Analysis of tungsten spectral-lines recorded from laser-target experiment

The paper is devoted to an analysis of selected experimental results obtained from space- and time-resolved spectroscopic measurements, which were performed during the interaction of an intense laser-beam (0.7 J, 2 ns) with a tungsten (W) target placed under high-vacuum conditions. The spectroscop...

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Published in:Вопросы атомной науки и техники
Date:2006
Main Authors: Tsarenko, A.V., Marchenko, A.K., Sadowski, M.J., Skladnik-Sadowska, E., Malinowski, K., Wolowski, J., Czarnecka, A., Gąsior, P., Parys, P., RosiĔski, M.
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Language:English
Published: Національний науковий центр «Харківський фізико-технічний інститут» НАН України 2006
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Online Access:https://nasplib.isofts.kiev.ua/handle/123456789/82155
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Cite this:Analysis of tungsten spectral-lines recorded from laser-target experiment / A.V. Tsarenko, A.K. Marchenko, M.J. Sadowski, E. Skladnik-Sadowska, K. Malinowski, J. Wolowski, A. Czarnecka, P. Gąsior, P. Parys, M. RosiĔski // Вопросы атомной науки и техники. — 2006. — № 6. — С. 150-152. — Бібліогр.: 5 назв. — англ.

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Digital Library of Periodicals of National Academy of Sciences of Ukraine
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author Tsarenko, A.V.
Marchenko, A.K.
Sadowski, M.J.
Skladnik-Sadowska, E.
Malinowski, K.
Wolowski, J.
Czarnecka, A.
Gąsior, P.
Parys, P.
RosiĔski, M.
author_facet Tsarenko, A.V.
Marchenko, A.K.
Sadowski, M.J.
Skladnik-Sadowska, E.
Malinowski, K.
Wolowski, J.
Czarnecka, A.
Gąsior, P.
Parys, P.
RosiĔski, M.
citation_txt Analysis of tungsten spectral-lines recorded from laser-target experiment / A.V. Tsarenko, A.K. Marchenko, M.J. Sadowski, E. Skladnik-Sadowska, K. Malinowski, J. Wolowski, A. Czarnecka, P. Gąsior, P. Parys, M. RosiĔski // Вопросы атомной науки и техники. — 2006. — № 6. — С. 150-152. — Бібліогр.: 5 назв. — англ.
collection DSpace DC
container_title Вопросы атомной науки и техники
description The paper is devoted to an analysis of selected experimental results obtained from space- and time-resolved spectroscopic measurements, which were performed during the interaction of an intense laser-beam (0.7 J, 2 ns) with a tungsten (W) target placed under high-vacuum conditions. The spectroscopic measurements were carried out by means of a Mechelle® 900 optical-spectrometer, and for the first time some tungsten spectral lines (WI and WII) were recorded. The most important parameters of a tungsten plasma plume were estimated using the fitting procedure. The appearance of the tungsten ions was also confirmed by a series of corpuscular measurements
first_indexed 2025-12-07T16:17:47Z
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fulltext 150 Problems of Atomic Science and Technology. 2006, 6. Series: Plasma Physics (12), p. 150-152 A.V. Tsarenko1 ANALYSIS OF TUNGSTEN SPECTRAL-LINES RECORDED FROM LASER-TARGET EXPERIMENT , A.K. Marchenko 1, M.J. Sadowski 2,3, E. Skladnik-Sadowska 2, K. Malinowski 2, J. Wolowski 3, A. Czarnecka 3, P. G sior 3, P. Parys 3, M. Rosi ski 3 1 Institute of Plasma Physics, NSC KIPT, Akademicheskaya Str.1, 61108 Kharkov, Ukraine; 2 The Andrzej Soltan Institute for Nuclear Studies (IPJ), 05-400 Otwock-Swierk, Poland; 3 Institute of Plasma Physics and Laser Microfusion (IPPLM), 00-908 Warsaw, Poland The paper is devoted to an analysis of selected experimental results obtained from space- and time-resolved spectroscopic measurements, which were performed during the interaction of an intense laser-beam (0.7 J, 2 ns) with a tungsten (W) target placed under high-vacuum conditions. The spectroscopic measurements were carried out by means of a Mechelle®900 optical-spectrometer, and for the first time some tungsten spectral lines (WI and WII) were recorded. The most important parameters of a tungsten plasma plume were estimated using the fitting procedure. The appearance of the tungsten ions was also confirmed by a series of corpuscular measurements. PACS: 52.50.Jm, 52.70.Kz, 52.70.Nc 1. INTRODUCTION Information about spectral lines emitted from tungsten (W) exited atoms and ions are of great importance for plasma research and fusion technology. Unfortunately such information is very scarce [1]. Therefore, it was decided to perform dedicated laser- target experiments under controlled experimental conditions. In general, studies of laser-produced plasmas are of importance for different branches of science and technology. The main aim of the described experiments was to record and analyze some optical W-spectra, which might be used e.g. for a comparison with results of spectroscopic measurements of plasma-target interactions inside various tokamak facilities. This study is important because tungsten is often used in different plasma facilities and it is the constructional material for ITER. 2. EXPERIMENTAL SET-UP AND SPECTROSCOPIC DIAGNOSTICS The experimental system used in our studies consisted of the main vacuum chamber, equipped with a movable target holder and ion diagnostic equipment, an external laser system and an optical spectrometer adapted for time-resolved measurements [2], as shown in Fig.1. Fig. 1. Experimental arrangement. The ion measuring equipment consisted of ion collectors and an electrostatic ion energy analyzer. The applied repetitive Nd- glass laser system could deliver a beam of = 1.06 m and E = 0.8 J in 3.5 ns pulses. The laser beam was introduced at an angle of 30o in relation to the target axis and focused upon the target center. During the experiments to be described the laser was operated with the repetition of = 10 Hz, and the power density upon the target amounted to about 1011 W/cm2. It was satisfactory to produce a W-plasma plume in front of the irradiated W-target. Each laser pulse had energy 540 mJ, and the focal spot had diameter equal to Df = 0.4 mm. The laser power density was IL= 1.4 x 1011 W/cm2. The spectroscopic measurements were carried out by means of a Mechelle®900 optical-spectrometer, which might be operated within the spectral range from 300 to 1100 nm. The system contained a special collimator, which was situated between a quartz observation window and a quartz optical cable coupled with the spectrometer. That collimator assured the spatial resolution of about 1 cm. The spectrometer had the spectral resolution equal to about 900 and the instrumental contour width of 0.5 nm within central region of the investigated spectrum. The applied exposure time was equal to 2 s. The recorded spectra were read with a cooled CCD camera coupled with a computer equipped with the GRAMS32-v.6.0 software, which made possible the fast and effective processing of the collected experimental data. 3. SPECTRAL ANALYSIS In order to obtain reliable information about W-plasma parameters a detailed analysis was performed using the well- known NIST database. Preliminary evaluations, which were performed on the basis of separate and randomly taken pairs of the recorded spectral lines, gave electron temperature (Te) values ranging from 0.5 to about 2 eV. Estimates of the electron concentration (Ne) gave values within the range from 1014 to 1019 cm-3 [3]. Although these estimates are close to those made in other laser-target experiments [4], one can easily notice considerable differences in the reported experiments. Our recent computational analysis of the recorded W spectra concerned normalized W-lines, which might be observed at different temperatures (Te = 0.1, 0.5, and 10 eV), as shown in Fig. 2. 151 Fig.2. Normalized W-spectra computed for different electron temperatures Te = 0.1 eV , 0.5 eV and 10 eV The performed analysis has indicated: • The strongest lines of WI and WII for the wide range of Te values; • The appearance of pure (separate) lines with the minimal overlapping; • The spectral lines (or groups of them), which are more or less sensitive to the electron temperature; • The lines undergoing the re-absorption (we selected the strongest lines with close energies of the excitation only). As for the observed spectra lines (and/or peaks) intensities have been verified with the object to self-absorption. Some peaks of the strongest lines, as expected, demonstrated a relatively high self- absorption. We took into consideration the lines having similar excitation energies only, because in such cases the intensity ratio is not a function of Te, but it depends on the Aki (or gf-values). For example, the WI 4294.6 and 4302.1 lines, for which the observed and calculated relative intensities were considerably different, are shown in Figs. 3,a and 3,b. The effects described above were taken into consideration during subsequent fitting procedures. It should, however, be noted that for the ion spectral lines it is in general very difficult to take into account the considered effects quantitatively. Some of the spectral lines with the strong self-absorption (e.g. WI 4008 Å peak) are shown above as those exceeding the limits of graphs. It should be noted that for a group of the W spectral lines within a wavelength range of 3572…3660 Å one can observe some discrepancy in the computed and recorded spectra (see Fig. 3a). For the shortest waves it might be explained by the fact that the transmission of the applied optical parts decreases in this range very sharply. In other wavelength regions the mentioned discrepancy might be due to differences in atomic (spectral) data from NIST and the spectroscopic data taken from other publications [5]. It seems that the observed spectral lines are closer to the old data. Fig.3. Recorded optical spectra and their fitting to those computed on the basis of the Saha-Boltzman equations. The rapid drop in the middle of the spectrum is an artificial effect induced by the spectrometer construction In the next phase of the analysis the most important parameters of a W-plasma plume were estimated using the fitting procedure as follows: in the first step we estimated electron temperature values to obtain a relatively good agreement for the recorded intensities of WI and WII spectral lines 4200 4400 4600 4800 5000 5200 0,01 0,1 1 wavelength, A In te ns ity , a .u . IntWI0.1 IntWI0.5 IntWI10 3500 3600 3700 3800 0,01 0,1 1 wavelenght, A In te ns ity , a .u . IntWII0.1 IntWII0.5 IntWII10 a) WI lines b) WII lines 4000 4100 4200 4300 4400 4000 5000 0 5000 10000 wavelength, A In te ns ity , a .u . spectrum411 (Counts) WI 1eV 8*10^16 WII 1eV 8*10^16 a) Te = 1 eV, Ne = 8 x 1016 cm-3 4000 4100 4200 4300 4400 4000 5000 0 40000 wavelength, A In te ns ity , a .u . spectrum411 (Counts) WI 0.8eV2*10^16 WII 0.8eV2*10^16 b) Te = 0.8 eV, Ne = 2 x 1016 cm-3 3500 3600 3700 3800 3900 4000 4100 0 1000 2000 3000 4000 5000 0 50000 In te ns ity , a .u . wavelength, A spectrum411 (Counts)WI 0.8eV2*10^16 WII 0.8eV2*10^16 c) Te = 0.8 eV, Ne = 2 x 1016 cm-3 152 . , . , separately; and in the second step the electron concentration value was determined to achieve the good agreement between the whole WI and WII spectra. As a result it was found that the most probable parameters of the investigated laser-produced W-plasma were as follows: Te 0.8…1 eV, Ne (2…8) x x 1016 cm-3. Using spectroscopic methods and it was also possible to estimate the concentration of the excited neutral W- atoms. Such an analysis is presented in Fig. 4. Fig.4. Distributions of ionization states of W-species computed on the basis of LTE relations Since, the estimated electron temperature was 0.8...1 eV, in the both considered cases one gets an approximated value N (WI) (1...3) x 1015 cm-3. The large uncertainty in the determination of Ne-values has been induced by a lack of additional experimental data. It is evident that more information about temporal evolutions of WI and WII spectral lines intensities or the total radiation is needed. 4. CONCLUSIONS The most important results of this study can be summarized as follows: 1. The tungsten spectral lines have been recorded and identified in the described laser-beam W-target experiments. 2. The electron temperature of W-plasma was estimated using the ratio of WII and WI spectral lines, and it was found that the most probable value was Te = 0.8…1 eV. It means that the recorded spectra were obtained from a late phase of that plasma expansion. 3. An estimate of the electron concentration value Ne (2…8) x 1016 cm-3 was performed using spectroscopic methods in order to achieve the good agreement between the whole recorded WI and WII spectra. 4. Information about the tungsten spectral lines and some procedures, which were used for the analysis, might be helpful in future studies, e.g., of the erosion of W-based constructional parts in fusion facilities. REFERENCES 1. A. Kallenbach et al.// Proc. 2nd GPPD, Cracow, Poland, Sept. 8-10, 2004, CD-issue, Inv05. 2. M.J. Sadowski, K. Malinowski et al.// Proc. SPIE Int. Congress on Optics & Optoelectronics, Warsaw 2005, SPIE Conf. Proc. 2005, v. 5948, p. 46-58. 3. M.J. Sadowski, E. Skladnik-Sadowska, et al.// Czech J. Phys. Suppl. B. 2006, v. 56, B550-B556. 4. S. S. Hariral, C. V. Bindhu et al.// J. Appl. Phys. 2003, v. 93, N 5, p. 2380-2388. 5. Ch. H. Cosliss and W. R. Bozman. Experimental transition probabilities for spectral lines of seventy elements. New York: Pergamon Press, 1962. , A.K. , . , . , . , . , A. , . , . , M. , (0.7 , 2 ) , . Mechelle®900 (WI WII). . . , A.K. , . , . , . , . , A. , . , . , . , (0.7 , 2 ) , . Mechelle®900 (WI WII). . . 0 0.2 0.4 0.6 0.8 1 1.2 1.4 1.6 1.8 2 2.2 2.40.1 0.2 0.3 0.4 0.5 0.6 0.7 0.8 0.9 WI WII WIII Electron temperature, eV Pa rti al d en si tie s 1 0.1 XI Te( ) XII Te( ) XIII Te( ) 2.40 Te a) Ne = 2 x 1016 cm-3 0 0.2 0.4 0.6 0.8 1 1.2 1.4 1.6 1.8 2 2.2 2.40.1 0.2 0.3 0.4 0.5 0.6 0.7 0.8 0.9 WI WII WIII Electron temperature, eV Pa rti al d en si tie s 1 0.1 XI Te( ) XII Te( ) XIII Te( ) 2.40 Te b) Ne = 8 x 1016 cm-3
id nasplib_isofts_kiev_ua-123456789-82155
institution Digital Library of Periodicals of National Academy of Sciences of Ukraine
issn 1562-6016
language English
last_indexed 2025-12-07T16:17:47Z
publishDate 2006
publisher Національний науковий центр «Харківський фізико-технічний інститут» НАН України
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spelling Tsarenko, A.V.
Marchenko, A.K.
Sadowski, M.J.
Skladnik-Sadowska, E.
Malinowski, K.
Wolowski, J.
Czarnecka, A.
Gąsior, P.
Parys, P.
RosiĔski, M.
2015-05-25T16:10:50Z
2015-05-25T16:10:50Z
2006
Analysis of tungsten spectral-lines recorded from laser-target experiment / A.V. Tsarenko, A.K. Marchenko, M.J. Sadowski, E. Skladnik-Sadowska, K. Malinowski, J. Wolowski, A. Czarnecka, P. Gąsior, P. Parys, M. RosiĔski // Вопросы атомной науки и техники. — 2006. — № 6. — С. 150-152. — Бібліогр.: 5 назв. — англ.
1562-6016
PACS: 52.50.Jm, 52.70.Kz, 52.70.Nc
https://nasplib.isofts.kiev.ua/handle/123456789/82155
The paper is devoted to an analysis of selected experimental results obtained from space- and time-resolved spectroscopic measurements, which were performed during the interaction of an intense laser-beam (0.7 J, 2 ns) with a tungsten (W) target placed under high-vacuum conditions. The spectroscopic measurements were carried out by means of a Mechelle® 900 optical-spectrometer, and for the first time some tungsten spectral lines (WI and WII) were recorded. The most important parameters of a tungsten plasma plume were estimated using the fitting procedure. The appearance of the tungsten ions was also confirmed by a series of corpuscular measurements
en
Національний науковий центр «Харківський фізико-технічний інститут» НАН України
Вопросы атомной науки и техники
Plasma dynamics and plasma wall interaction
Analysis of tungsten spectral-lines recorded from laser-target experiment
Article
published earlier
spellingShingle Analysis of tungsten spectral-lines recorded from laser-target experiment
Tsarenko, A.V.
Marchenko, A.K.
Sadowski, M.J.
Skladnik-Sadowska, E.
Malinowski, K.
Wolowski, J.
Czarnecka, A.
Gąsior, P.
Parys, P.
RosiĔski, M.
Plasma dynamics and plasma wall interaction
title Analysis of tungsten spectral-lines recorded from laser-target experiment
title_full Analysis of tungsten spectral-lines recorded from laser-target experiment
title_fullStr Analysis of tungsten spectral-lines recorded from laser-target experiment
title_full_unstemmed Analysis of tungsten spectral-lines recorded from laser-target experiment
title_short Analysis of tungsten spectral-lines recorded from laser-target experiment
title_sort analysis of tungsten spectral-lines recorded from laser-target experiment
topic Plasma dynamics and plasma wall interaction
topic_facet Plasma dynamics and plasma wall interaction
url https://nasplib.isofts.kiev.ua/handle/123456789/82155
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