Tuning of aggregation and film self-assembly of monomethincyanine dyes through variation of their monomer structure

Formation of condensed films and solution aggregates of four different monomethincyanine dyes has been studied using optical absorption spectroscopy and simulation methods, depending on variation of the dye monomer structure. The structure of the molecular dimer as a basic unit for the formation of...

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Veröffentlicht in:Semiconductor Physics Quantum Electronics & Optoelectronics
Datum:2019
Hauptverfasser: Sieryk, M.M., Dimitriev, O.P.
Format: Artikel
Sprache:Englisch
Veröffentlicht: Інститут фізики напівпровідників імені В.Є. Лашкарьова НАН України 2019
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Online Zugang:https://nasplib.isofts.kiev.ua/handle/123456789/215427
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Zitieren:Tuning of aggregation and film self-assembly of monomethincyanine dyes through variation of their monomer structure / M.M. Sieryk, O.P. Dimitriev // Semiconductor Physics Quantum Electronics & Optoelectronics. — 2019. — Т. 22, № 1. — С. 53-59. — Бібліогр.: 16 назв. — англ.

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Digital Library of Periodicals of National Academy of Sciences of Ukraine
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author Sieryk, M.M.
Dimitriev, O.P.
author_facet Sieryk, M.M.
Dimitriev, O.P.
citation_txt Tuning of aggregation and film self-assembly of monomethincyanine dyes through variation of their monomer structure / M.M. Sieryk, O.P. Dimitriev // Semiconductor Physics Quantum Electronics & Optoelectronics. — 2019. — Т. 22, № 1. — С. 53-59. — Бібліогр.: 16 назв. — англ.
collection DSpace DC
container_title Semiconductor Physics Quantum Electronics & Optoelectronics
description Formation of condensed films and solution aggregates of four different monomethincyanine dyes has been studied using optical absorption spectroscopy and simulation methods, depending on variation of the dye monomer structure. The structure of the molecular dimer as a basic unit for the formation of the condensed state was found to be largely dependent on heteroatoms in the dye structure and the presence of end hydrocarbon groups. The above factors mainly determine the mutual position of molecules in the dimer. It has been found that mutual orientation, intermolecular distance, and overlap of the adjacent molecules are the major factors influencing absorption spectra of dye aggregates. The dimer geometry that plays the primary role in film nucleation, however, has been shown to undergo changes depending on the temperature conditions or film thickness.
first_indexed 2026-03-23T19:02:11Z
format Article
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id nasplib_isofts_kiev_ua-123456789-215427
institution Digital Library of Periodicals of National Academy of Sciences of Ukraine
issn 1560-8034
language English
last_indexed 2026-03-23T19:02:11Z
publishDate 2019
publisher Інститут фізики напівпровідників імені В.Є. Лашкарьова НАН України
record_format dspace
spelling Sieryk, M.M.
Dimitriev, O.P.
2026-03-16T10:59:54Z
2019
Tuning of aggregation and film self-assembly of monomethincyanine dyes through variation of their monomer structure / M.M. Sieryk, O.P. Dimitriev // Semiconductor Physics Quantum Electronics & Optoelectronics. — 2019. — Т. 22, № 1. — С. 53-59. — Бібліогр.: 16 назв. — англ.
1560-8034
PACS: 78.40.Me, 81.16.Dn
https://nasplib.isofts.kiev.ua/handle/123456789/215427
https://doi.org/10.15407/spqeo22.01.53
Formation of condensed films and solution aggregates of four different monomethincyanine dyes has been studied using optical absorption spectroscopy and simulation methods, depending on variation of the dye monomer structure. The structure of the molecular dimer as a basic unit for the formation of the condensed state was found to be largely dependent on heteroatoms in the dye structure and the presence of end hydrocarbon groups. The above factors mainly determine the mutual position of molecules in the dimer. It has been found that mutual orientation, intermolecular distance, and overlap of the adjacent molecules are the major factors influencing absorption spectra of dye aggregates. The dimer geometry that plays the primary role in film nucleation, however, has been shown to undergo changes depending on the temperature conditions or film thickness.
We thank Dr. Yu. Slominskii for dyes granting, Dr. P. Lytvyn for the AFM studies, and Dr. K. Grytsenko for useful comments.
en
Інститут фізики напівпровідників імені В.Є. Лашкарьова НАН України
Semiconductor Physics Quantum Electronics & Optoelectronics
Hetero- and Low-Dimensional Structures
Tuning of aggregation and film self-assembly of monomethincyanine dyes through variation of their monomer structure
Article
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spellingShingle Tuning of aggregation and film self-assembly of monomethincyanine dyes through variation of their monomer structure
Sieryk, M.M.
Dimitriev, O.P.
Hetero- and Low-Dimensional Structures
title Tuning of aggregation and film self-assembly of monomethincyanine dyes through variation of their monomer structure
title_full Tuning of aggregation and film self-assembly of monomethincyanine dyes through variation of their monomer structure
title_fullStr Tuning of aggregation and film self-assembly of monomethincyanine dyes through variation of their monomer structure
title_full_unstemmed Tuning of aggregation and film self-assembly of monomethincyanine dyes through variation of their monomer structure
title_short Tuning of aggregation and film self-assembly of monomethincyanine dyes through variation of their monomer structure
title_sort tuning of aggregation and film self-assembly of monomethincyanine dyes through variation of their monomer structure
topic Hetero- and Low-Dimensional Structures
topic_facet Hetero- and Low-Dimensional Structures
url https://nasplib.isofts.kiev.ua/handle/123456789/215427
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