The peculiarities of the properties of ZnSxSe₁-x nanocrystals obtained by self-propagating high-temperature synthesis

ZnSxSe₁-x nanocrystals of all compounds were obtained by self-propagating high-temperature synthesis. It was found that the obtained samples had dimensions of 55±5 nm and were characterized by a mixed crystalline structure. With increase the x value the fraction of the hexagonal phase in nanocrystal...

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Veröffentlicht in:Functional Materials
Datum:2018
Hauptverfasser: Kovalenko, A.V., Plakhtii, Ye.G., Khmelenko, O.V.
Format: Artikel
Sprache:English
Veröffentlicht: НТК «Інститут монокристалів» НАН України 2018
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Online Zugang:https://nasplib.isofts.kiev.ua/handle/123456789/157188
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Zitieren:The peculiarities of the properties of ZnSxSe₁-x nanocrystals obtained by self-propagating high-temperature synthesis / A.V. Kovalenko, Ye.G. Plakhtii, O.V. Khmelenko // Functional Materials. — 2018. — Т. 25, № 4. — С. 665-669. — Бібліогр.: 15 назв. — англ.

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Digital Library of Periodicals of National Academy of Sciences of Ukraine
id nasplib_isofts_kiev_ua-123456789-157188
record_format dspace
spelling Kovalenko, A.V.
Plakhtii, Ye.G.
Khmelenko, O.V.
2019-06-19T17:13:00Z
2019-06-19T17:13:00Z
2018
The peculiarities of the properties of ZnSxSe₁-x nanocrystals obtained by self-propagating high-temperature synthesis / A.V. Kovalenko, Ye.G. Plakhtii, O.V. Khmelenko // Functional Materials. — 2018. — Т. 25, № 4. — С. 665-669. — Бібліогр.: 15 назв. — англ.
1027-5495
DOI:https://doi.org/10.15407/fm25.04.665
https://nasplib.isofts.kiev.ua/handle/123456789/157188
ZnSxSe₁-x nanocrystals of all compounds were obtained by self-propagating high-temperature synthesis. It was found that the obtained samples had dimensions of 55±5 nm and were characterized by a mixed crystalline structure. With increase the x value the fraction of the hexagonal phase in nanocrystals decreased from 65±5 % to 30±5 %, and the fraction of the cubic phase increased in the corresponding ratios. Despite the formation of ZnSxSe₁-x solid solutions, according to RCS data, the local environment of Mn2+ impurity ions is not mixed. At a value of 0.2<x&lq;1, the Mn²⁺ ions were surrounded by sulfur ions, and at x≤0.2 it was surrounded by selenium ions. The change of the Mn²⁺ ions local environment was accompanied by an abrupt change in the value of the RCS hyperfine structure of the Mn²⁺ ions from A = 6.88-6.91 mT to A = 6.55 mT. In ZnSxSe₁-x nanocrystals with x = 1 and x = 0.9, an EPR line with g = 1.9998 was detected, which is associated with an uncontrolled impurity - Cr⁺ ions.
en
НТК «Інститут монокристалів» НАН України
Functional Materials
Characterization and properties
The peculiarities of the properties of ZnSxSe₁-x nanocrystals obtained by self-propagating high-temperature synthesis
Article
published earlier
institution Digital Library of Periodicals of National Academy of Sciences of Ukraine
collection DSpace DC
title The peculiarities of the properties of ZnSxSe₁-x nanocrystals obtained by self-propagating high-temperature synthesis
spellingShingle The peculiarities of the properties of ZnSxSe₁-x nanocrystals obtained by self-propagating high-temperature synthesis
Kovalenko, A.V.
Plakhtii, Ye.G.
Khmelenko, O.V.
Characterization and properties
title_short The peculiarities of the properties of ZnSxSe₁-x nanocrystals obtained by self-propagating high-temperature synthesis
title_full The peculiarities of the properties of ZnSxSe₁-x nanocrystals obtained by self-propagating high-temperature synthesis
title_fullStr The peculiarities of the properties of ZnSxSe₁-x nanocrystals obtained by self-propagating high-temperature synthesis
title_full_unstemmed The peculiarities of the properties of ZnSxSe₁-x nanocrystals obtained by self-propagating high-temperature synthesis
title_sort peculiarities of the properties of znsxse₁-x nanocrystals obtained by self-propagating high-temperature synthesis
author Kovalenko, A.V.
Plakhtii, Ye.G.
Khmelenko, O.V.
author_facet Kovalenko, A.V.
Plakhtii, Ye.G.
Khmelenko, O.V.
topic Characterization and properties
topic_facet Characterization and properties
publishDate 2018
language English
container_title Functional Materials
publisher НТК «Інститут монокристалів» НАН України
format Article
description ZnSxSe₁-x nanocrystals of all compounds were obtained by self-propagating high-temperature synthesis. It was found that the obtained samples had dimensions of 55±5 nm and were characterized by a mixed crystalline structure. With increase the x value the fraction of the hexagonal phase in nanocrystals decreased from 65±5 % to 30±5 %, and the fraction of the cubic phase increased in the corresponding ratios. Despite the formation of ZnSxSe₁-x solid solutions, according to RCS data, the local environment of Mn2+ impurity ions is not mixed. At a value of 0.2<x&lq;1, the Mn²⁺ ions were surrounded by sulfur ions, and at x≤0.2 it was surrounded by selenium ions. The change of the Mn²⁺ ions local environment was accompanied by an abrupt change in the value of the RCS hyperfine structure of the Mn²⁺ ions from A = 6.88-6.91 mT to A = 6.55 mT. In ZnSxSe₁-x nanocrystals with x = 1 and x = 0.9, an EPR line with g = 1.9998 was detected, which is associated with an uncontrolled impurity - Cr⁺ ions.
issn 1027-5495
url https://nasplib.isofts.kiev.ua/handle/123456789/157188
citation_txt The peculiarities of the properties of ZnSxSe₁-x nanocrystals obtained by self-propagating high-temperature synthesis / A.V. Kovalenko, Ye.G. Plakhtii, O.V. Khmelenko // Functional Materials. — 2018. — Т. 25, № 4. — С. 665-669. — Бібліогр.: 15 назв. — англ.
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