The mathematical model for decay curve of the nuclei-delayed neutron precursors in experiment at a pulsed electron linear accelerator

On the basis of the notion about six groups of nuclei as delayed neutron precursors, radioactive decay laws and the pulsed mode of accelerator operation, a relationship has been derived to describe the decay curve of nuclei-delayed neutron precursors as a function of the pulse rate of the accelera...

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Опубліковано в: :Вопросы атомной науки и техники
Дата:2009
Автори: Buki, A.Yu., Gokov, S.P., Demeshko, O.A., Kasilov, V.I., Kokhnyuk, K.S., Kochetov, S.S., Mel’nitsky, I.V., Semisalov, I.L., Khomich, A.A., Shopen, O.A.
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Мова:Англійська
Опубліковано: Національний науковий центр «Харківський фізико-технічний інститут» НАН України 2009
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Онлайн доступ:https://nasplib.isofts.kiev.ua/handle/123456789/96514
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Цитувати:The mathematical model for decay curve of the nuclei-delayed neutron precursors in experiment at a pulsed electron linear accelerator / A.Yu. Buki, S.P. Gokov, O.A. Demeshko, V.I. Kasilov, K.S. Kokhnyuk, S.S. Kochetov, I.V. Mel’nitsky, I.L. Semisalov, A.A. Khomich, O.A. Shopen // Вопросы атомной науки и техники. — 2009. — № 5. — С. 95-100. — Бібліогр.: 9 назв. — англ.

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Digital Library of Periodicals of National Academy of Sciences of Ukraine
_version_ 1859717918441340928
author Buki, A.Yu.
Gokov, S.P.
Demeshko, O.A.
Kasilov, V.I.
Kokhnyuk, K.S.
Kochetov, S.S.
Mel’nitsky, I.V.
Semisalov, I.L.
Khomich, A.A.
Shopen, O.A.
author_facet Buki, A.Yu.
Gokov, S.P.
Demeshko, O.A.
Kasilov, V.I.
Kokhnyuk, K.S.
Kochetov, S.S.
Mel’nitsky, I.V.
Semisalov, I.L.
Khomich, A.A.
Shopen, O.A.
citation_txt The mathematical model for decay curve of the nuclei-delayed neutron precursors in experiment at a pulsed electron linear accelerator / A.Yu. Buki, S.P. Gokov, O.A. Demeshko, V.I. Kasilov, K.S. Kokhnyuk, S.S. Kochetov, I.V. Mel’nitsky, I.L. Semisalov, A.A. Khomich, O.A. Shopen // Вопросы атомной науки и техники. — 2009. — № 5. — С. 95-100. — Бібліогр.: 9 назв. — англ.
collection DSpace DC
container_title Вопросы атомной науки и техники
description On the basis of the notion about six groups of nuclei as delayed neutron precursors, radioactive decay laws and the pulsed mode of accelerator operation, a relationship has been derived to describe the decay curve of nuclei-delayed neutron precursors as a function of the pulse rate of the accelerator, the exposure time, the observation time, the time measurement interval and the number of measurement runs. A pilot experiment on thermal-neutron fission of 235U has been conducted. The aim of the experiment was to check the hardware and the information readout computer program. Based on the expressions derived, an analysis was performed and relative yields of delayed neutrons were determined. The present results are compared to the data obtained by other authors. For further development of the analysis, a question is brought up about the influence of additional conditions on the determination of relative delayedneutron yields. These additional conditions can be represented by certain expressions laid down when measuring delayed neutron yields directly between the accelerator pulses. Виходячи з представлення про шiсть груп ядер-попередникiв запiзнiлих нейтронiв, законiв радiоактивного розпаду, i iмпульсного режиму роботи прискорювача, отримано спiввiдношення, що описує криву розпаду ядер-попередникiв запiзнiлих нейтронiв у залежностi вiд частоти посилок прискорювача, часу експозицiї, часу спостереження, кроку вимiру за часом i кiлькостi циклiв вимiрiв. Проведено пробний експеримент з подiлу 235U тепловими нейтронами. Мета експерименту - перевiрка апаратури i комп’ютерної програми з’йому iнформацiї. На базi отриманих виражень проведено аналiз i визначено вiдноснi виходи запiзнiлих нейтронiв. Результати порiвнюються з iншими роботами. Як перспектива подальшого розвитку аналiзу, ставиться питання про вплив додаткових умов на визначення вiдносних виходiв запiзнiлих нейтронiв. Такими додатковими умовами можуть бути деякi вирази, сформульованi при вимiрi виходiв запiзнiлих нейтронiв безпосередньо мiж посилками прискорювача Исходя из представления о шести группах ядер-предшественников запаздывающих нейтронов, законов радиоактивного распада, и импульсного режима работы ускорителя, получено соотношение, описывающее кривую распада ядер предшественников запаздывающих нейтронов в зависимости от частоты посылок ускорителя, времени экспозиции, времени наблюдения, шага измерения по времени и количества циклов измерений. Проведен пробный эксперимент по делению 235U тепловыми нейтронами. Цель эксперимента - проверка аппаратуры и компьютерной программы съема информации. На базе полученных выражений проведен анализ и определены относительные выходы запаздывающих нейтронов. Результаты сравниваются с другими работами. Как перспектива дальнейшего развития анализа, ставится вопрос о влиянии дополнительных условий на определение относительных выходов запаздывающих нейтронов. Такими дополнительными условиями могут быть некоторые выражения, сформулированные при измерении выходов запаздывающих нейтронов непосредственно между посылками ускорителя.
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fulltext THE MATHEMATICAL MODEL FOR DECAY CURVE OF THE NUCLEI-DELAYED NEUTRON PRECURSORS IN EXPERIMENT AT A PULSED ELECTRON LINEAR ACCELERATOR A.Yu. Buki ∗, S.P. Gokov, O.A. Demeshko, V.I. Kasilov, K.S. Kokhnyuk, S.S. Kochetov, I.V. Mel’nitsky, I.L. Semisalov, A.A. Khomich, O.A. Shopen National Science Center ”Kharkov Institute of Physics and Technology”, 61108, Kharkov, Ukraine (Received July 24, 2009) On the basis of the notion about six groups of nuclei as delayed neutron precursors, radioactive decay laws and the pulsed mode of accelerator operation, a relationship has been derived to describe the decay curve of nuclei-delayed neutron precursors as a function of the pulse rate of the accelerator, the exposure time, the observation time, the time measurement interval and the number of measurement runs. A pilot experiment on thermal-neutron fission of 235U has been conducted. The aim of the experiment was to check the hardware and the information readout computer program. Based on the expressions derived, an analysis was performed and relative yields of delayed neutrons were determined. The present results are compared to the data obtained by other authors. For further development of the analysis, a question is brought up about the influence of additional conditions on the determination of relative delayed- neutron yields. These additional conditions can be represented by certain expressions laid down when measuring delayed neutron yields directly between the accelerator pulses. PACS: 28.20-v 1. INTRODUCTION The importance of the use of delayed neutrons in ap- plied nuclear physics is widely recognized [1]. Among the applications are the control and determination of small amounts of fissile elements (uranium and transuranium elements) in solid and liquid radioac- tive wastes, in spent fuel elements, and also the measurements of nuclear constants used in reac- tor engineering (relative yield and half-life period of certain groups of delayed neutrons). To determine the nuclear-physical constants, the world practice makes use of the fission processes of uranium, pluto- nium and other nuclei in neutron/gamma-ray beams. The beams may be both pulsed and continuous. The neutron/gamma-ray beams can be generated in different machines, including electron accelerators, through the use of targets-converters. Work [2] can serve an example of the use of a accelerator of con- tinuous action . The electrostatic accelerator was used there to obtain some nuclear-physical constants necessary for the development of nuclear reactor en- gineering. The research techniques for investigating the composition of transuranium wastes with the use of pulsed reactors are well developed in France [3]. Though the pulse techniques are more complicated as compared to the continuous methods, yet they have certain advantages. In the pulse technique, delayed neutrons can be registered by two methods during one measuring run. In the first method, de- layed neutrons are registered between the machine pulses in a certain time window chosen so as to reduce the background. In the second method, the sample is saturated with nuclei-delayed neutron precursors. Then the beam is switched off and the decay curve is measured. With machines of continuous action, only the measurement of the decay curve is possible. Since the delayed neutron yield registered between the pulses and the decay curve are described by the same parameters, the pulse technique is more infor- mative, because it provides a joint analysis of the data obtained by the two measuring methods. In our papers [4-9], we have developed the methods for de- termining fissile elements with the use of the pulsed electron accelerator. These methods can find their application in different countries (e.g., France, Rus- sia, etc.), where nuclear engineering is developing. Paper [8] was concerned with the first method of de- layed neutron registration (between the accelerator pulses). The present work is devoted to the second method (decay curve measurement). ∗Corresponding author. E-mail address: khomichaa@kipt.kharkov.ua PROBLEMS OF ATOMIC SCIENCE AND TECHNOLOGY, 2009, N5. Series: Nuclear Physics Investigations (52), p.95-100. 95 2. DERIVATION OF ANALYTIC DEPENDENCE FOR THE DELAYED NEUTRON YIELD UNDER THE DECAY CURVE 2.1. Main assumptions and definitions Let the accelerator pulse generate gi nuclei- delayed neutron precursors of group i = (1, 2, ... , 6); gi = const for all accelerator pulses; λi is the decay constant of the group i precursor; f is the acceler- ator pulse frequency (δt = 1/f is the time between the pulses). We assume the machine pulse dura- tion to be substantially shorter than the time be- tween the pulses, therefore it will be neglected in our further considerations. The last assumption follows from the fact that the pulse duration is ≈ 1 · 10−6s, while the interpulse interval at operating frequency of 50Hz makes 0.02s. The computer program of information readout and management is character- ized by the exposure time texp = µδt, µ being the number of pulses for the given time texp; the ob- servation time tobs (in the general case we assume texp 6= tobs); the time measurement interval tint (de- cay curve integration step or the time observation channel width), tint = const; the time observation channel number-k; the number of measurement runs- n. The measurement procedure includes the alter- nating cycles of accumulation of nuclei-precursors for the time texp = µδt and the cycles of observation of delayed neutrons for the time tobs. The accumu- lation cycle begins from the moment of accelerator beam switching and ends as the time texp elapses with the beam switched off. As the beam is switched off, the observation cycle begins and lasts tobs seconds. With the end of the observation cycle another accu- mulation cycle starts, and so on. Under the above- described assumptions, our task is to derive the ex- pression, which describes the delayed neutron yield of all groups in the k-th time channel for n cycles. We divide the task into two stages. The first stage con- sists in the derivation of expression for the number of accumulated nuclei-precursors of the i-th group in a certain arbitrary l-th cycle; the second stage lies in the derivation of the final formula. 2.2. The number of accumulated nuclei-precursors of the i-th group in an arbitrary l-th cycle We denote the unknown number of accumulated nuclei-precursors of the i-th group in an arbitrary l-th cycle as Nµl i (this symbol indicates that the ac- cumulation took place during µ accelerator pulses). Let Nµ i be the number of nuclei-precursors of the i- th group, which were accumulated for µ accelerator pulses in one cycle, and Nµ i = const for all the cy- cles. Then the number of precursors of group i, which were accumulated in the first cycle is Nµ1 i = Nµ i . The number of precursors accumulated in the second cycle is equal to Nµ2 i = Nµ i + Nµ i e−λitobs = Nµ i (1 + e−λitobs) . For the third cycle we have: Nµ3 i = Nµ i (1 + e−λitobs + e−λi2tobs) . Reasoning by induction, one can write down Nµl i = Nµ i (1+e−λitobs +e−λi2tobs +...+e−λi(l−1)tobs) . After finding the sum of geometrical progression, we have: Nµl i = Nµ i 1− e−λiltobs 1− eλitobs . (1) 2.3. Derivation of the final formula Using eq. (1), we find the number of i-th group de- layed neutrons that came to the timing channel k in the cycle l: 4Nµl ik = Nµ i 1− e−λiltobs 1− eλitobs (e−λi(k−1)tint − e−λiktint) . (2) Summing expression (2) over l = (1, 2, . . . , n), we ob- tain the number of i-th group delayed neutrons that came to the timing channel k during all the given n cycles: 4Nµ ikn = Nµ i e−λi(k−1)tint − e−λiktint 1− e−λitobs × (n− e−λitobs − e−λi(n+1)tobs 1− e−λitobs ) . (3) Summation of expression (3) over i gives the yield of all the groups of delayed neutrons in the arbitrary timing channel k for n measurement cycles 4Nµ kn = 6∑ i=1 Nµ i e−λi(k−1)tint − e−λiktint 1− e−λitobs × (n− e−λitobs − e−λi(n+1)tobs 1− e−λitobs ) . (4) It has been demonstrated in ref. [8] that Nµ i can be represented as: Nµ i = gi e−λi/f 1− e−λi/f (1− e−λiµδt) . (5) In the following, formula (4) will be the basis for the analysis of our preliminary experiment. If λi/f ¿ 1 for all neutron groups, then relation (5) can be rep- resented in the following form: Nµ i = gi f λi (1− e−λiµδt) = N0i(1− e−λiµδt), (6) where N0i = limtexp→∞Nµ i is the number of nuclei- precursors of group i accumulated in the sample at the cut-off time of the accelerator and at the start of measuring the decay curve at a sufficiently great texp. Practically, texp is approximately equal to 5T , where T is the half-life period of the most long-lived group. In our experiment, f = 50 Hz and the con- dition λi/f ¿ 1 can be fulfilled. So, in the analysis of our preliminary experiment by formula (4) the Nµ i parameter was taken in the form of expression (6). 96 The aim of the analysis has been to estimate the rel- ative yields of delayed neutrons under the decay curve Di = N0i/ ∑ N0i as well as the relative yields during fission ai = gi/ ∑ gi , and to compare them with the available data. For further discussion we note that at λi/f ¿ 1 these parameters can be represented as: Di = aiTi∑ aiTi , ai = N0iλi∑ N0iλi , where Ti is the half-life period of the i-th group, the other quantities being defined above. 3. EXPERIMENTAL SETUP AND THE MEASURING TECHNIQUE The experiment was performed at the NSC KIPT 300 MeV electron linear accelerator (LUE-300). The main units of the facility include: the linear accel- erator, the neutron-producing target, the sample to be studied (a mixture of 238U and 235U with 2% of 235U), a polyethylene warmer, the Mac-Kiben detec- tor to register neutrons (see for its details in ref. [9]). A new element of the setup, as compared with the cited work, is represented by a computer control of both the process of information readout and the ex- perimental conditions. The experiment on measuring the decay curve of nuclei-delayed neutron precursors was carried out at the energy of electrons incident on the neutron-producing target E = 16 MeV , beam current I = 34 µA, pulse frequency f = 50Hz. In front of the sample there was placed a warmer, which represented a polyethylene unit, 8cm in thickness. To detect neutrons, the all-wave Mac-Kiben detector was used. The program-controlled experimental condi- tions were as follows: exposure time texp = 300 s, the measurement interval tint = 1 s, the observation time tobs = 300 s, the number of cycles n = 4. Considering that the warmer was present in the experiment, in the treatment of the experimental data it was assumed that it was 235U which mainly fissioned. Figure shows the results of decay curve measurements ver- sus the time channel number (points with error bars). Fig. The results of decay curve measurements versus the time channel number 4. ANALYSIS OF THE EXPERIMENTAL DATA AND PROSPECTS FOR INVESTIGATIONS Two analytic treatments have been performed. The first treatment made use of the parameters ai taken from work [2]. The aim of the given analysis was to estimate N0i and the relative contributions from different groups of delayed neutrons under the decay curve Di = N0i/ΣN0i. The second direct determi- nation of N0i from the analysis of the decay curve made use of the least-squares method with a subse- quent estimation of Di and ai. A question has been brought up about additional conditions that exert an influence on the determination of the sought-for parameters. These additional conditions can be for- mulated when registering delayed neutrons between the accelerator pulses. 1. Using the relation ai = gi/ ∑6 1 gi we write down the parameters gi in terms of ai and substi- tute the resuly into expression (6). Then formula (4) takes on the form: 4Nµ kn = βf 6∑ i=1 ai λi (1− e−λitexp)× e−λi(k−1)tint − e−λiktint 1− e−λitobs × (n− e−λitobs − e−λi(n+1)tobs 1− e−λitobs ) , (7) where β = ∑6 1 gi With the ai parameters for 235U taken from ref. [2] and with the use of the least- squares method, the model dependence was brought into agreement with the experiment by varying the parameter β, which physically presents (to an ac- curacy of the proportionality factor) the number of nuclei-precursors of all six groups generated by one accelerator pulse. The fitting has resulted in β = 16.71 ± 0.12, ∑ χ2 k/(N − 1) = 1.57, N = 78 being the number of points under the decay curve (see Fig.1, solid curve). Note that in this analysis only 78 experimental points were involved (we had 300 experimental values). This is explained by the fact that the supplementation of experimental points (more than 78) produces no essential effect on the de- finable parameter β. With an increase in the number of experimental points up to 300, the β value changes only by 0.1%. and an experimental error in it of 0.7%. The analysis under discussion well predicts the total number of events under the decay curve. The ex- periment gives the total number of events under the decay curve to be 43087 ± 208. The model value of this parameter can be estimated by the formula: 4 ·∑6 1 N0i, where N0i is the second column of Tab.1 (N0i = fai ∑ gi/λi, ai, λi are taken from ref. [2],∑ gi - our analysis). The fourth column of Table1 gives the relative yields of delayed neutron groups under the decay curve: Di = N0i/ ∑ N0i (N0i is the second column of Table 1). 97 Table. 1. The number of nuclei-precursors of group i accumulated for one measurement cycle-N0i, and the relative yield of the i-th group delayed neutrons under the decay curve-Di. Here we used the following designations: Ng-Group number; N∗ 0i-Calculated, using parameters from [2]; N∗∗ 0i -Our data; D∗ i -Calculated, using parameters from [2]; D∗∗ i -Our data Ng N∗ 0i N∗∗ 0i D∗ i D∗∗ i 1 2476± 94 2469± 118 0.228± 0.09 0.246± 0.014 2 5685± 90 4941± 192 0.524± 0.010 0.492± 0.025 3 1523± 26 1561± 191 0.140± 0.003 0.155± 0.019 4 1078± 13 1007± 139 0.099± 0.002 0.100± 0.014 5 78± 2 68± 48 0.007± 0.0002 0.007± 0.005 6 6± 1 −3± 2.6 5± 4 0.0005± 0.0001 0.0005± 0.0004 2. For the analysis, formula (4) was taken in the following form: 4Nµ kn = 6∑ i=1 N0i ( 1− e−λitexp )× e−λi(k−1)tint − e−λiktint 1− e−λitobs × ( n− e−λitobs − e−λi(n+1)tobs 1− e−λitobs ) , (8) where N0i represents the sought-for parameters. From the condition: ∂χ2/∂N0i = 0 a set of lin- ear equations was formulated, and N0i was deter- mined with the least-squares method. This analysis has involved 240 experimental points. A further increase in the number of experimental points for the analysis does not change the N0i values. For control, the set was solved in two ways using the Cramer and the Gauss method. In this case, it ap- peared that the quality of agreement between the analytic curve and the experiment is characterized as∑ χ2 k/(N − P ) = 1, 1, (N = 240, P = 6). On finding N0i, relative yields of delayed neutrons were deter- mined both under the decay curve: Di = N0i/ ∑ N0i and under fission: ai = N0λi/ ∑ N0λi. The N0i val- ues are listed in the third column of Table 1. It can be seen from the table that N06 = −3 ± 2.6, this having, unfortunately, no physical meaning. The estimation of N06 with physical meaning was per- formed using the expression: N06 = N05λ5a6/λ6a5 , where N05 was taken from our analysis, while the other parameters were taken from ref. [2]. The Di values are presented in the fifth column of Table 1. The comparison of the N0i and Di values obtained in this section with similar values of the previous sec- tion (see table 1) shows them to be coincident within the experimental error (the exception is the second group). A comparatively great error is caused by the fact that in the preliminary experiment there were only 4 measurement cycles. Table 2 gives the values of relative yields ai. It is obvious from the table 2 that within the experimental error the ai values agree very closely with the results of ref. [2]. To conclude the analysis, we formulate below possible additional con- ditions for the search for the decay curve parameters. Table 2. Relative delayed neutron yields of six groups in thermal-neutron fission of 235U Ng ai − our data ai − from[2] 1 0.041± 0.003 0.038± 0.001 2 0.197± 0.014 0.211± 0.004 3 0.217± 0.026 0.197± 0.004 4 0.397± 0.064 0.396± 0.005 5 0.123± 0.081 0.132± 0.004 6 0.025± 0.020 0.026± 0.001 5. ADDITIONAL CONDITIONS ON THE SEARCH FOR THE DECAY CURVE PARAMETERS We now formulate additional conditions on the search for the decay curve parameters that can be obtained when registering neutrons between the accelerator pulses. In the preliminary experiment considered above, the measurements of delayed neutron yields between the pulses were not performed. Therefore, the conditions formulated below can be considered as a prospect for further investigations of the decay curve. At λi/f ¿ 1 , the following expressions are valid: ∑ N0i = fT ∑ gi/ln 2, where T = ∑ aiTi, ai are the relative yields of delayed neutrons, Ti are the half-lives of nuclei-precursors. It has been demon- strated in paper [8] that if, at least, two measure- ments of delayed neutron yields are made with regis- tration between the accelerator pulses with the times of exposure t1 >> 1/λi and t2 >> 1/λi (for definite- ness, we assume that t2 > t1), then T and ∑ gi can be determined from the following equations: N(t2) N(t1) = t2 ln 2− T t1 ln 2− T, , ∑ gi = (N(t2)−N(t1))δt (tend − tin)(t2 − t1)f , where N(t1) and N(t2) are the delayed neutron yields for the exposures t1 and t2, tend - tin is the time ob- servation channel width, tin is the start time, tend is the end time point (the time is computed from the moment of the accelerator pulse), the remaining parameters are described above. So, performing the 98 experiment between the pulses, we can formulate ad- ditional conditions on the search for the parameters of the decay curve in the following form: ∑ N0i − fT ∑ gi/ln 2 = 0, . Besides, the delayed neutron yield registered between the accelerator pulses for the time texp [8] can be an additional condition in the search of the decay curve parameters, because this yield and the decay curve are described by the same parameters: N(texp) = ∑ gi e−λitin − e−λitend 1− e−λi/f × ( f · texp − e−λi/f 1− e−λi/f ( 1− eλitexp )) . (9) In finding the parameters by the least-squares method at additional conditions, the accuracy of the sought-for parameters often gets improved. In future, we expect to investigate the influence of the men- tioned additional conditions obtained between the ac- celerator pulses on the accuracy of determination of decay curve parameters. Technically, the task is re- duced to finding the constrained minimum of the χ2 function and can be solved by the Lagrange method of undetermined coefficients. 6. CONCLUSIONS 1. An analytic representation of the decay curve has been obtained for the analysis and design of ex- periments. 2. A preliminary experiment has been performed to check the instrumentation and the computer infor- mation readout program. 3. The results of experimental data analysis are in agreement within the experimental error with the data of paper [2]. 4. The question has been brought up about ad- ditional conditions that exert influence on the deter- mination of decay curve parameters. References 1. V.V. Frolov. Nuclear techniques to control fissionable materials. M: ”Ehnergoatomizdat” 1989, 178p. (In Russian). 2. V.M. Piksaikin, L.E. Kazakov, G.G. Korolyov, S.G. Isayev, V.A. Roshchenko, M.Z. Tarasko. The relative yield and period of some delayed neutron groups at fission of 233U , 235U , 239Pu by epithermal neutrons // Atomnaya Ehnergiya. 2000, v.92, p.135-143 (In Russian). 3. A. Lyoossi, J. Romeyer-Dherbey, F. Jallu, et al. Transuranic waste detection by photon interro- gation and on-line delayed neutron counting // Nuclear Instruments and Methods in Physics Re- search. 2000, v.B160, p.280-289. 4. A.Yu. Buki, V.Y. Kasilov, V.V. Kirichenko, et al. Development of the industrial technique to deter- mine the fissionable material concentration using the electron linac as the base // Atomna Ehner- getika ta Promyslovist’ Ukrainy. 2000, N2, p.24- 25 (In Ukrainian). 5. V.I. Kasilov, V.V. Kirichenko, L.A. Makhnenko, et al. About possible determination of the 238U content in concrete samples by means of the elec- tron linac. Atomna Ehnergetika ta Promyslovist’ Ukrainy. 2000, N2, p.50-51 (In Russian). 6. R.P. Slabospitsky, S.S. Kochetov, V.V. Kirichenko. Rapid radioactive waste sorting system using the electron linac. Preprint KhFTI 2002-1. Kharkov, NSC KIPT , 2002, 19p.(In Russian). 7. S.S. Kochetov, R.P. Slabospitsky, V.V. Kirichenko. The use of the electron linac for determining fissionable materials in radioactive wastes // Visnyk Kharkivs’kogo Universytetu, ser. fizychna ”Yadra, chastynky, polya”. 2002, v.B.2(20), N.574, p.71-80 (In Russian). 8. A.A. Khomich, V.I. Kasilov, V.V. Kirichenko, et al. The model of delayed neutron yield in the experiment at the pulsed electron linac // Visnyk Kharkivs’kogo Universytetu, ser. fizychna ”Yadra, chastynky, polya”. 2006, v.B2(30), N732, p.87-95 (In Russian). 9. A.Yu. Buki , V.I.Kasilov , V.V. Kirichenko, et al. Method for defining the concentration of fissile materials in radioactive waste // Vo- prosy Atomnoj Nauki i Tekhniki. Ser. ”yaderno- fizicheskaya”. 2000, v. 2(36), p.64-65. МАТЕМАТИЧЕСКAЯ МОДЕЛЬ КРИВОЙ РАСПАДА ЯДЕР, ПРЕДШЕСТВЕННИКОВ ЗАПАЗДЫВАЮЩИХ НЕЙТРОНОВ, В ЭКСПЕРИМЕНТЕ НА ИМПУЛЬСНОМ ЛИНЕЙНОМ УСКОРИТЕЛЕ ЭЛЕКТРОНОВ А.Ю. Буки, С.П. Гоков, О.А. Демешко, В.И. Касилов, К.C. Кохнюк, С.С. Кочетов, И.В. Мельницкий, И.Л. Семисалов, А.A. Хомич, О.A. Шопен Исходя из представления о шести группах ядер-предшественников запаздывающих нейтронов, законов радиоактивного распада, и импульсного режима работы ускорителя, получено соотношение, описыва- 99 ющее кривую распада ядер предшественников запаздывающих нейтронов в зависимости от частоты посылок ускорителя, времени экспозиции, времени наблюдения, шага измерения по времени и коли- чества циклов измерений. Проведен пробный эксперимент по делению 235U тепловыми нейтронами. Цель эксперимента - проверка аппаратуры и компьютерной программы съема информации. На базе полученных выражений проведен анализ и определены относительные выходы запаздывающих ней- тронов. Результаты сравниваются с другими работами. Как перспектива дальнейшего развития ана- лиза, ставится вопрос о влиянии дополнительных условий на определение относительных выходов запаздывающих нейтронов. Такими дополнительными условиями могут быть некоторые выражения, сформулированные при измерении выходов запаздывающих нейтронов непосредственно между посыл- ками ускорителя. МАТЕМАТИЧНА МОДЕЛЬ КРИВОЇ РОЗПАДУ ЯДЕР, ПОПЕРЕДНИКIВ ЗАПIЗНIЛИХ НЕЙТРОНIВ, В ЕКСПЕРИМЕНТI НА IМПУЛЬСНОМУ ЛIНIЙНОМУ ПРИСКОРЮВАЧI ЕЛЕКТРОНIВ О.Ю. Букi, С.П. Гоков, О.О. Демешко, В.Й. Касилов, К.C. Кохнюк, С.С. Кочетов, I.В. Мельницький, I.Л. Семiсалов, А.A. Хомич, О.О. Шопен Виходячи з представлення про шiсть груп ядер-попередникiв запiзнiлих нейтронiв, законiв радiоак- тивного розпаду, i iмпульсного режиму роботи прискорювача, отримано спiввiдношення, що описує криву розпаду ядер-попередникiв запiзнiлих нейтронiв у залежностi вiд частоти посилок прискорюва- ча, часу експозицiї, часу спостереження, кроку вимiру за часом i кiлькостi циклiв вимiрiв. Проведено пробний експеримент з подiлу 235U тепловими нейтронами. Мета експерименту - перевiрка апаратури i комп’ютерної програми з’йому iнформацiї. На базi отриманих виражень проведено аналiз i визначено вiдноснi виходи запiзнiлих нейтронiв. Результати порiвнюються з iншими роботами. Як перспектива подальшого розвитку аналiзу, ставиться питання про вплив додаткових умов на визначення вiдносних виходiв запiзнiлих нейтронiв. Такими додатковими умовами можуть бути деякi вирази, сформульованi при вимiрi виходiв запiзнiлих нейтронiв безпосередньо мiж посилками прискорювача. 100
id nasplib_isofts_kiev_ua-123456789-96514
institution Digital Library of Periodicals of National Academy of Sciences of Ukraine
issn 1562-6016
language English
last_indexed 2025-12-01T08:35:45Z
publishDate 2009
publisher Національний науковий центр «Харківський фізико-технічний інститут» НАН України
record_format dspace
spelling Buki, A.Yu.
Gokov, S.P.
Demeshko, O.A.
Kasilov, V.I.
Kokhnyuk, K.S.
Kochetov, S.S.
Mel’nitsky, I.V.
Semisalov, I.L.
Khomich, A.A.
Shopen, O.A.
2016-03-17T20:49:39Z
2016-03-17T20:49:39Z
2009
The mathematical model for decay curve of the nuclei-delayed neutron precursors in experiment at a pulsed electron linear accelerator / A.Yu. Buki, S.P. Gokov, O.A. Demeshko, V.I. Kasilov, K.S. Kokhnyuk, S.S. Kochetov, I.V. Mel’nitsky, I.L. Semisalov, A.A. Khomich, O.A. Shopen // Вопросы атомной науки и техники. — 2009. — № 5. — С. 95-100. — Бібліогр.: 9 назв. — англ.
1562-6016
PACS: 28.20-v
https://nasplib.isofts.kiev.ua/handle/123456789/96514
On the basis of the notion about six groups of nuclei as delayed neutron precursors, radioactive decay laws and the pulsed mode of accelerator operation, a relationship has been derived to describe the decay curve of nuclei-delayed neutron precursors as a function of the pulse rate of the accelerator, the exposure time, the observation time, the time measurement interval and the number of measurement runs. A pilot experiment on thermal-neutron fission of 235U has been conducted. The aim of the experiment was to check the hardware and the information readout computer program. Based on the expressions derived, an analysis was performed and relative yields of delayed neutrons were determined. The present results are compared to the data obtained by other authors. For further development of the analysis, a question is brought up about the influence of additional conditions on the determination of relative delayedneutron yields. These additional conditions can be represented by certain expressions laid down when measuring delayed neutron yields directly between the accelerator pulses.
Виходячи з представлення про шiсть груп ядер-попередникiв запiзнiлих нейтронiв, законiв радiоактивного розпаду, i iмпульсного режиму роботи прискорювача, отримано спiввiдношення, що описує криву розпаду ядер-попередникiв запiзнiлих нейтронiв у залежностi вiд частоти посилок прискорювача, часу експозицiї, часу спостереження, кроку вимiру за часом i кiлькостi циклiв вимiрiв. Проведено пробний експеримент з подiлу 235U тепловими нейтронами. Мета експерименту - перевiрка апаратури i комп’ютерної програми з’йому iнформацiї. На базi отриманих виражень проведено аналiз i визначено вiдноснi виходи запiзнiлих нейтронiв. Результати порiвнюються з iншими роботами. Як перспектива подальшого розвитку аналiзу, ставиться питання про вплив додаткових умов на визначення вiдносних виходiв запiзнiлих нейтронiв. Такими додатковими умовами можуть бути деякi вирази, сформульованi при вимiрi виходiв запiзнiлих нейтронiв безпосередньо мiж посилками прискорювача
Исходя из представления о шести группах ядер-предшественников запаздывающих нейтронов, законов радиоактивного распада, и импульсного режима работы ускорителя, получено соотношение, описывающее кривую распада ядер предшественников запаздывающих нейтронов в зависимости от частоты посылок ускорителя, времени экспозиции, времени наблюдения, шага измерения по времени и количества циклов измерений. Проведен пробный эксперимент по делению 235U тепловыми нейтронами. Цель эксперимента - проверка аппаратуры и компьютерной программы съема информации. На базе полученных выражений проведен анализ и определены относительные выходы запаздывающих нейтронов. Результаты сравниваются с другими работами. Как перспектива дальнейшего развития анализа, ставится вопрос о влиянии дополнительных условий на определение относительных выходов запаздывающих нейтронов. Такими дополнительными условиями могут быть некоторые выражения, сформулированные при измерении выходов запаздывающих нейтронов непосредственно между посылками ускорителя.
en
Національний науковий центр «Харківський фізико-технічний інститут» НАН України
Вопросы атомной науки и техники
Ядернo-физические методы и обработка данных
The mathematical model for decay curve of the nuclei-delayed neutron precursors in experiment at a pulsed electron linear accelerator
Математична модель кривої розпаду ядер, попередникiв запiзнiлих нейтронiв, в експериментi на iмпульсному лiнiйному прискорювачi електронiв
Математическaя модель кривой распада ядер, предшественников запаздывающих нейтронов, в эксперименте на импульсном линейном ускорителе электронов
Article
published earlier
spellingShingle The mathematical model for decay curve of the nuclei-delayed neutron precursors in experiment at a pulsed electron linear accelerator
Buki, A.Yu.
Gokov, S.P.
Demeshko, O.A.
Kasilov, V.I.
Kokhnyuk, K.S.
Kochetov, S.S.
Mel’nitsky, I.V.
Semisalov, I.L.
Khomich, A.A.
Shopen, O.A.
Ядернo-физические методы и обработка данных
title The mathematical model for decay curve of the nuclei-delayed neutron precursors in experiment at a pulsed electron linear accelerator
title_alt Математична модель кривої розпаду ядер, попередникiв запiзнiлих нейтронiв, в експериментi на iмпульсному лiнiйному прискорювачi електронiв
Математическaя модель кривой распада ядер, предшественников запаздывающих нейтронов, в эксперименте на импульсном линейном ускорителе электронов
title_full The mathematical model for decay curve of the nuclei-delayed neutron precursors in experiment at a pulsed electron linear accelerator
title_fullStr The mathematical model for decay curve of the nuclei-delayed neutron precursors in experiment at a pulsed electron linear accelerator
title_full_unstemmed The mathematical model for decay curve of the nuclei-delayed neutron precursors in experiment at a pulsed electron linear accelerator
title_short The mathematical model for decay curve of the nuclei-delayed neutron precursors in experiment at a pulsed electron linear accelerator
title_sort mathematical model for decay curve of the nuclei-delayed neutron precursors in experiment at a pulsed electron linear accelerator
topic Ядернo-физические методы и обработка данных
topic_facet Ядернo-физические методы и обработка данных
url https://nasplib.isofts.kiev.ua/handle/123456789/96514
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