüêî¨ îáëàñòi, ùî âiäïîâiä๠ãóìiäíîìó òèïó êëiìàòó. Âèÿâëåíà âèñîêà ðóõëèâiñòü ðàäiþ ïî âiäíîøåííþ äî óðàíó i òîðiþ. Âèÿâëåíà âèñîêà êîðå- ëÿöiÿ ìiæ 40K vs 232Th, ÿêà ïiäòâåðäæó¹, ùî òîðié i êàëié âõîäÿòü äî ñêëàäó ìàòåðèíñüêèõ ìiíåðàëiâ ÷åðåç íèçüêó ðóõëèâîñòü òîðiþ. Êîðåëÿöiÿ 137Cs ç iíøèìè ðàäiîàêòèâíèìè içîòîïàìè íå ¹ ñóòò¹âîþ â ãðóíòi Õàðêiâñüêî¨ îáëàñòi. Öå, ìàáóòü, âêàçó¹ íà òå, ùî âèñîêîìîáiëüíi ãëèíèñòi ìiíåðàëè ìîæóòü ñîðáóâàòè öåçié. 59
id nasplib_isofts_kiev_ua-123456789-136096
institution Digital Library of Periodicals of National Academy of Sciences of Ukraine
issn 1562-6016
language English
last_indexed 2025-12-07T18:54:25Z
publishDate 2017
publisher Національний науковий центр «Харківський фізико-технічний інститут» НАН України
record_format dspace
spelling Dikiy, N.P.
Lyashko, Yu.V.
Medvedeva, E.P.
Medvedev, D.V.
Parhomenko, Yu.G.
Fedorets, I.D.
2018-06-15T19:07:49Z
2018-06-15T19:07:49Z
2017
The content of natural radioactive isotopes in soil of Kharkov region / N.P. Dikiy, Yu.V. Lyashko, E.P. Medvedeva, D.V. Medvedev, Yu.G. Parhomenko, I.D. Fedorets // Вопросы атомной науки и техники. — 2017. — № 3. — С. 55-59. — Бібліогр.: 10 назв. — англ.
1562-6016
PACS: 89.60.-k
https://nasplib.isofts.kiev.ua/handle/123456789/136096
The content and migration of natural radioactive isotopes in some lot of the surface soil of the Kharkiv region have been studied by the help of low background gamma spectroscopy. The migration series of radioactive elements (Ra > U > Th) in the soil of the Kharkiv region is determined, which corresponds to the humid type of climate. A high radium mobility as respect to uranium and thorium has been found. A high correlation between ⁴⁰K vs ²³²Th was found. Therefore, as a result of low mobility of thorium, it is possible to assume that thorium and potassium enter into the composition of the mother minerals. Correlation of ¹³⁷Cs with other radioactive isotopes was not significant in the soil of the Kharkiv region. This apparently indicates specifies in that a high mobility clay minerals can sorbing of cesium.
Вміст і міграція природних радіоактивних ізотопів у деяких ділянках поверхневого грунту Харківської області вивчалися за допомогою низькофонової гамма-спектроскопії. Визначена міграційна серія радіоактивних елементів (Ra > U > Th) у грунті Харківської області, що відповідає гумідному типу клімату. Виявлена висока рухливість радію по відношенню до урану і торію. Виявлена висока кореляція між ⁴⁰K vs ²³²Th, яка підтверджує, що торій і калій входять до складу материнських мінералів через низьку рухливость торію. Кореляція ¹³⁷Cs з іншими радіоактивними ізотопами не є суттєвою в грунті Харківської області. Це, мабуть, вказує на те, що високомобільні глинисті мінерали можуть сорбувати цезій.
Содержание и миграция природных радиоактивных изотопов в некоторых участках поверхностной почвы Харьковской области изучались с помощью низкофоновой гамма-спектроскопии. Определена миграционная серия радиоактивных элементов (Ra > U > Th) в почве Харьковской области, что соответствует гумидному типу климата. Обнаружена высокая подвижность радия по отношению к урану и торию. Обнаружена высокая корреляция между ⁴⁰K vs ²³²Th, которая подтверждает, что торий и калий входят в состав материнских минералов из-за низкой подвижности тория. Корреляция ¹³⁷Cs с другими радиоактивными изотопами не существенна в почве Харьковской области. Это, по-видимому, указывает на то, что высокомобильные глинистые минералы могут сорбировать цезий.
en
Національний науковий центр «Харківський фізико-технічний інститут» НАН України
Вопросы атомной науки и техники
Ядерно-физические методы и обработка данных
The content of natural radioactive isotopes in soil of Kharkov region
Вміст природних радіоактивних ізотопів у грунті Харківської області
Содержание природных радиоактивных изотопов в почве Харьковской области
Article
published earlier
spellingShingle The content of natural radioactive isotopes in soil of Kharkov region
Dikiy, N.P.
Lyashko, Yu.V.
Medvedeva, E.P.
Medvedev, D.V.
Parhomenko, Yu.G.
Fedorets, I.D.
Ядерно-физические методы и обработка данных
title The content of natural radioactive isotopes in soil of Kharkov region
title_alt Вміст природних радіоактивних ізотопів у грунті Харківської області
Содержание природных радиоактивных изотопов в почве Харьковской области
title_full The content of natural radioactive isotopes in soil of Kharkov region
title_fullStr The content of natural radioactive isotopes in soil of Kharkov region
title_full_unstemmed The content of natural radioactive isotopes in soil of Kharkov region
title_short The content of natural radioactive isotopes in soil of Kharkov region
title_sort content of natural radioactive isotopes in soil of kharkov region
topic Ядерно-физические методы и обработка данных
topic_facet Ядерно-физические методы и обработка данных
url https://nasplib.isofts.kiev.ua/handle/123456789/136096
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