On the possibility to detect acts of cluster decay of atomic nuclei by the methods of noise diagnostic

Cluster decay, as a special type of radioactive decay, up to date, is widely investigated. Nevertheless, until now, this activity is restricted: from one side by the possibilities of theoretical analysis, where some success is obtained for light nuclei only; and from another side only by experiments...

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Published in:Вопросы атомной науки и техники
Date:2020
Main Authors: Skorbun, A.D., Kuchmagra, O.A., Odinokin, G.I., Maslyuk, V.T., Romanyuk, M.I.
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Language:English
Published: Національний науковий центр «Харківський фізико-технічний інститут» НАН України 2020
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Online Access:https://nasplib.isofts.kiev.ua/handle/123456789/194533
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Cite this:On the possibility to detect acts of cluster decay of atomic nuclei by the methods of noise diagnostic / A.D. Skorbun, O.A. Kuchmagra, G.I. Odinokin, V.T. Maslyuk, M.I. Romanyuk // Problems of atomic science and tecnology. — 2020. — № 3. — С. 143-147. — Бібліогр.: 16 назв. — англ.

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Digital Library of Periodicals of National Academy of Sciences of Ukraine
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author Skorbun, A.D.
Kuchmagra, O.A.
Odinokin, G.I.
Maslyuk, V.T.
Romanyuk, M.I.
author_facet Skorbun, A.D.
Kuchmagra, O.A.
Odinokin, G.I.
Maslyuk, V.T.
Romanyuk, M.I.
citation_txt On the possibility to detect acts of cluster decay of atomic nuclei by the methods of noise diagnostic / A.D. Skorbun, O.A. Kuchmagra, G.I. Odinokin, V.T. Maslyuk, M.I. Romanyuk // Problems of atomic science and tecnology. — 2020. — № 3. — С. 143-147. — Бібліогр.: 16 назв. — англ.
collection DSpace DC
container_title Вопросы атомной науки и техники
description Cluster decay, as a special type of radioactive decay, up to date, is widely investigated. Nevertheless, until now, this activity is restricted: from one side by the possibilities of theoretical analysis, where some success is obtained for light nuclei only; and from another side only by experiments for nuclei defragmentation in searching for fission on magic nuclei. However, standard methods of radiometry and statistical analysis have not yet been applied. Such possibility can be realized by searching for acts of cluster decay as a rare event on an array of alpha-decay acts of actinides, which are recorded by industrial ionization fission chambers. The scheme of the experiment is discussed, which consists in the registration of every act of alpha-decay, against the background of which it is possible to detect the presence of nuclear clusters based on isotopes of ¹²,¹⁴С, ²⁰О, and others, which can be formed in the decay of ²³⁴,²³⁵U. The requirements for electronics and the background conditions for such an experiment are discussed in detail. Кластерний розпад, як особливий тип радіоактивного розпаду, на сьогоднішній день широко досліджується. Проте досі ця діяльність обмежена: з одного боку — можливостями теоретичного аналізу, де деякого успіху досягнуто лише для легких ядер, а з другого боку — лише експериментами з дефрагментації ядер у пошуках поділу на магічні ядра. Стандартні ж методи радіометрії і статистичного аналізу продуктів ядерних перетворень досі не застосовувались. Така можливість може бути реалізована шляхом пошуку актів кластерного розпаду, як рідкісних подій на масиві актів альфа-розпаду актинідних ядер, які фіксуються промисловими іонізаційними камерами поділу. Обговорюється схема експерименту, яка полягає в реєстрації кожного акту альфа-розпаду, на фоні яких можливо зафіксувати присутність ядерних кластерів ізотопів ¹²,¹⁴С, ²⁰О та інших, які можуть утворитися при розпаді ²³⁴,²³⁵U. Детально обговорюються вимоги до електроніки та фонові умови для такого експерименту. Кластерный распад, как особый тип радиоактивного распада, на сегодняшний день широко исследуется. Однако до сих пор эта деятельность ограничена: с одной стороны — возможностями теоретического анализа, где некоторых успехов достигли только для легких ядер, с другой стороны — только экспериментами по дефрагментации ядер в поисках деления на магические ядра. Стандартные же методы радиометрии и статистического анализа продуктов ядерных превращений до сих пор не применялись. Такая возможность может быть реализована путем поиска актов кластерного распада, как единичных событий на массиве актов альфа-распада актинидных ядер, которые фиксируются промышленными ионизационными камерами деления. Обсуждается схема эксперимента, состоящая в регистрации каждого акта альфа-распада, на фоне которых возможно зафиксировать присутствие ядерных кластеров изотопов ¹²,¹⁴С, ²⁰О и др., способных образоваться при распаде ²³⁴,²³⁵U. Детально обсуждаются требования к электронике и фоновые условия для такого эксперимента.
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fulltext ISSN 1562-6016. ВАНТ. 2020. №3(127) 143 ON THE POSSIBILITY TO DETECT ACTS OF CLUSTER DECAY OF ATOMIC NUCLEI BY THE METHODS OF NOISE DIAGNOSTIC A.D. Skorbun1, O.A. Kuchmagra1, G.I. Odinokin1, V.T. Maslyuk2, M.I. Romanyuk2 1Institute for safety problems of nuclear power plant NAS of Ukraine, Kyiv, Ukraine; 2Institute of Electron Physics, Uzhhorod, Ukraine E-mail: anskorbun@gmail.com; myk.romanyuk@gmail.com Cluster decay, as a special type of radioactive decay, up to date, is widely investigated. Nevertheless, until now, this activity is restricted: from one side by the possibilities of theoretical analysis, where some success is obtained for light nuclei only; and from another side only by experiments for nuclei defragmentation in searching for fission on magic nuclei. However, standard methods of radiometry and statistical analysis have not yet been applied. Such possibility can be realized by searching for acts of cluster decay as a rare event on an array of alpha-decay acts of actinides, which are recorded by industrial ionization fission chambers. The scheme of the experiment is discussed, which consists in the registration of every act of alpha-decay, against the background of which it is possible to detect the presence of nuclear clusters based on isotopes of 12,14С, 20О, and others, which can be formed in the decay of 234,235U. The requirements for electronics and the background conditions for such an experiment are discussed in detail. PACS: 21.60.Gx; 23.60.+e; 23.90.+w; 28.41.My INTRODUCTION The radioactivity phenomenon, which consists of the emission of elementary nuclear particles, or even indi- vidual nuclei, today is considered as a mainly intra- nuclear process. Investigation of these processes gives information about the stability of nuclear matter, the role of shell corrections, and also about the peculiarities of nucleons interaction in a nucleus. The last character- istics is especially crucial for explaining the cluster model of the nucleus [1], when, in addition to alpha- particles, more complex nuclear fragments, such as 12,14С, 20О can be emitted [2, 3]. There are even molecu- lar models of a nucleus [1], which analyzed the nature and possibilities for realization in the nucleus the cluster structures with different dimensionality. Experimental evidence of cluster radioactivity is looking for in the analysis of nuclei fission fragments [4]. In the last time, to this task the experiments for multi-fragmentation of atomic nuclei on the high-energy particle installations [5, 6] are recruited. These are enough complicated and expensive experiments with ambiguous results. Nevertheless, the main problem is that they are directed to evidence of the cluster structure of fissioning nuclei, not in the cluster decay. In our work, it is proposed to recruit to the task of cluster radioactivity investigation, in particular, the standard methods of radiometry, and statistical analysis of noise diagnostic data. In particular, one must be look- ing for acts of cluster decay of nuclei-actinides among acts of natural alpha-decay. The main idea of our pro- posal is based on a hypothesis that the energy of parti- cles as the result of cluster decay, will be proportional to their mass and, consequently, will be in several times higher, compared to the energy of alpha-particle during the standard alpha-decay process. This distinction and will be a required indication of cluster decay. The other requirement is in the necessity to organize an experi- ment, that long set of measurements will be fulfilled, for creating vast data array on the energy of particles, which can permit to carry out a reliable statistical analysis of the results. Technically the problem of cluster decay searching is reduced to known in nuclear physics the task to ex- tract or fixed rare events, using standard fission ioniza- tion chambers, for instance, KNT-31-1 [7], which are intended to measure neutron fluxes and use active ele- ments on the base of 234,235U. Such a device is a conven- tional apparatus of the system for control of the safety of nuclear power plants, and it is reliable with very well-known characteristics. In the article, requirements are discussed to stabili- zation of equipment for registrations and organizing long continuous measurements; characteristics of elec- tronics for such type of experiments; methods of re- ceived signals treatment, necessary for ensuring the reli- ability of registration of cluster decay acts. It is also dis- cussed the question of comparing cluster decay prob- abilities in the frames of the tunneling theory and the theory of spontaneous fission of actinides nuclei. CLUSTER RADIOACTIVITY: FROM TUNNELING TO SPONTANEOUS NUCLEUS FISSION The term "cluster radioactivity" is applied to a phe- nomenon of emission, or appearance among the prod- ucts of actinides nuclei transformations, high energy nucleon clusters, which are more massive, than alpha- particles. Cluster radioactivity was predicted and dis- covered in the 80-th of the last century [1], and more than eight nuclear clusters emitted from more than 25 heavy nuclei, from 114Ba to 241Аm, have now been ex- perimentally confirmed [8, 9]. Cluster radioactivity is considered as a phenomenon, intermediate between al- pha-decay and spontaneous fission of a nucleus. Com- mon for both of them is a barrier mechanism of realiza- tion of a final state: formation of alpha particle or en- semble of different fission fragments. In the first case it is Coulomb barrier with the height Bk  2Z/A1/3 МеV, which prevent to alpha particle tunneling; in the second one it is a potential barrier, which is determined by dif- ference between surface and Coulomb energies of fis- sion nucleus, and restrain transition of nucleus from ISSN 1562-6016. ВАНТ. 2020. №3(127) 144 spherical to ellipsoidal form (liquid drop model) in case of Z2/A < 48. For an explanation of cluster radioactivity, combining of adiabatic and non-adiabatic approaches are used, depending on a mass of the emitted cluster. At that, a mass Аf ~ 35 is becoming as a critical parameter [10, 11]. At A< Аf, parameters of cluster radioactivity (period of cluster decay, cluster energy) are satisfacto- rily described in the frame of an alpha-decay theory, but in another case, adiabatic mechanisms from the theory of nucleus fission are used. Therefore, for the problems of cluster radioactivity, it is interesting to investigate probabilities of the yield of heavy nuclei fission frag- ments and to establish influence factors. Such a task can be solved in the frame of after-fission approximation when particular characteristics of mass or charge distri- butions are determined according to the character of the thermodynamic ordering of the nucleus fission products [12]. Fig. 1 demonstrates the dependencies of probabili- ties, P, of the yields of different fission fragments with the atomic number Zi (charge spectrum) and the fine structure that is caused by the magical numbers 8, 20, 28, 50, and 82. It should be noted that similar trends take place for the charge spectrum for isotopes of 233- 238U. Note the strong dependence of the yields of the fission fragments on the excitation, or the fissile isotope 234U nuclear temperature, T. For example, the transition from "cold", T = 0.5 MeV to "hot" T = 2.0 MeV fission stages increases the probability of clusters contained, for example, of oxygen isotopes, Z = 8, in 10105, whereas for Si isotopes, such growth is only 1073. For Z = 6, C isotopes, such growth is already 10112! 0 20 40 60 80 100 -250 -200 -150 -100 -50 0 ln (Y ), ar b. un . Zi T=0,5 MeV T=1,0 MeV T=2,0 MeV 234U a 0 20 40 60 80 100 -16 -12 -8 -4 0 4 8 12 28 82 50 D er iv .,a rb .u n. Zi T=2,0 MeV T=1,0 MeV T=0,50 MeV 8 20 b Fig. 1. The temperature dependencies of the charge spectrum of the fission fragment yields for different values of nuclear temperature (a); fine structures, obtained by differentiating of the curves into (a). The features caused by the magic numbers of proton shells are highlighted (b) The given estimations were obtained within assump- tion on two-fragments fission and did not takes into ac- count the tunneling mechanism of nuclear transforma- tions. However, in case of strong excitation of the fissile nucleus by the high energy gamma quanta or neutron, this mechanism can give a contribution to cluster radio- activity occurrence. CHARACTERISTICS OF DETECTING SYSTEM Schematically standard ionization fission chambers for registration of neutron flows have such a construc- tion [7]. They are filled with gas into the working vol- ume with two electrodes are placed there. The thin layer of 235U covers one of the electrodes (cathode), and such construction is named as the radiator. Under neutron action, 235U is divided, and high-energetic fragments of fission ionize a gas. If to feed high voltage to the anode, then products of ionization – electrons and ions – are collected there. They form an electrical impulse, an am- plitude of which depends on the degree of ionization of the gas in working volume by fragments of 235U fission. The appearance of an impulse in the electrical circuit of the detecting system corresponds to an act of neutron registration. In a given scheme of experiments about cluster radioactivity, one must pay considerable atten- tion to the control of background conditions, or self- noise of an ionization chamber, against the background of which impulses from neutron registration are ob- served. The peculiarity of an ionization fission chamber, specifically the KNT-31-1 apparatus, which is proposed to use in the given work, is that their noises can have the two components: noises of electronics and the same, produced by spontaneous alpha-decay of uranium, coated on an electrode, so-called alpha-current or alpha- noise. This effect at neutron registration is considered as parasitic one. Furthermore, it can be easily eliminated, using the fact that the amplitude of impulse from alpha- particles is much less than from neutron impulses. Therefore, at using amplitude discriminator on the cor- responding level, the system will fix only impulses, ex- cited by neutrons. However, for our task, an ionization chamber can be considered as an ideal source of alpha-particles, with the complete and refined system of their registration. Statis- tical properties of alpha-current, to use it, have been investigated in our previous works [13], where it was shown, including, that it is possible to plainly distin- guish alpha-current and, correspondingly, to investigate its statistical properties. According to this, we consider a possibility to use an alpha-decay source inside of the ionization chamber, for the task of cluster decay searching. As it was pointed out, we will proceed from the assumption that as an in- dication of cluster decay will be impulses, amplitudes of which will exceed amplitudes of impulses from alpha- current. In this case, such conditions correspond to the known task of registering of neutron pulses on the of α- current’s background with the difference that the ampli- tudes of the single pulses from the cluster decay, as ex- pected, are comparable in order of magnitude to the am- plitudes of the pulses of α-current. ISSN 1562-6016. ВАНТ. 2020. №3(127) 145 Fig. 2. Oscillogrammes of ionization chamber signals from two parallel channels: 1 – in the first channel noises are hardly seen (at the given level of amplifying =0.5 V); 2 – neutron impulse in the second channel are seen practically without noises (a). Noisy signals (of alpha-current) are enough alike in both channels. The level of amplifying is 0.15 V (b) For more specific consideration, Fig. 2 presents re- sults about a neutron pulse, a, and α-current signals, b, illustrating the difference in such signal detection. As one can see, the neutron pulse is observed on a nearly flat path of the panel, while the α-current pulses must be separated from the noise background. However, it was shown in our works [13, 14] that electronics noise, α- current signals, and neutron pulses can be assuredly separated. EXPERIMENTS ON CLUSTER RADIOACTIVITY WITH USING NOISE DIAGNOSTICS METHODS In experimental studies for receiving necessary input information for statistical analyzing, equipment must be used, which is capable of fixing and of storing a chrono- logical sequence (time sets) of moments of registration of every neutron, which get into a detector, with some time resolution. It is essential to ensure automation and control of the measurement processes, raw data calculations, and processing according to developed methods and algo- rithms for different methods of noise diagnostics. Such a procedure gives the possibility of carrying out independent processing of accumulated data by us- ing different methods of statistical or correlation noise analysis. The main advantage of this approach to the measurement of noises is that analysis of data is carried over from the stage of on-line measurements to the stage of data processing that considerably simplifies and reduces the cost of the experiment, due to all measure- ments are carried out by the same, industrial and rela- tively simple equipment. Furthermore, for our task, this means the possibility to control parameters of impulses created by our equipment, in particular, their amplitude. During alpha-current measurements, impulses are sent to amplitude analyzer, in which they are sorted into 1024 channels according to their amplitudes. It was es- tablished that in the interval from first to 50-th channels, electronics noises are registered, and signals in the area of 50…80-th channels do not depend on neutron's pres- ence or absence (Fig. 3). Thus, in the area of 50…80-th channels, the alpha-current is registered (Fig. 4). Fig. 3. Typical appearance of an amplitude spectrum for the full set of measurements with the presence of neutrons (1) and in the absence of them (2). The up- per-scale demonstrates the correspondence between the level of discrimination and the number of a channel Fig. 4. The amplitude spectrum of impulses, which were registered in 50…80-th channels: the discriminator "cuts" impulses with amplitudes, less than the 50-th channel, and greater than 100-th channel (shown by the vertical line) If they use two amplitude discriminators to select this area of amplitudes, it is possible to investigate sta- tistics of alpha-current signals. In Fig. 3 the schematic image of amplitude depend- ences (or spectrum), which were received in the ex- periment with the given ionization chamber KNT-31-1, is presented. In this image it is possible to separate three areas: shaded area I, which includes 50…80-th chan- nels, where signals from detector practically do not de- pend on neutrons presence; also shaded area II on the right, where impulses from neutrons events are re- vealed; and an area from 80-th to 100-th channels be- tween them with the curve 2, where alpha-current is fixed. a b 1 2 1 2 ISSN 1562-6016. ВАНТ. 2020. №3(127) 146 As it was pointed earlier, due to some time is neces- sary to collect electrons and ions from ionization inside a fission chamber (“dead time”), the system can also register impulses of double or more amplitude, if ioniza- tion will be due to particles, which ionize the gas practi- cally simultaneously, that is during a dead time. Then signals from two or more alpha-particles will be re- ceived as a single one. The probability of such processes can be estimated if to consider them as Poisson ones. In our case, it is sug- gested that the time of ionization charges collection in chamber KNT-31-1 is equal to τ = 0.4∙10-6 s. Estimating the probability of occurrence of overlaps allows one to determine the number of expected events. It is possible to estimate the probability of events overlaps for alpha- particles during the time of measurement t according to the formula [15]:   0 ! )(),( 0 n n n e n nnP , where n is the number of alpha-particles, which create overlap; n0 is the number of alpha-particles, which is emitted by radiator in one second inside of fission chamber volume;  is the time, during which the overlap is possible. Then the number of overlapping for time unit is cal- culated according to formula )(0  npnN n (Table). Results of the standard calculations of the probability of simultaneous registration of alpha-particles n  0 ! nn n  0ne   pn N 1 0.25 0.778 0.1945 121 562 2 0.03125 0.778 0.0243 15 187 3 2.6∙10-3 0.778 2.0∙10-3 1 250 4 1.63∙10-4 0.778 1.27∙10-4 79 5 8.14∙10-6 0.778 6.33∙10-6 4 Thus calculations show that in ionization chamber KNT-31-1, the impulses from overlapping up to five alpha-particles can arise. It is considered that such summing impulses, in reality, are fixed by existing equipment. Their number is decreased with the increase of the amplitude of a summing impulse, hereupon an amplitude spectrum in Fig. 3 is not the straight line, but a diffuse area from 50-th to 100-th channels. According to reference data for 234U, which also is present on the cathode of KNT-31-1, it is an intensive source of alpha- particles, which have energy 4722.4 kеV (in 28.42% cases) and 4774.6 kеV (in 71.38% cases). In the case of five alpha-particle overlapping and full ionization charge accumulation inside an ionization chamber, the impulse with energy about 30 MeV is registered. This energy is comparable with the energy of a light nucleus at cluster radioactivity [2]. The amplitude of such an impulse is belonged to the range of values for fission fragment registration in the case of neutron detecting and can be fixed in an amplitudes spectrum. One can try to avoid this problem, taking into ac- count the peculiarity of the fission chamber, that a radia- tor of KNT-31-1 chamber, in reality, is a mixture of 235U+234U isotopes. The activity of 234U, despite its small concentration, is higher by several orders of mag- nitude than 235U. That is noise current or alpha-current of such chambers is mainly the result of 234U decay. Therefore, for the experiments on cluster radioactiv- ity searching, to reduce the number of background im- pulses, one should use the fission chamber [16], in which the radiator must be of exceptionally high en- richment (99.9% 235U, less than 0.03% 234U). Such a sort of fission chamber can be more expensive, but the intensity of alpha-current in them is much lesser. In this case, the probability the overlapping of impulses of α- particles under the experimental conditions decreases and increases the expectation for the possibility of regis- tration of cluster particles. Others possibilities for the success of such an ex- periment are as follows: 1. Equipment modernization, which consists of cre- ating high-quality electronics for registration impulses from the ionization fission chamber, which reduces an electronics component of dead time to the level of physical restrictions for the processes of ionization and charge collection, which we estimate as ~ 400 ns. 2. The necessity of theoretical modeling of multi- particle registration of alpha-current impulses, which should base on experimental data. 3. New theoretical investigations are necessary for the systematization of fission fragments of actinides. It is mainly concern the part of the selection and estima- tion of the probability of yields of the light magic nu- clei. It is necessary also to take into account the differ- ent versions of cluster decay mechanism. 4. Because the matter is of registration of single events, in the modernized experimental setup, the meas- ures must be taken to reducing and stabilization of background conditions in detecting system from neutron impulses, the equipment stabilization, and to provide long-time measurements. CONCLUSIONS Thus, registration of acts of atomic nuclei cluster de- cay by the noise diagnostics methods must take into account the fact that such events will be observed as an integral part of alpha-decay, including the presence of overlapping processes during measurements. The effect of overlapping impulses from practically simultaneously registered alpha-particles seems to be big enough, and it will be not simply to register the cluster decay impulses against this background. As an option, it is proposed to use ionization chambers, which have as a radiator’s ma- terial the isotope 235U, enriched comparatively to 234U. An essential item is decreasing of dead time of register- ing equipment employing by using high-quality elec- tronics. It is necessary also to carry out numerical esti- mations of amplitude spectral lines broadening, taking into account alpha particle energy at multi-particles im- pulses overlapping. The proposed approach can also bring success for the registration of more massive nuclei clusters, such as 34Si, in the case of their emission from uranium. A special task is the stabilization of power supply units and ensuring low background conditions of detect- ing system from neutrons in case of long-time meas- urements. ISSN 1562-6016. ВАНТ. 2020. №3(127) 147 REFERENCES 1. A. Sandulescu, D.N. Poenaru, and W. Greiner. New type of decay of heavy nuclei intermediate between fission and alpha-decay // Sov. J. Part. Nucl. 1980, № 11, p. 528-541. 2. R. Bonetti and A. Guglielmetti. Cluster radioactiv- ity: an overview after twenty years // Rom. Rep. Phys. 2007, v. 59, p. 301-310. 3. W.M. Seif, L.H. Amer. Systematic investigation of cluster radioactivity for uranium isotopes // Nuclear Physics A. 2017, v. 969, p. 254-268. 4. S.N. Kuklin, G.G. Adamian, N.V. Antonenko. 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Kuklin, G.G. Adamian, N.V. Antonenko. De- scription of Alpha-decay and Cluster Radioactivity in the Dinuclear System Model // Physics of Elemen- tary Particles and Atomic Nuclei. 2016, v. 47, № 2, p. 390-441. 11. A.A. Ogloblin et al. Observation of cluster decay of 242Cm // Phys. Rev. C. 2000, v. 61, p. 034301. 12. V.T. Maslyuk et al. Calculation of the fission- fragment yields of the pre-actinide by the example of the nat Pb isotopes // Nuclear Physics A. 2016, v. 955, p. 79. 13. О.A. Kuchmagra, G.I. Odinokin, A.D. Skorbun, S.M. Stadnyk, A.S. Sadovnikov. Using of alpha- activity of fission chamber radiator for control of workability of neutron measurement channel // Problems of safety of the atomic station and Chor- nobyl. 2006, v. 27, p. 97-101. 14. О.A. Kuchmagra, I.O. Maznyi, G.I. Odinokin, A.S. Sadovnikov, A.D. Skorbun, S.M. Stadnyk. Fis- sion Ionization Chamber as Reference Source in Neutron Flux Analysis // Nuclear and radiation safety. 2017, v. 4, № 76, p. 102-106. 15. Kalashnikova, M.S. Kozodayev. Detectors of ele- mentary particles. M.: “Nauka”, 1996, 407 p. 16. B. Dmitriev, E.K. Malishev. Neutron ionization chambers for reactor technics. M.: “Atomizdat”, 1975, 94 p. Article received 14.02.2020 О ВОЗМОЖНОСТИ РЕГИСТРАЦИИ АКТОВ КЛАСТЕРНОГО РАСПАДА АТОМНЫХ ЯДЕР МЕТОДАМИ ШУМОВОЙ ДИАГНОСТИКИ А.Д. Скорбун, О.А. Кучмагра, Г.И. Одинокин, В.Т. Маслюк, Н.И. Романюк Кластерный распад, как особый тип радиоактивного распада, на сегодняшний день широко исследуется. Однако до сих пор эта деятельность ограничена: с одной стороны – возможностями теоретического анализа, где некоторых успехов достигли только для легких ядер, с другой стороны – только экспериментами по де- фрагментации ядер в поисках деления на магические ядра. Стандартные же методы радиометрии и стати- стического анализа продуктов ядерных превращений до сих пор не применялись. Такая возможность может быть реализована путем поиска актов кластерного распада, как единичных событий на массиве актов альфа- распада актинидных ядер, которые фиксируются промышленными ионизационными камерами деления. Об- суждается схема эксперимента, состоящая в регистрации каждого акта альфа-распада, на фоне которых воз- можно зафиксировать присутствие ядерных кластеров изотопов 12,14С, 20О и др., способных образоваться при распаде 234,235U. Детально обсуждаются требования к электронике и фоновые условия для такого экспери- мента. ПРО МОЖЛИВІСТЬ РЕЄСТРАЦІЇ АКТІВ КЛАСТЕРНОГО РОЗПАДУ АТОМНИХ ЯДЕР МЕТОДАМИ ШУМОВОЇ ДІАГНОСТИКИ А.Д. Скорбун, О.А. Кучмагра, Г.І. Одинокін, В.Т. Маслюк, М.І. Романюк Кластерний розпад, як особливий тип радіоактивного розпаду, на сьогоднішній день широко досліджується. Проте досі ця діяльність обмежена: з одного боку – можливостями теоретичного аналізу, де деякого успіху досягнуто лише для легких ядер, а з другого боку – лише експериментами з дефрагментації ядер у пошуках поділу на магічні ядра. Стандартні ж методи радіометрії і статистичного аналізу продуктів ядерних перетворень досі не застосовувались. Така можливість може бути реалізована шляхом пошуку актів кластерного розпаду, як рідкісних подій на масиві актів альфа-розпаду актинідних ядер, які фіксуються промисловими іонізаційними камерами поділу. Обговорюється схема експерименту, яка полягає в реєстрації кожного акту альфа-розпаду, на фоні яких можливо зафіксувати присутність ядерних кластерів ізотопів 12,14С, 20О та інших, які можуть утворитися при розпаді 234,235U. Детально обговорюються вимоги до електро- ніки та фонові умови для такого експерименту.
id nasplib_isofts_kiev_ua-123456789-194533
institution Digital Library of Periodicals of National Academy of Sciences of Ukraine
issn 1562-6016
language English
last_indexed 2025-12-07T18:52:26Z
publishDate 2020
publisher Національний науковий центр «Харківський фізико-технічний інститут» НАН України
record_format dspace
spelling Skorbun, A.D.
Kuchmagra, O.A.
Odinokin, G.I.
Maslyuk, V.T.
Romanyuk, M.I.
2023-11-27T12:16:16Z
2023-11-27T12:16:16Z
2020
On the possibility to detect acts of cluster decay of atomic nuclei by the methods of noise diagnostic / A.D. Skorbun, O.A. Kuchmagra, G.I. Odinokin, V.T. Maslyuk, M.I. Romanyuk // Problems of atomic science and tecnology. — 2020. — № 3. — С. 143-147. — Бібліогр.: 16 назв. — англ.
1562-6016
PACS: 21.60.Gx; 23.60.+e; 23.90.+w; 28.41.My
https://nasplib.isofts.kiev.ua/handle/123456789/194533
Cluster decay, as a special type of radioactive decay, up to date, is widely investigated. Nevertheless, until now, this activity is restricted: from one side by the possibilities of theoretical analysis, where some success is obtained for light nuclei only; and from another side only by experiments for nuclei defragmentation in searching for fission on magic nuclei. However, standard methods of radiometry and statistical analysis have not yet been applied. Such possibility can be realized by searching for acts of cluster decay as a rare event on an array of alpha-decay acts of actinides, which are recorded by industrial ionization fission chambers. The scheme of the experiment is discussed, which consists in the registration of every act of alpha-decay, against the background of which it is possible to detect the presence of nuclear clusters based on isotopes of ¹²,¹⁴С, ²⁰О, and others, which can be formed in the decay of ²³⁴,²³⁵U. The requirements for electronics and the background conditions for such an experiment are discussed in detail.
Кластерний розпад, як особливий тип радіоактивного розпаду, на сьогоднішній день широко досліджується. Проте досі ця діяльність обмежена: з одного боку — можливостями теоретичного аналізу, де деякого успіху досягнуто лише для легких ядер, а з другого боку — лише експериментами з дефрагментації ядер у пошуках поділу на магічні ядра. Стандартні ж методи радіометрії і статистичного аналізу продуктів ядерних перетворень досі не застосовувались. Така можливість може бути реалізована шляхом пошуку актів кластерного розпаду, як рідкісних подій на масиві актів альфа-розпаду актинідних ядер, які фіксуються промисловими іонізаційними камерами поділу. Обговорюється схема експерименту, яка полягає в реєстрації кожного акту альфа-розпаду, на фоні яких можливо зафіксувати присутність ядерних кластерів ізотопів ¹²,¹⁴С, ²⁰О та інших, які можуть утворитися при розпаді ²³⁴,²³⁵U. Детально обговорюються вимоги до електроніки та фонові умови для такого експерименту.
Кластерный распад, как особый тип радиоактивного распада, на сегодняшний день широко исследуется. Однако до сих пор эта деятельность ограничена: с одной стороны — возможностями теоретического анализа, где некоторых успехов достигли только для легких ядер, с другой стороны — только экспериментами по дефрагментации ядер в поисках деления на магические ядра. Стандартные же методы радиометрии и статистического анализа продуктов ядерных превращений до сих пор не применялись. Такая возможность может быть реализована путем поиска актов кластерного распада, как единичных событий на массиве актов альфа-распада актинидных ядер, которые фиксируются промышленными ионизационными камерами деления. Обсуждается схема эксперимента, состоящая в регистрации каждого акта альфа-распада, на фоне которых возможно зафиксировать присутствие ядерных кластеров изотопов ¹²,¹⁴С, ²⁰О и др., способных образоваться при распаде ²³⁴,²³⁵U. Детально обсуждаются требования к электронике и фоновые условия для такого эксперимента.
en
Національний науковий центр «Харківський фізико-технічний інститут» НАН України
Вопросы атомной науки и техники
Experimental methods and processing of data
On the possibility to detect acts of cluster decay of atomic nuclei by the methods of noise diagnostic
Про можливість реєстрації актів кластерного розпаду атомних ядер методами шумової діагностики
О возможности регистрации актов кластерного распада атомных ядер методами шумовой диагностики
Article
published earlier
spellingShingle On the possibility to detect acts of cluster decay of atomic nuclei by the methods of noise diagnostic
Skorbun, A.D.
Kuchmagra, O.A.
Odinokin, G.I.
Maslyuk, V.T.
Romanyuk, M.I.
Experimental methods and processing of data
title On the possibility to detect acts of cluster decay of atomic nuclei by the methods of noise diagnostic
title_alt Про можливість реєстрації актів кластерного розпаду атомних ядер методами шумової діагностики
О возможности регистрации актов кластерного распада атомных ядер методами шумовой диагностики
title_full On the possibility to detect acts of cluster decay of atomic nuclei by the methods of noise diagnostic
title_fullStr On the possibility to detect acts of cluster decay of atomic nuclei by the methods of noise diagnostic
title_full_unstemmed On the possibility to detect acts of cluster decay of atomic nuclei by the methods of noise diagnostic
title_short On the possibility to detect acts of cluster decay of atomic nuclei by the methods of noise diagnostic
title_sort on the possibility to detect acts of cluster decay of atomic nuclei by the methods of noise diagnostic
topic Experimental methods and processing of data
topic_facet Experimental methods and processing of data
url https://nasplib.isofts.kiev.ua/handle/123456789/194533
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