DETERMINATION OF POLYLIGAND COMPLEXES OF COBALT (II) WITH CITRATE AND PYROPHOSPHATE IONS

In the work it is shown by the spectrophotometry method that depending on the concentration ratio of ligands [PPi4–]/[Cit3–] in the pyrophosphate-citrate electrolyte, cobalt (II) ions form not only citrate [Co(Cit)2]4– and pyrophosphate [Co(PPi)2]6–, but also polyligand complexes [Co(PPi)m(Cit)n]+2–...

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Дата:2022
Автори: Nikitenko, Vasyl, Kublanovsky, Valeriy, Yapontseva, Yuliya
Формат: Стаття
Мова:English
Опубліковано: V.I.Vernadsky Institute of General and Inorganic Chemistry 2022
Онлайн доступ:https://ucj.org.ua/index.php/journal/article/view/436
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Назва журналу:Ukrainian Chemistry Journal

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Ukrainian Chemistry Journal
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spelling oai:ojs2.1444248.nisspano.web.hosting-test.net:article-4362022-07-06T15:57:59Z DETERMINATION OF POLYLIGAND COMPLEXES OF COBALT (II) WITH CITRATE AND PYROPHOSPHATE IONS Nikitenko, Vasyl Kublanovsky, Valeriy Yapontseva, Yuliya cobalt (II), polyligand complex, composition, stability constant, spectro­photometry. In the work it is shown by the spectrophotometry method that depending on the concentration ratio of ligands [PPi4–]/[Cit3–] in the pyrophosphate-citrate electrolyte, cobalt (II) ions form not only citrate [Co(Cit)2]4– and pyrophosphate [Co(PPi)2]6–, but also polyligand complexes [Co(PPi)m(Cit)n]+2–(4m+3n). The composition of polyligand complexes [Co(PPi)Cit]5– was determined, and the equilibrium constant of the reaction of their formation and the constant of their stability were calculated (pβ=8.47). The dependence of the degree of formation of citrate, polyligand, and pyrophosphate complexes of cobalt (II) in the pyrophosphate-citrate electrolyte on the logarithm of the ratio of equilibrium concentrations of ligands is calculated. V.I.Vernadsky Institute of General and Inorganic Chemistry 2022-05-25 Article Article Physical chemistry Физическая xимия Фізична xімія application/pdf https://ucj.org.ua/index.php/journal/article/view/436 10.33609/2708-129X.88.04.2022.113-122 Ukrainian Chemistry Journal; Vol. 88 No. 4 (2022): Ukrainian Chemistry Journal; 113-122 Украинский химический журнал; Том 88 № 4 (2022): Ukrainian Chemistry Journal; 113-122 Український хімічний журнал; Том 88 № 4 (2022): Український хімічний журнал; 113-122 2708-129X 2708-1281 en https://ucj.org.ua/index.php/journal/article/view/436/224
institution Ukrainian Chemistry Journal
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datestamp_date 2022-07-06T15:57:59Z
collection OJS
language English
topic_facet cobalt (II)
polyligand complex
composition
stability constant
spectro­photometry.
format Article
author Nikitenko, Vasyl
Kublanovsky, Valeriy
Yapontseva, Yuliya
spellingShingle Nikitenko, Vasyl
Kublanovsky, Valeriy
Yapontseva, Yuliya
DETERMINATION OF POLYLIGAND COMPLEXES OF COBALT (II) WITH CITRATE AND PYROPHOSPHATE IONS
author_facet Nikitenko, Vasyl
Kublanovsky, Valeriy
Yapontseva, Yuliya
author_sort Nikitenko, Vasyl
title DETERMINATION OF POLYLIGAND COMPLEXES OF COBALT (II) WITH CITRATE AND PYROPHOSPHATE IONS
title_short DETERMINATION OF POLYLIGAND COMPLEXES OF COBALT (II) WITH CITRATE AND PYROPHOSPHATE IONS
title_full DETERMINATION OF POLYLIGAND COMPLEXES OF COBALT (II) WITH CITRATE AND PYROPHOSPHATE IONS
title_fullStr DETERMINATION OF POLYLIGAND COMPLEXES OF COBALT (II) WITH CITRATE AND PYROPHOSPHATE IONS
title_full_unstemmed DETERMINATION OF POLYLIGAND COMPLEXES OF COBALT (II) WITH CITRATE AND PYROPHOSPHATE IONS
title_sort determination of polyligand complexes of cobalt (ii) with citrate and pyrophosphate ions
description In the work it is shown by the spectrophotometry method that depending on the concentration ratio of ligands [PPi4–]/[Cit3–] in the pyrophosphate-citrate electrolyte, cobalt (II) ions form not only citrate [Co(Cit)2]4– and pyrophosphate [Co(PPi)2]6–, but also polyligand complexes [Co(PPi)m(Cit)n]+2–(4m+3n). The composition of polyligand complexes [Co(PPi)Cit]5– was determined, and the equilibrium constant of the reaction of their formation and the constant of their stability were calculated (pβ=8.47). The dependence of the degree of formation of citrate, polyligand, and pyrophosphate complexes of cobalt (II) in the pyrophosphate-citrate electrolyte on the logarithm of the ratio of equilibrium concentrations of ligands is calculated.
publisher V.I.Vernadsky Institute of General and Inorganic Chemistry
publishDate 2022
url https://ucj.org.ua/index.php/journal/article/view/436
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