Селективна дегідратація етиллактату до етилакрилату на NaY-фожазиті

Dehydration of lactic acid and its esters is a promising way for obtaining acrylate monomers. The transformation of 10 % ethyl lactate solution in ethanol into ethyl acrylate over NaY, NaX, NaA and L zeolites has been studied. It has been shown that NaY-faujasite is the most stable catalyst, which p...

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Збережено в:
Бібліографічні деталі
Дата:2017
Автори: Varvarin, A. M., Mylin, A. M., Brei, V. V.
Формат: Стаття
Мова:Українська
Опубліковано: Chuiko Institute of Surface Chemistry National Academy of Sciences of Ukraine 2017
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Онлайн доступ:https://www.cpts.com.ua/index.php/cpts/article/view/424
Теги: Додати тег
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Назва журналу:Chemistry, Physics and Technology of Surface

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Chemistry, Physics and Technology of Surface
Опис
Резюме:Dehydration of lactic acid and its esters is a promising way for obtaining acrylate monomers. The transformation of 10 % ethyl lactate solution in ethanol into ethyl acrylate over NaY, NaX, NaA and L zeolites has been studied. It has been shown that NaY-faujasite is the most stable catalyst, which provides 100 % conversion of ethyl lactate with 80–90 % selectivity towards ethyl acrylate at 350 °С and 0.1 MPa under LHSV= 3.4 h–1 for 3 h. It has been found that use of СО2 as carrier-gas and carrying out the reaction in ethanol steam allows prolonging time of stable work of the catalyst. Possible schemes of ethyl lactate transformations are discussed.