Дослідження ріст-стимулюючого впливу 1-(2-(додецилокси)-2-оксоетил)піридин-1-ій хлориду на проростки насіння пшениці

Ester-functionalized long-chain pyridinium salt 1-(2-(dodecyloxy)-2-oxoethyl)pyridin-1-ium chloride (1b) has been synthesized. The influence of the substance on morpho-physiological traits of wheat seedlings (germination, shoot and root length and biomass, chlorophylls and carotenoids content, as we...

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Дата:2023
Автори та афіліації:
  • Sergiy P. Rogalsky — V.P. Kukhar Institute of Bioorganic Chemistry and Petrochemistry of the NAS of Ukraine, Kyiv, Ukraine
  • Oksana P. Tarasyuk — V.P. Kukhar Institute of Bioorganic Chemistry and Petrochemistry of the NAS of Ukraine, Kyiv, Ukraine
  • Olga V. Bulko — Institute of Cell Biology and Genetic Engineering of the NAS of Ukraine, Kyiv, Ukraine
  • Lyudmila G. Lioshyna — Institute of Cell Biology and Genetic Engineering of the NAS of Ukraine, Kyiv, Ukraine
Ключові слова:keywords
Автори: Rogalsky, Sergiy P., Tarasyuk, Oksana P., Bulko, Olga V., Lioshyna, Lyudmila G.
Формат: Стаття
Мова:Англійська
Опубліковано: V.P. Kukhar Institute of Bioorganic Chemistry and Petrochemistry of the National Academy of Sciences of Ukraine 2023
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Онлайн доступ:https://bioorganica.com.ua/index.php/journal/article/view/76
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Назва журналу:Ukrainica Bioorganica Acta
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Ukrainica Bioorganica Acta
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author Rogalsky, Sergiy P.
Tarasyuk, Oksana P.
Bulko, Olga V.
Lioshyna, Lyudmila G.
author_facet Rogalsky, Sergiy P.
Tarasyuk, Oksana P.
Bulko, Olga V.
Lioshyna, Lyudmila G.
author_institution_txt_mv [ { "author": "Sergiy P. Rogalsky", "institution": "V.P. Kukhar Institute of Bioorganic Chemistry and Petrochemistry of the NAS of Ukraine, Kyiv, Ukraine" }, { "author": "Oksana P. Tarasyuk", "institution": "V.P. Kukhar Institute of Bioorganic Chemistry and Petrochemistry of the NAS of Ukraine, Kyiv, Ukraine" }, { "author": "Olga V. Bulko", "institution": "Institute of Cell Biology and Genetic Engineering of the NAS of Ukraine, Kyiv, Ukraine" }, { "author": "Lyudmila G. Lioshyna", "institution": "Institute of Cell Biology and Genetic Engineering of the NAS of Ukraine, Kyiv, Ukraine" } ]
author_sort Rogalsky, Sergiy P.
baseUrl_str https://bioorganica.com.ua/index.php/journal/oai
collection OJS
datestamp_date 2026-07-19T14:56:54Z
description Ester-functionalized long-chain pyridinium salt 1-(2-(dodecyloxy)-2-oxoethyl)pyridin-1-ium chloride (1b) has been synthesized. The influence of the substance on morpho-physiological traits of wheat seedlings (germination, shoot and root length and biomass, chlorophylls and carotenoids content, as well as flavonoid content) has been studied. The germination of seeds increased after their exposure to water solutions of pyridinium chloride 1b in the concentration range 0.001-0.1%. However, the concentration 0.1% has a negative effect on plant growth leading to reduced growth parameters in shoots and roots, plant mass, as well as pigments content. The exposure of wheat seeds to water solutions of pyridinium salt with lower concentrations (especially at 0.001%) significantly increased shoot and root length, as well as wet green mass in 7-day-old seedlings. At a concentration of 0.01%, the substance caused a significant increase of chlorophyll a, chlorophyll b, and carotenoids content thus revealing a positive effect on the photosynthetic apparatus of plant leaves. The flavonoid content in a green part of the plants also significantly increased which may indicate activating the plant defense system under mild stress conditions. The high growth-promoting effect of long-chain pyridinium chloride 1b on wheat plants, together with its broad range of antimicrobial activity and biodegradability, makes it an attractive product for various agrochemical applications
doi_str_mv 10.15407/bioorganica2023.02.041
first_indexed 2025-07-17T12:19:57Z
format Article
fulltext ISSN 1814-9758. Ukr. Bioorg. Acta, 2023, Vol. 18, N 2 UDC 547.821.3 + 57.017.64 + 58.04 DOI: https://doi.org/10.15407/bioorganica2023.02.041 41 SHORT COMMUNICATION Evaluation of growth-promoting effect of 1-(2-(dodecyloxy)-2-oxoethyl)pyridin-1-ium chloride on wheat seedlings Sergiy P. Rogalsky1*, Oksana P. Tarasyuk1, Olga V. Bulko2, Lyudmila G. Lioshyna2 1 V.P. Kukhar Institute of Bioorganic Chemistry and Petrochemistry of the NAS of Ukraine, Kyiv, Ukraine 2 Institute of Cell Biology and Genetic Engineering of the NAS of Ukraine, Kyiv, Ukraine Abstract: Ester-functionalized long-chain pyridinium salt 1-(2-(dodecyloxy)-2-oxoethyl)pyridin-1-ium chloride (1b) has been synthesized. The influence of the substance on morpho-physiological traits of wheat seedlings (germination, shoot and root length and biomass, chlorophylls and carotenoids content, as well as flavonoid content) has been studied. The germination of seeds increased after their exposure to water solutions of pyridinium chloride 1b in the concentration range 0.001-0.1%. However, the concentration 0.1% has a negative effect on plant growth leading to reduced growth parameters in shoots and roots, plant mass, as well as pigments content. The exposure of wheat seeds to water solutions of pyridinium salt with lower concentrations (especially at 0.001%) significantly increased shoot and root length, as well as wet green mass in 7-day-old seedlings. At a concentration of 0.01%, the substance caused a significant increase of chlorophyll a, chlorophyll b, and carotenoids content thus revealing a positive effect on the photosynthetic apparatus of plant leaves. The flavonoid content in a green part of the plants also significantly increased which may indicate activating the plant defense system under mild stress conditions. The high growth-promoting effect of long-chain pyridinium chloride 1b on wheat plants, together with its broad range of antimicrobial activity and biodegradability, makes it an attractive product for various agrochemical applications. Keywords: long-chain pyridinium salt; wheat seeds; growth-promoting effect; plant protection. Introduction Onium salts are a special type of water soluble plant growth regulators (PGRs) which are widely used in agronomic crops. Thus, 2-chloroethyltrimethyl- ammonium chloride (chlormequat chloride) and 1,1-dimethylpiperidinium chloride (mepiquat chloride) are known to reduce stem elongation in crops due to a reduction in the synthesis of gibberellic acid [1]. The use of these PGRs significantly mproves crop production even under environmental stresses. Nowadays, the onium salts, also called “ionic liquids” (ILs) are considered promising biologically active compounds for the development of new Received: Revised: Accepted: Published online: 03.10.2023 29.10.2023 26.11.2023 30.12.2023  Corresponding author. Tel.: +380-98-451-7569; e-mail: sergey.rogalsky@gmail.com (S.P. Rogalsky) ORCID: 0000-0002-5200-5247 phytopharmaceuticals. The “tunability” of ILs in the design of physicochemical properties and biological activity by modification of cation or anion structure creates enormous potential for their industrial use [2]. Thus, commercially available phenoxy herbicides having an acidic nature have been incorporated into ILs structure to develop a new group of compounds defined as herbicidal ILs [2, 3]. The combination of the herbicidal activity of the anion with different biological activity of the cation leads to dual- functions compounds with improved physicochemical properties, as well as antifungal activity against plant pathogens [3, 4]. At the same time, there is little data in the literature regarding the plant growth-promoting activity of common ILs comprising halogen anions. The biological activity of these compounds is greatly affected by the length of the aliphatic chain near the cation. From this point of view, long-chain ILs comprising heterocyclic cations seem especially attractive for plant protection since they combine good water solubility, high surface activity, and a broad range of antimicrobial activity [5]. However, the high ecotoxicity, as well as poor © Rogalsky S.P. et al. This is an open-access article distributed under the terms of the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are credited. Ukrainica Bioorganica Acta www.bi oorgan ica .org .ua https://www.scopus.com/affil/profile.uri?afid=60104367 https://orcid.org/0000-0002-5200-5247 ISSN 1814-9758. Ukr. Bioorg. Acta, 2023, Vol. 18, N 2 42 biodegradability of common ILs is a serious drawback limiting their practical applications [6, 7]. The introduction of polar functional groups such as hydroxyl, carboxyl, or ester into the hydrocarbon chains of ILs is an efficient approach to reducing their toxicity [6, 8]. In this work, long-chain pyridinium salt, 1-(2- (dodecyloxy)-2-oxoethyl)pyridin-1-ium chloride (1b) was synthesized (see Scheme 1), and evaluated for growth- promoting activity toward wheat seeds. Recent studies have shown that this ester-functionalized pyridinium salt has significantly reduced acute toxicity, as well as improved biodegradability compared to non-functionalized analogs [8]. At the same time, pyridinium chloride 1b was found to have moderate antibacterial activity and high antifungal activity that makes it a promising plant protection product. C12H25OH C6H6 K2CO3 N N Cl - 100 oC 1a 1b Cl Cl O Cl OC12H25 O Cl OC12H25 O O OC12H25 Scheme 1. Synthesis of 1-(2-(dodecyloxy)-2-oxoethyl)pyridin-1- ium chloride (1b). Results and Discussion The growth parameters of wheat seedlings after their treatment with water solutions of 1-(2-(dodecyloxy)-2- oxoethyl)pyridin-1-ium chloride (1b) are summarized in Table 1. Pyridinium salt increased germination in the concentration range of 0.001-0.1%. However, at the highest examined concentration of 0.1% significant reduction in shoot and root length was observed. It is worth noting that a similar adverse effect on wheat seedlings growth has been reported for short-chain imidazolium salts [9]. At lower concentrations, pyridinium chloride 1b has a positive effect on wheat growth parameters (Figure 1, Table 1). Thus, the maximum increase of shoot length (by 15%) and root length (by 7%) was determined for a substance concentration of 0.001%. Moreover, shoot and root dry mass increased by 18.3 and 24.6 %, respectively (Table 2). The hydration of seedlings changed slightly, which indicates the absence of any significant impact of the selected concentrations on this physiological indicator. The results of the analysis of pigments content in wheat seedlings are shown in Table 3. The treatment of wheat seeds with 1-(2-(dodecyloxy)-2-oxoethyl)pyridin-1-ium chloride (1b) in a concentration of 0.01% increased the content of chlorophylls and carotenoids by 25% (Ca), 20% (Cb) and 43% (Ccar). This indicates positive effect of pyridinium salt on photosynthetic system of plants. At the highest examined concentration of the compound (0.1%) a significant decrease in pigment content was determined (Table 3). The ratio of chlorophylls to carotenoids increased by 100% for plants treated with pyridinium chloride 1b at a concentration of 0.1%. For lower concentrations of 0.01 and 0.001%, the (Ca+Cb)/Ccar value was similar to control samples that indicates the absence of physiological stress in plants. Figure 1. 7-Days-old wheat seedlings after exposure to deionized water (1, control) and water solutions of 1-(2-(dodecyloxy)-2- oxoethyl)pyridin-1-ium chloride (1b) with concentrations of 0.01% (2) and 0.001% (3). Table 1. Growth parameters of wheat seedlings after treat- ment with water solutions of 1-(2-(dodecyloxy)-2-oxo- ethyl)pyridin-1-ium chloride (1b). Conc., % Germi- nation, % to control Shoot length, % to control Root length, % to control Root number, % to control 0.1 104±7.8 71.1±11.2 59.6±12.9 76.78±9.5 0.01 119.8±10.1 105.5±9.9 80.9±11.2 115.8±11.3 0.001 108.6±9.9 115.3±10.6 107.57±9.5 106.2±10.8 As one can see from Table 3, the main flavonoid content was in green part of plants. Antioxidant flavonoids are known to effectively control key stages of cell growth and differentiation, regulating the development of the entire plant and individual organs [10]. The content of flavonoids in shoots grown after treatment with pyridinium salt at a concentration of 0.1% was comparable to control samples. For wheat seedlings treated with lower concentrations of 0.01 and 0.001% the Cfl value increased by 60 and 40%, respectively. The last fact may indicate activating the plant defense system under mild stress conditions [10]. Overall, the obtained results clearly indicate that pyridinium salt 1b has pronounced growth-promoting effect on wheat seeds in the concentration range 0.001-0.01%. Similar results on the effect of the polymeric biocide polyhexamethylene guanidine hydrochloride on the morpho-physiological parameters of wheat seedlings have also been reported [11, 12]. At the same time, imidazolium-based ILs with alkyl chain length from 2 to 8 carbon atoms were found to reduce the germination and growth of wheat seeds even at low concentrations [9, 13]. Based on these results one can assume that both the nature of the cation and the structure of the alkyl chain are important factors determining the biological activity of onium salts toward plants. Thus, further studies of the effect of ester-functionalized pyridinium salts with different alkyl substituents on the morpho-physiological parameters of wheat seedlings are underway. S.P. Rogalsky, O.P. Tarasyuk et al. 43 Table 2. The effect of 1-(2-(dodecyloxy)-2-oxoethyl)pyridin-1-ium chloride (1b) on the mass and water content in the cells of wheat seedlings. Concentration, % Shoot Roots M wet, % to control М dry, % to control Hydration, % M wet, % to control М dry, % to control Hydration, % 0.1 94.6± 5.7 82.5±4.6 97.1±9.7 84.6± 10.7 71.5±14.4 89.1±13.6 0.01 113.1±8.5 109±7.1 96.9±12.4 101.7±9.6 102.6±7.1 96.9±11.2 0.001 129.3±9.9 118.3±7.9 101.8±14.4 116.1±8.7 124.6±7.9 100.5±14.7 Table 3. The effect of 1-(2-(dodecyloxy)-2-oxoethyl)pyridin-1-ium chloride (1b) on the pigments and flavonoids content in wheat seedlings. Concentration, % Ca, mg/g Cb, mg/g Са/Сb Сcar, mg/g (Сa+Cb) /Ccar Cfl, mg/g (green part) Cfl, mg/g (roots) 0 (control) 7.12±1.71 2.94±0.54 2.43±0.07 38.74±8.11 0.26±0.09 2.34±0.8 0.11±0.08 0.1 4.97±0.93 2.64±0.63 2.58±0.11 18.48±3.14 0.412±0.1 2.14±0.72 0.1±0.04 0.01 9.47±1.22 3.67±0.79 2.58±0.09 68.32±6.76 0.192±0.07 3.91±0.34 0.21±0.09 0.001 7.86±1.45 3.74±0.23 2.58±0.1 48.73±5.92 0.238±0.03 3.26±0.83 0.19±0.06 Conclusions In this work, a long-chain pyridinium salt 1b comprising polar ester group in the alkyl chain has been synthesized. The influence of the synthesized cationic surfactant on the morpho-physiological parameters of wheat seedlings has been studied. At a concentration of 0.1% the substance has inhibitory effect on plant growth. However, treating seeds with lower concentrations of pyridinium salt 1b (especially 0.001%) significantly increased growth parameters. In particular, the growth-promoting effect of 1b was manifest- ted in an increased seed germination, shoot and root length, as well as dry mass in 7-day-old seedlings. Moreover, the substance has a positive effect on the photosynthetic characteristics of plant leaves, increasing the synthesis of chlorophylls and carotenoids. At the same time, the ratio between chlorophylls and carotenoids remained close to control values, which indicates stability of the primary photochemical processes of photosystem II. Overall, the results of this research revealed pronounced positive effect of ester-functionalized cationic surfactant 1b on wheat seeds growth. The combination of antifungal activity of this compound with high biodegradability and growth-promoting activity toward plants makes it very promising for various agrochemical applications. Thus, further study of the biological activity of pyridinium salts with different structures of the alkyl radical is of significant interest. Experimental section General Following chemicals were used for the synthesis: pyridine (99%), chloroacetyl chloride (98%), 1-dodecanol (99%), benzene (99.8%), ethyl acetate (98%), potassium carbonate (99%). All chemicals were purchased from Sigma-Aldrich and used without further purification. Proton nuclear magnetic resonance (1H NMR) spectroscopy was used to confirm the structure of the synthesized compounds. Spectra were recorded in CDCl3 on a Varian Gemini-2000 (400 MHz) NMR spectrometer using tetramethyl silane as internal standard. Synthesis of dodecyl chloroacetate (1a) To the stirred mixture of 1-dodecanol (18.6 g, 0.1 mol) and potassium carbonate (13.8 g, 0.1 mol) in 100 ml of benzene was added chloroacetyl chloride (13.5 g, 0.12 mol) dropwise. The reaction was carried out for 6 h at room temperature. Then the solution was washed successively with water until a neutral pH was achieved. Then it was dried over calcium chloride overnight. The solvent was removed via distillation at normal pressure. The obtained oily product was additionally dried in vacuum 10 mbar at 60 ºC. 1H NMR (400 MHz, CDCl3) δ 4.18 (t, J = 6.8 Hz, 2H, COOCH2), 4.06 (s, 2H, CH2CO), 1.66 (m, 2H, ОCH2CH2), 1.27 (m, 18H, СH3(CH2)9), 0.89 (t, J = 6.7 Hz, 3H, CH3). Synthesis of 1-(2-(dodecyloxy)-2-oxoethyl)pyridin-1-ium chloride (1b) The mixture of 5 g (0.06 mol) of pyridine and 18.4 g (0.07 mol) of dodecyl chloroacetate was stirred at 100 ºC for 6 h. After cooling to room temperature the amorphous solid product was obtained. It was purified by recrystallization from ethyl acetate. Yield: 15.1 g (74%), white solid, mp 71-73 ºC. 1H NMR (400 MHz, CDCl3) δ 9.32 (d, J = 7.3 Hz, 2H, C2-H, C6-H), 8.50 (d, J = 7.8 Hz, 1H, C4-H), 8.06 (t, J = 6.9 Hz, 2H, C3-H, C5-H), 6.18 (s, 2H, NCH2), 4.19 (t, J = 7.0 Hz, 2H, ОCH2), 1.64 (p, J = 7.0 ISSN 1814-9758. Ukr. Bioorg. Acta, 2023, Vol. 18, N 2 44 Hz, 2H, ОCH2CH2), 1.26 (m, 18H, СH3(CH2)9), 0.85 (t, J = 6.7 Hz, 3H, CH3). Biological activity Seeds of wheat (Triticum aestivum L., cultivar “Podolyanka”, Ukraine) were germinated by hydroponic method in glass Petri dishes (Ø10 см) in deionized water (control) or in water solutions of of 1-(2-(dodecyloxy)-2- oxoethyl)pyridin-1-ium chloride (1b) with concentrations of 0.001 and 0.01%. In each Petri dish 20 seeds were sown, in two replications. The experiment was repeated three times. Germination was conducted in the dark at 25 ± 2 ºC. Number of germinated seeds was counted after 24 h. Germinated seeds were grown in a light box at 25 ± 2 ºC under 16/8 h (light/dark) photoperiod provided by cool- white fluorescent lamps (Philips TL-D 18W/54 T8 G13). Primary root length (L) and shoot length (l) was measured on 7-day-old-seedlings. Pigments and flavonoids were extracted from 0.1 g of dry mass (crushed and sieved through the sieve with pore size of 1.5 mm) with 1 ml of 70% ethanol for 24 hours at 24 ºC. Total chlorophyll (Ca and Cb) and carotenoids (Ccar) content was determined using a FLUOstar®Omega spectrophotometer (Germany) by measuring the absorbance of the ethanol extract of pigments at 649 and 665 nm (for chlorophylls) and at 479 nm (for carotenoids) [14]. Total flavonoid content of the plant extracts (Cfl) was determined using the aluminum chloride colorimetric assay at 415 nm [15]. Rutin was used as a reference compound. The statistical processing and analysis of the experimental data were conducted in Excel application of the standard Microsoft Office XP package (Microsoft, USA). If the samplings were subject to the normal distribution law, Student’s T-test was used for their comparison. The obtained results were considered reliable at the significance level, set at p<0.05. Notes The authors declare no conflict of interest. References 1. Pramanick, B.; Dubey, R.; Kesarwani, A.; Bera, A.; Bhutia, K.L.; Kumar, M.; Maitra, S. In Antibiotic stress in wheat; Advancement in mitigating the effects of waterlogging stress in wheat; Khan, M.K.; Pandey, A.; Hamurcu, M.; Gupta, O.P.; Gezgin, S.; Eds.; Academic Press, 2023; pp. 339-355. 2. Pernak, J.; Niemczak, M.; Materna, K.; Marcinkowska, K.; Praczyk, T. Ionic liquids as herbicides and plant growth regulators. Tetrahedron, 2013, 69, 4665-4669. 3. Pernak, J.; Giszter, R.; Biedziak, A.; Niemczak, M.; Olszewski, R.; Marcinkowska, K.; Praczyk, T. Alkyl (C16, C18, C22) trimethylammonium-based herbicidal ionic liquids. J. Agric. Food Chem., 2017, 65, 260-269. 4. Pernak, J.; Markiewicz, B.; Zgoła-Grzeskowiak, A.; Chrzanowski, Ł.; Gwiazdowski, R.; Marcinkowska, K.; Praczyk, T. Ionic liquids with dual pesticidal function. RSC Adv., 2014, 4, 39751-39754. 5. Zajac, A.; Kukawka, R.; Pawlowska-Zygarowicz, A.; Stolarska, O.; Smiglak, M. Ionic liquids as bioactive chemical tools for use in agriculture and the preservation of agricultural products. Green Chem., 2018, 20, 4764-4789. 6. Stolte, S.; Arning, J.; Bottin-Weber, U.; Müller, A.; Pitner, W.-R.; Welz-Biermann, U.; Jastorff, B.; Ranke, J. Effects of different head groups and functionalised side chains on the cytotoxicity of ionic liquids. Green Chem. 2007, 9, 760-767. 7. Pretti, C.; Chiappe, C.; Baldetti, I.; Brunini, S.; Monni, G.; Intorre, L. Acute toxicity of ionic liquids for three freshwater organisms: Pseudokirchneriella subcapitata, Daphnia magna and Danio rerio. Ecotoxicol. Environ. Saf. 2009, 72, 1170-1176. 8. Trush, M.; Metelytsia, L.; Semenyuta, I.; Kalashnikova, L.; Papeykin, O.; Venger, I.; Tarasyuk, O.; Bodachivska, L.; Blagodatnyi, V.; Rogalsky, S. Reduced ecotoxicity and improved biodegradability of cationic biocides based on ester-functionalized pyridinium ionic liquids. Environ. Sci. Pollut. Res. Int. 2019, 26, 4878-4889. 9. Tot, A.; Vraneš, M.; Maksimović, I.; Putnik-Delić, M.; Daničić, M.; Belić, S.; Gadžurić, S. The effect of imidazolium based ionic liquids on wheat and barley germination and growth: influence of length and oxygen functionalization of alkyl side chain. Ecotoxicol. Environ. Saf., 2018, 147, 401-406. 10. Agati, G.; Azzarello, E.; Pollastri, S.; Tattini, M. Flavonoids as antioxidants in plants: location and functional significance. Plant Sci. 2012, 196, 67-76. 11. Lysytsya, A.; Lyco, S.; Portuhaj, O. The polyhexamethylene- guanidine stimulation of seeds growing and cell proliferation. J. Mater. Sci. Eng. B, 2013, 3, 653-660. 12. Lyoshyna, L.; Tarasyuk, O.; Bulko, O.; Rogalsky, S.; Kamenieva, T.; Kuchuk, M. Effect of polymeric biocide polyhexamethylene guanidine hydrochloride on morpho-physiological and biochemical parameters of wheat seedlings under copper stress. Agric. Sci. Pract., 2020, 7, 49-58. 13. Xu, Y.; Wang, J.; Zhu, L.; Du, Z.; Wang, J.; Wei, K. Physiological and biochemical responses of wheat (Triticum aestivum L.) seedlings to three imidazolium-based ionic liquids in soil. Chemosphere, 2017, 191, 81-88. 14. Lichtenthaler, H.K. Chlorophylls and carotenoids: pigments of photosynthetic biomembranes. Method. Enzymol. 1987, 148, 350- 382. 15. Li, Y.; Ma, D.; Sun, D.; Wang, C.; Zhang, J.; Xie, Y.; Gu, T. Total phenolic, flavonoid content, and antioxidant activity of flour, noodles, and steamed bread made from different colored wheat grains by three milling methods. Crop. J. 2015, 3, 328-334. S.P. Rogalsky, O.P. Tarasyuk et al. 45 Дослідження ріст-стимулюючого впливу 1-(2-(додецилокси)-2-оксоетил)піридин- 1-ій хлориду на проростки насіння пшениці С.П. Рогальський1*, О.П. Тарасюк1, О.В. Булко2, Л.Г. Льошина2 1 Інститут біоорганічної хімії та нафтохімії ім. В.П. Кухаря НАН України, Київ, Україна. 2 Інститут клітинної біології та генетичної інженерії НАН України, Київ, Україна. Резюме: Синтезовано довголанцюгову піридинієву сіль 1-(2-(додецилокси)-2-оксоетил)піридин-1-ій хлорид (1b), що функціоналізована полярною естерною групою у складі алкільного радикала. Досліджено вплив цієї сполуки на морфо-фізіологічні характеристики проростків насіння пшениці (схожість, довжина пагона і кореня, біомаса, вміст пігментів і флавоноїдів). Після обробки насінин водними розчинами піридинієвої солі 1b з концентраціями 0.001-0.1% зростала їх схожість. Однак концентрація сполуки 0.1% має негативний вплив на ріст рослин і спричиняє зменшення ростових параметрів пагонів і коренів, маси і вмісту пігментів. В той же час, обробка насінин розчинами піридинієвої солі з меншими концентраціями (зокрема, 0.001%) сприяла зростанню довжини пагонів і коренів, а також зеленої біомаси у семиденних проростках пшениці. За концентрації 0.01% сполука спричиняє значне збільшення вмісту хлорофілів і каротиноїдів, що свідчить про її позитивний вплив на фотосинтетичний апарат рослин. Суттєве зростання вмісту флавоноїдів в зеленій частині рослин може свідчити про активацію захисної системи за умов помірного стресу. Ріст-стимулюючий вплив довголанцюгової піридинієвої солі 1b на насіння пшениці у поєднанні з широким спектром антимікробної активності та біодеструктивності сполуки свідчать про її перспективність для застосувань в агрохімічному секторі. Ключові слова: довголанцюгова піридинієва сіль; насіння пшениці; ріст-стимулюючий ефект; захист рослин.
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spelling oai:ojs2.bioorganica.com.ua:article-762026-07-19T14:56:54Z Evaluation of growth-promoting effect of 1-(2-(dodecyloxy)-2-oxoethyl)pyridin-1-ium chloride on wheat seedlings Дослідження ріст-стимулюючого впливу 1-(2-(додецилокси)-2-оксоетил)піридин-1-ій хлориду на проростки насіння пшениці Rogalsky, Sergiy P. Tarasyuk, Oksana P. Bulko, Olga V. Lioshyna, Lyudmila G. long-chain pyridinium salt wheat seeds growth-promoting effect plant protection довголанцюгова піридинієва сіль насіння пшениці ріст-стимулюючий ефект захист рослин Ester-functionalized long-chain pyridinium salt 1-(2-(dodecyloxy)-2-oxoethyl)pyridin-1-ium chloride (1b) has been synthesized. The influence of the substance on morpho-physiological traits of wheat seedlings (germination, shoot and root length and biomass, chlorophylls and carotenoids content, as well as flavonoid content) has been studied. The germination of seeds increased after their exposure to water solutions of pyridinium chloride 1b in the concentration range 0.001-0.1%. However, the concentration 0.1% has a negative effect on plant growth leading to reduced growth parameters in shoots and roots, plant mass, as well as pigments content. The exposure of wheat seeds to water solutions of pyridinium salt with lower concentrations (especially at 0.001%) significantly increased shoot and root length, as well as wet green mass in 7-day-old seedlings. At a concentration of 0.01%, the substance caused a significant increase of chlorophyll a, chlorophyll b, and carotenoids content thus revealing a positive effect on the photosynthetic apparatus of plant leaves. The flavonoid content in a green part of the plants also significantly increased which may indicate activating the plant defense system under mild stress conditions. The high growth-promoting effect of long-chain pyridinium chloride 1b on wheat plants, together with its broad range of antimicrobial activity and biodegradability, makes it an attractive product for various agrochemical applications Синтезовано довголанцюгову піридинієву сіль 1-(2-(додецилокси)-2-оксоетил)піридин-1-ій хлорид (1b), що функціоналізована полярною естерною групою у складі алкільного радикала. Досліджено вплив цієї сполуки на морфо-фізіологічні характеристики проростків насіння пшениці (схожість, довжина пагона і кореня, біомаса, вміст пігментів і флавоноїдів). Після обробки насінин водними розчинами піридинієвої солі 1b з концентраціями 0.001-0.1% зростала їх схожість. Однак концентрація сполуки 0.1% має негативний вплив на ріст рослин і спричиняє зменшення ростових параметрів пагонів і коренів, маси і вмісту пігментів. В той же час, обробка насінин розчинами піридинієвої солі з меншими концентраціями (зокрема, 0.001%) сприяла зростанню довжини пагонів і коренів, а також зеленої біомаси у семиденних проростках пшениці. За концентрації 0.01% сполука спричиняє значне збільшення вмісту хлорофілів і каротиноїдів, що свідчить про її позитивний вплив на фотосинтетичний апарат&amp;nbsp; рослин. Суттєве зростання вмісту флавоноїдів в зеленій частині рослин може свідчити про активацію захисної системи за умов помірного стресу. Ріст-стимулюючий вплив довголанцюгової піридинієвої солі 1b на насіння пшениці у поєднанні з широким спектром антимікробної активності та біодеструктивності сполуки свідчать про її перспективність для застосувань в агрохімічному секторі V.P. Kukhar Institute of Bioorganic Chemistry and Petrochemistry of the National Academy of Sciences of Ukraine 2023-12-30 Article Article application/pdf https://bioorganica.com.ua/index.php/journal/article/view/76 10.15407/bioorganica2023.02.041 Ukrainica Bioorganica Acta; Vol. 18 No. 2 (2023): Ukrainica Bioorganica Acta; 41-45 Ukrainica Bioorganica Acta; Том 18 № 2 (2023): Ukrainica Bioorganica Acta; 41-45 1814-9766 1814-9758 10.15407/bioorganica2023.02 en https://bioorganica.com.ua/index.php/journal/article/view/76/77 Copyright (c) 2023 Sergiy P. Rogalsky, Oksana P. Tarasyuk, Olga V. Bulko, Lyudmila G. Lioshyna https://creativecommons.org/licenses/by/4.0
spellingShingle довголанцюгова піридинієва сіль
насіння пшениці
ріст-стимулюючий ефект
захист рослин
Rogalsky, Sergiy P.
Tarasyuk, Oksana P.
Bulko, Olga V.
Lioshyna, Lyudmila G.
Дослідження ріст-стимулюючого впливу 1-(2-(додецилокси)-2-оксоетил)піридин-1-ій хлориду на проростки насіння пшениці
title Дослідження ріст-стимулюючого впливу 1-(2-(додецилокси)-2-оксоетил)піридин-1-ій хлориду на проростки насіння пшениці
title_alt Evaluation of growth-promoting effect of 1-(2-(dodecyloxy)-2-oxoethyl)pyridin-1-ium chloride on wheat seedlings
title_full Дослідження ріст-стимулюючого впливу 1-(2-(додецилокси)-2-оксоетил)піридин-1-ій хлориду на проростки насіння пшениці
title_fullStr Дослідження ріст-стимулюючого впливу 1-(2-(додецилокси)-2-оксоетил)піридин-1-ій хлориду на проростки насіння пшениці
title_full_unstemmed Дослідження ріст-стимулюючого впливу 1-(2-(додецилокси)-2-оксоетил)піридин-1-ій хлориду на проростки насіння пшениці
title_short Дослідження ріст-стимулюючого впливу 1-(2-(додецилокси)-2-оксоетил)піридин-1-ій хлориду на проростки насіння пшениці
title_sort дослідження ріст-стимулюючого впливу 1-(2-(додецилокси)-2-оксоетил)піридин-1-ій хлориду на проростки насіння пшениці
topic довголанцюгова піридинієва сіль
насіння пшениці
ріст-стимулюючий ефект
захист рослин
topic_facet long-chain pyridinium salt
wheat seeds
growth-promoting effect
plant protection
довголанцюгова піридинієва сіль
насіння пшениці
ріст-стимулюючий ефект
захист рослин
url https://bioorganica.com.ua/index.php/journal/article/view/76
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