Semiconductor sensors for dosimetry of epithermal neutrons

Minimum energy of neutron to displace atoms in silicon crystals are equal to 200 eV. Due to this fact testing our p-i-n diodes under irradiation by the epithermal neutrons was carried out. The more advanced p-i-n diodes on the base of high purity silicon were used at present work, and, as a result,...

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Date:1999
Main Authors: Litovchenko, P.G., Moss, R., Stecher-Rasmussen, F., Appelman, K., Barabash, L.I., Kibkalo, T.I., Lastovetsky, V.F., Litovchenko, A.P., Pinkovska, M.B.
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Language:English
Published: Інститут фізики напівпровідників імені В.Є. Лашкарьова НАН України 1999
Series:Semiconductor Physics Quantum Electronics & Optoelectronics
Online Access:https://nasplib.isofts.kiev.ua/handle/123456789/119067
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Cite this:Semiconductor sensors for dosimetry of epithermal neutrons / P.G. Litovchenko, R. Moss, F. Stecher-Rasmussen, K. Appelman, L.I. Barabash, T.I. Kibkalo, V.F. Lastovetsky, A.P. Litovchenko, M.B. Pinkovska // Semiconductor Physics Quantum Electronics & Optoelectronics. — 1999. — Т. 2, № 2. — С. 90-91. — Бібліогр.: 4 назв. — англ.

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Digital Library of Periodicals of National Academy of Sciences of Ukraine
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spelling nasplib_isofts_kiev_ua-123456789-1190672025-02-09T17:22:50Z Semiconductor sensors for dosimetry of epithermal neutrons Litovchenko, P.G. Moss, R. Stecher-Rasmussen, F. Appelman, K. Barabash, L.I. Kibkalo, T.I. Lastovetsky, V.F. Litovchenko, A.P. Pinkovska, M.B. Minimum energy of neutron to displace atoms in silicon crystals are equal to 200 eV. Due to this fact testing our p-i-n diodes under irradiation by the epithermal neutrons was carried out. The more advanced p-i-n diodes on the base of high purity silicon were used at present work, and, as a result, we have obtained considerably more sensitive sensors for more wide range of neutron doses. The sensitivity of sensors is 0.14 V/Gy for average neutron energy of 24 keV. 1999 Article Semiconductor sensors for dosimetry of epithermal neutrons / P.G. Litovchenko, R. Moss, F. Stecher-Rasmussen, K. Appelman, L.I. Barabash, T.I. Kibkalo, V.F. Lastovetsky, A.P. Litovchenko, M.B. Pinkovska // Semiconductor Physics Quantum Electronics & Optoelectronics. — 1999. — Т. 2, № 2. — С. 90-91. — Бібліогр.: 4 назв. — англ. 1560-8034 PACS 29.40.Wk https://nasplib.isofts.kiev.ua/handle/123456789/119067 en Semiconductor Physics Quantum Electronics & Optoelectronics application/pdf Інститут фізики напівпровідників імені В.Є. Лашкарьова НАН України
institution Digital Library of Periodicals of National Academy of Sciences of Ukraine
collection DSpace DC
language English
description Minimum energy of neutron to displace atoms in silicon crystals are equal to 200 eV. Due to this fact testing our p-i-n diodes under irradiation by the epithermal neutrons was carried out. The more advanced p-i-n diodes on the base of high purity silicon were used at present work, and, as a result, we have obtained considerably more sensitive sensors for more wide range of neutron doses. The sensitivity of sensors is 0.14 V/Gy for average neutron energy of 24 keV.
format Article
author Litovchenko, P.G.
Moss, R.
Stecher-Rasmussen, F.
Appelman, K.
Barabash, L.I.
Kibkalo, T.I.
Lastovetsky, V.F.
Litovchenko, A.P.
Pinkovska, M.B.
spellingShingle Litovchenko, P.G.
Moss, R.
Stecher-Rasmussen, F.
Appelman, K.
Barabash, L.I.
Kibkalo, T.I.
Lastovetsky, V.F.
Litovchenko, A.P.
Pinkovska, M.B.
Semiconductor sensors for dosimetry of epithermal neutrons
Semiconductor Physics Quantum Electronics & Optoelectronics
author_facet Litovchenko, P.G.
Moss, R.
Stecher-Rasmussen, F.
Appelman, K.
Barabash, L.I.
Kibkalo, T.I.
Lastovetsky, V.F.
Litovchenko, A.P.
Pinkovska, M.B.
author_sort Litovchenko, P.G.
title Semiconductor sensors for dosimetry of epithermal neutrons
title_short Semiconductor sensors for dosimetry of epithermal neutrons
title_full Semiconductor sensors for dosimetry of epithermal neutrons
title_fullStr Semiconductor sensors for dosimetry of epithermal neutrons
title_full_unstemmed Semiconductor sensors for dosimetry of epithermal neutrons
title_sort semiconductor sensors for dosimetry of epithermal neutrons
publisher Інститут фізики напівпровідників імені В.Є. Лашкарьова НАН України
publishDate 1999
url https://nasplib.isofts.kiev.ua/handle/123456789/119067
citation_txt Semiconductor sensors for dosimetry of epithermal neutrons / P.G. Litovchenko, R. Moss, F. Stecher-Rasmussen, K. Appelman, L.I. Barabash, T.I. Kibkalo, V.F. Lastovetsky, A.P. Litovchenko, M.B. Pinkovska // Semiconductor Physics Quantum Electronics & Optoelectronics. — 1999. — Т. 2, № 2. — С. 90-91. — Бібліогр.: 4 назв. — англ.
series Semiconductor Physics Quantum Electronics & Optoelectronics
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AT lastovetskyvf semiconductorsensorsfordosimetryofepithermalneutrons
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first_indexed 2025-11-28T13:37:36Z
last_indexed 2025-11-28T13:37:36Z
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fulltext 90 © 1999, Institute of Semiconductor Physics, National Academy of Sciences of Ukraine Semiconductor Physics, Quantum Electronics & Optoelectronics. 1999. V. 2, N 2. P. 90-91. PACS 29.40.Wk Semiconductor sensors for dosimetry of epithermal neutrons P. G. Litovchenko1, R. Moss2, F. Stecher-Rasmussen2, K. Appelman2, L. I. Barabash1, T. I. Kibkalo1, V. F. Lastovetsky1, A. P. Litovchenko1, M. B. Pinkovska1. 1 SC Institute for Nuclear Research of NASU, 47 prospect Nauki, 252028 Kiev, Ukraine. 2 ECN, Westerduinweg 3, P. O. Box 1,1755 ZG Petten, The Netherlands. Abstract. Minimum energy of neutron to displace atoms in silicon crystals are equal to 200 eV. Due to this fact testing our p-i-n diodes under irradiation by the epithermal neutrons was carried out. The more advanced p-i-n diodes on the base of high purity silicon were used at present work, and, as a result, we have obtained considerably more sensitive sensors for more wide range of neutron doses. The sensitivity of sensors is 0.14 V/Gy for average neutron energy of 24 keV. Keywords: dosimetry, semiconductor detectors, epithermal neutrons, silicon, converter. Paper received 17.05.98; revised manuscript received 26.06.98; accepted for publication 12.07.98. 1. Introduction The measurement of epithermal neutron flux is very signifi- cant task for Boron Neutron Capture Therapy (BNCT). In this paper semiconductor sensors were used for epithermal neutron flux measurement. These semiconductor sensors were produced by us. These are p-i-n diodes and semicon- ductor detectors with 235U converter. Possibilities for application of fast neutron dosime- ters using the p-i-n diodes as a base have been shown earlier [1]. The principle of detection is based on the cre- ation of radiation defects in semiconductors under the influence of fast neutrons, which change the electrical parameters (a diode voltage drop increases for a fixed current). It is known that the minimum energy of neu- tron to displace atoms in silicon crystals is equal to ~ 200 eV. Due to this fact there were all reasons to test the p-i-n diodes prepared by us under irradiation in the epithermal neutron energy range. 2. Experimental results At the beginning of investigation, our colleagues and we have made the detail analysis of all available dates, such as the KERMA damage and the total KERMA for silicon [2]. The results of experimental verification for monoenergetic neutrons in the energy range from 90 to 900 keV were ob- tained in [2]. In spite of the complicated view of the KERMA damage dependence, as evident from these data, a proper coincidence between the experimental results and theoreti- cal calculations of KERMA by Monte Karlo method was obtained. The presence of some hollow in the neutron ener- gy range from 100 to 300 eV partly makes difficulties to use the p-i-n diodes as tissue-equivalent sensors in practically used energy range of epithermal neutrons. There is doubt- less interest to test the offered by us semiconductor sen- sors intended for measurements of total tissue dose from the extremely complicated spectrum of Petten High Flux Re- actor, which was used in BNCT [3]. From these data, the fast neutrons (>10keV) make a considerable and undesirable contribution to damage KERMA. In our work [4], it was shown that p-i-n diodes, which were calibrated with a known energy, could be used to determine tissue doses, received in the courses of irradiation by neutrons with an unknown energy. Proceeding from this fact, we were able to determine a sensitivity of our sensors under the energy of 24 keV (the channel HB12) and intensity of 1.23.1012 n/m2.sec. The changes of a direct voltage drop (∆V) for p-i-n di- odes under fixed current of 1mA (at irradiation time 85 min, P.G. Litovchenko et al.: Semiconductor sensors for dosimetry of... 91SQO, 2(2), 1999 En = 24 keV, tissue KERMA 1Gy = 5.1015 n/m2) were mea- sured. The average changes of the direct voltage drop is ∆V = 0.175 V and the received dose is Φ = 1.25 Gy. The average sensitivity of sensors was ∆V/Φ = 0.140 V/Gy. Dose dependences of ∆V were obtained by means of additional irradiation of the same diodes up to the total 16 hours. Dose dependencies are presented in Fig. 1 for the sensors of numbers 2n and 3n with the best and the worst sensitivities, respectively. As one can see from Fig. 1, the changes of a direct voltage drop are very good fits to linear dependence ∆V vs Φ in the range of used irradiation doses. Mentioned sensors were calibrated in the channel HB12, and then irradiated in the channel HB11 for 1.8.103sec. Our sensors give the average tissue dose of neutrons as much as Φ = (2.76±0.16)Gy per hour. In this channel, besides neutrons, the gamma irradiation is presents, according to the HB11 channel technical char- acteristics, and gives the contribution to dose 1.2 Gy per hour. As the coefficient of discrimination for our neutron sensors in relation to the gamma irradiation is ~103 [2], then the determined above tissue dose entirely relates to the neu- tron spectrum of the channel HB 11. Proceeding from the HB11 technical characteristics one may appreciate the share of fast and epithermal neutrons into tissue KERMA. The epithermal neutron flux (0,414 eV-10 keV) is 3.3.1012 n/m2sec. If we suppose that all neutrons in this spectrum possess the energy as much as 10 keV (KERMA = 1016 n/m2), then the dose will correspond to Φ = 1.2 Gy per hour. Under assump- tion that both the average energy and flux of fast neutrons are 0.5MeV(KERMA = 5.6.108), and 4.7.107n/cm2/s (>10keV) respectively, we obtained Φ = 1.6 Gy. These appraisals of ours coincide with obtained by us results on the total dose (1.6+1.2)=2.8 Gy and confirm an undesirable contribution of fast neutrons (60%) in the total theraputical dose. The epithermal neutron flux at the HB11 channel was measured also by the silicon barrier-surface detectors with an attached 235U converter. The converter as 235U oxide- protoxide being enriched up to 99.92 % with the thickness of 1.5.10-4 m, mass 10-6 kg and alpha activity of 81 Bq was fabricated on Al- sublayer. We established that the detec- tors efficiency to epithermal neutrons the (HB11 neutron spectrum) is 1.82.10-5imp/n. Conclusions The use of p-i-n diodes made on the base of high purity silicon for registration of epithermal neutrons with the coefficient of gamma ray discrimination 103 is demon- strated. A good agreement of experimental data with theoretical calculations of the damage KERMA for sili- con has been shown. It is shown that p-i-n diodes can serve as tissue-equiv- alent dosimeters in the neutron energy range from 300 eV till 30 keV. The possibility of neutron flux monitoring by means of silicon detectors with 235U converter was shown. References 1. A. B. Rosenfeld, L. I.Barabash, P. G. Litovchenko, V. I. Khivrich, P-i-n Diode with a Wide Measurement Range of Fast Neutron Dos- es., Rad. Prot. Dos., 33(l/4), pp. 175-178 (1990). 2. M. G. Carolan, A. B. Rosenfeld, S. Wallace, H. Mariaty, G. J. Storr, V. I. Khivrich, R. Moss, B. J. Alien, Silicon Dosime- ter Diode for BNCT Using Epithermal Neutron Sources. Proc. of 1-st Intern. Workshop on Accelerator-Based Neutron Sources for BNCT, l, September 11-14, 1994, Jacson, Wyoming, pp. 299-309. 3. Boron Neutron Capture Therapy, Proc. of Intern. Workshop and plenary meeting, Petten The Netherlands, 1991, Edited by D. Gabel and R. Moss, p.47. 4. V. I. Khivrich, M. D. Varentsov, P. G. Litovchenko, A. I. Ano- khin, A. B. Rosenfeld, M. G. Carolan, O. S. Zinets, M. I. Rein- hard, D. Alexiev, High Purity Silicon as a Basic Material for Man- ufacturing of Radiation Defects and Integral Neutron Dosimeters, IEEE Trans. on Nucl. Sci., NS-43, N6, pp. 2687-2692 (1996). Fig. 1. Dose dependence as a function of change of voltage (∆V) at p-i-n diodes with big (2n) and little (3n) sensitivity under irradiation of neutron with energy of 24 keV. 1 10 1 10 1 1 0.1 0.1 ΦΦΦΦΦ, Gy ∆∆∆∆ ∆V , V