Photo-spintronics of spin-orbit active electric weak links

We show that a carbon nanotube can serve as a functional electric weak link performing photo-spintronic transduction. A spin current, facilitated by strong spin-orbit interactions in the nanotube and not accompanied by a charge current, is induced in a device containing the nanotube weak link by cir...

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Published in:Физика низких температур
Date:2017
Main Authors: Shekhter, R.I., Entin-Wohlman, O., Jonson, M., Aharony, A.
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Language:English
Published: Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України 2017
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Online Access:https://nasplib.isofts.kiev.ua/handle/123456789/174618
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Cite this:Photo-spintronics of spin-orbit active electric weak links / R.I. Shekhter, O. Entin-Wohlman, M. Jonson, A. Aharony // Физика низких температур. — 2017. — Т. 43, № 8. — С. 1137-1140. — Бібліогр.: 7 назв. — англ.

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Digital Library of Periodicals of National Academy of Sciences of Ukraine
id nasplib_isofts_kiev_ua-123456789-174618
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spelling Shekhter, R.I.
Entin-Wohlman, O.
Jonson, M.
Aharony, A.
2021-01-26T07:49:05Z
2021-01-26T07:49:05Z
2017
Photo-spintronics of spin-orbit active electric weak links / R.I. Shekhter, O. Entin-Wohlman, M. Jonson, A. Aharony // Физика низких температур. — 2017. — Т. 43, № 8. — С. 1137-1140. — Бібліогр.: 7 назв. — англ.
0132-6414
PACS: 71.70.E, 75.70.Tj, 75.76.+j
https://nasplib.isofts.kiev.ua/handle/123456789/174618
We show that a carbon nanotube can serve as a functional electric weak link performing photo-spintronic transduction. A spin current, facilitated by strong spin-orbit interactions in the nanotube and not accompanied by a charge current, is induced in a device containing the nanotube weak link by circularly polarized microwaves. Nanomechanical tuning of the photo-spintronic transduction can be achieved due to the sensitivity of the spinorbit interaction to geometrical deformations of the weak link.
This work was partially supported by the Swedish Research Council (VR), by the Israel Science Foundation (ISF) and by the infrastructure program of Israel Ministry of Science and Technology under Contract No. 3-11173.
en
Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України
Физика низких температур
Low dimensionality and inhomogeneity effects in quantum matter
Photo-spintronics of spin-orbit active electric weak links
Article
published earlier
institution Digital Library of Periodicals of National Academy of Sciences of Ukraine
collection DSpace DC
title Photo-spintronics of spin-orbit active electric weak links
spellingShingle Photo-spintronics of spin-orbit active electric weak links
Shekhter, R.I.
Entin-Wohlman, O.
Jonson, M.
Aharony, A.
Low dimensionality and inhomogeneity effects in quantum matter
title_short Photo-spintronics of spin-orbit active electric weak links
title_full Photo-spintronics of spin-orbit active electric weak links
title_fullStr Photo-spintronics of spin-orbit active electric weak links
title_full_unstemmed Photo-spintronics of spin-orbit active electric weak links
title_sort photo-spintronics of spin-orbit active electric weak links
author Shekhter, R.I.
Entin-Wohlman, O.
Jonson, M.
Aharony, A.
author_facet Shekhter, R.I.
Entin-Wohlman, O.
Jonson, M.
Aharony, A.
topic Low dimensionality and inhomogeneity effects in quantum matter
topic_facet Low dimensionality and inhomogeneity effects in quantum matter
publishDate 2017
language English
container_title Физика низких температур
publisher Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України
format Article
description We show that a carbon nanotube can serve as a functional electric weak link performing photo-spintronic transduction. A spin current, facilitated by strong spin-orbit interactions in the nanotube and not accompanied by a charge current, is induced in a device containing the nanotube weak link by circularly polarized microwaves. Nanomechanical tuning of the photo-spintronic transduction can be achieved due to the sensitivity of the spinorbit interaction to geometrical deformations of the weak link.
issn 0132-6414
url https://nasplib.isofts.kiev.ua/handle/123456789/174618
citation_txt Photo-spintronics of spin-orbit active electric weak links / R.I. Shekhter, O. Entin-Wohlman, M. Jonson, A. Aharony // Физика низких температур. — 2017. — Т. 43, № 8. — С. 1137-1140. — Бібліогр.: 7 назв. — англ.
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AT entinwohlmano photospintronicsofspinorbitactiveelectricweaklinks
AT jonsonm photospintronicsofspinorbitactiveelectricweaklinks
AT aharonya photospintronicsofspinorbitactiveelectricweaklinks
first_indexed 2025-11-24T11:40:19Z
last_indexed 2025-11-24T11:40:19Z
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fulltext Low Temperature Physics/Fizika Nizkikh Temperatur, 2017, v. 43, No. 8, pp. 1137–1140 Photo-spintronics of spin-orbit active electric weak links R.I. Shekhter1, O. Entin-Wohlman2,3, M. Jonson1,4, and A. Aharony2,3 1Department of Physics, University of Gothenburg, SE-412 96 Göteborg, Sweden E-mail: mats.jonson@physics.gu.se 2Raymond and Beverly Sackler School of Physics and Astronomy, Tel Aviv University, Tel Aviv 69978, Israel 3Physics Department, Ben Gurion University, Beer Sheva 84105, Israel 4SUPA, Institute of Photonics and Quantum Sciences, Heriot-Watt University, Edinburgh, EH14 4AS, Scotland, UK Received January 18, 2017, published online June 26, 2017 We show that a carbon nanotube can serve as a functional electric weak link performing photo-spintronic transduction. A spin current, facilitated by strong spin-orbit interactions in the nanotube and not accompanied by a charge current, is induced in a device containing the nanotube weak link by circularly polarized microwaves. Nanomechanical tuning of the photo-spintronic transduction can be achieved due to the sensitivity of the spin- orbit interaction to geometrical deformations of the weak link. PACS: 71.70.Ej Spin-orbit coupling, Zeeman and Stark splitting, Jahn-Teller effect; 75.70.Tj Spin-orbit effects; 75.76.+j Spin transport effects. Keywords: spin-orbit interactions, spintronics. 1. Introduction Spintronics is a rapidly developing research area of modern solid state physics. In contrast to traditional elec- tronics, where the electric charge of electrons is in focus, the field of spintronics relies on another fundamental prop- erty of electrons, viz. their magnetic moment, which is as- sociated with their spin degree of freedom. Issues related to the electrical control of spin currents as well as to spin control of charge currents are at the heart of spintronics research today, both from a fundamental and an applied perspective [1]. Recently it has been suggested that such controls may be effectively implemented in nano- devices containing an electric weak link with strong spin- orbit interactions (SOI) that bridges bulk electrodes [2–4]. In [2] it was demonstrated that a spin-orbit coupling results in a “splitting” of the spin of electrons passing through such a weak link (Rashba spin splitting), which under cer- tain conditions may generate a spin current. This was shown to occur if an imbalance of the population of spin states in the electrodes is established by spin-flip assisted electronic transitions due to the absorption (or emission) of circularly polarized photons created by microwave pump- ing [5]. The SOI-induced spin generation inside the weak link makes it a point-like source of a spin current due to a photo-spintronic effect on the nanometer length scale. Es- timations show, however, that if the SOI is caused by an external electric field, as implicitly assumed in [2], that field has to be quite strong for the induced Rashba spin splitting to be significant. The aim of the present work is to demonstrate that a much stronger photo-spintronic trans- duction effect can be achieved if a material with an intrin- sic SOI, here assumed to be induced by stresses, is used for the weak link. The precise form of the stress-induced SOI depends on the material used for the electric weak link and the type of strains involved. In a single-wall carbon nanotube, which will be considered here, the strain can be thought of as occurring when a graphene ribbon is rolled up to form a tube. The strain-induced SOI in a simple one-dimensional model of such a nanotube is described by the Hamiltonian strain strain so so ˆ ˆ= ,F k ⋅n v σ (1) where Fv is the Fermi velocity, strain sok is a phenomenolog- ical parameter that gives the strength of the SOI in units of inverse length, σ is a vector whose components are the Pauli matrices , ,x y zσ , and n̂ is a unit vector pointing along the longitudinal axis of the nanotube in the direction of electron propagation ( ˆˆ =n k ). Equation (1), which was used in Ref. 3, is a simplified form of the SOI Hamiltonian previ- ously derived for a realistic model of such a nanotube [6]. © R.I. Shekhter, O. Entin-Wohlman, M. Jonson, and A. Aharony, 2017 mailto:mats.jonson@physics.gu.se R.I. Shekhter, O. Entin-Wohlman, M. Jonson, and A. Aharony The SOI active weak-link device shown in Fig. 1 com- prises a nanowire that bridges two bulk electronic reser- voirs. The spin-orbit interaction described by Eq. (1) is restricted to the nanowire and has the effect of scattering the spins of electrons that pass through the wire. Following the approach developed in Refs. 2–4 we will describe the transfer of electrons through the nanowire-based weak link with the help of a spin-dependent tunnel Hamiltonian. Hence, the total Hamiltonian of the system can be written as a sum of three parts, ˆ ˆ ˆ ˆ= ,L R T+ +    (2) where † ( ) ( ) ( )( ) ( ) ˆ =L R k p c c σσ σ ε∑ k pk p k p  (3) are Hamiltonians that describe the electrons in the left and right leads. These electrons are characterized by the mo- mentum quantum numbers k and p, respectively, and by the spin projection on the ẑ -axis. We label the latter by = 1σ ± , so that the spin projections are = /2s σ . The tun- nel Hamiltonian is expressed in terms of the probability amplitudes , ,[ ]W ′σ σp k for electron transmission through the wire, † , , , , ˆ = ( [ ] h. .).T c W c c′σ σ σ′σ ′σ σ +∑∑ p k kp k p  (4) These amplitudes have to be calculated taking the spin dynamics given by Hamiltonian (1) into account. 2. Spin-biased electric weak link Electronic transport through the weak link shown in Fig. 1 can be induced in a number of different ways. The standard method would be to apply a voltage bias V across the link, so that the chemical potentials for electrons in the left and right reservoirs are shifted by a small amount eV with respect to each other. The result of such charge bias- ing is that excess charge of opposite polarity is accumulat- ed on either side of the link, which leads to an electrical current through the link in a direction that counters the bias-induced charge imbalance. Another method, which will be in focus here and which is illustrated in Fig. 1, is to arrange for the chemical poten- tial to be different for the two possible projections of the electron spin along a certain axis. Such spin biasing can be achieved by illuminating the entire device with circularly- polarized microwave radiation of a frequency that enables electron spin-flip assisted photon absorption. This photonic pumping of the electronic spin creates an imbalance be- tween the number of electrons with opposite spin projec- tions on an axis defined by the direction of the radiation and leads to a spin-dependent shift in the chemical poten- tials for electrons with opposite spin projections. The mag- nitude of the shift, which extends throughout the device, depends on the intensity of the radiation and on the spin relaxation rate. If we assume that the SOI, which is re- stricted to the weak link, is the dominant spin relaxation mechanism the SOI becomes a source of a spin current, which flows out of the weak link into the two reservoirs and which counteracts the spin pumping. Referring to Fig. 1, we note that both the orientation of the plane that contains the weak link with respect to the pumped spin orientation and the bending angle of the link can be used to tune the gener- ated spin current. The spin bias U can be defined by noting that for ˆ = 0T the electron spin reservoirs are described by Fer- mi–Dirac distributions with different chemical potentials, † ˆ( ) ( ) ( )( ) =0= = ( ),FT f c c nσ σ σσ〈 〉 ε −µk p k p k pk p  (5) where = /2, = 1,Uσµ µ −σ σ ± (6) and µ is the chemical potential of both leads at equilibri- um. The spin current generated by electrons tunneling out of the SOI-active weak link can be obtained as the time derivative of the total spin, Ŝ〈 〉 , of the electrons, spin = 1 ˆˆ = = , 2 dd SJ dt dt σ σ ± 〈 〉 σ 〈 〉∑   (7) where † ( ) ( )( ) ( ) ˆ ˆ ˆ ˆ= , = .L R L R c cσ σ σ σ σσ+ ∑ k pk p k p     (8) Fig. 1. (Сolor online) Schematic picture of the device considered. A bent nanowire with a strong spin-orbit interaction bridges two bulk reservoirs. The bent nanowire is modeled by two equal- length straight wire segments which form angles θ and −θ with the x̂ -axis, respectively, while the plane that contains the nan- owire is tilted by an angle γ away from the ŷ -axis towards the ẑ- axis. The device is irradiated by circularly-polarized microwave radiation (wavy arrows) that creates a difference in the population of spin-up and spin-down electrons (thick vertical arrows) corre- sponding to a “spin biasing” of the device. Spin-flip transitions induced by the spin-orbit interaction in the nanowire create a spin current spin spin spin= L RJ J J+ traveling out from the wire with a magnitude that depends on the angles θ and γ . 1138 Low Temperature Physics/Fizika Nizkikh Temperatur, 2017, v. 43, No. 8 Photo-spintronics of spin-orbit active electric weak links A straightforward calculation of the spin current (7) can be done using the tunnel Hamiltonian (1) to lowest order in perturbation theory [2]. Then, one finds for the spin con- ductance spinG (defined in analogy with the electrical con- ductance G) the relation spin spin= / for 0.G J U U → (9) 3. Rashba spin splitting as a source of spin generation in an SOI active weak link In order to calculate the spin current given by Eq. (7) one needs to evaluate the electronic transmission amplitudes , ,[ ]W ′σ σp k , which appear in the tunnel Hamiltonian (4), and specifically their dependence on the spin-orbit interaction as given by Eq. (1). In our simple model the weak link consists of two straight parts of equal length | |=| | = /2L R dR R joined by a bend. Neglecting the momentum (but not the spin) dependence, the probability amplitude for an electron of ener- gy E to pass from, say, the left to the right lead can be written as a product of five factors, = ( , ) ( , ) .R R L LW T G E G E TR R (10) Here W is a 2×2 matrix in spin space, ( )L RT is the proba- bility amplitude to tunnel from the wire to the left (right) lead and  is the transfer matrix through the bend in the wire. In Ref. 4 the Green’s function ( )( ; )L RG ER for the straight segments of the wire, in which the SOI interaction takes place, was evaluated for a Hamiltonian of the form 2 2 * ˆ = ( ) . 2 k m + ⋅Q k  σ (11) A comparison with Eq. (1) shows that in the present case strain so ˆ( ) = F kQ k nv . Hence, from Eqs. (A12) and (A13) of Ref. 4 we conclude that ( ) 0 ( )( , ) = ( , )L R L RG E G E ×R R ( )ˆ[cos( ) sin( ) ],L Ri× α − α ⋅n σ (12) where we have used the short-hand notation strain so /2k d ≡ α, which is a measure of the strength of the SOI, and where 2* 0 ( ) 0 0 ( )( , ) = ( / ) exp[ | |],L R L RG E i m k ikπR R (13) with 2 1/2* 0 = (2 / )k m E  , is the propagator on the left (right) segment in the absence of SOI. It follows that we can factor out the dependence on the SOI and write the amplitude given by Eq. (10) as 0= ,W W  (14) where 0 0 0= (| |, ) (| |, )R R L LW T G E G E TR R (15) is the SOI-independent part and ˆ ˆ= [cos( ) sin( ) ][cos( ) sin( ) ]R Li iα − α ⋅ α − α ⋅n n σ σ (16) contains the effect of the SOI. In our geometry the ẑ -axis is the spin quantization ax- is, and the bent wire lies in a plane that (i) contains the x̂-axis and (ii) is rotated by an angle γ away from the ŷ-axis towards the ẑ -axis. In the plane of the wire, the left (right) straight leg of the wire forms an angle θ (−θ) with the x̂-axis. In other words, ˆ ˆ ˆ ˆ= cos( ) sin( )[cos( ) sin( ) ],L θ + θ γ + γn x y z ˆ ˆ ˆ ˆ= cos( ) sin( )[cos( ) sin( ) ] ,R θ − θ γ + γn x y z (17) which means that we can write Eq. (16) in a matrix form, = ,W A i− ⋅B σ (18) where 2 2 ˆ ˆ= ( ) ( )cos sin R LA α − α ⋅ =n n 2 2= ( ) ( ) cos(2 ) ,cos sinα − α θ (19) and 2ˆ ˆ ˆ ˆ= sin( ) cos( )( ) ( )sinR L R Lα α + + α × =B n n n n 2ˆ ˆ= sin(2 )cos( ) sin ( )sin(2 )sin( )α θ − α θ γ +x y 2ˆ sin ( )sin(2 )cos( ) .+ α θ γz (20) Hence, the probability for a SOI-induced spin-flip transi- tion is 2 2 2| | = | | | |x yw B B↑↓ ↑↓≡ + = 2 2 4 2 2= sin (2 )cos ( ) sin ( )sin (2 )sin ( ) .α θ + α θ γ (21) The spin conductance can now be expressed in terms of the spin-flip probability w↑↓ as spin 2= ( , ). / GG w e ↑↓ θ γ  (22) Equations (21) and (22) represent the main results of the paper. The strength of the SOI, characterized by the di- mensionless parameter strain so= /2k dα , determines the amount of photo-spintronic transduction that can be achieved by the studied Rashba spin-splitter device. The sensitivity of the effect to the geometry of the experimental set-up opens the possibility for tuning the device nano- mechanically, by varying the angles γ and θ. The depend- ence of the spin conductance on these experimentally ac- cessible device parameters is illustrated in Figs. 2 and 3. The photo-spintronic transduction occurs even for a straight wire (i.e., when = 0θ ). However, wire deformation provides a tool for a nanomechanical control of the gener- ated spin current. Depending on the strength of SOI cou- pling α, both a monotonic and a non-monotonic depend- ence of the dimensionless spin-conductance w↑↓ on mechanical deformations can be achieved. Figure 2 illustrates that the dimensionless conductance, w↑↓ , is an oscillatory function of the angle γ . As is clear Low Temperature Physics/Fizika Nizkikh Temperatur, 2017, v. 43, No. 8 1139 R.I. Shekhter, O. Entin-Wohlman, M. Jonson, and A. Aharony from Eq. (21), the maximal [minimal] value, m ( )axwα θ m[ ( )]inwα θ , of = ( )w w↑↓ ↑↓ γ is achieved when the normal to the plane containing the nanowire weak link is perpendicu- lar [parallel] to the spin quantization axis, i.e. when = / 2γ ±π [ = 0γ or π] and therefore 2( ) = 1sin γ 2[ ( ) = 0]sin γ , inde- pendent of the values of α and θ. For a strong enough SOI, i.e., when 2sin ( ) 1/2α ≥ , the largest possible value, max ( ) = 1wα θ , is reached when the bending angle is = αθ θ , where 2 2cos ( ) = 1/[2sin ( )]αθ α , as illustrated in Fig. 3. On the other hand, for 2sin ( ) < 1/2α the effect is smaller since then 2 max ( ) < sin (2 ) < 1wα θ α . 4. Conclusions In this paper we have shown that a nanowire, in which the electrons are subjected to a spin-orbit interaction (SOI), can be used as a functional electric weak link between SOI-inactive leads and serve as an essentially point-like source of a spin-current induced by circularly-polarized microwave radiation. This spin current is not accompanied by a charge current. The possibility to concentrate such “pure” spin-currents at the nanometer length scale suggests novel spintronic devices. Whether realistic applications are feasible crucially de- pends on how strong a photo-spintronic effect can be real- ized in practice, which in turn depends on the strength of the SOI that can be achieved. Consider, for instance, a sin- gle-wall carbon nanotube. Its strain-induced SO energy gap strain so∆ has been measured to be around 0.4 meV [7]. Since strain strain so so= 2 F k∆ v , this value corresponds to strain 6 so 0.4 10k ≈ ⋅ m–1 for 60.5 10F ≈ ⋅v m/s. For nanowire lengths d of the order of a µm, strain sok d can therefore be of order 1, which is large enough to allow the dimensionless spin conductance to be tuned near to its maximal value = 1w↑↓ . This work was partially supported by the Swedish Re- search Council (VR), by the Israel Science Foundation (ISF) and by the infrastructure program of Israel Ministry of Science and Technology under contract 3-11173. 1. D.D. Awschalom, L.C. Bassett, A.S. Dzurak, E.L. Hu, and J.R. Petta, Science 339, 1174 (2013). 2. R.I. Shekhter, O. Entin-Wohlman, and A. Aharony, Phys. Rev. Lett. 111, 176602 (2013); R.I. Shekhter, O. Entin- Wohlman, and A. Aharony, Phys. Rev. B 90, 045401 (2014). 3. R.I. Shekhter, O. Entin-Wohlman, M. Jonson, and A. Aharony, Phys. Rev. Lett. 116, 217001 (2016). 4. R.I. Shekhter, O. Entin-Wohlman, M. Jonson, and A. Aharony, Fiz. Niz. Temp. 43, 368 (2017) [Low Temp. Phys. 43, 309 (2017)]. 5. K. Koyama and H. Merz, Z. Physik B 20, 131 (1975); M. Wohlecke and G. Borstel, Phys. Status Solidi B 106, 593 (1981). 6. M.S. Rudner and E.I. Rashba, Phys. Rev. B 81, 125426 (2010); K. Flensberg and C.M. Marcus, Phys. Rev. B 81, 195418 (2010). 7. F. Kuemmeth, S. Ilani, D.C. Ralph, and P.L. McEuen, Nature 452, 448 (2008). Fig. 2. The dimensionless spin conductance ( , )w↑↓ θ γ defined in Eqs. (21) and (22), plotted as a function of the tilt angle γ of the plane that contains the nanowire weak link (see Fig. 1). The spin conductance oscillates between a maximal value max ( )wα θ and a minimal value min ( )wα θ , which both depend on the bend angle θ and the strength α of the spin-orbit interaction in the wire. Here = = /4α θ π for which max ( ) = 0.75wα θ and min ( ) = 0.50wα θ . Fig. 3. The maximal value max ( )wα θ of the dimensionless spin conductance ( , )w↑↓ θ γ [obtained for 2sin ( ) = 1γ ] and the minimal value min ( )wα θ of ( , )w↑↓ θ γ [obtained for 2sin ( ) = 0γ ] plotted as functions of the nanowire bend angle θ defined in Fig. 1. The two pairs of curves are for two different values of the spin-orbit inter- action strength α in the nanowire: the upper pair pertains for = /3α π , for which 2sin > 1/2α , and the lower one pertains for = /8α π , for which 2sin ( ) < 1/2α . Note that when 2sin ( ) 1/2α ≥ the maximal spin conductance max ( )wα θ reaches the value 1 for 2 2cos ( ) = 1/[2sin ( )]θ α . When 2sin ( ) < 1/2α both max ( )wα θ and min ( )wα θ decrease monotonically from 2sin (2 )α to 0. 1140 Low Temperature Physics/Fizika Nizkikh Temperatur, 2017, v. 43, No. 8 1. Introduction 2. Spin-biased electric weak link 3. Rashba spin splitting as a source of spin generation in an SOI active weak link 4. Conclusions