Simulation of phase diagrams in LaNi₅-H₂(D₂) system and inversion of isotopic effect

Simulation of phase transitions in IMC-hydrogen systems based on modified scheme of perturbation theory provides correct description of main characteristics of phase diagrams within a wide pressure range of hydrogen isotopes (6 decimal orders and wider). The obtained data on thermodynamic parameters...

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Published in:Functional Materials
Date:2007
Main Authors: Marinin, V.S., Shmalko, Yu.F., Umerenkova, K.R.
Format: Article
Language:English
Published: НТК «Інститут монокристалів» НАН України 2007
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Online Access:https://nasplib.isofts.kiev.ua/handle/123456789/136969
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Journal Title:Digital Library of Periodicals of National Academy of Sciences of Ukraine
Cite this:Simulation of phase diagrams in LaNi₅-H₂(D₂) system and inversion of isotopic effect / V.S. Marinin, Yu.F. Shmalko, K.R. Umerenkova // Functional Materials. — 2007. — Т. 14, № 4. — С. 492-497. — Бібліогр.: 8 назв. — англ.

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Digital Library of Periodicals of National Academy of Sciences of Ukraine
id nasplib_isofts_kiev_ua-123456789-136969
record_format dspace
spelling Marinin, V.S.
Shmalko, Yu.F.
Umerenkova, K.R.
2018-06-16T18:17:28Z
2018-06-16T18:17:28Z
2007
Simulation of phase diagrams in LaNi₅-H₂(D₂) system and inversion of isotopic effect / V.S. Marinin, Yu.F. Shmalko, K.R. Umerenkova // Functional Materials. — 2007. — Т. 14, № 4. — С. 492-497. — Бібліогр.: 8 назв. — англ.
1027-5495
https://nasplib.isofts.kiev.ua/handle/123456789/136969
Simulation of phase transitions in IMC-hydrogen systems based on modified scheme of perturbation theory provides correct description of main characteristics of phase diagrams within a wide pressure range of hydrogen isotopes (6 decimal orders and wider). The obtained data on thermodynamic parameters of α-β transition allows to describe inversion of isotopic effect in LaNi₅-H₂(D₂) system. Data on solubility of hydrogen isotopes in LaNi₅ at pressures up to 500 atm. have been obtained; data on parameters of the critical points of α-β equilibrium (for which experimental data are absent) have been also obtained. The proposed calculation scheme does not use any fitting parameters or empirical correlations and is based on atomic characteristics of the hydrogen subsystem and metallic matrix which are physically meaningful.
en
НТК «Інститут монокристалів» НАН України
Functional Materials
Modeling and simulation
Simulation of phase diagrams in LaNi₅-H₂(D₂) system and inversion of isotopic effect
Моделювання фазових діаграм у системі LaNi₅-H₂(D₂) та інверсія ізотопного ефекту
Article
published earlier
institution Digital Library of Periodicals of National Academy of Sciences of Ukraine
collection DSpace DC
title Simulation of phase diagrams in LaNi₅-H₂(D₂) system and inversion of isotopic effect
spellingShingle Simulation of phase diagrams in LaNi₅-H₂(D₂) system and inversion of isotopic effect
Marinin, V.S.
Shmalko, Yu.F.
Umerenkova, K.R.
Modeling and simulation
title_short Simulation of phase diagrams in LaNi₅-H₂(D₂) system and inversion of isotopic effect
title_full Simulation of phase diagrams in LaNi₅-H₂(D₂) system and inversion of isotopic effect
title_fullStr Simulation of phase diagrams in LaNi₅-H₂(D₂) system and inversion of isotopic effect
title_full_unstemmed Simulation of phase diagrams in LaNi₅-H₂(D₂) system and inversion of isotopic effect
title_sort simulation of phase diagrams in lani₅-h₂(d₂) system and inversion of isotopic effect
author Marinin, V.S.
Shmalko, Yu.F.
Umerenkova, K.R.
author_facet Marinin, V.S.
Shmalko, Yu.F.
Umerenkova, K.R.
topic Modeling and simulation
topic_facet Modeling and simulation
publishDate 2007
language English
container_title Functional Materials
publisher НТК «Інститут монокристалів» НАН України
format Article
title_alt Моделювання фазових діаграм у системі LaNi₅-H₂(D₂) та інверсія ізотопного ефекту
description Simulation of phase transitions in IMC-hydrogen systems based on modified scheme of perturbation theory provides correct description of main characteristics of phase diagrams within a wide pressure range of hydrogen isotopes (6 decimal orders and wider). The obtained data on thermodynamic parameters of α-β transition allows to describe inversion of isotopic effect in LaNi₅-H₂(D₂) system. Data on solubility of hydrogen isotopes in LaNi₅ at pressures up to 500 atm. have been obtained; data on parameters of the critical points of α-β equilibrium (for which experimental data are absent) have been also obtained. The proposed calculation scheme does not use any fitting parameters or empirical correlations and is based on atomic characteristics of the hydrogen subsystem and metallic matrix which are physically meaningful.
issn 1027-5495
url https://nasplib.isofts.kiev.ua/handle/123456789/136969
citation_txt Simulation of phase diagrams in LaNi₅-H₂(D₂) system and inversion of isotopic effect / V.S. Marinin, Yu.F. Shmalko, K.R. Umerenkova // Functional Materials. — 2007. — Т. 14, № 4. — С. 492-497. — Бібліогр.: 8 назв. — англ.
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first_indexed 2025-12-07T13:23:29Z
last_indexed 2025-12-07T13:23:29Z
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