Specific features of thermal expansion and polyamorphism in CH4–C60 solutions at low temperatures

The temperature dependence of the linear thermal expansion coefficient α(T) has been investigated in the temperature range of 2.5 to 23 K for two different CH4–C60 solutions in which CH4 molecules occupied 24 and 50% of the octahedral interstitial sites of the C60 lattice. In both cases, α(T) exhibi...

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Date:2007
Main Authors: Dolbin, A.V., Esel’son, V.B., Gavrilko, V.G., Manzhelii, V.G., Vinnikov, N.A., Gadd, G.E., Moricca, S., Cassidy, D., Sundqvist, B.
Format: Article
Language:English
Published: Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України 2007
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Online Access:https://nasplib.isofts.kiev.ua/handle/123456789/7775
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Journal Title:Digital Library of Periodicals of National Academy of Sciences of Ukraine
Cite this:Specific features of thermal expansion and polyamorphism in CH4–C60 solutions at low temperatures / A.V. Dolbin, V.B. Esel’son, V.G. Gavrilko, V.G. Manzhelii, N.A. Vinnikov, G.E. Gadd, S. Moricca, D. Cassidy, B. Sundqvist // Физика низких температур. — 2007. — Т. 33, № 12. — С.1401-1405. — Бібліогр.: 16 назв. — англ.

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Digital Library of Periodicals of National Academy of Sciences of Ukraine
id nasplib_isofts_kiev_ua-123456789-7775
record_format dspace
spelling Dolbin, A.V.
Esel’son, V.B.
Gavrilko, V.G.
Manzhelii, V.G.
Vinnikov, N.A.
Gadd, G.E.
Moricca, S.
Cassidy, D.
Sundqvist, B.
2010-04-12T13:16:20Z
2010-04-12T13:16:20Z
2007
Specific features of thermal expansion and polyamorphism in CH4–C60 solutions at low temperatures / A.V. Dolbin, V.B. Esel’son, V.G. Gavrilko, V.G. Manzhelii, N.A. Vinnikov, G.E. Gadd, S. Moricca, D. Cassidy, B. Sundqvist // Физика низких температур. — 2007. — Т. 33, № 12. — С.1401-1405. — Бібліогр.: 16 назв. — англ.
0132-6414
https://nasplib.isofts.kiev.ua/handle/123456789/7775
The temperature dependence of the linear thermal expansion coefficient α(T) has been investigated in the temperature range of 2.5 to 23 K for two different CH4–C60 solutions in which CH4 molecules occupied 24 and 50% of the octahedral interstitial sites of the C60 lattice. In both cases, α(T) exhibits hysteresis, suggesting the existence of two types of orientational glass associated with these solutions. The temperature of the first-order phase transition between these two glasses was estimated and the behavior of these two glasses compared. The characteristic times of thermalization τ1, reorientation of the C60 molecules τ2, and of the phase transformation between the glasses τ', have been estimated for these solutions. Both the temperature dependence of α(T) and the characteristic thermalization time τ1are found to have features near the phase transition temperature and an explanation has been put forward to explain these observed features.
en
Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України
Динамика кристаллической решетки
Specific features of thermal expansion and polyamorphism in CH4–C60 solutions at low temperatures
Article
published earlier
institution Digital Library of Periodicals of National Academy of Sciences of Ukraine
collection DSpace DC
title Specific features of thermal expansion and polyamorphism in CH4–C60 solutions at low temperatures
spellingShingle Specific features of thermal expansion and polyamorphism in CH4–C60 solutions at low temperatures
Dolbin, A.V.
Esel’son, V.B.
Gavrilko, V.G.
Manzhelii, V.G.
Vinnikov, N.A.
Gadd, G.E.
Moricca, S.
Cassidy, D.
Sundqvist, B.
Динамика кристаллической решетки
title_short Specific features of thermal expansion and polyamorphism in CH4–C60 solutions at low temperatures
title_full Specific features of thermal expansion and polyamorphism in CH4–C60 solutions at low temperatures
title_fullStr Specific features of thermal expansion and polyamorphism in CH4–C60 solutions at low temperatures
title_full_unstemmed Specific features of thermal expansion and polyamorphism in CH4–C60 solutions at low temperatures
title_sort specific features of thermal expansion and polyamorphism in ch4–c60 solutions at low temperatures
author Dolbin, A.V.
Esel’son, V.B.
Gavrilko, V.G.
Manzhelii, V.G.
Vinnikov, N.A.
Gadd, G.E.
Moricca, S.
Cassidy, D.
Sundqvist, B.
author_facet Dolbin, A.V.
Esel’son, V.B.
Gavrilko, V.G.
Manzhelii, V.G.
Vinnikov, N.A.
Gadd, G.E.
Moricca, S.
Cassidy, D.
Sundqvist, B.
topic Динамика кристаллической решетки
topic_facet Динамика кристаллической решетки
publishDate 2007
language English
publisher Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України
format Article
description The temperature dependence of the linear thermal expansion coefficient α(T) has been investigated in the temperature range of 2.5 to 23 K for two different CH4–C60 solutions in which CH4 molecules occupied 24 and 50% of the octahedral interstitial sites of the C60 lattice. In both cases, α(T) exhibits hysteresis, suggesting the existence of two types of orientational glass associated with these solutions. The temperature of the first-order phase transition between these two glasses was estimated and the behavior of these two glasses compared. The characteristic times of thermalization τ1, reorientation of the C60 molecules τ2, and of the phase transformation between the glasses τ', have been estimated for these solutions. Both the temperature dependence of α(T) and the characteristic thermalization time τ1are found to have features near the phase transition temperature and an explanation has been put forward to explain these observed features.
issn 0132-6414
url https://nasplib.isofts.kiev.ua/handle/123456789/7775
citation_txt Specific features of thermal expansion and polyamorphism in CH4–C60 solutions at low temperatures / A.V. Dolbin, V.B. Esel’son, V.G. Gavrilko, V.G. Manzhelii, N.A. Vinnikov, G.E. Gadd, S. Moricca, D. Cassidy, B. Sundqvist // Физика низких температур. — 2007. — Т. 33, № 12. — С.1401-1405. — Бібліогр.: 16 назв. — англ.
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