STRUCTURE AND SPECTRAL-LUMUINESCENT PROPERTIES OF LANTHANIDE-CONTAINING COMPLEXES WITH AZACROWN CALIXARENES

Lanthanide complexes with calix[4]arenes lower rim substituted with two azacrown ether fragments are reported. The size of the substituent cavity varied from 4 to 6 heteroatoms. The complexes were analyzed by means of IR, NMR, ESI mass spectroscopy. It is assumed that the coordination of Ln(III) ion...

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Бібліографічні деталі
Дата:2021
Автори: Smola, Serhii, Rusakova, Natalia, Alekseeva, Olena, Basok, Stepan, Kirichenko, Tatiana, Korovin, Oleksandr, Malinka, Olena, Semenishyn, Nikolay
Формат: Стаття
Мова:English
Опубліковано: V.I.Vernadsky Institute of General and Inorganic Chemistry 2021
Онлайн доступ:https://ucj.org.ua/index.php/journal/article/view/372
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Назва журналу:Ukrainian Chemistry Journal

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Ukrainian Chemistry Journal
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spelling oai:ojs2.1444248.nisspano.web.hosting-test.net:article-3722021-12-16T12:12:21Z STRUCTURE AND SPECTRAL-LUMUINESCENT PROPERTIES OF LANTHANIDE-CONTAINING COMPLEXES WITH AZACROWN CALIXARENES Smola, Serhii Rusakova, Natalia Alekseeva, Olena Basok, Stepan Kirichenko, Tatiana Korovin, Oleksandr Malinka, Olena Semenishyn, Nikolay lanthanide complexes, calix[4]arenes, azacrown ethers, luminescence. Lanthanide complexes with calix[4]arenes lower rim substituted with two azacrown ether fragments are reported. The size of the substituent cavity varied from 4 to 6 heteroatoms. The complexes were analyzed by means of IR, NMR, ESI mass spectroscopy. It is assumed that the coordination of Ln(III) ions occurs through the donor atoms of the lower rim; the counter anion and solvent molecule are also coordinated. Lanthanide-centered characteristic luminescence was observed in Eu(III), Tb(III) and Yb(III) complexes. The most efficient 4f-luminescence is observed for terbium-containing complexes with benzo-crown-derived ligands. The pathways of the sensitization of 4f-luminescence are discussed. V.I.Vernadsky Institute of General and Inorganic Chemistry 2021-11-26 Article Article Inorganic Chemistry Неорганическая химия Неорганічна хімія application/pdf https://ucj.org.ua/index.php/journal/article/view/372 10.33609/2708-129X.87.10.2021.103-115 Ukrainian Chemistry Journal; Vol. 87 No. 10 (2021): Ukrainian Chemistry Journal; 103-115 Украинский химический журнал; Том 87 № 10 (2021): Ukrainian Chemistry Journal; 103-115 Український хімічний журнал; Том 87 № 10 (2021): Український хімічний журнал; 103-115 2708-129X 2708-1281 en https://ucj.org.ua/index.php/journal/article/view/372/193
institution Ukrainian Chemistry Journal
baseUrl_str
datestamp_date 2021-12-16T12:12:21Z
collection OJS
language English
topic_facet lanthanide complexes
calix[4]arenes
azacrown ethers
luminescence.
format Article
author Smola, Serhii
Rusakova, Natalia
Alekseeva, Olena
Basok, Stepan
Kirichenko, Tatiana
Korovin, Oleksandr
Malinka, Olena
Semenishyn, Nikolay
spellingShingle Smola, Serhii
Rusakova, Natalia
Alekseeva, Olena
Basok, Stepan
Kirichenko, Tatiana
Korovin, Oleksandr
Malinka, Olena
Semenishyn, Nikolay
STRUCTURE AND SPECTRAL-LUMUINESCENT PROPERTIES OF LANTHANIDE-CONTAINING COMPLEXES WITH AZACROWN CALIXARENES
author_facet Smola, Serhii
Rusakova, Natalia
Alekseeva, Olena
Basok, Stepan
Kirichenko, Tatiana
Korovin, Oleksandr
Malinka, Olena
Semenishyn, Nikolay
author_sort Smola, Serhii
title STRUCTURE AND SPECTRAL-LUMUINESCENT PROPERTIES OF LANTHANIDE-CONTAINING COMPLEXES WITH AZACROWN CALIXARENES
title_short STRUCTURE AND SPECTRAL-LUMUINESCENT PROPERTIES OF LANTHANIDE-CONTAINING COMPLEXES WITH AZACROWN CALIXARENES
title_full STRUCTURE AND SPECTRAL-LUMUINESCENT PROPERTIES OF LANTHANIDE-CONTAINING COMPLEXES WITH AZACROWN CALIXARENES
title_fullStr STRUCTURE AND SPECTRAL-LUMUINESCENT PROPERTIES OF LANTHANIDE-CONTAINING COMPLEXES WITH AZACROWN CALIXARENES
title_full_unstemmed STRUCTURE AND SPECTRAL-LUMUINESCENT PROPERTIES OF LANTHANIDE-CONTAINING COMPLEXES WITH AZACROWN CALIXARENES
title_sort structure and spectral-lumuinescent properties of lanthanide-containing complexes with azacrown calixarenes
description Lanthanide complexes with calix[4]arenes lower rim substituted with two azacrown ether fragments are reported. The size of the substituent cavity varied from 4 to 6 heteroatoms. The complexes were analyzed by means of IR, NMR, ESI mass spectroscopy. It is assumed that the coordination of Ln(III) ions occurs through the donor atoms of the lower rim; the counter anion and solvent molecule are also coordinated. Lanthanide-centered characteristic luminescence was observed in Eu(III), Tb(III) and Yb(III) complexes. The most efficient 4f-luminescence is observed for terbium-containing complexes with benzo-crown-derived ligands. The pathways of the sensitization of 4f-luminescence are discussed.
publisher V.I.Vernadsky Institute of General and Inorganic Chemistry
publishDate 2021
url https://ucj.org.ua/index.php/journal/article/view/372
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