ФЛЮОРЕСЦЕНТНІ ХАРАКТЕРИСТИКИ РОЗЧИНІВ РОДАМІНУ 6Ж ТА РОДАМІНУ С У ВОДНО-МІЦЕЛЯРНИХ СЕРЕДОВИЩАХ ПАР

The influence of cationic, anionic, nonionic surfactants and their mixtures on the fluorescence characteristics of rhodamine 6G and Rho-damine C solutions has been investigated. The fluorescence intensity of aqueous solutions of rhodamine 6G and in the presence of cetylpyr...

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Дата:2019
Автори: Zaporozhets, Olga, Kulichenko, Sergey, Lelyushok, Sergey, Klovak, Viktoriia
Формат: Стаття
Мова:English
Опубліковано: V.I.Vernadsky Institute of General and Inorganic Chemistry 2019
Онлайн доступ:https://ucj.org.ua/index.php/journal/article/view/106
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Назва журналу:Ukrainian Chemistry Journal

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Ukrainian Chemistry Journal
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spelling oai:ojs2.1444248.nisspano.web.hosting-test.net:article-1062019-12-24T08:25:03Z FLUORESCENCE CHARACTERISTICS OF RHODAMINE 6G AND RHODAMINE C IN WATER-MICELLAR SURFACTANT ENVIRONMENTS ФЛУОРЕСЦЕНТНЫЕ ХАРАКТЕРИСТИКИ РАСТВОРОВ РОДАМИНА 6Ж И РОДАМИНА С В ВОДНО-МИЦЕЛЛЯРНЫХ СРЕДАХ ПАВ ФЛЮОРЕСЦЕНТНІ ХАРАКТЕРИСТИКИ РОЗЧИНІВ РОДАМІНУ 6Ж ТА РОДАМІНУ С У ВОДНО-МІЦЕЛЯРНИХ СЕРЕДОВИЩАХ ПАР Zaporozhets, Olga Kulichenko, Sergey Lelyushok, Sergey Klovak, Viktoriia fluorescence, surfactants, rhodamine 6G, rhodamine C, sodium dodecyl sulfate, cetylpyridinium chloride, Triton X-100. The influence of cationic, anionic, nonionic surfactants and their mixtures on the fluorescence characteristics of rhodamine 6G and Rho-damine C solutions has been investigated. The fluorescence intensity of aqueous solutions of rhodamine 6G and in the presence of cetylpyridinium chloride and sodium dodecyl sulfate has almost unchanged throughout the pH range. The fluorescence intensity of aqueous and water-micellar rhodamine C solutions has been increased in the pH 1-4 range; the signal has been remained unchanged at high pH values. The studies have been carried out at pH 4 for rhodamine 6G and at pH 10 for rhodamine C. The fluorescence characteristics of water-micellar dye - surfactant - non-ionic surfactant systems have been performed at a concentration of Triton X-100 of 3.4·10‑2 mol/l. The interaction with cationic surfactants has shown differences character between the I=f(n) dependences for aqueous solutions of highly hydrophobic rhodamine 6G and more hydrophilic rhodamine C. The study of the effect of the hydrocarbon radical length on the intensity of the fluorescence of rhodamine 6G and rhodamine C has been carried out at two concentrations of cationic surfactants: under the condition of the formation of stoichiometric associates dye with cationic surfactant and in the region of the micellar concentrations of cationic surfactants. The character of the influence of the length of the hydrocarbon radical cationic surfactants on the fluorescence intensity of the dyes can be explained by the increasing role of hydrophobic interactions and the enhancement of solubilization in systems involving long-chain surfactants. The difference in the nature of the associates of rhodamine 6G and rhodamine C with hydrophobic and moderately hydrophobic cationic surfactants has been counterbalanced in the presence of Triton X-100. Reduction of fluorescence intensity of rhodamine 6G in domicile solutions of anionic sodium dodecyl sulfate has been established. The method of fluorescence detection of sodium dodecyl sulfate in reaction with rhodamine 6G has been proposed. The method has been tested in determining of anionic surfactants in the waters after washing clothes. V.I.Vernadsky Institute of General and Inorganic Chemistry 2019-12-16 Article Article Physical chemistry Физическая xимия Фізична xімія application/pdf https://ucj.org.ua/index.php/journal/article/view/106 10.33609/0041-6045.85.11.2019.84-95 Ukrainian Chemistry Journal; Vol. 85 No. 12 (2019): Ukrainian Chemistry Journal; 84-95 Украинский химический журнал; Том 85 № 12 (2019): Украинский химический журнал; 84-95 Український хімічний журнал; Том 85 № 12 (2019): Український хімічний журнал; 84-95 2708-129X 2708-1281 en https://ucj.org.ua/index.php/journal/article/view/106/70
institution Ukrainian Chemistry Journal
baseUrl_str
datestamp_date 2019-12-24T08:25:03Z
collection OJS
language English
topic_facet fluorescence
surfactants
rhodamine 6G
rhodamine C
sodium dodecyl sulfate
cetylpyridinium chloride
Triton X-100.
format Article
author Zaporozhets, Olga
Kulichenko, Sergey
Lelyushok, Sergey
Klovak, Viktoriia
spellingShingle Zaporozhets, Olga
Kulichenko, Sergey
Lelyushok, Sergey
Klovak, Viktoriia
ФЛЮОРЕСЦЕНТНІ ХАРАКТЕРИСТИКИ РОЗЧИНІВ РОДАМІНУ 6Ж ТА РОДАМІНУ С У ВОДНО-МІЦЕЛЯРНИХ СЕРЕДОВИЩАХ ПАР
author_facet Zaporozhets, Olga
Kulichenko, Sergey
Lelyushok, Sergey
Klovak, Viktoriia
author_sort Zaporozhets, Olga
title ФЛЮОРЕСЦЕНТНІ ХАРАКТЕРИСТИКИ РОЗЧИНІВ РОДАМІНУ 6Ж ТА РОДАМІНУ С У ВОДНО-МІЦЕЛЯРНИХ СЕРЕДОВИЩАХ ПАР
title_short ФЛЮОРЕСЦЕНТНІ ХАРАКТЕРИСТИКИ РОЗЧИНІВ РОДАМІНУ 6Ж ТА РОДАМІНУ С У ВОДНО-МІЦЕЛЯРНИХ СЕРЕДОВИЩАХ ПАР
title_full ФЛЮОРЕСЦЕНТНІ ХАРАКТЕРИСТИКИ РОЗЧИНІВ РОДАМІНУ 6Ж ТА РОДАМІНУ С У ВОДНО-МІЦЕЛЯРНИХ СЕРЕДОВИЩАХ ПАР
title_fullStr ФЛЮОРЕСЦЕНТНІ ХАРАКТЕРИСТИКИ РОЗЧИНІВ РОДАМІНУ 6Ж ТА РОДАМІНУ С У ВОДНО-МІЦЕЛЯРНИХ СЕРЕДОВИЩАХ ПАР
title_full_unstemmed ФЛЮОРЕСЦЕНТНІ ХАРАКТЕРИСТИКИ РОЗЧИНІВ РОДАМІНУ 6Ж ТА РОДАМІНУ С У ВОДНО-МІЦЕЛЯРНИХ СЕРЕДОВИЩАХ ПАР
title_sort флюоресцентні характеристики розчинів родаміну 6ж та родаміну с у водно-міцелярних середовищах пар
title_alt FLUORESCENCE CHARACTERISTICS OF RHODAMINE 6G AND RHODAMINE C IN WATER-MICELLAR SURFACTANT ENVIRONMENTS
ФЛУОРЕСЦЕНТНЫЕ ХАРАКТЕРИСТИКИ РАСТВОРОВ РОДАМИНА 6Ж И РОДАМИНА С В ВОДНО-МИЦЕЛЛЯРНЫХ СРЕДАХ ПАВ
description The influence of cationic, anionic, nonionic surfactants and their mixtures on the fluorescence characteristics of rhodamine 6G and Rho-damine C solutions has been investigated. The fluorescence intensity of aqueous solutions of rhodamine 6G and in the presence of cetylpyridinium chloride and sodium dodecyl sulfate has almost unchanged throughout the pH range. The fluorescence intensity of aqueous and water-micellar rhodamine C solutions has been increased in the pH 1-4 range; the signal has been remained unchanged at high pH values. The studies have been carried out at pH 4 for rhodamine 6G and at pH 10 for rhodamine C. The fluorescence characteristics of water-micellar dye - surfactant - non-ionic surfactant systems have been performed at a concentration of Triton X-100 of 3.4·10‑2 mol/l. The interaction with cationic surfactants has shown differences character between the I=f(n) dependences for aqueous solutions of highly hydrophobic rhodamine 6G and more hydrophilic rhodamine C. The study of the effect of the hydrocarbon radical length on the intensity of the fluorescence of rhodamine 6G and rhodamine C has been carried out at two concentrations of cationic surfactants: under the condition of the formation of stoichiometric associates dye with cationic surfactant and in the region of the micellar concentrations of cationic surfactants. The character of the influence of the length of the hydrocarbon radical cationic surfactants on the fluorescence intensity of the dyes can be explained by the increasing role of hydrophobic interactions and the enhancement of solubilization in systems involving long-chain surfactants. The difference in the nature of the associates of rhodamine 6G and rhodamine C with hydrophobic and moderately hydrophobic cationic surfactants has been counterbalanced in the presence of Triton X-100. Reduction of fluorescence intensity of rhodamine 6G in domicile solutions of anionic sodium dodecyl sulfate has been established. The method of fluorescence detection of sodium dodecyl sulfate in reaction with rhodamine 6G has been proposed. The method has been tested in determining of anionic surfactants in the waters after washing clothes.
publisher V.I.Vernadsky Institute of General and Inorganic Chemistry
publishDate 2019
url https://ucj.org.ua/index.php/journal/article/view/106
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