Mолекулярна ізомеризація димерів n-пропанолу

The molecular isomerization has been studied in n-propanol dimers by quantum-chemical calculations with the DFT method. 25 combinations of molecular pairs are calculated with and without consideration of the dielectric constant of n-propanol. Such approach allowed us to determine the most stable con...

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Bibliographic Details
Date:2020
Main Authors: Doroshenko, I., Vaskivskyi, Ye., Chernolevska, Ye., Meyliev, L., Kuyliev, B.
Format: Article
Language:English
Published: Publishing house "Academperiodika" 2020
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Online Access:https://ujp.bitp.kiev.ua/index.php/ujp/article/view/2019602
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Journal Title:Ukrainian Journal of Physics

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Ukrainian Journal of Physics
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Summary:The molecular isomerization has been studied in n-propanol dimers by quantum-chemical calculations with the DFT method. 25 combinations of molecular pairs are calculated with and without consideration of the dielectric constant of n-propanol. Such approach allowed us to determine the most stable configurations of alcohol dimers. It has been shown that dimers of n-propanol are mostly (77.1%) formed by only 5 of 25 possible configurations at room temperature and by 2 combinations (87.3%) at the melting point. The size distribution of dimers and the spectral dispersion in the region of free and bonded O–H stretching vibrations are calculated.