Electronic structure and magnetic properties of graphite intercalated with 3d-metals

Electronic structure and magnetic properties of graphite-based systems with intercalated 3d-transition metal atoms (V, Cr, Mn, Fe, Co, Ni) were calculated ab initio using the density functional theory. The presence of different magnetic states depending on the type of inserted M atoms is revealed f...

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Datum:2014
Hauptverfasser: Grechnev, G.E., Lyogenkaya, A.A., Kolesnichenko, Yu.A., Prylutskyy, Yu.I., R., Hayn
Format: Artikel
Sprache:English
Veröffentlicht: Фізико-технічний інститут низьких температур ім. Б.І. Вєркіна НАН України 2014
Schriftenreihe:Физика низких температур
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Online Zugang:https://nasplib.isofts.kiev.ua/handle/123456789/119495
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Назва журналу:Digital Library of Periodicals of National Academy of Sciences of Ukraine
Zitieren:Electronic structure and magnetic properties of graphite intercalated with 3d-metals / G.E. Grechnev, A.A. Lyogenkaya, Yu.A. Kolesnichenko, Yu.I. Prylutskyy, R. Hayn // Физика низких температур. — 2014. — Т. 40, № 5. — С. 580-584. — Бібліогр.: 17 назв. — англ.

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Digital Library of Periodicals of National Academy of Sciences of Ukraine
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Zusammenfassung:Electronic structure and magnetic properties of graphite-based systems with intercalated 3d-transition metal atoms (V, Cr, Mn, Fe, Co, Ni) were calculated ab initio using the density functional theory. The presence of different magnetic states depending on the type of inserted M atoms is revealed for hexagonal P6/mmm and P6 3/mmc crystall structures. The values of magnetic moments appeared to be governed by the p–d hybridization, and by variations of exchange interactions with intercalation. The results of calculations clearly indicate itinerancy of the 3d-electrons of inserted M atoms.