Особливості теплового руху в кристалах, утворених молекулами броміду цетилтриметиламонію

Phase transformations in CTAB polycrystals are investigated with the use of the thermophysical, dielectric, and spectroscopic techniques. A molecular model of these transformations is proposed. According to this model, the free volume in the intercrystalline layer of CTAB polycrystals starts to grow...

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Datum:2025
Hauptverfasser: Alekseev, O.M., Lazarenko, M.M., Puchkovska, G.O., Bezrodnaya, T.V., Sendzyuk, A.A.
Format: Artikel
Sprache:Ukrainian
English
Veröffentlicht: Publishing house "Academperiodika" 2025
Schlagworte:
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Online Zugang:https://ujp.bitp.kiev.ua/index.php/ujp/article/view/2022236
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Назва журналу:Ukrainian Journal of Physics

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Ukrainian Journal of Physics
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Zusammenfassung:Phase transformations in CTAB polycrystals are investigated with the use of the thermophysical, dielectric, and spectroscopic techniques. A molecular model of these transformations is proposed. According to this model, the free volume in the intercrystalline layer of CTAB polycrystals starts to grow at 10 °С, and Br− ions bound with the –N(CH3)3 terminal groups increase their mobility. At 55 °С, topological solitons of the “one-unit constriction with 180° reorientation” type appear. They arise at terminal methyl groups, pass by the molecules, and are reflected from–N(CH3)3 groups. In this case, CTAB crystals pass to the orthorhombic rotation-crystalline phase. At 92 °С, topological solitons change the orientation of the terminal –N(CH3)3 groups, which results in the melting of nonpolar aliphatic layers.