Rashba proximity states in superconducting tunnel junctions

We consider a new kind of superconducting proximity effect created by the tunneling of “spin split” Cooper pairs between two conventional superconductors connected by a normal conductor containing a quantum dot. The difference compared to the usual superconducting proximity effect is that the spin s...

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Опубліковано в: :Физика низких температур
Дата:2018
Автори: Entin-Wohlman, O., Shekhter, R.I., Jonson, M., Aharony, A.
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Опубліковано: Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України 2018
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Цитувати:Rashba proximity states in superconducting tunnel junctions / O. Entin-Wohlman, R.I. Shekhter, M. Jonson, A. Aharony // Физика низких температур. — 2018. — Т. 44, № 6. — С. 701-710. — Бібліогр.: 31 назв. — англ.

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Digital Library of Periodicals of National Academy of Sciences of Ukraine
_version_ 1860097300116799488
author Entin-Wohlman, O.
Shekhter, R.I.
Jonson, M.
Aharony, A.
author_facet Entin-Wohlman, O.
Shekhter, R.I.
Jonson, M.
Aharony, A.
citation_txt Rashba proximity states in superconducting tunnel junctions / O. Entin-Wohlman, R.I. Shekhter, M. Jonson, A. Aharony // Физика низких температур. — 2018. — Т. 44, № 6. — С. 701-710. — Бібліогр.: 31 назв. — англ.
collection DSpace DC
container_title Физика низких температур
description We consider a new kind of superconducting proximity effect created by the tunneling of “spin split” Cooper pairs between two conventional superconductors connected by a normal conductor containing a quantum dot. The difference compared to the usual superconducting proximity effect is that the spin states of the tunneling Cooper pairs are split into singlet and triplet components by the electron spin-orbit coupling, which is assumed to be active in the normal conductor only. We demonstrate that the supercurrent carried by the spin-split Cooper pairs can be manipulated both mechanically and electrically for strengths of the spin-orbit coupling that can realistically be achieved by electrostatic gates.
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fulltext Low Temperature Physics/Fizika Nizkikh Temperatur, 2018, v. 44, No. 6, pp. 701–710 Rashba proximity states in superconducting tunnel junctions O. Entin-Wohlman1,2, R.I. Shekhter3, M. Jonson3, and A. Aharony1,2 1Raymond and Beverly Sackler School of Physics and Astronomy, Tel Aviv University, Tel Aviv 69978, Israel 2Physics Department, Ben Gurion University, Beer Sheva 84105, Israel E-mail: oraentin@bgu.ac.il 3Department of Physics, University of Gothenburg, SE-412 96 Göteborg, Sweden Received January 15, 2018, published online April 25, 2018 We consider a new kind of superconducting proximity effect created by the tunneling of “spin split” Cooper pairs between two conventional superconductors connected by a normal conductor containing a quantum dot. The difference compared to the usual superconducting proximity effect is that the spin states of the tunneling Cooper pairs are split into singlet and triplet components by the electron spin-orbit coupling, which is assumed to be active in the normal conductor only. We demonstrate that the supercurrent carried by the spin-split Cooper pairs can be manipulated both mechanically and electrically for strengths of the spin-orbit coupling that can real- istically be achieved by electrostatic gates. PACS: 72.25.Hg Electrical injection of spin polarized carriers; 72.25.Rb Spin relaxation and scattering. Keywords: spin-orbit interaction, Rashba spin splitter, Josephson effect, electric weak link. 1. Introduction The prominent role that the electronic spin plays in de- termining the properties of solid-state devices has been at the forefront of experimental and theoretical research during the last decade. The topological surface electronic states, that are formed due to a strong spin-orbit coupling, with their vast potential for quantum computations [1,2] and spintronic applications [3] of spin-polarized currents, are just a few conspicuous examples. Conducting nanostructures, e.g., quantum dots, nanowires and nanorings, where the mesoscopic behavior of the electrons is dominated by Cou- lomb correlations and quantum-phase coherence, are by now the tools of choice for studying spin-related phenom- ena, in particular effects induced by the spin-orbit cou- pling. Composite mesoscopic structures comprising such nanometer-sized elements are currently of considerable interest due to their applicability in quantum communica- tion systems [4–6]. The hope is to provide a coherent plat- form for flying qubits: moving two-state spinors, which may represent the electronic spin [7] or any other pseudo-spin state, e.g., of particles moving in two coupled wires [8]. Clearly, spin-state decoherence is detrimental to spin- tronics applications involving, e.g., flying qubits. Reducing the scattering rate of spin-polarized electrons in order to pre- serve spin coherence is therefore essential, and is the rea- son why using superconducting materials have been con- sidered. However, while electron transport in a supercon- ductor is indeed fully coherent, the supercurrent carried by spin-singlet Cooper pairs in a conventional superconductor conducts charge but not spin. If, on the other hand, the Cooper pairs could be spin polarized it would mean that a coherent, dissipationless spin current could be generated. Hence, it is highly desirable to find methods for generating spin-polarized Cooper pairs. Recently, such a method — involving the creation of spin-polarized Cooper pairs in superconducting weak links made of materials with a strong spin-orbit interaction (SOI) — was proposed. It was shown that the spin-structure of the Cooper pairs, injected into a non-superconducting material in which the spin-orbit inter- action is significant, can be “predesigned” in such a way that a net electronic spin-polarization is carried through an SOI- active weak link that connects the superconducting leads. The physics behind this phenomenon is the splitting of the transferred electronic states within the weak link with re- spect to spin — the so-called “Rashba spin-splitting” [9]. As a consequence of this spin splitting, the electronic spin expe- riences quantum fluctuations that lead to a “triplet-channel” for Cooper-pair transport through the link. © O. Entin-Wohlman, R.I. Shekhter, M. Jonson, and A. Aharony, 2018 O. Entin-Wohlman, R.I. Shekhter, M. Jonson, and A. Aharony The ability to inject electrons paired in a spin-triplet state into a conventional BCS superconductor from an SOI-active superconducting weak link, opens a route to all kinds of spintronics applications that can be implemented by using a dissipationless spin current. However, the ap- pearance of spin-triplet Cooper pairs in a conventional BCS superconductor is a so-called proximity effect, and spin-polarized Cooper pairs are present only in the vicinity of the weak link. In addition, the triplet states are vulnera- ble to any spin-relaxation mechanism in the superconduc- tor. A clever composite device-design is therefore required to allow for the accumulation of paired electrons with a non-zero net spin, while significantly blocking their spin relaxation. In the present paper we suggest such a design, and pro- pose a new type of a superconducting weak link in which Rashba spin-split states involving pairs of time-reversed (“Cooper pair”) states can be established through the prox- imity effect. The generic component of the device is a quantum dot coupled to two superconductors through SOI- active weak links in the form of nanowires, as illustrated in Fig. 1. A significant advantage of the device is its relative- ly low spin relaxation rate — a well-known property of quantum dots [10–14]. The extent to which spin is accu- mulated on the dot can be controlled by electric fields that modify the SOI strength [15–18]. Another handle on the device is the possibility to tune mechanically the physical location of the dot, and thus affect the amount of tunneling between the two reservoirs [19,20]. The paper is organized as follows. Section 2 introduces the Hamiltonian of our model and details the calculation of the transmission of Cooper pairs between two supercon- ductors connected by a weak link on which the transferred electrons are subjected to a spin-orbit interaction. We in- clude in the calculation two important effects. (i) The SOI on the left wire can differ from the one on the right wire (see Fig. 1), both in strength and in the direction of the effective magnetic field that characterizes this interaction. (ii) The passage of a Cooper pair through the weak link can take place either by sequential tunneling, during which the two electrons tunnel one by one and the dot is at most sin- gly occupied, or by events in which the two electrons hap- pen to reside simultaneously on the dot during the tunnel- ing. In the latter case, one has to account for the Coulomb interaction on the dot. Obviously these two processes con- tribute disparately to the transport. We dwell on the two separate contributions and their dependence on the geome- try of the junction in Sec. 3. Since we consider in Sec. 2 the transfer of Cooper pairs, in which the two electrons are in time-reversed states, we need to construct the relation between the (spin-dependent) tunneling amplitudes in the- se two states. This task is accomplished in Appendix A. The transmission of Cooper pairs is analyzed by studying the equilibrium Josephson current between the two reser- voirs. In particular, we analyze the manner by which the spins of the tunneling electrons precess as they pass through the weak link. Technical details of this calculation are relegated to Appendix B. Section 3 presents the results. We derive there explicit expressions for the spin-precession factor of each of the two processes alluded to above, and explain the way the disparity between the two reflects the coherence of the sequential single-electron tunneling process, and the inco- herence of the double-electron one, during which the dot is doubly occupied. We also analyze there the dependence of the Cooper pairs’ transmission on the relative angle be- tween the two directions of the SOI’s on the two wires. Our conclusions are discussed in Sec. 4. 2. Tunneling of Cooper pairs 2.1. Description of the model The spin splitting of electrons that flow through a weak link in which the Rashba [21,22] spin-orbit interaction is active, can be understood within a semiclassical picture. As the electrons pass through the weak link, their spins precess around an effective magnetic field associated with the SOI. This spin dynamics splits the electron wave func- tion into different spin states and yields a certain probabil- ity, which can be controlled externally, for the spins to be flipped as they emerge from the weak link [23]. The spin- splitting phenomenon becomes more complicated when the transmission of a pair of electrons in two time-reversed states through an SOI-active weak link is considered. In that case there are two types of tunneling events, those where the electrons are transferred one by one sequentially, and those in which the dot is doubly occupied during the tunneling. This is taken into account in our model by rep- resenting the quantum dot as a single localized level of energy ε which can accommodate two electrons in two spin states (“up” and “down”). In our simple model the reservoirs that supply the electrons are two bulk BCS su- perconductors; these are coupled together by a nanowire on which the quantum dot is located. When on the dot, the spin state of one electron of the Cooper pair is projected on the spin-up state of the dot, and that of the other on the spin-down state [24]. We find that the projection breaks the coherent evolution of the spin states. The Pauli princi- Fig. 1. (Color online) Spin-orbit active superconducting weak- link. The quantum dot is represented by a single localized level of energy ε , and the superconducting reservoirs are denoted LS and RS . The tunneling amplitude (a matrix in spin space) between the dot and the left (right) lead is denoted kt ( pt ). 702 Low Temperature Physics/Fizika Nizkikh Temperatur, 2018, v. 44, No. 6 Rashba proximity states in superconducting tunnel junctions ple is assumed to be effective only on the quantum dot; elsewhere the passage of the electrons in and out of the dot is viewed as a single-electron tunneling event, whose am- plitude includes the electronic spin precession [25]. The Hamiltonian of the junction illustrated in Fig. 1 reads 0 tun= .+   (1) The Hamiltonian 0 pertains to the decoupled system, and includes the Hamiltonian of the quantum dot and that of the superconducting leads, † †† 0 lead = , = . L R d d Ud d d d α σ σ ↑ ↓↑ ↓ σ α ε + +∑ ∑  (2) The operator dσ ( †dσ) annihilates (creates) an electron in the spin state | σ〉 on the dot, and U denotes the Coulomb repulsion. The BCS leads are described by the annihilation (creation) operators of the electrons there, ( )c σk p ( † ( )c σk p ). [k (p) enumerates the single-particle orbital states on the left (right) lead.] Denoting by ( )k pε the single-electron energy measured relative to the common chemical poten- tial of the device, the Hamiltonian of the leads is = ( ) † ( ) ( )lead ( ) ( ), =L R k p c cα σσ σ ε −∑ k pk p k p  † †( ) ( ) ( ) ( ) ( ) (e H.c.), i L R L R c c ϕ ↑ − − ↓ −∆ +∑ k p k p k p (3) where ( )L R∆ and ( )L Rϕ are the amplitude and the phase of the superconducting order parameters. The tunneling Hamiltonian is the key component of our model, tun = H.c. ,LD RD+ +   (4) where ( )† ( ) ( ) ( ) ( ), , = [t ] .L R D L R D c d′ ′σσ σσ ′σ σ ∑ k p k p k p  (5) The probability amplitude for the transfer of an electron from the spin state | ′σ 〉 on the dot to the state | ( ),σ〉k p in the left (right) reservoir is ( ) ( )[t ]L R D ′σσk p , which allows for spin flips during the tunneling. This amplitude is conven- iently separated into a (scalar) orbital amplitude, and a unitary matrix (in spin space), denoted W, that contains the effects of the SOI (whether of the Rashba [21,22] or the Dresselhaus [26] type), and also the dependence on the spatial direction of the SOI-active wire. The spin-orbit in- teraction associated with strains is briefly mentioned in Sec. 3. For the linear SOI [9], the tunneling amplitude can be presented in the form ( ) ( )( ) ( )t = e , ikL R D L R DF L R L R d it − k W (6) where Fk is the Fermi wave vector in the leads, and ( )L Rd is the length of the bond between the left (right) lead and the dot. The generic form of W is [27,28] ( ) ( ) ( )= ,L R D L R L Ra i+ ⋅W bσ (7) where ( )L Ra is a real scalar and ( )L Rb is a real vector (de- termined by the symmetry axis of the SOI and the spatial direction of the weak link), with 2 ( ) ( ) ( ) = 1L R L R L Ra + ⋅b b (σ is the vector of the Pauli matrices). In the absence of the spin-orbit interaction ( )L RW is just the unit matrix, name- ly, ( ) = 1L Ra and ( ) = 0L Rb . Explicit expressions for the spin-orbit coupling are discussed in Sec. 3. Since the two electrons of a Cooper pair are in two states connected by the time-reversal transformation, one has to consider also the tunneling amplitude between the time-reversed states of | ′σ 〉 and | ( ),σ〉k p , which we denote by an overline, i.e., | ( ) |yi′ ′σ 〉 ≡ σ σ 〉 and | ( ), .− − σ〉k p The corresponding amplitude, ( ) ( )[ ]L R D ′σσk pt , describes the trans- fer of an electron from the spin state | ′σ 〉 on the dot to the state | ( ),− − σ〉k p in the left (right) lead. It is given by ( ) ( ) 1 ( ) ( ) ˆ ˆ; = ( ) ,L R D L R D yK i−≡ σk p k pt Tt T T (8) ( yσ is a Pauli matrix, and K is the complex conjugation operator). We derive in Appendix A the relation ( ) ( ) ( ) ( )[ ] = [( ) ] ,L R D L R D ∗ ′ ′σσ σσk p k pt t (9) which is of paramount importance in our considerations. 2.2. The particle current The flow of electrons between the two superconductors is analyzed by studying the equilibrium Josephson current, i.e., the rate by which electrons leave the left (or the right) superconductor, when the chemical potentials of the two reservoirs are identical (and therefore a flow of quasi- particles is prohibited by the gap in the quasiparticle densi- ty of states in the superconducting leads). Using units in which = 1 , this rate is † , = ( / ) = 2Im ( ) ,LDJ d dt c c tσσ σ − 〈 〉 − 〈 〉∑ kk k  (10) where the angular brackets denote quantum averaging. It is evaluated using the S-matrix, 1( ) = ( , ) ( ) ( , ) ,LD LDt S t t S t−〈 〉 〈 −∞ −∞ 〉  (11) with 0 0( ) = exp[ ] exp[ ]LD LDt i t i t−    , and the quan- tum average is with respect to 0 . As the leading-order contribution to J is fourth-order in the tunneling Hamilto- nian, it is found from the expansion up to third order of the S-matrix [29], Low Temperature Physics/Fizika Nizkikh Temperatur, 2018, v. 44, No. 6 703 O. Entin-Wohlman, R.I. Shekhter, M. Jonson, and A. Aharony 1 1 2 1 tun 1 1 2 tun 1 tun 2 1 2 3 tun 1 tun 2 tun 3 ( , ) =1 ( ) ( ) ( ) ( ) ( ) ( ) . tt t t tt S t i dt t dt dt t t i dt dt dt t t t −∞ −∞ −∞ −∞ −∞ −∞ −∞ − − + + ∫ ∫ ∫ ∫ ∫ ∫       (12) The energy level on the dot is assumed to lie well above the chemical potential of the leads, and thus the small pa- rameter of the expansion is /Γ ε , where = L RΓ Γ +Γ is the total width of the resonance level created on the dot due to the coupling with the bulk reservoirs (each coupling induc- es a partial width ( )L RΓ , see Appendix B). This implies that the perturbation expansion is carried out on a dot which is empty when decoupled [30]. We list and discuss the relevant terms in the expansion of J in Appendix B. As mentioned, the total Josephson current in our junc- tion is due to the two processes available for the tunneling pairs. In the first, whose contribution is denoted sJ , double occupancy on the dot does not occur, and the transfer of the electron pair is accomplished by a sequential tunneling of the paired electrons one by one. In the second process that contributes dJ , the dot is doubly occupied during the tunneling. The (lengthy but straightforward) calculation presented in Appendix B yields ,s dJ J J= + (13) where 0 0 ( / ) , 2 ( / , / ) . s s s d d d J I F J I F U = ε ∆ = ε ∆ ∆   (14) These results are obtained, for simplicity, in the zero- temperature limit, and for =L R∆ ∆ ≡ ∆. The common fac- tor 0I in the expressions for sJ and dJ is the Josephson amplitude of the interface between the two superconduc- tors (i.e., when the localized level on the dot as well as the SOI are ignored), 0 = 2sin( )[ / ]R L L RI ϕ −ϕ Γ Γ ∆ . The dis- parity of the two tunneling processes comes into play in the other two factors in Eqs. (14). The functions sF and dF [31], given in Eqs. (B5) and (B9) and reproduced here for convenience, 1( ) cosh 1 1 , , cosh cosh cosh ps k k k p p dd F ∞ ∞ −∞ −∞ ζζ ε = × π π ζ + ε ε × ε = ζ + ζ ζ + ε ∆ ∫ ∫    (15) and 1( , ) cosh 1 1 , , , cosh2 pd k k p dd F U UU U ∞ ∞ −∞ −∞ ζζ ε = × π π ζ + ε ε × ε = = ζ + ε ∆ ∆ε + ∫ ∫       (16) convey the effect of the resonance on the dot, and the Cou- lomb repulsion there. As seen, the Pauli principle tends to reduce the contribution of the second tunneling process. The last factors, s and d , describe the amount of spin precession. Their detailed analysis is the topic of the next subsection. These two factors become 1 in the absence of the SOI. It follows that in the absence of the SOI, the Jo- sephson current of our junction, 0J , is 0 0= [ ( / ) 2 ( / , / )] .s dJ I F F Uε ∆ + ε ∆ ∆ (17) The normalized Josephson current, i.e., J of Eq. (13) di- vided by 0J , is 0 ( / ) 2 ( / , / ) . ( / ) 2 ( / , / ) s s d d s d J F F U J F F U ε ∆ + ε ∆ ∆ = ε ∆ + ε ∆ ∆   (18) 2.3. Spin precession In the sequential tunneling process, where the pair of electrons tunnel one by one, their spin-precession factor is , , 1= sgn ( )sgn ( ) 2 [( ) ] [ ] [( ) ] [ ] , s L R L R LD LD DR DR L L R R ′σ σ σ σ ∗ ∗ ′ ′σ σ σ σ σ σ σσ σ σ × × ∑ ∑ W W W W  (19) while the spin-precession factor of the tunneling process during which the dot is doubly occupied is , 1= sgn( )sgn ( ) 2 [( ) ] [ ] [( ) ] [ ] . d L R L R LD LD DR DR L L R R σ σ σ ∗ ∗ σ σ σ σ σσ σσ σ σ × × ∑ ∑ W W W W  (20) [See the derivation in Appendix B that leads to Eqs. (B4) and (B8), reproduced in Eqs. (19) and (20) for convenience.] It is illuminating to scrutinize the summations over the spin indices. The factor s can be written as , 2 2 1= sgn( )sgn( )[( ) ] [ ] 2 = |[ ] | |[ ] | , s LR LR L R L R L R L R LR LR ∗ σ σ σ σ σ σ ↑↑ ↑↓ σ σ = − ∑ W W W W  (21) where the direct spin part of the tunneling amplitude from the right lead to left one is [ ] = [ ] [ ] .LR LD DR L R L Rσ σ σ σ σσ σ ∑W W W (22) In contrast, the spin-precession factor of the double- occupancy channel cannot be expressed in terms of the direct amplitudes; we find 2 2 2 2 = (| [ ] | | [ ] | ) (| [ ] | | [ ] | ) . d LD LD DR DR ↑↑ ↑↓ ↑↑ ↑↓ − × × − W W W W  (23) 704 Low Temperature Physics/Fizika Nizkikh Temperatur, 2018, v. 44, No. 6 Rashba proximity states in superconducting tunnel junctions One notes that d , Eq. (23), is a product of two factors of the same structure as the single factor in s , Eq. (21). Our interpretation is that s describes the coherent transfer of a Cooper pair from the right to the left lead, while d de- scribes first a coherent Cooper pair transfer from the right lead to the dot, where coherence is lost, then a second co- herent transfer from the dot to the left lead. Both contribu- tions to the Josephson current, sJ and dJ [see Eqs. (13) and (14)], are suppressed to a certain extent by the spin- precession (as compared with their respective values in the absence of the SOI). Which of them is more severely af- fected is determined by the geometry of the junction and the symmetry direction of the SOI. This feature is dis- cussed in Sec. 3. The effect of the spin-orbit coupling on the super- current is embedded in the precession of the spins it in- duces. It is therefore natural to express the current, in particular the precession factors, in terms of orientations of the effective magnetic fields responsible for the pre- cession in the left and right SOI-active nanowires. In- deed, upon carrying out the spin summations in Eqs. (18) and (20) within each reservoir [i.e., on Lσ and Rσ using Eq. (7) for W], one finds that these factors can be ex- pressed in terms of the vectors LV and RV , that represent the effective magnetic fields, sgn ( )[( ) ] [ ] [ ] , sgn ( )[ ] [( ) ] [ ] . LD LD L LL L L DR DR R RR R R ∗ ′ ′σ σ σ σ σ σ σ ∗ ′ ′σσ σ σ σσ σ σ ≡ ⋅ σ ≡ ⋅ ∑ ∑ W W V W W V σ σ (24) The vectors ( )L RV are determined by the detailed form of the SOI, Eq. (7), ( ) ( ) ( ) 2 ( ) ( ) ( ) = 2 ˆ ˆ2 (1 2 ). L R L R z L R L R L R L R b a b + + × + − V b b z z (25) Inserting Eqs. (24) into the spin-precession factors Eqs. (19) and (20), one finds = , = . s L R d Lz RzV V ⋅V V  (26) It is thus seen that due to the Pauli exclusion principle, only the components of the vectors LV and RV that are parallel to the quantization axis on the dot contribute to the spin-precession factor arising from the tunneling pro- cess in which the dot is doubly occupied, whereas all components of these vectors participate in the spin- precession factor of the sequential transmission. We also note that the difference between the two spin-precession factors disappears when either of the vectors ( )L RV or both are directed along z-axis (which is the situation in the absence of the SOI coupling). 3. Results Although it is possible in principle to calculate an effec- tive SOI ab initio, it is rather ubiquitous to adopt the phe- nomenological Hamiltonian proposed in Ref. 22. This Hamiltonian (named after Rashba) is valid for systems with a single high-symmetry axis that lack spatial inver- sion symmetry. For an electron of an effective mass m∗ and momentum p propagating along a wire where the SOI is active, it reads Rashba ˆ= ( ).so so k m∗ σ ⋅ ×p n (27) Here n̂ is a unit vector along the symmetry axis (the c-axis in hexagonal wurtzite crystals, the growth direction in a semiconductor heterostructure, the direction of an external electric field), and Rashba sok is the strength of the SOI in units of inverse length, which is usually taken from exper- iments [16,18]. By exploiting the Hamiltonian (27) to find the propagator along a one-dimensional wire, one obtains that the tunneling amplitude is [19,27] Rashba ˆ= e exp[ ],ikF LL so L rit ik × ⋅kt r n σ (28) with an analogous form for pt . Here ( )L Rr is the radius vector pointing from the dot to the left (right) reservoir along the wire, and Fk is the Fermi wave vector of an elec- tron traversing this nanowire. The linear Dresselhaus SOI [26] gives rise to a comparable form for so [28]. Another source for SOI’s are strains, created for instance when a single flat graphene ribbon is rolled up to form a tube. This type of SOI was modeled by the Hamiltonian strain strain ˆ= ,F so so k k m∗ ⋅n σ (29) where strain sok is a phenomenological parameter that gives the strength of the SOI in units of inverse length and the unit vector n̂ points along the nanotube [14,17]. In the case of the Rashba SOI, the spin-dependent fac- tor in the tunneling amplitude Eq. (28) can be written in the form ˆ ˆ= exp[ ] = cos ( ) sin ( ) ,i iα ⋅ α + α ⋅W v v  σ σ (30) where α is proportional to the strength of the spin-orbit coupling and both α and the unit vector v̂ are determined by the symmetry direction of the SOI and the geometrical configuration of the junction: Rashba= sinsok dα ϕ , where d is the length of the SOI-active bridge, and ϕ is the angle between the wire direction and n̂, the symmetry axis of the interaction. Low Temperature Physics/Fizika Nizkikh Temperatur, 2018, v. 44, No. 6 705 O. Entin-Wohlman, R.I. Shekhter, M. Jonson, and A. Aharony The parameters that characterize the spin-orbit coupling can be controlled experimentally. The capability to tune the strength of the spin-orbit interaction electrostati- cally was first demonstrated in Ref. 15 on inverted In0.53Ga0.47As/In0.52Al0.48As heterostructures. A more recent experimental evidence is found in Ref. 16, that describes measurements on the inversion layer of a In0.75Ga0.25As/In0.75Al0.25As semiconductor heterostruc- ture, and in Ref. 18, which reports on a dual-gated InAs/GaSb quantum well. The electrodes in these experi- ments are two-dimensional electron (or hole) gas bulk conductors; two gate electrodes are used to tune both the carriers’ concentration and the strength of the SOI. The spin-orbit coupling is characterized by the “Rashba param- eter” Rα , whose relation to Rashba sok is Rashba 2= / ,so Rk m∗α  (31) where Rα is measured in [meV⋅Å] (we keep  in the ex- perimental estimations). In Ref. 16, the spin-orbit coupling constant α varied with the gate voltage between roughly 150 and 300 meV⋅Å. Attributing α mainly to the Rashba SOI parameter Rα , and using = 0.04m m∗ (m is the free- electron mass), one concludes that if a weak link were to be electrostatically defined in such a system, then Rashba sok d could be varied from ~ 8 to ~ 16 for d = 1 µm. The ratio of the effective mass to the free-electron mass quoted in Ref. 18 is comparable; in this quantum well the Dresselhous SOI was kept constant while Rα could be varied between 53 and 75 meV Å, leading to Rashba sok d that varies from ~ 8 to ~ 16 for d = 1 µm. As an explicit example, we consider a weak link of the form of two straight segments, whose SOI’s parameters are ( )L Rα and ( )ˆ L Rv . One then finds that the two spin- precession factors, Eqs. (26), are [see Eqs. (25) and (30)] 2 2= [cos (2 ) 2 ][cos(2 ) 2 ],d L Lz R Rz′ ′α + α +  v v (32) and = 4sin( )sin( ) ˆ ˆ{[ ] [cos( ) cos( ) ] [cos( ) cos( ) ]} , s d L R L R z R Lz L Rz L R L R Lz Rz⊥ ⊥ + α α × ′ ′× × α − α + ′ ′+ ⋅ α α + v v v v         v v v v (33) where ( ) ( ) ( )= sin( ).L R z L R z L R′ αv v (34) (The notation ⊥ indicates the part of the vector normal to ˆ.)z For instance, when both ˆ Lv and ˆ Rv are along ẑ , then 1s d= =  , and the effect of the SOI disappears. On the other hand, when the spin-orbit coupling is due to the Rashba interaction with an electric field directed along ẑ and the junction is lying in the XY plane (see Fig. 1), then ˆ Lv and ˆ Rv are in the XY plane. In that case the spin- precession factors are cos (2 )cos (2 ) , sin (2 )sin (2 )cos ( ) , d L R s d L R = α α = + α α θ        (35) where θ is the angle between ˆ Lv and ˆ Rv . We plot in Fig. 2 the normalized Josephson current, Eq. (18), for = =R Lα α α   and the spin-precession factors as given in Eqs. (35), as a function of the angle θ, for various values of the spin- orbit strength α . One notes the change of sign of the normalized Josephson current, as a function of the angle θ between ˆ Lv and ˆ Rv . Figure 3 displays the normalized Josephson current as a function of both θ and the spin-orbit coupling constant α . Fig. 2. (Color online) The normalized Josephson current, Eq. (18), as a function of the angle θ between ˆ Lv and ˆ Rv [see Eqs. (35)] for various values of = =R Lα α α   . Straight (black) line — = 0α (1), tiny-dashed (blue) curve — = 0.2α (2), medium-dashed (magenta) curve — = 0.4α (3), large-dashed (red) curve — = 0.6α (4), dot- ted (brown) curve — = 0.8α (5), dot-dashed (black) curve — = 1α (6), dot-dashed (orange) curve — = 1.2α (7). The parame- ters that determine Eqs. (15) and (16) are / = 0ε ∆ and / = 5U ∆ . Fig. 3. (Color online) A density plot of the normalized Josephson current, Eq. (18), as a function of the angle θ between ˆ Lv and ˆ Rv and the spin-orbit coupling constant, α [see Eqs. (35)]. The parame- ters that determine Eqs. (15) and (16) are / = 0ε ∆ and / = 5U ∆ . 706 Low Temperature Physics/Fizika Nizkikh Temperatur, 2018, v. 44, No. 6 Rashba proximity states in superconducting tunnel junctions Here one notes the conspicuous oscillations as a func- tion of ,α which arise from the trigonometric functions in Eqs. (35). Figures 2 and 3 exemplify the possibility to vary the supercurrent in our device mechanically, by bending the bridge (and thus changing θ) connecting the superconductors. As mentioned, the coupling constant of the SOI can be manipulated experimentally by varying gate voltages. Additional functionality is obtained when the orienta- tions of these electric fields (induced by the gates) in the two arms of the bridge are made to be different. The simplest example is when the two arms of the bridge lie along the x-axis, with the electric field on the left nan- owire directed along z, while that on the right one is in the YZ-plane, making an angle γ with the electric field on the left wire. In this configuration, ˆ ˆ=L −v y and ˆ ˆ ˆ= cos ( ) sin ( ).R − γ + γv y z Using these expressions in Eqs. (32), (33), and (34) gives 2 2 2 cos(2 )[cos (2 ) 2sin ( )sin ( )] , sin (2 )cos ( ) , d s = α α + α γ = + α γ        (36) where for simplicity we have assumed that Rashba=L so Lk dα and Rashba=R so Rk dα coincide, i.e., =L Rα α ≡ α   . The nor- malized Josephson current pertaining to this configuration, as a function of the angle γ between the electric fields, is shown in Fig. 4 for various values of α . Its oscillation with respect to both γ and α is displayed in Fig. 5. Importantly, all our illustrations are based on gate-controlled SOI strengths that are amenable in experiment. 4. Discussion We have considered the spin splitting of Cooper pairs that carry a supercurrent through a weak-link Josephson junction. Our main result, illustrated in Figs. 2–5, is the rich oscillatory dependence of the normalized Josephson current, 0/J J [see Eq. (18)], on both the spin-orbit cou- pling constant α and the geometrical properties of the junction. In the example illustrated in Fig. 1, the latter var- iation is manifested in the dependence of 0/J J on the bending angle θ between ˆ Lv and ˆ Rv , which are normal to the wires connecting the dot with the left and right res- ervoirs, respectively, and are lying in the the plane of the junction. As seen in Fig. 2, for certain specific values of θ and the spin-orbit coupling strength α the current vanish- es. Another possibility to manipulate the geometry is to ‘mis-orient’ the electric fields that give rise to the spin- orbit interactions on the weak link. Figures 4 and 5 display the dependence of the supercurrent on the angle in- between these two fields. The oscillatory dependence of the supercurrent on the SOI strength (i.e., the dependence on α in Figs. 2–5) re- sults from a rather complex interference between different transmission events: the single-electron transmission one, that yields sJ , and the double-electron transmission that gives dJ , Eqs. (14). In the single-electron transmission channel the two electrons are transferred sequentially one by one, so that at any time during the tunneling there is only one electron on the bridge. By contrast, in the other transmission channel both electrons appear in the link for some period of time, which means that in the Coulomb- blockade limit the transfer of Cooper pairs in this channel Fig. 4. (Color online) The normalized Josephson current, Eq. (18), as a function of the angle γ , the ‘mis-orientation’ of the electric fields on the left and right nanowires [see Fig. 1 and Eqs. (36)] for various values of = =R Lα α α   . Straight (black) line — = 0α (1), tiny- dashed (blue) curve — = 0.2α (2), medium-dashed (magenta) curve — = 0.4α (3), large-dashed (red) curve — = 0.6α (4), dotted (brown) curve — = 0.8α (5), dot-dashed (black) curve — = 1α (6), dot-dashed (orange) curve — = 1.2α (7). The parameters that deter- mine Eqs. (15) and (16) are / = 0ε ∆ and / = 5U ∆ . Fig. 5. (Color online) A density plot of the normalized Joseph- son current, Eq. (18), as a function of the angle γ between in- dicating the ‘mis-orientation’ of the electric fields on the two nanowires, and the spin-orbit coupling constant, α [see Eqs. (36)]. The parameters that determine Eqs. (15) and (16) are / = 0ε ∆ and / = 5U ∆ . Low Temperature Physics/Fizika Nizkikh Temperatur, 2018, v. 44, No. 6 707 O. Entin-Wohlman, R.I. Shekhter, M. Jonson, and A. Aharony is completely suppressed. As the Coulomb blockade is lifted, the probability of pairs to be transferred in the dou- ble-electron tunneling increases. As seen from Eqs. (21), (22), and (23), the Pauli principle operating on the dot breaks the coherence of the pair transfer in the double- electron tunneling process, but does not ruin completely the contribution to the Josephson current. The pronounced oscillations of the supercurrent and the sign reversal can be observed for plausible lengths of the weak link, of the order of a micron, supposedly achievable by suitably-designed geometries of the gates. The magni- tude of the Josephson current through a quantum dot is set by the functions sF and dF , Eqs. (15) and (16), that are derived for short weak links [31]. However, whereas the restriction on the length d of the bridge might be strict, d << ξ for the orbital part (ξ is the superconducting coher- ence length), it is far weaker for the spin-dependent part: Rashba so Fk d k<< ξ, since the spin-precession factors s and d are not sensitive to the energy dependence of the transmission amplitude [9]. Our results indicate interesting phenomena caused by SOI-induced spin polarization of Cooper pairs. An intriguing feature of our result concerns the spin- polarization created on the dot due to the superconducting proximity effect in conjunction with the spin-orbit cou- pling. Calculating this polarization may require higher- orders in the tunneling, which are beyond the scope of the present analysis. Acknowledgment We thank the Computational Science Research Center in Beijing for the hospitality that allowed for the accom- plishment of this project. RIS and MJ thank the IBS Cen- ter for Theoretical Physics of Complex Systems, Daejeon, Rep. of Korea, and OEW and AA thank the Dept. of Physics, Univ. of Gothenburg, for hospitality. This work was partially supported by the Swedish Research Council (VR), by the Israel Science Foundation (ISF), by the in- frastructure program of Israel’s Ministry of Science and Technology under contract 3-11173, by the Pazi Founda- tion, and by the Institute for Basic Science, Rep. of Korea (IBS-R024-D1). Appendix A: Time-reversal symmetry and the tunneling amplitudes Here we discuss the effect of the time-reversal trans- formation on the tunneling amplitudes of Eq. (5) as given in Eqs. (6) and (7), and prove Eq. (9). Consider for in- stance [ ]LD ′σσkt , the probability amplitude for an electron to go from the the state | ′σ 〉 on the dot to the state | ,σ〉k on the left lead. We denote by an overline the quantities relat- ed to the time-reversed process. Thus, [ ]LD ′σσkt is the probability amplitude for the time-reversed process which takes an electron from the time-reversed state of | ′σ 〉 on the dot, — i.e., from | ′σ 〉 — to the time-reversed state of | ,σ〉k in the left lead, that is, to | ,− σ〉k . The time-reversal trans- formation is given in Eq. (8), and is reproduced here for clarity, 1ˆ ˆ= ,LD LD − k kt Tt T (A1) where ˆ = ( )yK iσT is the time-reversal operator; K is the complex conjugation operator, and yσ is the Pauli matrix. Hence, | ( ) | = | , | ( ) | =| . y y i i ↑〉 ≡ σ ↑〉 − ↓〉 ↓〉 ≡ σ ↓〉 ↑〉 (A2) The spin-orbit interaction by itself is time-reversal sym- metric, i.e., its matrix part W [see Eqs. (6) and (7)] is in- variant under the time-reversal transformation, =W W, while the scalar factor (i.e., ( ) ( )exp[ ]L R F L Rit ik d− is com- plex-conjugated. It remains to find the tunneling amplitude in the basis of the time-reversed states. To this end we use the generic form of the linear SOI, W [see Eq. (7)]. Using Eqs. (A2), one finds ( ) ( )[ ] = [( ) ] , L R D L R D ∗ ′ ′σσ σσW W (A3) which leads to the relation Eq. (9). Appendix B: Expansion of the particle current Upon using the expansion Eq. (12) in the expression (10) for the particle current, one finds quite a number of terms. However, only four of them describe the transfer of Cooper pairs at thermal equilibrium, ____________________________________________________ 1 2 2 1 1 2 3 1 2 3 1 2 3 1 2 3 1 2 3 1 2 3 2 3 [ ( ) ( ) ( ) ( ) ( ) ( ) ( ) ( ) ] ( ) ( ) ( ) ( ) ( ) ( ) ( ) ( ) . t tt LD DR LD DR LD LD DR DR t tt t t t LD LD DR DR LD DR LD DR i dt dt dt t t t t t t t t i dt dt dt t t t t i dt dt dt t t t t −∞ −∞ −∞ −∞ −∞ −∞ −∞ −∞ −∞ 〈 〉 + 〈 〉 − − 〈 〉 + 〈 〉 ∫ ∫ ∫ ∫ ∫ ∫ ∫ ∫ ∫                 (B1) _______________________________________________ Recall that the dot is empty in the decoupled state of the junction [30]. Examining the expressions in Eq. (B1) in conjunction with Eq. (5) shows the following fea- tures. (i) Each of the terms corresponds to the annihila- tion of a pair of electrons in the right reservoir and the creation of a pair in the left reservoir. [Note that the 708 Low Temperature Physics/Fizika Nizkikh Temperatur, 2018, v. 44, No. 6 Rashba proximity states in superconducting tunnel junctions particle current, Eq. (10), requires the imaginary part of (B1), which means that it includes also analogous terms corresponding to a pair creation in the right reservoir, and a pair annihilation in the left one.] As the electrons in each pair are in two time-reversed states, the two tun- neling amplitudes are related according to Eq. (9). For in- stance, the first term in Eq. (B1) is ____________________________________________________ 1 2 , , , , † † 1 2 3 1 1 2 2 3 3 [ ] [ ] [ ] [ ] † †( ) ( ) ( ) ( ) ( ) ( ) ( ) ( ) . L R L R RL LD DR LD DR L R t tt L i dt dt dt c t d t d t c t c t d t d t c t ′ ′ ′σ σ σ σ σ σ σ σ ′σ σ σ σ ′ ′σ − σ σ σ′ ′σ σ− σ σ −∞ −∞ −∞ × × 〈 〉 ∑ ∑ ∫ ∫ ∫ k p k p k p p pk k t t t t (B2) _______________________________________________ (ii) Two of the terms in Eq. (B1), the first and the fourth, correspond to sequential tunneling, in which the dot is only singly occupied in the intermediate state. In the other two terms, the dot is doubly occupied in the intermediate state, and therefore the evolution of the spin states of the tunneling pair is disrupted. (iii) The quantum averages of the operators of the reservoirs are nonzero only in the superconducting state, i.e., when both leads are superconducting. The remaining part of the calculation is routine: using the Bogoliubov transformation, one derives the time-dependent quantum average of the operators of the reservoirs. Those on the dot are calculated using the Hamiltonian of the decoupled dot [the first two terms on the right hand-side of Eq. (2)]. In this way, the expression in Eq. (B2) becomes ( 2 2 , )2e | | | | 1 1 1 . 2 2 i R L sL R k p k k p p t t E E E E E E ϕ −ϕ− × ∆ ∆ × + ε + + ε ∑ k p k p  (B3) where 2 2 2 ( ) ( ) ( )=k p k p L RE ε + ∆ . For simplicity, the tempera- ture is set to zero. In deriving this expression, we have made use of Eq. (9), that relates the tunneling amplitudes of two time-reversed events. The factor s describes the spin precession in the sequential tunneling processes [i.e., the first and the fourth terms in Eq. (B2)]. Explicitly, , , , 1= sgn ( )sgn ( )[( ) ] 2 [ ] [( ) ] [ ] . L L R L s LD L R LD DR DR R R ∗ ′σ σ ′σ σ σ σ ∗ ′σ σ σ σ σσ σ σ × × ∑ ∑ W W W W  (B4) As in the absence of the SOI the matrices W are all just the unit matrix, the spin-precession factor s becomes then 1. The sums over k and p are carried out assuming that 2 ( )| |tk p and the single-particle density of states of the leads can be approximated by their respective values at the Fermi energy, 2 ( )| |L Rt and ( )L RN . For a short weak link with =L R∆ ∆ ≡ ∆ [31], these sums then give s( / ) ( / )L R FΓ Γ ∆ ε ∆ , where 2 ( ) ( ) ( )= | |L R L R L RN tΓ π , and the function sF is 1 ( ) = [(cosh )(cosh cosh )(cosh )] , = / . s k p k k p p d F d ∞ −∞ ∞ − −∞ ζ ε × π ζ × ζ + ε ζ + ζ ζ + ε π ε ε ∆ ∫ ∫ (B5) An identical result is obtained for the fourth term in the expansion (B1). The imaginary part of the expression in Eq. (B3) consists of three factors, the Josephson amplitude of the interface between the two superconductors (i,e., in the absence of the resonant level on the dot and the SOI), 0 = 2sin( )[ / ]R L L RI ϕ −ϕ Γ Γ ∆ , the function sF that con- veys the effect of the localized level on the dot, and the spin-precession factor, s . The two latter factors are dis- cussed in Sec. 3. The second term in Eq. (B1), which pertains to the situ- ation where during the tunneling process the dot is doubly occupied, reads 1 2 , , , † 1 2 3 1 1 2 † 2 3 3 [ ] [ ] [ ] [ ] † †( ) ( ) ( ) ( ) ( ) ( ) ( ) ( ) , L R L R R L L R R LD DR LD DR L t tt i dt dt dt c t d t c t d t d t c t d t c t σ σ σσ σ σ σσ σ σ σ σ σ σ− σ σ −∞ −∞ −∞ − σ σ σ × × 〈 × × 〉 ∑ ∑ ∫ ∫ ∫ k p k p k p k k p p t t t t (B6) where we have taken into account the Pauli principle, and therefore there are only three summations over the spin indices [c.f. Eq. (B2)]. In this case we obtain ( 2 2 , 1 1 1)4e | | | | , 2 2 2 i dL RR L k p k p t t E E E U E ϕ ∆ ∆−ϕ− +ε ε+ +ε∑ k p k p  (B7) where d describes the spin precession in the tunneling processes in which the two electrons reside simultaneously on the dot in the intermediate sate [i.e., the second and the third terms in Eq. (B2)]. Its explicit form is Low Temperature Physics/Fizika Nizkikh Temperatur, 2018, v. 44, No. 6 709 O. Entin-Wohlman, R.I. Shekhter, M. Jonson, and A. Aharony , 1= sgn ( )sgn ( )[( ) ] 2 [ ] [( ) ] [ ] . L L R L R R d LD L R LD DR DR ∗ σ σ σ σ σ ∗ σ σ σσ σσ σ σ × × ∑ ∑ W W W W  (B8) Similar to s , this factor also becomes 1 in the absence of the SOI. The sums over k and p are carried out as ex- plained above. Because of the double occupancy of the dot, the energy denominators in Eq. (B7) differ from those in Eq. (B3). These summations give rise to another function, ( / , / )dF Uε ∆ ∆ , of the energies on the dot [31] 1 ( , ) = [(cosh )(2 )(cosh )] , = / , = / . d pk k p F U dd U U U ∞ ∞ − −∞ −∞ ε ζζ = ζ + ε ε + ζ + ε π π ε ε ∆ ∆ ∫ ∫         (B9) Since the third term in the expansion (B1) turns out to be identical to Eq. (B7), it follows that the contribution from these tunneling processes to the Josephson current is again a product of three factors, 0I , dF , and d . _______ 1. J. Lehmann, A. Gaita-Arino, E. Coronado, and D. Loss, Nanotechnology 2, 312 (2007). 2. C. Kloeffel and D. Loss, Annu. Rev. Condens. 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Introduction 2. Tunneling of Cooper pairs 2.1. Description of the model 2.2. The particle current 2.3. Spin precession 3. Results 4. Discussion Acknowledgment Appendix A: Time-reversal symmetry and the tunneling amplitudes Appendix B: Expansion of the particle current
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2021-02-03T19:05:44Z
2018
Rashba proximity states in superconducting tunnel junctions / O. Entin-Wohlman, R.I. Shekhter, M. Jonson, A. Aharony // Физика низких температур. — 2018. — Т. 44, № 6. — С. 701-710. — Бібліогр.: 31 назв. — англ.
0132-6414
PACS: 72.25.Hg, 72.25.Rb
https://nasplib.isofts.kiev.ua/handle/123456789/176152
We consider a new kind of superconducting proximity effect created by the tunneling of “spin split” Cooper pairs between two conventional superconductors connected by a normal conductor containing a quantum dot. The difference compared to the usual superconducting proximity effect is that the spin states of the tunneling Cooper pairs are split into singlet and triplet components by the electron spin-orbit coupling, which is assumed to be active in the normal conductor only. We demonstrate that the supercurrent carried by the spin-split Cooper pairs can be manipulated both mechanically and electrically for strengths of the spin-orbit coupling that can realistically be achieved by electrostatic gates.
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Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України
Физика низких температур
Специальный выпуск К 90-летию со дня рождения A.A. Абрикосова
Rashba proximity states in superconducting tunnel junctions
Article
published earlier
spellingShingle Rashba proximity states in superconducting tunnel junctions
Entin-Wohlman, O.
Shekhter, R.I.
Jonson, M.
Aharony, A.
Специальный выпуск К 90-летию со дня рождения A.A. Абрикосова
title Rashba proximity states in superconducting tunnel junctions
title_full Rashba proximity states in superconducting tunnel junctions
title_fullStr Rashba proximity states in superconducting tunnel junctions
title_full_unstemmed Rashba proximity states in superconducting tunnel junctions
title_short Rashba proximity states in superconducting tunnel junctions
title_sort rashba proximity states in superconducting tunnel junctions
topic Специальный выпуск К 90-летию со дня рождения A.A. Абрикосова
topic_facet Специальный выпуск К 90-летию со дня рождения A.A. Абрикосова
url https://nasplib.isofts.kiev.ua/handle/123456789/176152
work_keys_str_mv AT entinwohlmano rashbaproximitystatesinsuperconductingtunneljunctions
AT shekhterri rashbaproximitystatesinsuperconductingtunneljunctions
AT jonsonm rashbaproximitystatesinsuperconductingtunneljunctions
AT aharonya rashbaproximitystatesinsuperconductingtunneljunctions