СТМ-дослідження впорядкування молекул діарилетенів на поверхні Аu(111)

The self-organisation of terphenylthiazole based diarylethene on Au(111) is studied using scanning tunnelling microscopy (STM). The observations of thickness variation of monolayer of molecules revealed process of molecular geometry changing on Au (111). The signs of molecular ordering on the basis...

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Bibliographische Detailangaben
Datum:2014
Hauptverfasser: Snegir, S. V., Kapitanchuk, A. L., Koshova, O. O., Marchenko, A. A.
Format: Artikel
Sprache:Ukrainisch
Veröffentlicht: Chuiko Institute of Surface Chemistry National Academy of Sciences of Ukraine 2014
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Online Zugang:https://www.cpts.com.ua/index.php/cpts/article/view/287
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Назва журналу:Chemistry, Physics and Technology of Surface

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Chemistry, Physics and Technology of Surface
Beschreibung
Zusammenfassung:The self-organisation of terphenylthiazole based diarylethene on Au(111) is studied using scanning tunnelling microscopy (STM). The observations of thickness variation of monolayer of molecules revealed process of molecular geometry changing on Au (111). The signs of molecular ordering on the basis of regularly repeated protrusions are detected. The unit cell of molecular packing is found to be equivalent for monolayers build by molecules in open- and closed-ring forms. For the purpose of interpretation of STM images, quantum chemical calculations of the spatial and electronic structures of the free molecule in neutral state are performed.