Electrostatics of the nanowire radial -- diode

In this paper, the electrostatic theory of the nanowire radial core-shell -- homojunction has been considered. The calculations carried out show that, in contrast to a planar -- diode, the built-in electric field of the nanowire radial -- diode proves to be inhomogeneous. This field reaches its maxi...

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Автор: Borblik, V.L.
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Опубліковано: Інститут фізики напівпровідників імені В.Є. Лашкарьова НАН України 2019
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Цитувати:Electrostatics of the nanowire radial -- diode / V.L. Borblik // Semiconductor Physics Quantum Electronics & Optoelectronics. — 2019. — Т. 22, № 2. — С. 201-205. — Бібліогр.: 16 назв. — англ.

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Digital Library of Periodicals of National Academy of Sciences of Ukraine
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author Borblik, V.L.
author_facet Borblik, V.L.
citation_txt Electrostatics of the nanowire radial -- diode / V.L. Borblik // Semiconductor Physics Quantum Electronics & Optoelectronics. — 2019. — Т. 22, № 2. — С. 201-205. — Бібліогр.: 16 назв. — англ.
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description In this paper, the electrostatic theory of the nanowire radial core-shell -- homojunction has been considered. The calculations carried out show that, in contrast to a planar -- diode, the built-in electric field of the nanowire radial -- diode proves to be inhomogeneous. This field reaches its maximum in the region of the i-layer adjoining the core. When moving away the i-layer from the nanowire center, the degree of field inhomogeneity decays, and both edge values of the field in the i-layer eventually reach the magnitude, which takes place in an analogous planar -- diode. This magnitude can be both higher and lower than the maximal field in the nanowire -- diode (depending on doping conditions). Simultaneously, the capacitance of the nanowire p-i-n diode can both increase and decrease in its value, going, at the same time, to weak voltage dependence inherent to the planar -- diode.
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fulltext ISSN 1560-8034, 1605-6582 (On-line), SPQEO, 2019. V. 22, N 2. P. 201-205. © 2019, V. Lashkaryov Institute of Semiconductor Physics, National Academy of Sciences of Ukraine 201 Hetero- and low-dimensional structures Electrostatics of the nanowire radial p-i-n diode V.L. Borblik V. Lashkaryov Institute of Semiconductor Physics, NAS of Ukraine, 41, prospect Nauky, 03680 Kyiv, Ukraine E-mail: borblik@isp.kiev.ua Abstract. In this paper, the electrostatic theory of the nanowire radial core-shell p-i-n homojunction has been considered. The carried out calculations show that, in contrast to planar p-i-n diode, the built-in electric field of the nanowire radial p-i-n diode proves to be inhomogeneous. This field reaches its maximum in the region of the i-layer adjoining to the core. When moving away the i-layer from the nanowire center, the degree of field inhomogeneity decays, and both edge values of the field in the i-layer reach eventually the magnitude, which takes place in analogous planar p-i-n diode. This magnitude can be both higher and lower than the maximal field in the nanowire p-i-n diode (depending on doping conditions). Simultaneously, the capacitance of the nanowire p-i-n diode can both increase and decrease in its value, going, at the same time, to weak voltage dependence inherent to the planar p-i-n diode. Keywords: nanostructures, core-shells nanowire, radial p-i-n junction, capacitance. https://doi.org/10.15407/spqeo22.02.201 PACS 61.46.Km, 62.23.St, 85.30.Kk Manuscript received 06.03.19; revised version received 24.03.19; accepted for publication 19.06.19; published online 27.06.19. 1. Introduction In the recent time, a great interest of the investigators is attracted to semiconductor nanowires, especially to the multilayer ones, whose layers are either doped in different ways or form a heterostructure. On the base of these objects, principally new constructions of the core- shell devices are created, which use both transverse (radial) transport of the current carriers (radial solar cells [1], radial photodiodes [2], radial light emitting devices [3]) and their longitudinal transport (field-effect transistor [4], high electron mobility transistor [5]). Cylindrical symmetry inherent to these nanostructures introduces a number of peculiarities to their electrophysical properties. In particular, depletion widths of the radial p-n junction depend on its radius in a rather nonstandard way: as radius of the p-n junction decreases, depletion width of the core increases [6], but that of the shell, on the contrary, decreases [7, 8]. As a result, in the devices where the heterostructure p-n junction is used, this fact results in changing the relative contribution to the device performance characteristics from different constituent materials. Namely, the lesser radius of the heterostructure p-n junction, the larger is contribution from the core material. In the radial p-n junction, the dependence 1/C 2 versus U (C is the barrier capacitance, U – applied voltage) proves to be nonlinear [6, 8]. Furthermore, strong asymmetry in injection from the core to shell and from the shell to core appears [9]. These studies concern nanowire p-n junction structures. At the same time, radial nanowire structures use often not p-n but p-i-n junctions [10-14]. In particular, this makes it possible to broaden the region of strong electric field in the junction, which is additional advantageous in materials with short minority carrier diffusion lengths [15]. Electrostatics of these structures was not studied so far. In this paper, electrostatics of the radial p-i-n homojunction has been investigated theoretically. 2. Theory Schematic view of the structure under consideration is presented in Fig. 1. Here rp is the depletion region boundary in the core, rn – depletion region boundary in the shell, and i-layer is located between r1 and r2. In the depletion approximation, we have Poisson’s equations   S AqN rE dr d r   1 , 1rrrp  , (1a)   0 1 rE dr d r , 21 rrr  , (1b) mailto:borblik@isp.kiev.ua SPQEO, 2019. V. 22, N 2. P. 201-205. Borblik V.L. Electrostatics of the nanowire radial p-i-n diode 202 0 rn p n rp r1 r2 i Fig. 1. Schematic view of the nanowire structure under consideration.   S DqN rE dr d r   1 , nrrr 2 , (1c) where q is the electron charge, εS – dielectric constant of the semiconductor, NA and ND are the concentrations of acceptors and donors, respectively. Solution of these equations gives the electric field distribution in the structure r rrqN E p S A 22 2    , 1rrrp  , (2a) r A E  , 21 rrr  , (2b) r rrqN E n S D 22 2    , nrrr 2 , (2c) where A is the integration constant. Matching the electric fields at r1 and r2, we obtain    22 2 22 1 22 n S D p S A rr qN rr qN A      , (3) whence it follows    2 2 222 1 rrNrrN nDpA  . (4) The second integration of Eq. (2) gives the potentials                       r r r rrqN rV p p p S A ln 22 2 22 , 1rrrp  , (5a)     constln  rArV , 21 rrr  , (5b) bi n n n S D V r r r rrqN rV                    ln 22 )( 2 22 , nrrr 2 , (5c) where the following boundary conditions are used   0prV ,   bin VrV  , (6) Vbi is the built-in potential of the junction. Matching of the potentials at r = r1 and r = r2 allows us to exclude const and obtain equation bi n n S Dp p S A V r r A r r r qN r r r qN                           1 2 2 2 1 2 lnln 2 ln 2 . (7) Equations (4) and (7) have to be solved jointly in order to obtain rp and rn. All the rest quantities are expressed through them. The barrier capacitance dU dQ C p  , where Qp is the electric charge concentrated in the depleted p-region of the junction. This charge is given by  LrrqNQ pAp 22 1  (8) where rp is voltage-dependent and L is length of the nanowire. Inasmuch as  pnpA Sp rrrqNdU dr ln 1  , (9) the capacitance per unit area of the p-i-n junction is  pn S rrr C ln 1 1   . (10) 3. Numerical results For numerical solution of Eqs. (4) and (7), the parameters of silicon at room temperature have been chosen. Three doping situations have been considered: NA = ND, NA >> ND, and NA << ND. The calculation results for the electric field distribution in the structure are presented in Fig. 2. The characteristic feature of these distributions is inhomogeneity of the field in the i-layer, which sharply differs from the case of planar p-i-n diode, where electric field in the i-layer is homogeneous [16]. The field inhomogeneity is especially strong when NA = ND or NA >> ND and diminishes with thickening of the i-layer. In any case, the electric field is maximal near the nanowire core. SPQEO, 2019. V. 22, N 2. P. 201-205. Borblik V.L. Electrostatics of the nanowire radial p-i-n diode 203 10 20 30 40 50 60 70 0.0 2.0x10 5 4.0x10 5 6.0x10 5 8.0x10 5 30,40 nm r, nm E , V /c m 30,50 nm N A = N D = 5x10 18 cm -3 30,60 nm a 30,30 nm 20 30 40 50 60 70 80 1x10 5 2x10 5 3x10 5 4x10 5 5x10 5 30,30 nm N A = 5x10 18 cm -3, N D = 5x10 17 cm -3 30,60 nm 30,50 nm E , V /c m r, nm 30,40 nm b 10 20 30 40 50 60 70 80 90 100 0 1x10 5 2x10 5 3x10 5 N A = 5x10 17 cm -3, N D = 5x10 18 cm -3 80,95 nm 80,85 nm 80,90 nm r, nm E , V /c m c 80,80 nm Fig. 2. Electric field distribution in the nanowire p-i-n diode at NA = ND (a), NA >> ND (b), and NA << ND (c); numbers near the curves are radial coordinates of the i-layer showing its extent, dashed lines corresponds to the i-layer of zero extent (p-n diode). 20 40 60 80 100 120 0 1x10 5 2x10 5 3x10 5 4x10 5 5x10 5 6x10 5 N A = N D = 5x10 18 cm -3 E , V /c m 807060 r 1 = 20 nm 30 40 r, nm 50 r 2 - r 1 = 20 nma inf 0 20 40 60 80 100 120 140 0 1x10 5 2x10 5 3x10 5 4x10 5 5x10 5 N A = 5x10 18 cm -3, N D = 5x10 17 cm -3 60 r, nm E , V /c m r 2 - r 1 = 20 nm 80 70 50 40 r 1 = 20 nm 30 b inf 20 40 60 80 100 120 140 160 0.0 5.0x10 4 1.0x10 5 1.5x10 5 2.0x10 5 2.5x10 5 N A = 5x10 17 cm -3, N D = 5x10 18 cm -3 r, nm E , V /c m r 2 - r 1 = 20 nm 120110 r 1 = 60 nm 70 80 90 100 c inf Fig. 3. Electric field distribution in the nanowire p-i-n diode depending on radial position of the i-layer at NA = ND (a), NA >> ND (b), and NA << ND (c); dashed lines shows to what magnitude both edge values of the field in the i-layer go, when the nanowire p-i-n diode becomes the planar one. SPQEO, 2019. V. 22, N 2. P. 201-205. Borblik V.L. Electrostatics of the nanowire radial p-i-n diode 204 -0.4 -0.2 0.0 0.2 0.4 0.6 2.5x10 5 3.0x10 5 3.5x10 5 4.0x10 5 4.5x10 5 5.0x10 5 5.5x10 5 r 1 = 20 nm r 2 - r 1 = 20 nm N A = N D = 5x10 18 cm -3 C , p F /c m 2 U, V 70 30 40 50 100 200 500 a -0.4 -0.2 0.0 0.2 0.4 0.6 1.5x10 5 2.0x10 5 2.5x10 5 3.0x10 5 3.5x10 5 4.0x10 5 4.5x10 5 r 2 - r 1 = 20 nm N A = 5x10 18 cm -3, N D = 5x10 17 cm -3 U, V C , p F /c m 2 r 1 = 20 nm 30 40 50 60 80 120 200 300 500 b -0.6 -0.4 -0.2 0.0 0.2 0.4 0.6 5.0x10 4 1.0x10 5 1.5x10 5 2.0x10 5 2.5x10 5 r 2 - r 1 = 20 nm N A = 5x10 17 cm -3, N D = 5x10 18 cm -3 C , p F /c m 2 500 300 200 150 120 U, V r 1 = 60 nm 70 80 90 100 c Fig. 4. Voltage dependences of the nanowire p-i-n diode capacitance at NA = ND (a), NA >> ND (b), and NA << ND (c) as a function of the distance between the i-layer and the nanowire center. It is of interest to study dependence of the electric field distributions on radial position of the i-layer in this nanowire. Fig. 3 represents such dependences for three doping situations at the same thickness of the i-layer equal to 20 nm. It is seen that, as the i-layer moves away from a center of the nanowire, inhomogeneity of the electric field distribution becomes more and more weak, i.e., the field goes to homogeneous one inherent to planar p-i-n diodes. The dash lines in these figures demonstrate asymptotical confluence of both edge values of the field in the i-layer, when r1 goes to infinity, i.e., the nanowire curvature becomes ignorable. It is seen also that the maximum electric field in the i-layer of nanowire proves to be higher than that in an analogous planar diode at NA = ND and NA >> ND and, on the contrary, is lower at NA << ND. Fig. 4 represents the voltage dependences of the nanowire p-i-n diode capacitance given by the formula (10) for three doping combinations as a function of the distance between the i-layer and center of the nanowire at the same value of the i-layer thickness equal to 20 nm. As it follows from these figures, the capacitance of the nanowire p-i-n diode decreases with moving away the i-layer from the nanowire center at NA = ND and NA >> ND and, on the contrary, increases at NA << ND. In any case, the voltage dependence of the capacitance diminishes as it has to be in planar p-i-n diode [16]. 4. Conclusions Being used as solar cells or photodiodes, the nanowire radial p-i-n diodes have certain advantages as compared with the planar analogs. In particular, at Ncore = Nshell or Ncore >> Nshell, the maximal built-in electric field in the i- layer proves to be higher than that in planar p-i-n diode under other equal conditions. But one has to keep in mind that the highest electric field is localized in the region of the i-layer adjoining to the core. It should be also noted that the capacitance of the nanowire p-i-n diode can be both larger and smaller than that of its planar analog at the same parameter values. Acknowledgement This work was supported by the National Academy of Sciences of Ukraine [project 2.2.6.34]. References 1. Tian B., Zheng X., Kempa T.J., Fang Y., Yu N., Yu G., Huang J., and Lieber C.M. Coaxial silicon nanowires as solar cells and nanoelectronic power sources. Nature. 2007. 449. P. 885–890. https://doi.org/10.1038/nature06181. 2. Soci C., Zhang A., Bao X.-Y., Kim H., Lo Y., and Wang D. Nanowire photodetectors. J. Nanosci. Nanotechnol. 2010. 10, No 3. P. 1430–1449. https://doi.org/10.1038/nature06181 SPQEO, 2019. V. 22, N 2. P. 201-205. Borblik V.L. Electrostatics of the nanowire radial p-i-n diode 205 3. Hua B., Motohisa J., Kobayashi Y., Hara S., and Fukui T. Single GaAs/GaAsP coaxial core-shell nanowire lasers. Nano Lett. 2009. 9, No 1. P. 112– 116. https://doi.org/10.1021/nl802636b. 4. Xiang J., Lu W., Hu Y., Wu Y., Yan H., and Lieber C.M. Ge/Si nanowire heterostructures as high- performance field-effect transistors. Nature. 2006. 441. P. 489–493. https://doi.org/ 10.1038/nature04796. 5. Jiang X., Xiong Q., Nam S., Qian F., Li Y., and Lieber C.M. InAs/InP radial nanowire heterostructures as high electron mobility devices. Nano Lett. 2007. 7, No 10. P. 3214–3218. https://doi.org/10.1021/nl072024a. 6. Petrosyan S., Yesayan A., and Nersesyan S. Theory of nanowire radial p-n-junction. World Academy of Science, Engineering and Technology, International Science Index 71, International Journal of Mathematical, Computational, Physical, Electrical and Computer Engineering. 2012. 6, No 11. P. 1065–1070. 7. Borblik V.L. Concerning the depletion width of a radial p-n junction and its influence on electrical properties of the diode. Semiconductor Physics, Quantum Electronics & Optoelectronics. 2017. 20, No 2. P. 168–172. http://doi.org/10.15407/spqeo20.02.168. 8. Borblik V.L. Electrostatics of nanowire radial p–n heterojunctions. J. Electron. Mater. 2018. 47, No 7. P. 4022–4027. https://doi.org/10.1007/s11664-018-6288-4. 9. Borblik V.L. Effect of circular p-n junction curvature on the diode current density. J. Electron. Mater. 2016. 45, No 8. P. 4117–4121. https://doi.org/10.1007/s11664-016-4597-z. 10. Tian B., Kempa T.J., and Lieber C.M. Single nanowire photovoltaics. Chem. Soc. Rev. 2009. 38, No 1. P. 16–24. https://doi.org/10.1039/b718703n. 11. Colombo C., Heiβ M., Grätzel M., Fontcuberta i Morral A. Gallium arsenide p-i-n radial structures for photovoltaic applications. Appl. Phys. Lett. 2009. 94, No 17. P. 173108. https://doi.org/10.1063/1.3125435. 12. Yoo J., Dayeh S.A., Tang W., and Picraux S.T. Epitaxial growth of radial Si p-i-n junctions for photovoltaic applications. Appl. Phys. Lett. 2013. 102, No 9. P. 093113. https://doi.org/10.1063/1.4794541. 13. Zhang Y., Sanchez A.M., Aagesen M. et al. Growth and fabrication of high-quality single nanowire devices with radial p-i-n junctions. Small. 2019. 15. P. 1803684 (7 p.). https://doi.org/10.1002/smll.201803684. 14. Qian F., Li Y., Gradečak S., Wang D., Barrelet C.J., and Lieber C.M. Gallium nitride-based nanowire radial heterostructures for nanophotonics. Nano Lett. 2004. 4, No 10. P. 1975–1979. https://doi.org/10.1021/nl0487774. 15. Abdellatif S. and Kirah K. Numerical modeling and simulation for a radial p-i-n nanowire photovoltaic device. Energy Procedia. 2013. 36. P. 488–491. https://doi.org/10.1016/j.egypro.2013.07.055. 16. Sze S.M. Physics of Semiconductor Devices. John Wiley & Sons, 1981. Authors and CV Dr. Vitalii L. Borblik graduated from Kiev State University in 1968. He received his PhD in physics and mathematics from the Institute of Semiconductors in Kiev (National Academy of Sciences of Ukraine) in 1978. At present, he is senior scien- tific researcher in the Department of Electric and Galvanomagnetic Pro- perties of Semiconductors at the V. Lashkaryov Institute of Semiconductor Physics. His researches include electron transport in semiconductor heterostructures, dynamical concentration lattices in bipolar semiconductor plasma, injection and exclusion phenomena in semiconductor devices and physics of the diode temperature sensors. Recent scientific interests of V.L. Borblik are electric and optic properties of nanostructured materials. ORSiD 0000-0002-8224-9170 https://doi.org/10.1038/nature04796 https://doi.org/10.1063/1.3125435 https://doi.org/10.1063/1.4794541 https://doi.org/10.1016/j.egypro.2013.07.055
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institution Digital Library of Periodicals of National Academy of Sciences of Ukraine
issn 1560-8034
language English
last_indexed 2026-03-23T18:52:40Z
publishDate 2019
publisher Інститут фізики напівпровідників імені В.Є. Лашкарьова НАН України
record_format dspace
spelling Borblik, V.L.
2026-03-18T11:39:09Z
2019
Electrostatics of the nanowire radial -- diode / V.L. Borblik // Semiconductor Physics Quantum Electronics &amp; Optoelectronics. — 2019. — Т. 22, № 2. — С. 201-205. — Бібліогр.: 16 назв. — англ.
1560-8034
PACS: 61.46.Km, 62.23.St, 85.30.Kk
https://nasplib.isofts.kiev.ua/handle/123456789/215464
https://doi.org/10.15407/spqeo22.02.201
In this paper, the electrostatic theory of the nanowire radial core-shell -- homojunction has been considered. The calculations carried out show that, in contrast to a planar -- diode, the built-in electric field of the nanowire radial -- diode proves to be inhomogeneous. This field reaches its maximum in the region of the i-layer adjoining the core. When moving away the i-layer from the nanowire center, the degree of field inhomogeneity decays, and both edge values of the field in the i-layer eventually reach the magnitude, which takes place in an analogous planar -- diode. This magnitude can be both higher and lower than the maximal field in the nanowire -- diode (depending on doping conditions). Simultaneously, the capacitance of the nanowire p-i-n diode can both increase and decrease in its value, going, at the same time, to weak voltage dependence inherent to the planar -- diode.
This work was supported by the National Academy of Sciences of Ukraine [project 2.2.6.34].
en
Інститут фізики напівпровідників імені В.Є. Лашкарьова НАН України
Semiconductor Physics Quantum Electronics &amp; Optoelectronics
Hetero- and Low-Dimensional Structures
Electrostatics of the nanowire radial -- diode
Article
published earlier
spellingShingle Electrostatics of the nanowire radial -- diode
Borblik, V.L.
Hetero- and Low-Dimensional Structures
title Electrostatics of the nanowire radial -- diode
title_full Electrostatics of the nanowire radial -- diode
title_fullStr Electrostatics of the nanowire radial -- diode
title_full_unstemmed Electrostatics of the nanowire radial -- diode
title_short Electrostatics of the nanowire radial -- diode
title_sort electrostatics of the nanowire radial -- diode
topic Hetero- and Low-Dimensional Structures
topic_facet Hetero- and Low-Dimensional Structures
url https://nasplib.isofts.kiev.ua/handle/123456789/215464
work_keys_str_mv AT borblikvl electrostaticsofthenanowireradialdiode