STRUCTURE AND SPECTRAL-LUMUINESCENT PROPERTIES OF LANTHANIDE-CONTAINING COMPLEXES WITH AZACROWN CALIXARENES

Lanthanide complexes with calix[4]arenes lower rim substituted with two azacrown ether fragments are reported. The size of the substituent cavity varied from 4 to 6 heteroatoms. The complexes were analyzed by means of IR, NMR, ESI mass spectroscopy. It is assumed that the coordination of Ln(III) ion...

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Дата:2021
Автори: Smola, Serhii, Rusakova, Natalia, Alekseeva, Olena, Basok, Stepan, Kirichenko, Tatiana, Korovin, Oleksandr, Malinka, Olena, Semenishyn, Nikolay
Формат: Стаття
Мова:Англійська
Опубліковано: V.I.Vernadsky Institute of General and Inorganic Chemistry 2021
Онлайн доступ:https://ucj.org.ua/index.php/journal/article/view/372
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Назва журналу:Ukrainian Chemistry Journal

Репозитарії

Ukrainian Chemistry Journal
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author Smola, Serhii
Rusakova, Natalia
Alekseeva, Olena
Basok, Stepan
Kirichenko, Tatiana
Korovin, Oleksandr
Malinka, Olena
Semenishyn, Nikolay
author_facet Smola, Serhii
Rusakova, Natalia
Alekseeva, Olena
Basok, Stepan
Kirichenko, Tatiana
Korovin, Oleksandr
Malinka, Olena
Semenishyn, Nikolay
author_sort Smola, Serhii
baseUrl_str
collection OJS
datestamp_date 2021-12-16T12:12:21Z
description Lanthanide complexes with calix[4]arenes lower rim substituted with two azacrown ether fragments are reported. The size of the substituent cavity varied from 4 to 6 heteroatoms. The complexes were analyzed by means of IR, NMR, ESI mass spectroscopy. It is assumed that the coordination of Ln(III) ions occurs through the donor atoms of the lower rim; the counter anion and solvent molecule are also coordinated. Lanthanide-centered characteristic luminescence was observed in Eu(III), Tb(III) and Yb(III) complexes. The most efficient 4f-luminescence is observed for terbium-containing complexes with benzo-crown-derived ligands. The pathways of the sensitization of 4f-luminescence are discussed.
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spelling oai:ojs2.1444248.nisspano.web.hosting-test.net:article-3722021-12-16T12:12:21Z STRUCTURE AND SPECTRAL-LUMUINESCENT PROPERTIES OF LANTHANIDE-CONTAINING COMPLEXES WITH AZACROWN CALIXARENES Smola, Serhii Rusakova, Natalia Alekseeva, Olena Basok, Stepan Kirichenko, Tatiana Korovin, Oleksandr Malinka, Olena Semenishyn, Nikolay lanthanide complexes, calix[4]arenes, azacrown ethers, luminescence. Lanthanide complexes with calix[4]arenes lower rim substituted with two azacrown ether fragments are reported. The size of the substituent cavity varied from 4 to 6 heteroatoms. The complexes were analyzed by means of IR, NMR, ESI mass spectroscopy. It is assumed that the coordination of Ln(III) ions occurs through the donor atoms of the lower rim; the counter anion and solvent molecule are also coordinated. Lanthanide-centered characteristic luminescence was observed in Eu(III), Tb(III) and Yb(III) complexes. The most efficient 4f-luminescence is observed for terbium-containing complexes with benzo-crown-derived ligands. The pathways of the sensitization of 4f-luminescence are discussed. V.I.Vernadsky Institute of General and Inorganic Chemistry 2021-11-26 Article Article Inorganic Chemistry Неорганическая химия Неорганічна хімія application/pdf https://ucj.org.ua/index.php/journal/article/view/372 10.33609/2708-129X.87.10.2021.103-115 Ukrainian Chemistry Journal; Vol. 87 No. 10 (2021): Ukrainian Chemistry Journal; 103-115 Украинский химический журнал; Том 87 № 10 (2021): Ukrainian Chemistry Journal; 103-115 Український хімічний журнал; Том 87 № 10 (2021): Український хімічний журнал; 103-115 2708-129X 2708-1281 en https://ucj.org.ua/index.php/journal/article/view/372/193
spellingShingle Smola, Serhii
Rusakova, Natalia
Alekseeva, Olena
Basok, Stepan
Kirichenko, Tatiana
Korovin, Oleksandr
Malinka, Olena
Semenishyn, Nikolay
STRUCTURE AND SPECTRAL-LUMUINESCENT PROPERTIES OF LANTHANIDE-CONTAINING COMPLEXES WITH AZACROWN CALIXARENES
title STRUCTURE AND SPECTRAL-LUMUINESCENT PROPERTIES OF LANTHANIDE-CONTAINING COMPLEXES WITH AZACROWN CALIXARENES
title_full STRUCTURE AND SPECTRAL-LUMUINESCENT PROPERTIES OF LANTHANIDE-CONTAINING COMPLEXES WITH AZACROWN CALIXARENES
title_fullStr STRUCTURE AND SPECTRAL-LUMUINESCENT PROPERTIES OF LANTHANIDE-CONTAINING COMPLEXES WITH AZACROWN CALIXARENES
title_full_unstemmed STRUCTURE AND SPECTRAL-LUMUINESCENT PROPERTIES OF LANTHANIDE-CONTAINING COMPLEXES WITH AZACROWN CALIXARENES
title_short STRUCTURE AND SPECTRAL-LUMUINESCENT PROPERTIES OF LANTHANIDE-CONTAINING COMPLEXES WITH AZACROWN CALIXARENES
title_sort structure and spectral-lumuinescent properties of lanthanide-containing complexes with azacrown calixarenes
topic_facet lanthanide complexes
calix[4]arenes
azacrown ethers
luminescence.
url https://ucj.org.ua/index.php/journal/article/view/372
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