Target unit for radiation test of materials under bremsstrahlung of electron accelerator

There is a necessity to provide an immobilization of the long-lived radioactive waste into radiation-resistant structure (a cement matrix, container capsule, geological disposal environment and so on) for it safely disposal. The material of the every of these barriers should have resistance correspo...

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Published in:Вопросы атомной науки и техники
Date:2001
Main Authors: Yeran, L.V., Karasyov, S.P., Pomatsalyuk, R.I., Sayenko, S.Yu., Shevchenko, V.A., Shlyakhov, I.N., Tenishev, A.Eh., Uvarov, V.L.
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Language:English
Published: Національний науковий центр «Харківський фізико-технічний інститут» НАН України 2001
Online Access:https://nasplib.isofts.kiev.ua/handle/123456789/79031
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Cite this:Target unit for radiation test of materials under bremsstrahlung of electron accelerator / L.V. Yeran, S.P. Karasyov, R.I. Pomatsalyuk, S.Yu. Sayenko, V.A. Shevchenko, I.N. Shlyakhov, A.Eh. Tenishev, V.L. Uvarov // Вопросы атомной науки и техники. — 2001. — № 5. — С. 206-208. — Бібліогр.: 5 назв. — англ.

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Digital Library of Periodicals of National Academy of Sciences of Ukraine
id nasplib_isofts_kiev_ua-123456789-79031
record_format dspace
spelling Yeran, L.V.
Karasyov, S.P.
Pomatsalyuk, R.I.
Sayenko, S.Yu.
Shevchenko, V.A.
Shlyakhov, I.N.
Tenishev, A.Eh.
Uvarov, V.L.
2015-03-24T18:51:56Z
2015-03-24T18:51:56Z
2001
Target unit for radiation test of materials under bremsstrahlung of electron accelerator / L.V. Yeran, S.P. Karasyov, R.I. Pomatsalyuk, S.Yu. Sayenko, V.A. Shevchenko, I.N. Shlyakhov, A.Eh. Tenishev, V.L. Uvarov // Вопросы атомной науки и техники. — 2001. — № 5. — С. 206-208. — Бібліогр.: 5 назв. — англ.
1562-6016
PACS number: 81.70.-q
https://nasplib.isofts.kiev.ua/handle/123456789/79031
There is a necessity to provide an immobilization of the long-lived radioactive waste into radiation-resistant structure (a cement matrix, container capsule, geological disposal environment and so on) for it safely disposal. The material of the every of these barriers should have resistance corresponding to the absorbed dose value up to 10⁸ Gy for the period of time up to 1000 years. The method of imitation exposure of the materials under bremsstrahlung of the high-current Linac was developed for prediction behavior and material selection. For realization of this method in a wide range of exposure conditions (by temperature, humidity, rate and amount of the doze) the special target unit was designed. It has a modular construction and includes two chambers for samples (one for exposure in liquid and another one – in the atmosphere) that are placed along the irradiation axis and integrated together spatially. Also, the target unit has plane-parallel ionization chamber for continuous monitoring of the photon flux intensity and absorbed doze. The copper thermistor is used as a temperature probe. The structure and characteristics of measurement channels are described as well.
Work is supported by STCU under contract N 1580.
en
Національний науковий центр «Харківський фізико-технічний інститут» НАН України
Вопросы атомной науки и техники
Target unit for radiation test of materials under bremsstrahlung of electron accelerator
Мишенное устройство для радиационных испытаний материалов в поле тормозного излучения ускорителя электронов
Article
published earlier
institution Digital Library of Periodicals of National Academy of Sciences of Ukraine
collection DSpace DC
title Target unit for radiation test of materials under bremsstrahlung of electron accelerator
spellingShingle Target unit for radiation test of materials under bremsstrahlung of electron accelerator
Yeran, L.V.
Karasyov, S.P.
Pomatsalyuk, R.I.
Sayenko, S.Yu.
Shevchenko, V.A.
Shlyakhov, I.N.
Tenishev, A.Eh.
Uvarov, V.L.
title_short Target unit for radiation test of materials under bremsstrahlung of electron accelerator
title_full Target unit for radiation test of materials under bremsstrahlung of electron accelerator
title_fullStr Target unit for radiation test of materials under bremsstrahlung of electron accelerator
title_full_unstemmed Target unit for radiation test of materials under bremsstrahlung of electron accelerator
title_sort target unit for radiation test of materials under bremsstrahlung of electron accelerator
author Yeran, L.V.
Karasyov, S.P.
Pomatsalyuk, R.I.
Sayenko, S.Yu.
Shevchenko, V.A.
Shlyakhov, I.N.
Tenishev, A.Eh.
Uvarov, V.L.
author_facet Yeran, L.V.
Karasyov, S.P.
Pomatsalyuk, R.I.
Sayenko, S.Yu.
Shevchenko, V.A.
Shlyakhov, I.N.
Tenishev, A.Eh.
Uvarov, V.L.
publishDate 2001
language English
container_title Вопросы атомной науки и техники
publisher Національний науковий центр «Харківський фізико-технічний інститут» НАН України
format Article
title_alt Мишенное устройство для радиационных испытаний материалов в поле тормозного излучения ускорителя электронов
description There is a necessity to provide an immobilization of the long-lived radioactive waste into radiation-resistant structure (a cement matrix, container capsule, geological disposal environment and so on) for it safely disposal. The material of the every of these barriers should have resistance corresponding to the absorbed dose value up to 10⁸ Gy for the period of time up to 1000 years. The method of imitation exposure of the materials under bremsstrahlung of the high-current Linac was developed for prediction behavior and material selection. For realization of this method in a wide range of exposure conditions (by temperature, humidity, rate and amount of the doze) the special target unit was designed. It has a modular construction and includes two chambers for samples (one for exposure in liquid and another one – in the atmosphere) that are placed along the irradiation axis and integrated together spatially. Also, the target unit has plane-parallel ionization chamber for continuous monitoring of the photon flux intensity and absorbed doze. The copper thermistor is used as a temperature probe. The structure and characteristics of measurement channels are described as well.
issn 1562-6016
url https://nasplib.isofts.kiev.ua/handle/123456789/79031
citation_txt Target unit for radiation test of materials under bremsstrahlung of electron accelerator / L.V. Yeran, S.P. Karasyov, R.I. Pomatsalyuk, S.Yu. Sayenko, V.A. Shevchenko, I.N. Shlyakhov, A.Eh. Tenishev, V.L. Uvarov // Вопросы атомной науки и техники. — 2001. — № 5. — С. 206-208. — Бібліогр.: 5 назв. — англ.
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first_indexed 2025-11-27T04:07:15Z
last_indexed 2025-11-27T04:07:15Z
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fulltext TARGET UNIT FOR RADIATION TEST OF MATERIALS UNDER BREMSSTRAHLUNG OF ELECTRON ACCELERATOR L.V. Yeran, S.P. Karasyov, R.I. Pomatsalyuk, S.Yu. Sayenko, V.A. Shevchenko, I.N. Shlyakhov, A.Eh. Tenishev, V.L. Uvarov NSC KIPT, Kharkov, Ukraine uvarov@kipt.kharkov.ua There is a necessity to provide an immobilization of the long-lived radioactive waste into radiation-resistant struc- ture (a cement matrix, container capsule, geological disposal environment and so on) for it safely disposal. The ma- terial of the every of these barriers should have resistance corresponding to the absorbed dose value up to 108 Gy for the period of time up to 1000 years. The method of imitation exposure of the materials under bremsstrahlung of the high-current Linac was developed for prediction behavior and material selection. For realization of this method in a wide range of exposure conditions (by temperature, humidity, rate and amount of the doze) the special target unit was designed. It has a modular construction and includes two chambers for samples (one for exposure in liquid and another one – in the atmosphere) that are placed along the irradiation axis and integrated together spatially. Also, the target unit has plane-parallel ionization chamber for continuous monitoring of the photon flux intensity and ab- sorbed doze. The copper thermistor is used as a temperature probe. The structure and characteristics of measurement channels are described as well. PACS number: 81.70.-q 1 INTRODUCTION The main goal of imitation exposure of the materials that are used for the immobilization of radionuclides is a creation of absorbed doze up to 108 Gy in investigated samples during acceptable period of the time (no more than 1 year) at monitoring parameters of radiation ef- fect. These parameters in the first instance are an ab- sorbed doze rate and a temperature of the samples. Namely these parameters define the annealing rate of the radiation defects, and thus, representability of the re- sults obtained. It is easy to make sure that the radiation heating of samples is no more than ~10° under absorbed doze rate noted above, i.e. contribution of the tempera- ture to annealing of defects in the process of imitation exposure can be ignored. However, the specified param- eters and also spectral characteristics of radiation are ba- sic objects of metrological accompaniment of the imita- tion exposure. The gamma-ray unit with radionuclide sources (basi- cally, Со-60) is a traditional radiation source for testing in doze range up to 108 Gy. The advantage of such tests is stability of influence conditions to the sample. There- with, the setup with activity up to 1 MCi is needed to provide the absorbed doze rate (ADR) about 10 Gy/s [2]. The electron accelerator can provide the same con- ditions with converting its beam to bremsstrahlung (BR) [3]. The value of the BR ADR in a sample of about 10 Gy/s for electrons with the energy 10 MeV is reached by converting a beam with the power 10 kW, that corresponds to parameters of modern industrial ac- celerators (see, for example, [4]). A possibility of the electron energy and flux control provides an expansion of range of the influence parameters to the sample dur- ing its test. The results of development of the special target unit for sample exposure under bremsstruhlung of high-cur- rent electron accelerator are presented in this report. 2 TARGET UNIT COMPONENTS 2.1. The target unit (TU) has a parallelepiped shape and consists of three chambers (Fig. 1). Beam scanning axis Iion T° ,C 2 1 3 4 5 Fig. 1. TU components. Upper hermetically sealed chamber 1 is designed for placement of samples, being irradiated in liquid (throat 2 is made to pass samples in liquid), and central cham- ber 3 – in air. The free-air ionization chamber (IC-1) is placed in volume 4 for continuously monitoring of pho- ton stream through the samples. The passage with tube 5 for the ionization chamber feed and signal cables is made in ceramic insulator. 2.2. The linear sweep of the electron beam within limits of the output accelerator window is performed by the electromagnet EM (see Fig. 2). The scanned beam is directed to the converter of bremsstruhlung C, that is a plate from material with a high atomic number (tantalum, tungsten) and placed into a tank being cooled by the running water. The thickness of the water layer under the plate is chosen so that the part of accelerated electrons passed through the plate is absorbed in this layer. The TU is placed under the bottom of the tank symmetrically to the line of the beam scan. An irregularity of the photon flow density on a surface of the TU is defined by distribution of the electron flow density on a surface C, and also by the width of TU and typically is less than ±5%. 206 mailto:uvarov@kipt.kharkov.ua e- A EM C Н2О TU γ Fig. 2. TU geometry placement. 3 COMPUTER SIMULATION As known, granite is the promising geological envi- ronment for radioactive waste disposal [4]. Therefore, the samples from granite (that consists of more than 70% of SiO2) was chosen as one from objects to study. The preliminary calculations showed that replacement of the real matrix from granite to pure SiO2 when simu- lating the radiation effect gives the results varied no mo- re than 3%, but the calculation time is reduced conside- rably in this case. Version of the TU analyzed with a method of the computer simulation is presented in Fig. 3. e- e- dН2О dAIR dSiО2 dCONV dSiО2 dIC Fig. 3. Geometry and parameters of simulation. dconv,cm dH2O,cm dair,cm dSiO2,cm dIC,cm 2 15 5 2 2 The calculations were made for three values of the ac- celerated electron energy: 10, 15 and 20 MeV with the average beam current 1mA (see Table 1). Analysis of the data obtained shows that the version of the TU under consideration provided an irradiation of the samples by “pure” braking photon flow in all the range of the accel- erated electron energy. Table 1. Simulation results Electron energy, MeV 10 15 20 Electron energy flux, kW 10 15 20 Number of absorbed elec- trons, % in converter in water filter 99.5 - 92.79 6.92 49.07 50.73 Photon energy flux at TU, kW 1.07 2.76 5.08 Average energy of photons, MeV 0.82 1.12 1.44 Absorbed power P of pho- ton radiation in SiO2, W 16.32 50.18 110.8 Ionization current I in IC, µ А 60 191 419 k=I/P, µА/W 3.64 3.80 3.78 The average photon energy Еγ by spectrum occurs near the values for such representative components of the radioactive waste as Cs-137 (Еγ=0.662 MeV) and Со-60 (Еγ=1.25 MeV), and ADR in SiO2 is ≥10 Gy/s, that satisfy the conditions of the imitation exposure. Close linear dependence of ionization current on ab- sorbed power of the braking photon radiation in SiO2 is observed in the investigated energy range of accelerated electrons. That can be explained by realization of the electron balance conditions for the given relation of electron energy and also the thickness of the water filter and irradiated samples [5]. This result gives a reason to carry out continuous nondestructive monitoring of the absorbed doze in irradiated samples from ionization charge in IC. 4 MEASUREMENT CHANNEL 4.1. In the context of the results noted above the measurement channel for the TU (Fig. 4.) was develo- ped and designed for on-line monitoring of absorbed doze and ADR of the photon radiation and also for mea- suring the temperature of samples under irradiation. The channel provides measurements both in the stand-alone mode and in the remote mode controlling by computer using RS-232 interface. Measurement circuit of photon radiation parameters Temperature measurement circuit IC-1 ТР-1 CPU module Power supply TU Fig. 4. Block-diagram of measurement channel. The channel includes two measurement circuits. The free-air ionization chamber IC-1 is used as a primary sensor in the measurement circuit of the braking radia- tion parameters. The thermal probe TP-1 is used in the measurement circuit of the sample temperature. 4.2 Technical data The measurement channel of photon radiation: - current range of the IC-1, µА - 5…5000 - relative measurement error of the IC-1 current, % - ≤ 3 The measurement channel of the sample tempera- ture: - temperature range, °С - 0…80 - relative measurement error, % - ≤ 3 The power supply produces a stabilized DC voltage ВОПРОСЫ АТОМНОЙ НАУКИ И ТЕХНИКИ. 2001. №5. Серия: Ядерно-физические исследования (39), с. 207-208. 207 +/-15 V to feed the measurement circuits and +5 V to feed the central-processing unit (CPU) module. 4.3 The measurement circuit of the photon radiation parameters A signal from the ionization chamber IC-1 (Fig. 5) directs to the input of the current-to-voltage converter (CVC). The voltage with the amplitude proportional to the input current is produced at the output of the CVC. Then a signal through the optoisolation and amplifier goes to the input 1 of the analog-to-digital converter (ADC). The CVC is made on a base of the operational amplifier (OA) type AD711. The resistors of type С2-29ОС ±0.5% are used to increase the time and tem- perature stability. IC-1 CVC Opto- isolation Amplifier Output U1 Fig. 5. Block-diagram of measurement circuit of ionization current. 4.4 The temperature measurement circuit The thermal probe TP-1 (Fig. 6.) is feed from the stable current generator with a magnitude of 1 mA. A signal from the thermistor TP-1 is going to the input of the thermostable differential amplifier (DA). The input of the DA has the filter for suppression of an HF noise. The DA is made on a base of OA type AD623 with the resistors С2-29. The CVC, the stable current generator and DA are placed into the thermostat from the foam plastic. ТР-1 Differential amplifier Opto- isolation Amplifier Output U2 Current generator Fig. 6. Block-diagram of temperature measurement circuit. 4.5 CPU module The CPU module (Fig. 7) consists of the following components: - ADC; - CPU; - data memory (RAM); - program memory(ROM); - indication module (IM); - control keypad (CK); - level translator of the serial interface (LT). ADC CPU Display unit Keypad ROM RAM RS-232 level translator INPUT1 INPUT2 To remote computer Fig. 7. Block-diagram of the CPU module. The basic functions performed by the CPU module are: - conversion of analogue signals from the measure- ment circuit to the digital code by the ADC; - storing the results of the measurements and con- verting them to physical units; - measurement data display; control of the operation mode by using the keypad; - data exchange between the CPU module and re- mote computer using a serial interface RS-232. 4.6 Measurement procedure After starting a measurement the CPU produces the control signals for the ADC during 10 ms with 1 s peri- od. The scan rate of ADC is 10 kHz. The values of ana- logue signals converted to the digital code from one of the measurement circuits are stored into the data me- mory RAM. Then these data are averaged, converted to physical units and output to the display unit. Every se- cond the measurement circuit is switched to another one. One time per second the increment of the measu- rement values are calculated and stored. The timer is started from the begining of measurement process for calculation of measurement time. The measurement pro- cess is stopped after a corresponded key has been pressed on the keypad. There are two mode of the CPU module operation: from the keypad control (stand-alone mode) and under control from the remote computer using a serial inter- face RS-232. In last case the data transfer to the remote computer. 5 CONCLUSION The special target unit to provide radiation tests of the material samples in bremsstrahlung field of the elec- tron accelerator has been developed with the follow pa- rameters range: - absorbed doze rate of photon radiation, Gy/s- 1…100; - absorbed doze, Gy - 103...1010; - average photon energy , MeV - 0.8…1.4; - samples temperature, Т°С - 0...80. The device has the measurement channel linked to the remote computer that provides on-line monitoring of the photon radiation parameters and temperature of the samples. Work is supported by STCU under contract N 1580. REFERENCES 1. N.P.Dikiy, S.Yu.Sayenko, V.L.Uvarov, E.P.Shevya- kova. Application of Nuclear-Physics Methods for Studying the Radionuclide Transport in Granite Rocks // Voprosy atomnij Nauki i Tekhniki. Seriya: “Yaderno-Fizicheskiye issledovaniya” (36). 2000, № 2, p. 54-57. 2. A.K.Krasin et al. Powerful gamma-setup UGU-200 // Atomnaya Ehnergiya. 1971, v. 31, N. 3, p. 205-207. 3. V.V.Kluyev et al. Nondistructive Control with the High-Energy Sources. Moscow: Energoatomizdat, 1989, 176 p. (in Russian). 4. Z.M.Deconik et al. Investigation of Possibility of Ra- 208 dioactive Waste Disposal in Deep Geological Forma- tion // Bulletin of Ecological State of Chernobyl Zone. 1999, v. 13, p. 64-66 (in Ukrainian). 5. V.Vexler et al. Ionization Methods for Investigation of Radiations. Moscow: GITTL, 1949, 424 p. ВОПРОСЫ АТОМНОЙ НАУКИ И ТЕХНИКИ. 2001. №5. Серия: Ядерно-физические исследования (39), с. 209-208. 209